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RESEARCH PAPER · Journal of Solid State Chemistry · 2012

BaGa2GeX6(X=S, Se): New mid-IR nonlinear optical crystals with large band gaps

Xinsong Lin, Yifeng Guo, Ning Ye

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BaGa2GeX6(X=S, Se): New mid-IR nonlinear optical crystals with large band gapsOriginalDisconnection Enhances the Second Harmonic Generation Response: Synthesis and Characterization of Ba23Ga8Sb2S38247Sulfides with Strong Nonlinear Optical Activity and Thermochromism: ACd4Ga5S12 (A = K, Rb, Cs)172Molecular Germanium Selenophosphate Salts: Phase-Change Properties and Strong Second Harmonic Generation85ChemInform Abstract: BaGa2GeX6 (X: S, Se): New mid‐IR Nonlinear Optical Crystals with Large Band Gaps.0Na2Cd7B8O20: a new noncentrosymmetric compound with special [B3O7] units20Synthesis, structure, optical property, and electronic structure of Ba7AgGa5Se159Syntheses, Structures, and Nonlinear Optical Properties of Quaternary Chalcogenides: Pb4Ga4GeQ12 (Q = S, Se)60Functionalization Based on the Substitutional Flexibility: Strong Middle IR Nonlinear Optical Selenides AXII4XIII5Se12219Metal Chalcogenides: A Rich Source of Nonlinear Optical Materials680Ba8Sn4S15: A Strong Second Harmonic Generation Sulfide with Zero-Dimensional Crystal Structure106Synthesis, Structure and Bonding, Optical Properties of Ba4MTrQ6 (M=Cu, Ag; Tr=Ga, In; Q=S, Se)18Ag 3 Ga 3 SiSe 8 : a new infrared nonlinear optical material with a chalcopyrite structure34Synthesis and characterization of ternary glasses in the system Na2Se-Ga2Se3-GeSe2111-[4-(methylsulfanyl) phenyl]-3-(4-nitropshenyl) prop-2-en-1-one: A reverse saturable absorption based optical limiter37Syntheses, Structures, and Nonlinear-Optical Properties of Metal Sulfides Ba2Ga8MS16 (M = Si, Ge)94Designing the syntheses and photophysical simulations of noncentrosymmetric compounds17Infrared nonlinear optical properties of lithium-containing diamond-like semiconductors Li 2 ZnGeSe 4 and Li 2 ZnSnSe 457SnGa 2 GeS 6 : synthesis, structure, linear and nonlinear optical properties46Second Harmonic Generation Response Optimized at Various Optical Wavelength Ranges through a Series of Cubic Chalcogenides Ba6Ag2.67+4δSn4.33−δS16–xSex41Phase-Change Behavior and Nonlinear Optical Second and Third Harmonic Generation of the One-Dimensional K(1–x)CsxPSe6 and Metastable β-CsPSe662Syntheses, crystal structures, and NLO properties of the quaternary sulfides RE3Sb0.33SiS7 (RE=La, Pr)24Synthesis, crystal structure and optical property of a novel metal chalcohalide: ZnHg3Se2Cl47Structure and properties of off-stoichiometric Ba–Ga–Ge selenide glasses5BaCdSnS 4 and Ba 3 CdSn 2 S 8 : syntheses, structures, and non-linear optical and photoluminescence properties97Quaternary BaGa2GeS6 and BaGa2GeSе6 Nonlinear Crystals for the Mid-IR Spectral Range0Ba4Ga2Se8: A ternary selenide containing chains and discrete Se22− units14Syntheses and structural characterization of non-centrosymmetric Na2M2M'S6 (M, M′=Ga, In, Si, Ge, Sn, Zn, Cd) sulfides36Hydrazine-hydrothermal syntheses, characterizations and photoelectrochemical properties of two quaternary chalcogenidoantimonates(III) BaCuSbQ3 (Q = S, Se)51Na 2 ZnGe 2 S 6 : A New Infrared Nonlinear Optical Material with Good Balance between Large Second-Harmonic Generation Response and High Laser Damage Threshold302Noncentrosymmetric selenide Ba4Ga4GeSe12: Synthesis, structure, and optical properties9Crystal growth and characterization of new quaternary chalcogenide nonlinear crystals for the mid-IR: BaGa_2GeS_6 and BaGa_2GeSe_6101Recent studies of nonlinear chalcogenide crystals for the mid-IR148A new quaternary semiconductor compound (Ba2Sb4GeS10): Ab initio study7Centrosymmetric to noncentrosymmetric structural transformation of new quaternary selenides induced by isolated dimeric [Sn 2 Se 4 ] units: from Ba 8 Ga 2 Sn 7 Se 18 to Ba 10 Ga 2 Sn 9 Se 2210Tailored synthesis of nonlinear optical quaternary chalcohalides: Ba 4 Ge 3 S 9 Cl 2 , Ba 4 Si 3 Se 9 Cl 2 and Ba 4 Ge 3 Se 9 Cl 252Second harmonic