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RESEARCH PAPER · Advanced Functional Materials · 2018

MgSiAs: An Unexplored System with Promising Nonlinear Optical Properties

Katherine E. Woo, Jian Wang, Kui Wu, Kathleen Lee, Juli‐Anna Dolyniuk, Shilie Pan, Kirill A. Kovnir

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MgSiAs: An Unexplored System with Promising Nonlinear Optical PropertiesOriginalSynthesis of Saucer Shaped Manganese Oxide Nanoparticles by Co-precipitation Method and the Application as Fuel Additive53Crystal and Electronic Structure and Optical Properties of AE2SiP4 (AE = Sr, Eu, Ba) and Ba4Si3P823First-principles study of intrinsic point defects in MgSiAs 23Pb4B6O13: A Polar Lead Oxyborate with Uncommon ∞(B6O12)6– Layers Exhibiting a Large Second Harmonic Generation Response15The role of cobalt doping on the optical and structural properties of Mn3O4 nanostructured thin films obtained by SILAR technique25New compounds Mg3IV6V8 (IV=Si, Ge, Sn; V=P, As, Sb) and their potential application to photovoltaic materials3MnSiP2: A New Mid-IR Ternary Phosphide with Strong SHG Effect and Ultrabroad Transparency Range66Ba2Si3P6: 1D Nonlinear Optical Material with Thermal Barrier Chains99Chemical Flexibility of Mg in Pnictide Materials: Structure and Properties Diversity27From NaZn4Sb3 to HT-Na1–xZn4–ySb3: Panoramic Hydride Synthesis, Structural Diversity, and Thermoelectric Properties28Li[LiCs2Cl][Ga3S6]: A Nanoporous Framework of GaS4 Tetrahedra with Excellent Nonlinear Optical Performance172Li[LiCs2Cl][Ga3S6]: A Nanoporous Framework of GaS4 Tetrahedra with Excellent Nonlinear Optical Performance40BaGe 2 Pn 2 (Pn = P, As): Two Congruent-Melting Non-chalcopyrite Pnictides as Mid- and Far-Infrared Nonlinear Optical Materials Exhibiting Large Second Harmonic Generation Effects54Chemically driven superstructural ordering leading to giant unit cells in unconventional clathrates Cs 8 Zn 18 Sb 28 and Cs 8 Cd 18 Sb 2818LiSi 3 As 6 and Li 2 SiAs 2 with flexible SiAs 2 polyanions: synthesis, structure, bonding, and ionic conductivity9Flux Growth of Phosphide and Arsenide Crystals40Dilute magnetism in Co-doped spinel Mg3Si6As81Anionic Aliovalent Substitution from Structure Models of ZnS: Novel Defect Diamond‐like Halopnictide Infrared Nonlinear Optical Materials with Wide Band Gaps and Large SHG Effects78Anionic Aliovalent Substitution from Structure Models of ZnS: Novel Defect Diamond‐like Halopnictide Infrared Nonlinear Optical Materials with Wide Band Gaps and Large SHG Effects19Sn2B5O9Br as an Outstanding Bifunctional Material with Strong Second‐Harmonic Generation Effect and Large Birefringence84Synthesis, Crystal and Electronic Structure of La2SiP414Improving sensitivity and resolution in solid-state nuclear magnetic resonance0Synthesis-enabled exploration of chiral and polar multivalent quaternary sulfides37Third time's the charm: intricate non-centrosymmetric polymorphism in Ln SiP 3 ( Ln = La and Ce) induced by distortions of phosphorus square layers26New Noncentrosymmetric Tetrel Pnictides Composed of Square‐Planar Gold(I) with Peculiar Bonding13Noncentrosymmetric Tetrel Pnictides RuSi4P4 and IrSi3P3: Nonlinear Optical Materials with Outstanding Laser Damage Threshold47Zintl Compounds7Mg 2 In 3 Si 2 P 7 : A Quaternary Diamond-like Phosphide Infrared Nonlinear Optical Material Derived from ZnGeP 2130A3Te(Zn2Ge)Ge2O14 (A = Sr, Ba, and Pb): New Langasite Mid-infrared Nonlinear Optical Materials by Rational Chemical Substitution32The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks36Add a Pinch of Tetrel: The Transformation of a Centrosymmetric Metal into a Nonsymmorphic and Chiral Semiconductor8Pnictides: An emerging class of infrared nonlinear optical material candidates47Cs2Bi2OSi2O7: A Promising Bismuth Silicate Nonlinear Optical Crystal with Face-Sharing BiO5 Polyhedra Exhibiting Strengthened Second Harmonic Generation Response and Birefringence43Uncovering a Vital Band Gap Mechanism of Pnictides49Additive‐Triggered Polar Polymorph Formation: β‐Sc(IO 3 ) 3 , a Promising Next‐Generation Mid‐Infrared Nonlinear Optical Material42Additive‐Triggered Polar Polymorph Formation: β‐Sc(IO3)3, a Promising Next‐Generation Mid‐Infrared Nonlinear Optical Material3An overview of Mg-based IR nonlinear optical materials22IrSi 3 As 3 : a first transition metal arsenide non-linear optical material10MgSiP2: An Infrared Nonlinear Optical Crystal with a Large Non‐Resonant Phase‐Matchable Second Harmonic Coefficient and High Laser Damage Threshold18“Three‐in‐One”: A New Hg‐Based Selenide Hg 7 P 2 Se 12 Exhibiting Wide Infrared Transparency Range and Strong Nonlinear Optical Effect80Direct Band Gap Semiconductors with Two‐ and Three‐Dimensional Triel‐Phosphide Frameworks (Triel=Al, Ga, In)3FeSi4P4 and CoSi3P3: Hidden Gems of Ternary Tetrel Pnictides with Outstanding Nonlinear Optical Properties11Achieving strong optical nonlinearity and wide bandgap of pnictides via ionic motif–driven directed assembly of covalent groups39Cd5As2Br4: A Ternary Arsenide with Nonlinear Optical Property3Prediction of lanthanide-containing ternary compounds2Bismuth as reactive and non-reactive flux medium for the synthesis and crystal growth of intermetallics9Pnictides: An Overview of Crystal Structures, Properties and Applications5From Centrosymmetric Ca3Ge2O3S4 to Noncentrosymmetric Ca3Ge2O4Se3: A Nonlinear Optical Ca-Based Oxyselenide5Harnessing tetrahedral diversity: The path to superior diamond-like IR NLO crystals13Design of a High-Performance Infrared Nonlinear Optical Crystal via a Multiple Flexible-Group Synergistic Polarization Strategy10The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 115The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 110Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0

