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RESEARCH PAPER · Semiconductor Science and Technology · 2016

Recent studies of nonlinear chalcogenide crystals for the mid-IR

L. I. Isaenko, Alexander Yèlisseyev

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Recent studies of nonlinear chalcogenide crystals for the mid-IROriginalElectronic structure and optical properties of noncentrosymmetric LiGaSe 2 : Experimental measurements and DFT band structure calculations36First-principles study lone-pair effects of Sb (III)-S chromophore influence on SHG response in quaternary potassium containing silver antimony sulfides12Mid-Infrared Nonlinear Optical Materials Based on Metal Chalcogenides: Structure–Property Relationship338Growth, Properties, and Theoretical Analysis of M2LiVO4 (M = Rb, Cs) Crystals: Two Potential Mid-Infrared Nonlinear Optical Materials36LiGaTe2 (LGT) nonlinear crystal: Synthesis and crystal growth processes exploration10Negative thermal expansion and electronic structure variation of chalcopyrite type LiGaTe 249Optimized oriented seed growth and optical properties of high-quality LiInSe 2 crystals13Research progress of mid-and far-infrared nonlinear optical crystals10Ultrasensitive photodetectors based on a high-quality LiInSe 2 single crystal11PbGa2GeS6 crystal as a novel nonlinear optical material: Band structure aspects36Electronic structure and optical properties of LiGa0.5In0.5Se2 single crystal, a nonlinear optical mid-IR material12Laser detection of explosives based on differential absorption and scattering17Prediction and Characterization of NaGaS2, A High Thermal Conductivity Mid-Infrared Nonlinear Optical Material for High-Power Laser Frequency Conversion38A review on the development of infrared nonlinear optical materials with triangular anionic groups38Recherche et élaboration de nouveaux matériaux pour les applications laser non-linéaires du moyen infrarouge0ZnGa2Se4, a nonlinear material with wide mid infrared transparency and good thermomechanical properties4MnSiP2: A New Mid-IR Ternary Phosphide with Strong SHG Effect and Ultrabroad Transparency Range66Hierarchy in nonlinear optical responses induced by metal cation tailoring effect in the In-containing chalcogenide compounds4Dislocations that Decrease Size Mismatch within the Lattice Leading to Ultrawide Band Gap, Large Second‐Order Susceptibility, and High Nonlinear Optical Performance of AgGaS229Dislocations that Decrease Size Mismatch within the Lattice Leading to Ultrawide Band Gap, Large Second‐Order Susceptibility, and High Nonlinear Optical Performance of AgGaS2186Lattice Dynamics and Electronic Properties of a BaGa2GeS6 Nonlinear Crystal: Raman Scattering, IR Reflection, and ab initio Calculations6LiBa2MIIIQ4 (MIII = Al, Ga, In; Q = S, Se): A Series of Metal Chalcogenides with a Structural Transition12Rb4Li2TiOGe4O12: A Titanyl Nonlinear Optical Material with the Widest Transparency Range68Rb4Li2TiOGe4O12: A Titanyl Nonlinear Optical Material with the Widest Transparency Range29Designing excellent mid-infrared nonlinear optical materials with fluorooxo-functional group of d0 transition metal oxyfluorides64ВПЛИВ РОЗМІРІВ ЗЕРЕН КРИСТАЛІЧНОГО ПОРОШКУ НА ІНТЕНСИВНІСТЬ ГЕНЕРАЦІЇ ДРУГОЇ ГАРМОНІКИ0Matériaux chalcogénures innovants pour l’optique non linéaire intégrée dans le moyen infra rouge0Parametric upconversion imaging and its applications127Li2K4TiOGe4O12: A Stable Mid-Infrared Nonlinear Optical Material69Ba 6 In 6 Zn 4 Se 19 : a high performance infrared nonlinear optical crystal with [InSe 3 ] 3− trigonal planar functional motifs22Lead Mixed Oxyhalides Satisfying All Fundamental Requirements for High‐Performance Mid‐Infrared Nonlinear Optical Materials164Lead Mixed Oxyhalides Satisfying All Fundamental Requirements for High‐Performance Mid‐Infrared Nonlinear Optical Materials55Rb21.89W32.66O108: An Excellent Mid- and Far-IR Nonlinear-Optical Material with a Wide Band Gap4Theoretical Study