generation response of the cubic chalcogenides Ba(6−x)Srx[Ag(4−y)Sn(y/4)](SnS4)49Noncentrosymmetric chalcogenides BaZnSiSe4 and BaZnGeSe4 featuring one-dimensional structures56Discovery-Synthesis, Design, and Prediction of Chalcogenide Phases208Mid-Infrared Nonlinear Optical Materials Based on Metal Chalcogenides: Structure–Property Relationship338Numerical analysis of СО laser frequency conversion efficiency in BaGa 2 GeSe 6 crystal6Phase-matching properties of BaGa2GeSe6 for three-wave interactions in the 0778–105910 μm spectral range29Synthesis, crystal structures and nonlinear optical properties of polymorphism: α- and β-RbHgI3·H2O18A review on structure-performance relationship toward the optimal design of infrared nonlinear optical materials with balanced performances253BaB2S4: An Efficient and Air-Stable Thioborate as Infrared Nonlinear Optical Material with High Laser Damage Threshold85Recent progress on new infrared nonlinear optical materials with application prospect133Li 2 ZnGeS 4 : a promising diamond-like infrared nonlinear optical material with high laser damage threshold and outstanding second-harmonic generation response43Theoretical investigation on the promotion of second harmonic generation from chalcopyrite family A I GaS 2 to A II Ga 2 S 47Sum frequency conversion of multiline CO laser emission in BaGa2GeSe6 crystal of one cm long1The exploration of new infrared nonlinear optical crystals2Effect of S and Se replacement on electronic and thermoelectric features of BaCu2GeQ4 (Q = S, Se) chalcogenide crystals27Polycrystal Synthesis, Crystal Growth, Structure, and Optical Properties of AgGaGe n S 2( n +1) ( n = 2, 3, 4, and 5) Single Crystals for Mid-IR Laser Applications27Mixed-Anion Inorganic Compounds: A Favorable Candidate for Infrared Nonlinear Optical Materials140Synthesis and characterization of new quaternary polyselenide Ba4TMSbSe12 (TM = Nb, Ta)2Lattice Dynamics and Electronic Properties of a BaGa2GeS6 Nonlinear Crystal: Raman Scattering, IR Reflection, and ab initio Calculations6Crystal Growth and Characterization of a New Quaternary Chalcogenide Nonlinear Crystal for the Mid-Infrared: PbGa2GeSe611BaGe 2 Pn 2 (Pn = P, As): Two Congruent-Melting Non-chalcopyrite Pnictides as Mid- and Far-Infrared Nonlinear Optical Materials Exhibiting Large Second Harmonic Generation Effects54Quaternary rare-earth sulfide LaSnGa3S7: Synthesis, structure, thermal and optical properties5Effective nonlinearity of the new quaternary chalcogenide crystal BaGa 2 GeSe 624LiBa4Ga5Q12 (Q = S, Se): Noncentrosymmetric Metal Chalcogenides with a Cesium Chloride Topological Structure Displaying a Remarkable Laser Damage Threshold32BaGa 2 GeS 6 and BaGa 2 GeSe 6 crystals for nonlinear optical frequency conversion6Anionic Aliovalent Substitution from Structure Models of ZnS: Novel Defect Diamond‐like Halopnictide Infrared Nonlinear Optical Materials with Wide Band Gaps and Large SHG Effects78Anionic Aliovalent Substitution from Structure Models of ZnS: Novel Defect Diamond‐like Halopnictide Infrared Nonlinear Optical Materials with Wide Band Gaps and Large SHG Effects19Recent Advances in Oxide‐based Nonlinear Optical Materials with Wide Infrared Transparency Beyond 6 μm38Capability of frequency conversion in BGGS and BGGSe crystals0The effect of volume inclusions of the ZnGeP2 single-crystal on the dispersion of the refraction index and the absorption coefficient in mid-IR and terahertz ranges of wavelengths4α-CdP2: Large SHG Effect Originating from the Synergism of Parallel ∞1[P–] Polyanion Chains and Distorted CdP4 Tetrahedra21A review on the recently developed promising infrared nonlinear optical materials103Halonitrides Zn 2 NX (X=Cl,Br): Novel Mid-Infrared Nonlinear Optical Materials30LaSiP3 and LaSi2P6: Two Excellent Rare‐Earth Pnictides with Strong SHG Responses as Mid‐ and Far‐Infrared Nonlinear Optical Crystals36Barium nonlinear optical crystals for the mid-IR: characterization and some applications75Mg 2 In 3 Si 2 P 7 : A Quaternary Diamond-like Phosphide Infrared Nonlinear Optical Material Derived from ZnGeP 