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RESEARCH PAPER · Chemistry of Materials · 2019

MnSiP2: A New Mid-IR Ternary Phosphide with Strong SHG Effect and Ultrabroad Transparency Range

Tongtong Yu, Shanpeng Wang, Xiang Zhang, Chenning Li, Jie Qiao, Ning Jia, Bing Q. Han, Sheng‐Qing Xia, Xutang Tao

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MnSiP2: A New Mid-IR Ternary Phosphide with Strong SHG Effect and Ultrabroad Transparency RangeOriginalBa2Si3P6: 1D Nonlinear Optical Material with Thermal Barrier Chains99LiBa2MIIIQ4 (MIII = Al, Ga, In; Q = S, Se): A Series of Metal Chalcogenides with a Structural Transition12Chemical Flexibility of Mg in Pnictide Materials: Structure and Properties Diversity27Li[LiCs2Cl][Ga3S6]: A Nanoporous Framework of GaS4 Tetrahedra with Excellent Nonlinear Optical Performance172Li[LiCs2Cl][Ga3S6]: A Nanoporous Framework of GaS4 Tetrahedra with Excellent Nonlinear Optical Performance40BaGe 2 Pn 2 (Pn = P, As): Two Congruent-Melting Non-chalcopyrite Pnictides as Mid- and Far-Infrared Nonlinear Optical Materials Exhibiting Large Second Harmonic Generation Effects54Abnormal bandgap enlargement resulted in a promising mid-infrared nonlinear optical material Rb 2 CdBrI 3 with an ultrahigh laser damage threshold10Sr 4 Pb 1.5 Sb 5 O 5 Se 8 : a new mid-infrared nonlinear optical material with a moderate SHG response22(Na0.60Ba0.70)Ga2Se4: An Infrared Nonlinear Optical Crystal Designed using AgGaSe2 as the Template38Flux Growth of Phosphide and Arsenide Crystals40LiBa4Ga5Q12 (Q = S, Se): Noncentrosymmetric Metal Chalcogenides with a Cesium Chloride Topological Structure Displaying a Remarkable Laser Damage Threshold32KInSi1.32Sn0.68Se6: An Infrared Nonlinear Optical Material Containing Three Types of Tetrahedral Units19Crystal chemistry, second-order nonlinear optical, and magnetic properties of Eu8Sn4Se2014[ABa2Cl][Ga4S8] (A = Rb, Cs): Wide-Spectrum Nonlinear Optical Materials Obtained by Polycation-Substitution-Induced Nonlinear Optical (NLO)-Functional Motif Ordering269Inherent laws between tetrahedral arrangement pattern and optical performance in tetrahedron-based mid-infrared nonlinear optical materials130Nanostructured metal phosphides: from controllable synthesis to sustainable catalysis324Synthesis-enabled exploration of chiral and polar multivalent quaternary sulfides37New Noncentrosymmetric Tetrel Pnictides Composed of Square‐Planar Gold(I) with Peculiar Bonding13Noncentrosymmetric Tetrel Pnictides RuSi4P4 and IrSi3P3: Nonlinear Optical Materials with Outstanding Laser Damage Threshold47LaSiP3 and LaSi2P6: Two Excellent Rare‐Earth Pnictides with Strong SHG Responses as Mid‐ and Far‐Infrared Nonlinear Optical Crystals36α-Ca2CdP2 and β-Ca2CdP2: Two Polymorphic Phosphide-Based Infrared Nonlinear Crystals with Distorted NLO-Active Tetrahedral Motifs Realizing Large Second Harmonic Generation Effects and Suitable Band Gaps30Mg 2 In 3 Si 2 P 7 : A Quaternary Diamond-like Phosphide Infrared Nonlinear Optical Material Derived from ZnGeP 2130A3Te(Zn2Ge)Ge2O14 (A = Sr, Ba, and Pb): New Langasite Mid-infrared Nonlinear Optical Materials by Rational Chemical Substitution32Li2MTeO6 (M=Ti, Sn): Mid‐Infrared Nonlinear Optical Crystal with Strong Second Harmonic Generation Response and Wide Transparency Range72Li2MTeO6 (M=Ti, Sn): Mid‐Infrared Nonlinear Optical Crystal with Strong Second Harmonic Generation Response and Wide Transparency Range4The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks36Design of metal silicide nanoparticles in molten salts : electrocatalytic and magnetic properties0Cd7SiAs6, a Nonchalcopyrite Arsenide with a Strong Nonlinear-Optical Response9Add a Pinch of Tetrel: The Transformation of a Centrosymmetric Metal into a Nonsymmorphic and Chiral Semiconductor8Perovskite Quantum Dot‐Ta 2 NiSe 5 Mixed‐Dimensional Van Der Waals Heterostructures for High‐Performance Near‐Infrared Photodetection61Pnictides: