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RESEARCH PAPER · Angewandte Chemie International Edition · 2025

Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene Hydrogenolysis

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Tandem Catalysis for Plastic Depolymerization: In Situ Hydrogen Generation via Methanol Aqueous Phase Reforming for Sustainable Polyethylene HydrogenolysisOriginalAdvances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design6Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites14Single-atom alloys for sustainability-related electrocatalytic applications1CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor20Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics3Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Sustainable polyolefin upcycling using liquid organic hydrogen carrier based hydrogen delivery and hydrocracking11Research progress of high value utilization of waste polyethylene plastics6Catalytic transfer reductive conversion of plastic wastes into fuel and chemicals0Steering C–C bond cleavage and hydrogenation in polystyrene hydrocracking through external Brønsted acid sites over Ni/zeolites1Enhancing Hydrogen Spillover via Crystalline-Phase Engineering of Ru/ZrO 2 for Selective Liquid Alkane Production in Polyethylene Hydrogenolysis6Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling1Tandem hydropyrolysis–hydrogenolysis of polyolefin wastes over morphology‐tuned Co 3 O 4 for jet‐fuel hydrocarbons0Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Carbonylolysis of waste polyesters into high-value organic acids5Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis0Lattice Hydroxyl‐Assisted Platinum Single Atom Catalyst Toward Hydrogen Production From Methanol Aqueous Reforming4Piezocatalytic reforming of plastics into high-value chemicals5Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis0Catalytic Microwave Pyrolysis of Plastic Waste for Hydrogen and Nanocarbons0A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Atomically precise catalysts design toward efficient waste plastic hydrogenolysis2Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products0Light‐Driven Coupled Upcycling of Polyethylene and CO 2 to Aromatics over Zeolite–Ni/CeO 2 Composite Catalysts0Coupling Polyolefin Conversion and Methanol Reduction for C 9 –C 10 Alkylaromatic Production1

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  1. Advances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design

    Chemical Communications · 2025-01-01

    M.J. Kim, Insoo Ro

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  2. Complementary acid site mechanisms in hydrogen-free polyethylene upcycling: elucidating the distinct roles of Brønsted and Lewis sites in Ce-modified zeolites

    Green Chemistry · 2025-01-01

    Taeeun Kwon, J. S. PARK, Ki Hyuk Kang, Dae-Sung Jung, Wangyun Won, Insoo Ro

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  3. Single-atom alloys for sustainability-related electrocatalytic applications

    Frontiers of Chemical Science and Engineering · 2025-06-16

    Mingming Yin, Yunfei Gao, Chenchen Cui, Wei Ma, Lili Zhang, Zhen Ping Zhou

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  4. CO-promoted polyethylene hydrogenolysis with renewable formic acid as hydrogen donor

    Nature Communications · 2025-08-21

    Yuqi Wang, Qikun Hu, Shuairen Qian, Jiayang Zhao, Yi Cheng, Jun Ma, Jing Zhang, Zhiqiang Niu

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  5. Hydrogen-Free Catalytic Strategies for the Upcycling of Polyolefin Plastics

    Korean Journal of Chemical Engineering · 2025-10-20

    Taeeun Kwon, Jae Woo Kim, Insoo Ro

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  6. Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives

    Advanced Functional Materials · 2025-11-10

    Yanan Diao, Xuetao Qin, Chengxin Hou, Bingbing Chen, Tianqi Yun, Xinwen Guo, Ding Ma, Chuan Shi

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  7. Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion

    ACS Catalysis · 2025-12-10

    Fan Yuan, Hongshun Ran, Tingxi Chen, Yaxuan Jing

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  8. Sustainable polyolefin upcycling using liquid organic hydrogen carrier based hydrogen delivery and hydrocracking

    Nature Communications · 2025-12-24

    Taeeun Kwon, Seoyoung Ahn, Taehyup Kim, Jong Hun Kang, Soo-Hwa Jeong, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  9. Research progress of high value utilization of waste polyethylene plastics

    Green Chemistry · 2025-12-30

    Mingjun Xiao, Xihang Dai

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  10. Catalytic transfer reductive conversion of plastic wastes into fuel and chemicals

    Green Chemistry · 2026-01-01

    Yinghui Chen, Huayang Lin, Ruixing Wang, Jiaqi Qiao, Sibao Liu, Guozhu Liu

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  11. Steering C–C bond cleavage and hydrogenation in polystyrene hydrocracking through external Brønsted acid sites over Ni/zeolites

    Catalysis Science & Technology · 2026-01-01

    Jonghyun Park, Taeeun Kwon, Ki Hyuk Kang, Wangyun Won, Insoo Ro

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  12. Enhancing Hydrogen Spillover via Crystalline-Phase Engineering of Ru/ZrO 2 for Selective Liquid Alkane Production in Polyethylene Hydrogenolysis