2130β-BaGa 4 Se 7 : a promising IR nonlinear optical crystal designed by predictable structural rearrangement46Pnictides: An emerging class of infrared nonlinear optical material candidates47Crystal growth and characterization of a new quaternary hexagonal nonlinear crystal for the mid-IR: Ba2Ga8GeS1619Optical and generation characteristics of new nonlinear Ba2Ga8GeS16 and Ba2Ga8(GeSe2)S14 crystals for the mid-IR range10Uncovering a Vital Band Gap Mechanism of Pnictides49Ba2MAsQ5 (Q = S and Se) Family of Polar Structures with Large Second Harmonic Generation and Phase Matchability23Crystal Growth and Chirality - Technologies and Applications12AeMg6Ga6S16 (Ae = Ca, Sr, Ba): The First Double Alkaline‐Earth Metal Chalcogenides with Excellent Performances29Temperature-dependent phase-matching properties of BaGa 2 GeS 6 in the 0.767–10.5910 µm spectral range13Trade-Off for Better Balanced Nonlinear Optical Performance with Disordered Si in ZnGeP217Recent Advances in Infrared Nonlinear Optical Crystal7A non-centrosymmetric chalcohalide synthesized through the combination of chemical tailoring with aliovalent substitution12Honeycomb layered topology construction for exceptional long-wave infrared nonlinear optical crystals29Polar Phosphorus Chalcogenide Cage Molecules: Enhancement of Nonlinear Optical Properties in Adducts39Polar Phosphorus Chalcogenide Cage Molecules: Enhancement of Nonlinear Optical Properties in Adducts1Remarkable phase-matchable second-harmonic generation realized by strong polarities of [PbSe3] and [GaSe4] functional motifs in PbGa4Se718Thermo-mechanical properties of BaGa2GeS(e)6 nonlinear optical crystals15Growth of the new high-performance NLO crystal BaGa2GeSe6 via the controlled vapor pressure method2BaCu2SiS4: A New Member of the AIIBI2MIVQ4 Chalcogenide Family with a Chiral Crystal Structure6Hg 3 AsS 4 X (X = Cl and Br): two Hg-based chalcogenides as long-wave infrared nonlinear optical crystals with superior comprehensive performances33Barium Chalcogenide Crystals: A Review27Infrared nonlinear optical materials with multiple strongly ionic cations5Barium chalcogenides for nonlinear optics in the mid-IR: Properties and applications15Homoatomic Polychalcogenide Nonlinear Optical Anionic Groups with Ultra-Large Optical Anisotropy31Insights into the optoelectronic, thermodynamic, and thermoelectric properties of novel BaYCuX3 (X = Se, Te) semiconductors from first-principles investigation3Unlocking superior performance of broadband powerful mid-IR optical parametric amplifiers with a BaGa2GeS6 crystal pumped at 1.24 µm14Effective nonlinearity of trigonal BaGa 2 GeS 65Widely Tunable BaGa 2 GeSe 6 Optical Parametric Amplifier Pumped by a Mode-Locked Nd: YAG Laser4Nonlinear absorption and refraction study of barium chalcogenide crystals3The electronic structure, optical, and transport properties of novel SrScCu3M4 (M = Se, Te) semiconductors4A Study of Effective Nonlinearity of BaGa2GeS6 Crystal by CO Laser Sum-Frequency Generation with Type-I and Type-II Phase Matching6Design of a high-performance infrared birefringent crystal Ba 4 HgP 2 Se 10 via a low-dimensional motif intercalation strategy2High-energy MIR picosecond optical parametric amplifier with ultra-wide tunability spanning from 3 to 14 µm based on BaHgGeSe 4 crystal8Five Transition Metal-Mixed Germanium Chalcogenide Materials: Solvothermal Syntheses, Crystal Structures, Photoelectric Response Properties, and Ion-Exchange Properties3Theoretical material properties of the nonlinear optical crystals: disordered barium gallium chalcogenides0Modulating Nonlinear Optical Performances in α/β-SnGa2GeS6 Polymorphs via Atomic Coordination Engineering1Ba-based IR nonlinear optical materials: synthesis, growth, structures, and properties6Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0Synthesis, structure, optical properties, and magnetic behavior of layered heavy rare-earth thiogermanates CsDyGeS4 and CsErGeS40Homologous lattice coupling drives the formation of tetrahedra-ordered phase exhibiting enhanced optical nonlinearity and band gap0