An emerging class of infrared nonlinear optical material candidates47A DFT Study for Analyzing Opto-electronic Behavior of ZnCN20Broad transparency and wide band gap achieved in a magnetic infrared nonlinear optical chalcogenide by suppressing d–d transitions41Optimized Bridgman growth and quality improvement of LiInSe2 crystal by annealing in Li2Se vapor atmosphere12Balance of Deep-Ultraviolet Transparency and Large Second Harmonic Generation Response in a Silicate Crystal9Shedding Light on the Structure and Characterization of K2ZnGe2O6: A Phase-Matchable Nonlinear Optical Crystal19The Coming Age of Pnictide and Chalcogenide Ternary Crystals in the Terahertz Frequency Regime12Trade-Off for Better Balanced Nonlinear Optical Performance with Disordered Si in ZnGeP217AIn 3 Si 4 P 9 (A = Ca, Sr): quaternary phosphides with double-helix structures exhibiting high laser-induced damage thresholds19Recent Advances in Infrared Nonlinear Optical Crystal7A new stable polymorph of Li 2 TeMo 3 O 12 with wide mid-infrared transparency and a large Raman response17Atomic structures and carrier dynamics of defects in a ZnGeP2 crystal6Nitrides: a promising class of nonlinear optical material candidates9Cs4Zn5P6S18I2: the Largest Birefringence in Chalcohalide Achieved by Highly Polarizable Nonlinear Optical Functional Motifs21Excellent Nonlinear Optical M[M4Cl][Ga11S20] (M = A/Ba, A = K, Rb) Achieved by Unusual Cationic Substitution Strategy20K4ZnV5O15Cl: A Congruent‐Melting Mid‐Infrared Nonlinear Optical Crystal Combined with Strong Second‐Harmonic Generation and High Laser‐Induced Damage Threshold14“Three‐in‐One”: A New Hg‐Based Selenide Hg 7 P 2 Se 12 Exhibiting Wide Infrared Transparency Range and Strong Nonlinear Optical Effect80Direct Band Gap Semiconductors with Two‐ and Three‐Dimensional Triel‐Phosphide Frameworks (Triel=Al, Ga, In)3Structural strategy for advancing nonlinear optical effects in 1D-[MX 2 ] ∞ chains: internal distortion and atomic types2FeSi4P4 and CoSi3P3: Hidden Gems of Ternary Tetrel Pnictides with Outstanding Nonlinear Optical Properties11Polar-Layer-Driven Reconstruction of a Noncentrosymmetric Vandate Mid-Infrared Nonlinear-Optical Crystal10Achieving strong optical nonlinearity and wide bandgap of pnictides via ionic motif–driven directed assembly of covalent groups39Numerical simulation and modified Bridgman growth of high-quality and large-sized LiGaS 2 mid-infrared optical crystals1First-Principles High-Throughput Screening Combined with Experimental Synthesis to Find Vanadate Nonlinear Optical Material BiCa2VO64In and Out: Shuttling Atoms in Covalent Nanocrystals, from Synthesis in Molten Salts to Water-Splitting Electrocatalysis5Nonlinear Optical Series A(VO2)3(SeO3)2 (A = NH4+, K+, and H3O+) with Large Birefringence Derived from High-Anisotropic VO6 Octahedra and SeO3 Pyramids8Pnictides: An Overview of Crystal Structures, Properties and Applications5Optimized growth and anisotropic physical properties of a promising mid-infrared nonlinear optical crystal Li2TiTeO63Single-Crystal Growth and Characterization of High-Entropy Phosphides ASiP20[Cd 4 P 2 ][I 3 ] and [Cd 2 P][CdCl 3 ]: two Millon's phase phosphides exhibiting wide band gaps and large birefringence0Optimized seeded-Bridgman growth and characterization of LiGaS 2 crystals0Topology-Guided Discovery of BaIn 2 Si 7 P 12 : A Quaternary Diamond-like Framework Phosphide with Giant Second-Harmonic Generation and High Laser-Induced Damage Threshold22Design of a High-Performance Infrared Nonlinear Optical Crystal via a Multiple Flexible-Group Synergistic Polarization Strategy10Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0First‐Principles Investigation of the Structural, Electronic, Optical, Elastic, and Thermal Properties of Defect Diamond‐Like Hg 3 P 2 S 80Beyond the bandgap bottleneck: structure–property design principles for infrared nonlinear optical phosphides0