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  1. Synthesis of Saucer Shaped Manganese Oxide Nanoparticles by Co-precipitation Method and the Application as Fuel Additive

    Journal of Cluster Science · 2018-07-09

    Saba Jamil, Shanza Rauf Khan, Bushra Sultana, Maria Hashmi, Muhammad Hamza Haroon, Muhammad Ramzan Saeed Ashraf Janjua

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  2. Crystal and Electronic Structure and Optical Properties of AE2SiP4 (AE = Sr, Eu, Ba) and Ba4Si3P8

    Zeitschrift für anorganische und allgemeine Chemie · 2018-11-19

    Justin Mark, Juli‐Anna Dolyniuk, Nhon Tran, Kirill A. Kovnir

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  3. First-principles study of intrinsic point defects in MgSiAs 2

    Physical Chemistry Chemical Physics · 2019-01-01

    Ping Tuo, Bicai Pan

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  4. Pb4B6O13: A Polar Lead Oxyborate with Uncommon ∞(B6O12)6– Layers Exhibiting a Large Second Harmonic Generation Response

    Inorganic Chemistry · 2019-01-14

    Lingyun Dong, Ying Wang, Bingbing Zhang, Zhihua Yang, Xusheng Ge, Kai Liu, Shigang Shen

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  5. The role of cobalt doping on the optical and structural properties of Mn3O4 nanostructured thin films obtained by SILAR technique

    Superlattices and Microstructures · 2019-01-28

    Özkan Bayram, Erdal İgman, Harun Güney, Önder Şimşek

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  6. New compounds Mg3IV6V8 (IV=Si, Ge, Sn; V=P, As, Sb) and their potential application to photovoltaic materials

    Journal of Alloys and Compounds · 2019-02-02

    Ping Tuo, Bicai Pan

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  7. MnSiP2: A New Mid-IR Ternary Phosphide with Strong SHG Effect and Ultrabroad Transparency Range

    Chemistry of Materials · 2019-02-12

    Tongtong Yu, Shanpeng Wang, Xiang Zhang, Chenning Li, Jie Qiao, Ning Jia, Bing Q. Han, Sheng‐Qing Xia, Xutang Tao

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  8. Ba2Si3P6: 1D Nonlinear Optical Material with Thermal Barrier Chains

    Journal of the American Chemical Society · 2019-07-05

    Justin Mark, Jian Wang, Kui Wu, Jeane Gladys Lo, Shannon Lee, Kirill A. Kovnir

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  9. Chemical Flexibility of Mg in Pnictide Materials: Structure and Properties Diversity