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  1. Disconnection Enhances the Second Harmonic Generation Response: Synthesis and Characterization of Ba23Ga8Sb2S38

    Journal of the American Chemical Society · 2012-03-28

    Mei‐Chun Chen, Li‐Ming Wu, Hua Lin, Liujiang Zhou, Ling Chen

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  2. Sulfides with Strong Nonlinear Optical Activity and Thermochromism: ACd4Ga5S12 (A = K, Rb, Cs)

    Chemistry of Materials · 2012-08-18

    Hua Lin, Liujiang Zhou, Ling Chen

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  3. Molecular Germanium Selenophosphate Salts: Phase-Change Properties and Strong Second Harmonic Generation

    Journal of the American Chemical Society · 2012-11-16

    Collin D. Morris, In Jae Chung, Sungoh Park, Connor M. Harrison, Daniel J. Clark, Joon Ik Jang, Mercouri G. Kanatzidis

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  4. ChemInform Abstract: BaGa2GeX6 (X: S, Se): New mid‐IR Nonlinear Optical Crystals with Large Band Gaps.

    ChemInform · 2012-12-18

    Xinsong Lin, Yifeng Guo, Ning Ye

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  5. Na2Cd7B8O20: a new noncentrosymmetric compound with special [B3O7] units

    CrystEngComm · 2013-01-01

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  6. Synthesis, structure, optical property, and electronic structure of Ba7AgGa5Se15

    Journal of Alloys and Compounds · 2013-03-14

    Wenlong Yin, Ran He, Kai Feng, Wenyu Hao, Jiyong Yao, Yicheng Wu

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  7. Syntheses, Structures, and Nonlinear Optical Properties of Quaternary Chalcogenides: Pb4Ga4GeQ12 (Q = S, Se)

    Inorganic Chemistry · 2013-07-12

    Yu‐Kun Chen, Mei‐Chun Chen, Liujiang Zhou, Ling Chen, Li‐Ming Wu

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  8. Functionalization Based on the Substitutional Flexibility: Strong Middle IR Nonlinear Optical Selenides AXII4XIII5Se12

    Journal of the American Chemical Society · 2013-07-31

    Hua Lin, Ling Chen, Liujiang Zhou, Li‐Ming Wu

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  9. Metal Chalcogenides: A Rich Source of Nonlinear Optical Materials

    Chemistry of Materials · 2013-08-09

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  10. Ba8Sn4S15: A Strong Second Harmonic Generation Sulfide with Zero-Dimensional Crystal Structure

    Chemistry of Materials · 2013-12-17

    Zhong‐Zhen Luo, Chensheng Lin, Weilong Zhang, Hao Zhang, Zhangzhen He, Wen‐Dan Cheng

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  11. Synthesis, Structure and Bonding, Optical Properties of Ba4MTrQ6 (M=Cu, Ag; Tr=Ga, In; Q=S, Se)