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  1. Ba2Si3P6: 1D Nonlinear Optical Material with Thermal Barrier Chains

    Journal of the American Chemical Society · 2019-07-05

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  2. LiBa2MIIIQ4 (MIII = Al, Ga, In; Q = S, Se): A Series of Metal Chalcogenides with a Structural Transition

    Inorganic Chemistry · 2019-09-12

    Ailijiang Abudurusuli, Kui Wu, Junjie Li, Alimujiang Yalikun, Zhihua Yang, Shilie Pan

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  3. Chemical Flexibility of Mg in Pnictide Materials: Structure and Properties Diversity

    Chemistry of Materials · 2019-09-17

    Jian Wang, Justin Mark, Katherine E. Woo, Jackson Voyles, Kirill A. Kovnir

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  4. Li[LiCs2Cl][Ga3S6]: A Nanoporous Framework of GaS4 Tetrahedra with Excellent Nonlinear Optical Performance

    Angewandte Chemie International Edition · 2019-10-26

    Bin‐Wen Liu, Xiao‐Ming Jiang, Bingxuan Li, Hui‐Yi Zeng, Guo‐Cong Guo

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  5. Li[LiCs2Cl][Ga3S6]: A Nanoporous Framework of GaS4 Tetrahedra with Excellent Nonlinear Optical Performance

    Angewandte Chemie · 2019-10-26

    Bin‐Wen Liu, Xiao‐Ming Jiang, Bingxuan Li, Hui‐Yi Zeng, Guo‐Cong Guo

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  6. BaGe 2 Pn 2 (Pn = P, As): Two Congruent-Melting Non-chalcopyrite Pnictides as Mid- and Far-Infrared Nonlinear Optical Materials Exhibiting Large Second Harmonic Generation Effects

    Chemistry of Materials · 2019-11-21

    Jindong Chen, Chensheng Lin, Guang Peng, Feng Xu, Min Luo, Shunda Yang, Shuangshuang Shi, Yingshuang Sun, Tao Yan, Bingxuan Li, Ning Ye

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  7. Abnormal bandgap enlargement resulted in a promising mid-infrared nonlinear optical material Rb 2 CdBrI 3 with an ultrahigh laser damage threshold

    Journal of Materials Chemistry C · 2020-01-01

    Qi Wu, Xian Liu, Yeshuang Du, Chunlin Teng, Fei Liang

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  8. Sr 4 Pb 1.5 Sb 5 O 5 Se 8 : a new mid-infrared nonlinear optical material with a moderate SHG response

    CrystEngComm · 2020-01-01

    Yang Wang, Mengjia Luo, Pei Zhao, Xiangli Che, Yunzhen Cao, Fuqiang Huang

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  9. (Na0.60Ba0.70)Ga2Se4: An Infrared Nonlinear Optical Crystal Designed using AgGaSe2 as the Template

    Inorganic Chemistry · 2020-03-03

    Yanan Li, Huaiguo Xue, Sheng‐Ping Guo

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  10. Flux Growth of Phosphide and Arsenide Crystals

    Frontiers in Chemistry · 2020-04-02

    Jian Wang, Philip Yox, Kirill A. Kovnir

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  11. LiBa4Ga5Q12 (Q = S, Se): Noncentrosymmetric Metal Chalcogenides with a Cesium Chloride Topological Structure Displaying a Remarkable Laser Damage Threshold

    Inorganic Chemistry · 2020-04-04

    Ailijiang Abudurusuli, Junjie Li, Tinghao Tong, Zhihua Yang, Shilie Pan

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  12. KInSi1.32Sn0.68Se6: An Infrared Nonlinear Optical Material Containing Three Types of Tetrahedral Units