    Chemistry of Materials · 2019-09-17

    Jian Wang, Justin Mark, Katherine E. Woo, Jackson Voyles, Kirill A. Kovnir

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  10. From NaZn4Sb3 to HT-Na1–xZn4–ySb3: Panoramic Hydride Synthesis, Structural Diversity, and Thermoelectric Properties

    Chemistry of Materials · 2019-10-03

    Volodymyr Gvozdetskyi, Bryan Owens‐Baird, Sangki Hong, Tori Cox, Gourab Bhaskar, Colin P. Harmer, Yang Sun, Feng Zhang, Cai‐Zhuang Wang, Kai‐Ming Ho, Julia V. Zaikina

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  11. Li[LiCs2Cl][Ga3S6]: A Nanoporous Framework of GaS4 Tetrahedra with Excellent Nonlinear Optical Performance

    Angewandte Chemie International Edition · 2019-10-26

    Bin‐Wen Liu, Xiao‐Ming Jiang, Bingxuan Li, Hui‐Yi Zeng, Guo‐Cong Guo

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  12. Li[LiCs2Cl][Ga3S6]: A Nanoporous Framework of GaS4 Tetrahedra with Excellent Nonlinear Optical Performance

    Angewandte Chemie · 2019-10-26

    Bin‐Wen Liu, Xiao‐Ming Jiang, Bingxuan Li, Hui‐Yi Zeng, Guo‐Cong Guo

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  13. BaGe 2 Pn 2 (Pn = P, As): Two Congruent-Melting Non-chalcopyrite Pnictides as Mid- and Far-Infrared Nonlinear Optical Materials Exhibiting Large Second Harmonic Generation Effects

    Chemistry of Materials · 2019-11-21

    Jindong Chen, Chensheng Lin, Guang Peng, Feng Xu, Min Luo, Shunda Yang, Shuangshuang Shi, Yingshuang Sun, Tao Yan, Bingxuan Li, Ning Ye

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  14. Chemically driven superstructural ordering leading to giant unit cells in unconventional clathrates Cs 8 Zn 18 Sb 28 and Cs 8 Cd 18 Sb 28

    Chemical Science · 2020-01-01

    Bryan Owens‐Baird, Philip Yox, Shannon Lee, Xian B. Carroll, SuYin Grass Wang, Yu‐Sheng Chen, Oleg I. Lebedev, Kirill A. Kovnir

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  15. LiSi 3 As 6 and Li 2 SiAs 2 with flexible SiAs 2 polyanions: synthesis, structure, bonding, and ionic conductivity

    Journal of Materials Chemistry A · 2020-01-01

    Justin Mark, Kathleen Lee, Maxwell A. T. Marple, Shannon Lee, Sabyasachi Sen, Kirill A. Kovnir

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  16. Flux Growth of Phosphide and Arsenide Crystals

    Frontiers in Chemistry · 2020-04-02

    Jian Wang, Philip Yox, Kirill A. Kovnir

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  17. Dilute magnetism in Co-doped spinel Mg3Si6As8

    Journal of Applied Physics · 2020-07-20

    Ping Tuo, Bicai Pan

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  18. Anionic Aliovalent Substitution from Structure Models of ZnS: Novel Defect Diamond‐like Halopnictide Infrared Nonlinear Optical Materials with Wide Band Gaps and Large SHG Effects

    Angewandte Chemie International Edition · 2020-09-04

    Jindong Chen, Chensheng Lin, Dan Zhao, Min Luo, Guang Peng, Bingxuan Li, Shunda Yang, Yingshuang Sun, Ning Ye

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  19. Anionic Aliovalent Substitution from Structure Models of ZnS: Novel Defect Diamond‐like Halopnictide Infrared Nonlinear Optical Materials with Wide Band Gaps and Large SHG Effects

    Angewandte Chemie · 2020-09-04

    Jindong Chen, Chensheng Lin, Dan Zhao, Min Luo, Guang Peng, Bingxuan Li, Shunda Yang, Yingshuang Sun, Ning Ye

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  20. Sn2B5O9Br as an Outstanding Bifunctional Material with Strong Second‐Harmonic Generation Effect and Large Birefringence

    Advanced Optical Materials · 2020-12-16

    Jingyu Guo, Shichao Cheng, Shujuan Han, Zhihua Yang, Shilie Pan

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  21. Synthesis, Crystal and Electronic Structure of La2SiP4

    Zeitschrift für anorganische und allgemeine Chemie · 2020-12-18

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  22. Improving sensitivity and resolution in solid-state nuclear magnetic resonance