    Chemistry - An Asian Journal · 2014-02-12

    Xiao‐Wu Lei, Min Yang, Sheng‐Qing Xia, Xiao‐Cun Liu, Mingyan Pan, Xin Li, Xu‐Tang Tao

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  12. Ag 3 Ga 3 SiSe 8 : a new infrared nonlinear optical material with a chalcopyrite structure

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    Dajiang Mei, Pifu Gong, Zheshuai Lin, Kai Feng, Jiyong Yao, Fuqiang Huang, Yicheng Wu

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  13. Synthesis and characterization of ternary glasses in the system Na2Se-Ga2Se3-GeSe2

    Journal of Non-Crystalline Solids · 2014-08-15

    Alvin W. Mao, Steven Currie, Bruce G. Aitken, Sabyasachi Sen

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  14. 1-[4-(methylsulfanyl) phenyl]-3-(4-nitropshenyl) prop-2-en-1-one: A reverse saturable absorption based optical limiter

    Materials Chemistry and Physics · 2014-11-16

    S. Raghavendra, Chandraju Sadolalu Chidan Kumar, A. Jayarama, S.M. Dharmaprakash

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  15. Syntheses, Structures, and Nonlinear-Optical Properties of Metal Sulfides Ba2Ga8MS16 (M = Si, Ge)

    Inorganic Chemistry · 2014-11-20

    Bin‐Wen Liu, Hui‐Yi Zeng, Ming‐Jian Zhang, Yuhang Fan, Guo‐Cong Guo, Jin‐Shun Huang, Zhen‐Chao Dong

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  16. Designing the syntheses and photophysical simulations of noncentrosymmetric compounds

    Inorganic Chemistry Frontiers · 2014-12-01

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  17. Infrared nonlinear optical properties of lithium-containing diamond-like semiconductors Li 2 ZnGeSe 4 and Li 2 ZnSnSe 4

    Dalton Transactions · 2015-01-01

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  18. SnGa 2 GeS 6 : synthesis, structure, linear and nonlinear optical properties

    Dalton Transactions · 2015-01-01

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  19. Second Harmonic Generation Response Optimized at Various Optical Wavelength Ranges through a Series of Cubic Chalcogenides Ba6Ag2.67+4δSn4.33−δS16–xSex

    Chemistry of Materials · 2015-01-30

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  20. Phase-Change Behavior and Nonlinear Optical Second and Third Harmonic Generation of the One-Dimensional K(1–x)CsxPSe6 and Metastable β-CsPSe6

    Chemistry of Materials · 2015-02-12

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  21. Syntheses, crystal structures, and NLO properties of the quaternary sulfides RE3Sb0.33SiS7 (RE=La, Pr)

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  22. Synthesis, crystal structure and optical property of a novel metal chalcohalide: ZnHg3Se2Cl4

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  23. Structure and properties of off-stoichiometric Ba–Ga–Ge selenide glasses

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  24. BaCdSnS 4 and Ba 3 CdSn 2 S 8 : syntheses, structures, and non-linear optical and photoluminescence properties

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  25. Quaternary BaGa2GeS6 and BaGa2GeSе6 Nonlinear Crystals for the Mid-IR Spectral Range

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  26. Ba4Ga2Se8: A ternary selenide containing chains and discrete Se22− units

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  27. Syntheses and structural characterization of non-centrosymmetric Na2M2M'S6 (M, M′=Ga, In, Si, Ge, Sn, Zn, Cd) sulfides

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  28. Hydrazine-hydrothermal syntheses, characterizations and photoelectrochemical properties of two quaternary chalcogenidoantimonates(III) BaCuSbQ3 (Q = S, Se)

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  29. Na 2 ZnGe 2 S 6 : A New Infrared Nonlinear Optical Material with Good Balance between Large Second-Harmonic Generation Response and High Laser Damage Threshold

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  30. Noncentrosymmetric selenide Ba4Ga4GeSe12: Synthesis, structure, and optical properties

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  31. Crystal growth and characterization of new quaternary chalcogenide nonlinear crystals for the mid-IR: BaGa_2GeS_6 and BaGa_2GeSe_6

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  32. Recent studies of nonlinear chalcogenide crystals for the mid-IR

    Semiconductor Science and Technology · 2016-10-26

    L. I. Isaenko, Alexander Yèlisseyev

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  33. A new quaternary semiconductor compound (Ba2Sb4GeS10): Ab initio study