on the Intrinsic Source of the Large Thermal Conductivity of Li-Based Chalcogenide Nonlinear Optical Crystals: From AgGaS2 to LiGaS215Broadened effect of Dy around 3 μm of Yb/Er/Dy: PbF 2 crystal for broadband tunable lasers5A review on phase transition and structure-performance relationship of second-order nonlinear optical polymorphs107Measuring the nonlinear optical properties of indium tin oxide thin film using femtosecond laser pulses64Structure-property survey and computer-assisted screening of mid-infrared nonlinear optical chalcohalides11450-µJ level, 20-picosecond, narrowband difference-frequency generation at 4.6, 5.4, 7.5, 9.2, and 10.8 µm in LiGaS2 and LiGaSe2 at Nd:YAG laser pumping and various crystalline Raman laser seedings19Ba2[MoO3(OH)(IO3)2]IO3: A Promising SHG Material Featuring a Λ-Shaped Functional Motif Achieved by Universal Mono-Site Substitution50LiGaS2 crystal growth under low temperature gradient conditions by the modified Bridgman method4Finding Optimal Mid-Infrared Nonlinear Optical Materials in Germanates by First-Principles High-Throughput Screening and Experimental Verification79Study of LiInSe2 Single Crystals for the Thermal Neutron Detection4Growth and optical properties of nonlinear optical crystal Rb4Li2TiOGe4O128Study on precipitates in AgGaSe2 single crystal grown by vertical gradient freezing method5A review on the recently developed promising infrared nonlinear optical materials103Review of thermal parameters of Li-based nonlinear crystals for high power 8 µm sources1Role of lone-pair electrons in determining the thermal transport behavior of LiAsS 2 : first-principles investigation5Thermophysical properties of lithium thiogallate that are important for optical applications12Optical properties of Li-based nonlinear crystals for high power mid-IR OPCPA pumped at 1 µm under realistic operational conditions12Hybrid high spectral resolution broadband mid-infrared SFG spectrometer development and demonstration4Li 4 MgGe 2 S 7 : The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap214Li4MgGe2S7: The First Alkali and Alkaline‐Earth Diamond‐Like Infrared Nonlinear Optical Material with Exceptional Large Band Gap16Hg 3 P 2 S 8 : A New Promising Infrared Nonlinear Optical Material with a Large Second-Harmonic Generation and a High Laser-Induced Damage Threshold111High refractive index (Dy) doped (GeTe)80(InTe)20 thin films for sub-THz and millimeter-wave applications29Structure Tuning, Strong Second Harmonic Generation Response, and High Optical Stability of the Polar Semiconductors Na1–xKxAsQ234Giant Non‐Resonant Infrared Second Order Nonlinearity in γ ‐NaAsSe229Halogen-Ion-Induced Structural Phase Transition Giving a Polymorph of HgBr2 with Balanced Nonlinear Optical Properties8Na+/Ag+ substitution induced birefringence enhancement from AgGaS2 to NaGaS218Mid-infrared photon pair generation in AgGaS217Li-Free ternary sulphide Cs 5 Ga 9 S 16 with excellent nonlinear optical performance similar to classic LiGaS 213Optical and defect properties of mid-IR laser crystal Dy 3+ : PbGa 2 S 4 : a DFT and XPS study5Phase matching achieved by isomorphous substitution in IR nonlinear optical material Ba 2 SnSSi 2 O 7 with an undiscovered [SnO 4 S] functional motif47Pd and octahedra do not get along: Square planar [PdS4] units in non-centrosymmetric La6PdSi2S1419Inorganic nonlinear optical materials7Analysis of broadband mid-infrared optical parametric amplification based on LiGaS2, LiGaSe2, LiInS2, and LiInSe2 crystals6Simultaneously Wavelength- and Temperature-Insensitive Mid-Infrared Optical Parametric Amplification with LiGaS2 Crystal1Impact of structure complexity on optoelectronic and non-linear optical properties in quaternary Ag(Pb)–Ga(In)–Si(Ge)–S(Se) systems13Non‐Linear Optical Properties of the (RE)3CuGeS7 Family of Compounds16The Combination of Structure Prediction and Experiment for the Exploration of Alkali‐Earth Metal‐Contained Chalcopyrite‐Like IR Nonlinear