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  23. Synthesis-enabled exploration of chiral and polar multivalent quaternary sulfides

    Chemical Science · 2021-01-01

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  24. Third time's the charm: intricate non-centrosymmetric polymorphism in Ln SiP 3 ( Ln = La and Ce) induced by distortions of phosphorus square layers

    Dalton Transactions · 2021-01-01

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  25. New Noncentrosymmetric Tetrel Pnictides Composed of Square‐Planar Gold(I) with Peculiar Bonding

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  26. Noncentrosymmetric Tetrel Pnictides RuSi4P4 and IrSi3P3: Nonlinear Optical Materials with Outstanding Laser Damage Threshold

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  27. Zintl Compounds

    Encyclopedia of Inorganic and Bioinorganic Chemistry · 2021-03-26

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  28. Mg 2 In 3 Si 2 P 7 : A Quaternary Diamond-like Phosphide Infrared Nonlinear Optical Material Derived from ZnGeP 2

    Journal of the American Chemical Society · 2021-07-01

    Jindong Chen, Hongxiang Chen, Feng Xu, Liling Cao, Xiaotian Jiang, Shunda Yang, Yingshuang Sun, Xin Lei Zhao, Chensheng Lin, Ning Ye

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  29. A3Te(Zn2Ge)Ge2O14 (A = Sr, Ba, and Pb): New Langasite Mid-infrared Nonlinear Optical Materials by Rational Chemical Substitution

    Chemistry of Materials · 2021-07-25

    Kaichuang Chen, Chensheng Lin, Shengzi Zhang, Guang Peng, Yu Chen, Dan Zhao, Huixin Fan, Shunda Yang, Xin Wen, Min Luo, Zheshuai Lin, Ning Ye

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  30. The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks

    Chemistry - An Asian Journal · 2021-09-01

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  31. Add a Pinch of Tetrel: The Transformation of a Centrosymmetric Metal into a Nonsymmorphic and Chiral Semiconductor

    Chemistry - A European Journal · 2021-12-09

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  32. Pnictides: An emerging class of infrared nonlinear optical material candidates

    Journal of Alloys and Compounds · 2021-12-22

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  33. Cs2Bi2OSi2O7: A Promising Bismuth Silicate Nonlinear Optical Crystal with Face-Sharing BiO5 Polyhedra Exhibiting Strengthened Second Harmonic Generation Response and Birefringence

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  34. Uncovering a Vital Band Gap Mechanism of Pnictides

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  35. Additive‐Triggered Polar Polymorph Formation: β‐Sc(IO 3 ) 3 , a Promising Next‐Generation Mid‐Infrared Nonlinear Optical Material

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  36. Additive‐Triggered Polar Polymorph Formation: β‐Sc(IO3)3, a Promising Next‐Generation Mid‐Infrared Nonlinear Optical Material

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  37. An overview of Mg-based IR nonlinear optical materials

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  38. IrSi 3 As 3 : a first transition metal arsenide non-linear optical material

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  39. MgSiP2: An Infrared Nonlinear Optical Crystal with a Large Non‐Resonant Phase‐Matchable Second Harmonic Coefficient and High Laser Damage Threshold

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  40. “Three‐in‐One”: A New Hg‐Based Selenide Hg 7 P 2 Se 12 Exhibiting Wide Infrared Transparency Range and Strong Nonlinear Optical Effect

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  41. Direct Band Gap Semiconductors with Two‐ and Three‐Dimensional Triel‐Phosphide Frameworks (Triel=Al, Ga, In)

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  42. FeSi4P4 and CoSi3P3: Hidden Gems of Ternary Tetrel Pnictides with Outstanding Nonlinear Optical Properties

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  43. Achieving strong optical nonlinearity and wide bandgap of pnictides via ionic motif–driven directed assembly of covalent groups

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  44. Cd5As2Br4: A Ternary Arsenide with Nonlinear Optical Property

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  45. Prediction of lanthanide-containing ternary compounds

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  46. Bismuth as reactive and non-reactive flux medium for the synthesis and crystal growth of intermetallics

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  47. Pnictides: An Overview of Crystal Structures, Properties and Applications

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  48. From Centrosymmetric Ca3Ge2O3S4 to Noncentrosymmetric Ca3Ge2O4Se3: A Nonlinear Optical Ca-Based Oxyselenide

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  49. Harnessing tetrahedral diversity: The path to superior diamond-like IR NLO crystals

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  50. Design of a High-Performance Infrared Nonlinear Optical Crystal via a Multiple Flexible-Group Synergistic Polarization Strategy

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