    ACS Sustainable Chemistry & Engineering · 2026-01-07

    Qingming Fan, Jiaojiao Gao, Xintian Luo, Zeyu He, Boran Wang, Jing Ming Xu

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  13. Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling

    Discover Chemistry. · 2026-01-20

    Haokun Wang, Dermot O’Hare

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  14. Tandem hydropyrolysis–hydrogenolysis of polyolefin wastes over morphology‐tuned Co 3 O 4 for jet‐fuel hydrocarbons

    AIChE Journal · 2026-02-05

    Dongxian Li, Xiaocao Shan, Xianzhi Meng, Jia Wang, Jianchun Jiang, Arthur J. Ragauskas

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  15. Thermo-chemical upgrading of waste polyethylene and polypropylene plastics

    Scientia Sinica Chimica · 2026-02-26

    Wanying Han, Longfei Lin, Buxing Han

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  16. Carbonylolysis of waste polyesters into high-value organic acids

    Nature Communications · 2026-03-10

    Dongxu Liu, Siming Zhu, Qingqing Mei

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  17. Preparing methane‐resistant Ru catalysts via moderate metal‐support interactions for polyethylene hydrogenolysis

    AIChE Journal · 2026-03-16

    Yiwei Fang, Yundao Jing, Jinquan Ming, Wenjie Wang, Weixiao Sun, Xiaohu Ge, Wenyao Chen, Gang Qian, Yueqiang Cao, Xuezhi Duan, Xinggui Zhou, Jing Zhang

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  18. Lattice Hydroxyl‐Assisted Platinum Single Atom Catalyst Toward Hydrogen Production From Methanol Aqueous Reforming

    Angewandte Chemie International Edition · 2026-04-07

    Hao Meng, Shaoteng Yuan, Zhiming Yin, Tianyao Shen, Kai Ming Feng, Haisong Feng, Linlin Wang, Lirong Zheng, Song Ki Hong, Yusen Yang, Jian Zhang, Xin Zhang, Min Wei

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  19. Piezocatalytic reforming of plastics into high-value chemicals

    Nature Communications · 2026-04-16

    Z. D. Sha, Fang Chen, Cheng Hu, Hongwei Huang

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  20. Engineering Interfacial Compatibility and Dynamic Active Hydrogen Pools to Accelerate Polyolefin Hydrogenolysis

    ACS Catalysis · 2026-04-23

    Tao Guo, S T Zhang, Zhuangzhuang Lai, Zihui He, Hongshun Ran, Shourong Zheng, Yaxuan Jing, Xiaolei Qu

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  21. Catalytic Microwave Pyrolysis of Plastic Waste for Hydrogen and Nanocarbons

    Chemical Engineering & Technology · 2026-05-01

    K Karthik, Viyat Varun Upadhyay, Puppala Satyavathi, Frederick Sidney Correa, Saravanan Arumugam, Jagtej Singh, Shree Jayaram Kalyanaraman, Ramya Maranan, Anand Rajendran, Rohini Thimmapura Venkatesh

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  22. A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways

    Advanced Materials · 2026-05-12

    Chang‐Jie Yang, Xin-Yu Wang, Mei‐Qi Zhu, Tianyou Zhao, Yong-Zhou Pan, Yuhai Dou, Jie Yang, Zechao C. Zhuang, Zhenglong Li, Zhijun Wu, Wen‐Gang Cui, Hongge Pan, Weiwei Li, Dingsheng S. Wang

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  23. Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications

    Advanced Materials · 2026-05-22

    Minhao Tang, Ji Shen, Zhimin Liu

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  24. Atomically precise catalysts design toward efficient waste plastic hydrogenolysis

    Nature Communications · 2026-06-06

    Zedong Zhang, Shijie Shen, Wenwu Zhong, Wen‐Gang Cui, Yaxiong Yang, Jia Wang, Shule Wang, Hongge Pan, Dingsheng S. Wang

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  25. Advances in Catalytic Hydrogenolysis of Waste Plastics to Value-Added Products

    Industrial & Engineering Chemistry Research · 2026-06-08

    Xiaofan Zhou, Feng Xing Niu, Zeyuan Wu, Siji Wu, Ziqi Dong, Junyan Li, Da Chen

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  26. Light‐Driven Coupled Upcycling of Polyethylene and CO 2 to Aromatics over Zeolite–Ni/CeO 2 Composite Catalysts

    ChemSusChem · 2026-06-13

    Weiwei Li, Q Feng, Zhiyi Wu, Yuxuan Zhou, Jiahui Shen, Yihe Huang, Xiaohan Jin, Liu Cao, Kai Ming Feng, Xingda An, Ning Zhang, Chaoran Li, Le He

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  27. Coupling Polyolefin Conversion and Methanol Reduction for C 9 –C 10 Alkylaromatic Production

    Angewandte Chemie International Edition · 2026-07-11

    Sheng-Ren Li, Richard L. Smith, Janusz A. Koziński, Zhen Fang

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