Optical Material105Second-Harmonic Generation-Positive Na 2 Ga 2 SiS 6 with a Broad Band Gap and a High Laser Damage Threshold14Ba2MAsQ5 (Q = S and Se) Family of Polar Structures with Large Second Harmonic Generation and Phase Matchability23NaBaBS3: A Promising Infrared Functional Material with Large Birefringence Induced by π-Conjugated [BS3] Units32Crystal Growth and Chirality - Technologies and Applications12Design of Infrared Nonlinear Optical Compounds with Diamond-like Structures and Balanced Optical Performance9The Coming Age of Pnictide and Chalcogenide Ternary Crystals in the Terahertz Frequency Regime12Ultrashort near-infrared pulse generation by non-collinear optical parametric amplification in LiInS22Transparent Lead‐Free Ferroelectric (K, Na)NbO3 Single Crystal with Giant Second Harmonic Generation and Wide Mid‐Infrared Transparency Window21Ternary AGa5S8 (A = K, Rb, Cs): Promising infrared nonlinear optical materials rationally realized by “one-for-multiple substitution” strategy37Growth and Characterization of a Nonlinear Optical Crystal Cd3Te2WO10 Decorated by WO4 Tetrahedra Showing a Large Band Gap9Li x Ag 1– x GaSe 2 : Interplay Between Lithium and Silver in Mid‐Infrared Nonlinear Optical Chalcogenides33LiAlS2: A promising infrared frequency-conversion material with ultrawide band gap and high laser-induced damage threshold19Nonlinear Optical Properties of Zinc Oxide Nanoparticle Colloids Prepared by Pulsed Laser Ablation in Distilled Water22Recent Advances in Infrared Nonlinear Optical Crystal7Fourth-generation solar cells: a review126Recent advances in F-containing iodate nonlinear optical materials6Synthesis of chiral high-entropy sulfides for non-linear optical applications13近红外激光泵浦的可调谐中红外固体激光器研究进展（特邀）3Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates51Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates7Antireflection microstructures fabricated on the surface of a LiGaSe2 nonlinear crystal12Machine Learning Regression Model for Predicting the Formation Energy of Nonlinear Optical Crystals5Unbiased Screening of Novel Infrared Nonlinear Optical Materials with High Thermal Conductivity: Long‐neglected Nitrides and Popular Chalcogenides12Unbiased Screening of Novel Infrared Nonlinear Optical Materials with High Thermal Conductivity: Long‐neglected Nitrides and Popular Chalcogenides48Theoretical Prediction‐Assisted Synthesis and Characterization of Infrared Nonlinear Optical Material NaSrBS324[Ba4(S2)][ZnGa4S10]: Design of an Unprecedented Infrared Nonlinear Salt‐Inclusion Chalcogenide with Disulfide‐Bonds36Zn 2 HgP 2 S 8 : A Wide Bandgap Hg‐Based Infrared Nonlinear Optical Material with Large Second‐Harmonic Generation Response75BaCu2SiS4: A New Member of the AIIBI2MIVQ4 Chalcogenide Family with a Chiral Crystal Structure6Theoretical investigations on ternary defective diamond-like infrared nonlinear optical materials in Be-Ga-Se system18A Machine Learning Study on High Thermal Conductivity Assisted to Discover Chalcogenides with Balanced Infrared Nonlinear Optical Performance59Robust Type‐II Band Alignment and Stacking‐Controlling Second Harmonic Generation in GaN/ZnO vdW Heterostructure17Cascade picosecond optical parametric amplification for generating radiation in the 2.1 μ m0“Three‐in‐One”: A New Hg‐Based Selenide Hg 7 P 2 Se 12 Exhibiting Wide Infrared Transparency Range and Strong Nonlinear Optical Effect80Novel cesium cerium( iv ) iodate Cs 2 Ce(IO 3 ) 6 : hydrothermal synthesis, crystal structures and thermal stability2Barium Chalcogenide Crystals: A Review27Evaluation and prospect of Mid-Infrared nonlinear optical materials in f0 rare earth (RE = Sc, Y, La) chalcogenides45Tunable Optical Parametric Oscillator Based on MgO:PPLN and HgGa2S4 Crystals Pumped by an Nd:YAG Laser with Increased Energy Characteristics0Advances in the development of few-cycle gigawatt-peak-power mid-IR optical parametric amplifiers pumped by Cr:Forsterite laser using non-oxide