    The Philosophical Magazine A Journal of Theoretical Experimental and Applied Physics · 2016-12-22

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  34. Centrosymmetric to noncentrosymmetric structural transformation of new quaternary selenides induced by isolated dimeric [Sn 2 Se 4 ] units: from Ba 8 Ga 2 Sn 7 Se 18 to Ba 10 Ga 2 Sn 9 Se 22

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  35. Tailored synthesis of nonlinear optical quaternary chalcohalides: Ba 4 Ge 3 S 9 Cl 2 , Ba 4 Si 3 Se 9 Cl 2 and Ba 4 Ge 3 Se 9 Cl 2

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  36. Second harmonic generation response of the cubic chalcogenides Ba(6−x)Srx[Ag(4−y)Sn(y/4)](SnS4)4

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  37. Noncentrosymmetric chalcogenides BaZnSiSe4 and BaZnGeSe4 featuring one-dimensional structures

    Journal of Alloys and Compounds · 2017-03-05

    Wenlong Yin, Abishek K. Iyer, Chao Li, Jiyong Yao, Arthur Mar

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  38. Discovery-Synthesis, Design, and Prediction of Chalcogenide Phases

    Inorganic Chemistry · 2017-03-09

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  39. Mid-Infrared Nonlinear Optical Materials Based on Metal Chalcogenides: Structure–Property Relationship

    Crystal Growth & Design · 2017-03-15

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  40. Numerical analysis of СО laser frequency conversion efficiency in BaGa 2 GeSe 6 crystal

    Laser Physics · 2018-02-01

    А. А. Ионин, I. O. Kinyaevskiy, V. A. Mozhaeva

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  41. Phase-matching properties of BaGa2GeSe6 for three-wave interactions in the 0778–105910 μm spectral range

    Applied Optics · 2018-08-30

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  42. Synthesis, crystal structures and nonlinear optical properties of polymorphism: α- and β-RbHgI3·H2O

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  43. A review on structure-performance relationship toward the optimal design of infrared nonlinear optical materials with balanced performances

    Coordination Chemistry Reviews · 2018-09-20

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  44. BaB2S4: An Efficient and Air-Stable Thioborate as Infrared Nonlinear Optical Material with High Laser Damage Threshold

    Chemistry of Materials · 2018-10-16

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  45. Recent progress on new infrared nonlinear optical materials with application prospect

    Journal of Solid State Chemistry · 2018-12-20

    Xiaoyu Luo, Zhuang Li, Yangwu Guo, Jiyong Yao, Yicheng Wu

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  46. Li 2 ZnGeS 4 : a promising diamond-like infrared nonlinear optical material with high laser damage threshold and outstanding second-harmonic generation response

    Dalton Transactions · 2019-01-01

    Yi Huang, Kui Wu, Jianian Cheng, Yu Chu, Zhihua Yang, Shilie Pan

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  47. Theoretical investigation on the promotion of second harmonic generation from chalcopyrite family A I GaS 2 to A II Ga 2 S 4

    RSC Advances · 2019-01-01

    Alimujiang Yalikun, Ming‐Hsien Lee, Mamatrishat Mamat

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  48. Sum frequency conversion of multiline CO laser emission in BaGa2GeSe6 crystal of one cm long

    Journal of Physics Conference Series · 2019-03-01

    Dmitrii V. Badikov, Valeriy V. Badikov, А. А. Ионин, I. O. Kinyaevskiy, Yu. M. Klimachëv, А. А. Котков, V. A. Mozhaeva, Adilya M. Sagitova

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  49. The exploration of new infrared nonlinear optical crystals

    Chinese Science Bulletin (Chinese Version) · 2019-03-01

    Huimin Zhou, Li‐Ming Wu

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  50. Effect of S and Se replacement on electronic and thermoelectric features of BaCu2GeQ4 (Q = S, Se) chalcogenide crystals

    Journal of Alloys and Compounds · 2019-03-19

    Sikander Azam, Muhammad Irfan, Zeesham Abbas, Saleem Ayaz Khan, Ivan V. Kityk, Tanzila Kanwal, M. Sohail, Shabbir Muhammad, Abdullah Godran Al-Sehemi

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