nonlinear crystals8Ag 2 GeS 3 : A Diamond‐Like Chalcogenide as an IR Nonlinear Optical Material with Outstanding Second‐Harmonic Generation Response28Enhanced third-order nonlinear optical properties of ZnO@C-N composite microspheres10Lattice Dynamics and Thermoelectric Properties of 2D LiAlTe2, LiGaTe2, and LiInTe2 Monolayers4K2HgGe3Se8: A Quaternary Hg-Based Selenide with Nonlinear Optical Properties6Extending mid-infrared wavelength to 6.84 μm in oxide nonlinear optical crystal via birefringence dispersion management4Synthesis of ZnGa2Se4 by the Reaction of GaI3 and ZnI2 with Selenium0Enhanced Anisotropic Second Harmonic Generation in Type-II van der Waals Heterostructures of g-C3N4/BiVO40Balanced IR Nonlinear Optical Performance Achieved by Cation–Anion Module Cosubstitution in V-Based Salt-Inclusion Oxychalcogenides22Computer‐Aided Development of New Nonlinear Optical Materials38Computer‐Aided Development of New Nonlinear Optical Materials14Prospects of using novel nonlinear crystals in SU(1,1) interferometry4A wide band gap selenohalide Cs 9 Si 8 Se 20 Cl with unprecedented [CsSe 7 Cl] mixed anionic units2Alkali triel chalcogenide nanocrystals: a molecular reactivity approach to ternary phase selectivity2Numerical simulation and modified Bridgman growth of high-quality and large-sized LiGaS 2 mid-infrared optical crystals1Structural, Vibrational and Elastic Properties of Lims2 (M = B, Al, Ga, in, Tl) Chalcopyrite-Type Crystals0新型非线性光学晶体和双折射晶体的研究进展（特邀）4Prediction and Evaluation of Li 2 ZnS 2 Crystals as Mid‐Infrared Nonlinear Optical Material with High Thermal Conductivity7Synergically Assembling Advantageous Groups toward High‐Performance Infrared Nonlinear Optical Materials A II CdSiSe 4 (A II = Sr, Ba)41Synergistic Machine Learning Guided Discovery of ABa 3 (BSe 3 ) 2 X (A = Rb, Cs; X = Cl, Br, I): A Promising Family as Property‐Balanced IR Functional Materials10Parametric Down-Conversion of Near-IR Laser Radiation into the Mid-IR Range Using Nonlinear LiGaSe2 and LiGaS2 Crystals with Antireflection Microstructures1Dimensional Reduction Guides Electronic Structure Evolution in the A n Cu 4– n SnS 4 Semiconductor Series9Investigation of optical parametric amplification properties of B2GGS crystals under Type-I phase-matching0First-principles study of properties of hypothetical chalcopyrite-structured disulfides0Tuning birefringence in alkaline-earth metal oxyhalides through diverse mixed-cation coordination architectures1ABCQ4型硫属化物红外非线性光学材料的构效关系（特邀）0Laser-induced damage threshold comparison of untreated, antireflection-coated and antireflection-microstructured LiGaS 2 nonlinear crystals1Optimized seeded-Bridgman growth and characterization of LiGaS 2 crystals0Polyhedral replacement-guided design of Ce3MnGaSe7 featuring strong second-harmonic genera-tion and high laser-induced damage threshold0中红外上转换多维成像技术研究进展（特邀）0高性能硫属化物红外非线性光学材料构效关系（特邀）0Harnessing tetrahedral diversity: The path to superior diamond-like IR NLO crystals15The Effects of Anions on the Structural and Nonlinear Optical Properties in Mixed LiGa x In 1– x C 2 (C = S, Se, Te) Compounds0Effects of gamma ray irradiation on the structural, linear and nonlinear optical properties of perovskite structure0From Centrosymmetric Mg 2 GeS 4 to Noncentrosymmetric CdMg 3 Ge 2 S 8 : Cation-Mixing-Driven Symmetry Reduction4Femtosecond laser fabrication of antireflection microstructures on LiInS 2 and LiInSe 2 nonlinear crystals0Synthesis and Characterization of RE 3 LiSiSe 7 (RE = La–Nd, Sm, Gd, and Tb) Exhibiting Enhanced Nonlinear Optical (NLO) Properties0Photodarkening in crystalline BaGa4Se70Solution-Grown Cs2HgI4 Bulk Crystals: Achieving Strong SHG and High Damage Threshold Synergistically for IR Nonlinear Optics1KCuBi4S7: An Expanded Bi2S3 Structure Type with a Narrow Band Gap and Ultralow Thermal Conductivity0AlGaS3: a wide band gap ternary diamond-like infrared nonlinear optical material with high laser-induced damage threshold1

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  4. Growth, Properties, and Theoretical Analysis of M2LiVO4 (M = Rb, Cs) Crystals: Two Potential Mid-Infrared Nonlinear Optical Materials

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  5. LiGaTe2 (LGT) nonlinear crystal: Synthesis and crystal growth processes exploration

    Materials Science in Semiconductor Processing · 2017-09-28

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  6. Negative thermal expansion and electronic structure variation of chalcopyrite type LiGaTe 2

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  7. Optimized oriented seed growth and optical properties of high-quality LiInSe 2 crystals

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  10. PbGa2GeS6 crystal as a novel nonlinear optical material: Band structure aspects

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  11. Electronic structure and optical properties of LiGa0.5In0.5Se2 single crystal, a nonlinear optical mid-IR material

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  19. Dislocations that Decrease Size Mismatch within the Lattice Leading to Ultrawide Band Gap, Large Second‐Order Susceptibility, and High Nonlinear Optical Performance of AgGaS2

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  25. Designing excellent mid-infrared nonlinear optical materials with fluorooxo-functional group of d0 transition metal oxyfluorides

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  31. Lead Mixed Oxyhalides Satisfying All Fundamental Requirements for High‐Performance Mid‐Infrared Nonlinear Optical Materials

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  32. Lead Mixed Oxyhalides Satisfying All Fundamental Requirements for High‐Performance Mid‐Infrared Nonlinear Optical Materials

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  33. Rb21.89W32.66O108: An Excellent Mid- and Far-IR Nonlinear-Optical Material with a Wide Band Gap

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  34. Theoretical Study on the Intrinsic Source of the Large Thermal Conductivity of Li-Based Chalcogenide Nonlinear Optical Crystals: From AgGaS2 to LiGaS2

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  35. Broadened effect of Dy around 3 μm of Yb/Er/Dy: PbF 2 crystal for broadband tunable lasers

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  36. A review on phase transition and structure-performance relationship of second-order nonlinear optical polymorphs

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  37. Measuring the nonlinear optical properties of indium tin oxide thin film using femtosecond laser pulses

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  38. Structure-property survey and computer-assisted screening of mid-infrared nonlinear optical chalcohalides

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  39. 50-µJ level, 20-picosecond, narrowband difference-frequency generation at 4.6, 5.4, 7.5, 9.2, and 10.8 µm in LiGaS2 and LiGaSe2 at Nd:YAG laser pumping and various crystalline Raman laser seedings

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  40. Ba2[MoO3(OH)(IO3)2]IO3: A Promising SHG Material Featuring a Λ-Shaped Functional Motif Achieved by Universal Mono-Site Substitution

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  41. LiGaS2 crystal growth under low temperature gradient conditions by the modified Bridgman method

    Materials Science and Engineering B · 2020-08-27

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  42. Finding Optimal Mid-Infrared Nonlinear Optical Materials in Germanates by First-Principles High-Throughput Screening and Experimental Verification

    ACS Applied Materials & Interfaces · 2020-09-14

    Jin Yu, Bingbing Zhang, Xiaodong Zhang, Ying Wang, Kui Wu, Ming‐Hsien Lee

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  43. Study of LiInSe2 Single Crystals for the Thermal Neutron Detection

    Journal of Surface Investigation X-ray Synchrotron and Neutron Techniques · 2020-10-01

    Α. V. Belushkin, A.A. Bogdzel, Alina A. Goloshumova, L. I. Isaenko, Sergey I. Lobanov, V. M. Milkov, Alexandra Yu. Tarasova, Alexander Yèlisseyev

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  44. Growth and optical properties of nonlinear optical crystal Rb4Li2TiOGe4O12

    Journal of Crystal Growth · 2020-11-21

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  45. Study on precipitates in AgGaSe2 single crystal grown by vertical gradient freezing method

    Materials Research Express · 2020-11-25

    Denghui Yang, Xin-Ling Cao, Ling Yang, Yong-Ling Zhou

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  46. A review on the recently developed promising infrared nonlinear optical materials

    Dalton Transactions · 2021-01-01

    Ailijiang Abudurusuli, Junjie Li, Shilie Pan

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  47. Review of thermal parameters of Li-based nonlinear crystals for high power 8 µm sources

    Conference on Lasers and Electro-Optics · 2021-01-01

    Mahesh Namboodiri, Torsten Golz, Jan Heye Buß, Michael Schulz, Robert Riedel, Tim Laarmann, Mark J. Prandolini

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  48. Role of lone-pair electrons in determining the thermal transport behavior of LiAsS 2 : first-principles investigation

    CrystEngComm · 2021-01-01

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  49. Thermophysical properties of lithium thiogallate that are important for optical applications

    RSC Advances · 2021-01-01

    Alexey Kurus, Alexander Yèlisseyev, Sergei I. Lobanov, Pavel E. Plyusnin, Мaxim S. Моlokeev, Leonid A. Solovyev, Dmitry A. Samoshkin, С. В. Станкус, S. V. Mel’nikova, Lyudmila I. Isaenko

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  50. Optical properties of Li-based nonlinear crystals for high power mid-IR OPCPA pumped at 1 µm under realistic operational conditions

    Optical Materials Express · 2021-01-05

    M.N. Namboodiri, Cheng Luo, Gregor Indorf, Torsten Golz, Ivanka Grguraš, Jan Heye Buß, Michael Schulz, Robert Riedel, Mark J. Prandolini, Tim Laarmann

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