    Inorganic Chemistry · 2020-04-21

    Xiaohui Li, Yiting Chen, Huaiguo Xue, Sheng‐Ping Guo

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  13. Crystal chemistry, second-order nonlinear optical, and magnetic properties of Eu8Sn4Se20

    Journal of Solid State Chemistry · 2020-05-08

    Sihan Yang, Xiaohui Li, Wen‐Dong Yao, Qian-Ting Xu, Sheng‐Ping Guo

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  14. [ABa2Cl][Ga4S8] (A = Rb, Cs): Wide-Spectrum Nonlinear Optical Materials Obtained by Polycation-Substitution-Induced Nonlinear Optical (NLO)-Functional Motif Ordering

    Journal of the American Chemical Society · 2020-05-29

    Bin‐Wen Liu, Xiao‐Ming Jiang, Hui‐Yi Zeng, Guo‐Cong Guo

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  15. Inherent laws between tetrahedral arrangement pattern and optical performance in tetrahedron-based mid-infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2020-06-29

    Weikang Wang, Dajiang Mei, Fei Liang, Jun Zhao, Yuandong Wu, Zheshuai Lin

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  16. Nanostructured metal phosphides: from controllable synthesis to sustainable catalysis

    Chemical Society Reviews · 2021-01-01

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  17. Synthesis-enabled exploration of chiral and polar multivalent quaternary sulfides

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    Georgiy Akopov, Nethmi W. Hewage, Philip Yox, Gayatri Viswanathan, Shannon Lee, Liam Hulsebosch, Sarah D. Cady, Alexander L. Paterson, Frédéric A. Perras, Wenqian Xu, Kui Wu, Yaroslav Mudryk, Kirill A. Kovnir

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  18. New Noncentrosymmetric Tetrel Pnictides Composed of Square‐Planar Gold(I) with Peculiar Bonding

    Chemistry - A European Journal · 2021-02-02

    Shannon Lee, Juyeon Won, Lin‐Lin Wang, Dapeng Jing, Colin P. Harmer, Justin Mark, Georgiy Akopov, Kirill A. Kovnir

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  19. Noncentrosymmetric Tetrel Pnictides RuSi4P4 and IrSi3P3: Nonlinear Optical Materials with Outstanding Laser Damage Threshold

    Advanced Functional Materials · 2021-02-17

    Shannon Lee, Scott L. Carnahan, Georgiy Akopov, Philip Yox, Linlin Wang, Aaron J. Rossini, Kui Wu, Kirill A. Kovnir

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  20. LaSiP3 and LaSi2P6: Two Excellent Rare‐Earth Pnictides with Strong SHG Responses as Mid‐ and Far‐Infrared Nonlinear Optical Crystals

    Advanced Optical Materials · 2021-03-05

    Yingshuang Sun, Jindong Chen, Shunda Yang, Bingxuan Li, Guoliang Chai, Chensheng Lin, Min Luo, Ning Ye

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  21. α-Ca2CdP2 and β-Ca2CdP2: Two Polymorphic Phosphide-Based Infrared Nonlinear Crystals with Distorted NLO-Active Tetrahedral Motifs Realizing Large Second Harmonic Generation Effects and Suitable Band Gaps

    Inorganic Chemistry · 2021-05-03

    Yingshuang Sun, Chensheng Lin, Jindong Chen, Feng Xu, Shunda Yang, Bingxuan Li, Guangsai Yang, Min Luo, Ning Ye

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  22. Mg 2 In 3 Si 2 P 7 : A Quaternary Diamond-like Phosphide Infrared Nonlinear Optical Material Derived from ZnGeP 2

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  23. A3Te(Zn2Ge)Ge2O14 (A = Sr, Ba, and Pb): New Langasite Mid-infrared Nonlinear Optical Materials by Rational Chemical Substitution

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  24. Li2MTeO6 (M=Ti, Sn): Mid‐Infrared Nonlinear Optical Crystal with Strong Second Harmonic Generation Response and Wide Transparency Range

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  25. Li2MTeO6 (M=Ti, Sn): Mid‐Infrared Nonlinear Optical Crystal with Strong Second Harmonic Generation Response and Wide Transparency Range

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  26. The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks

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  27. Design of metal silicide nanoparticles in molten salts : electrocatalytic and magnetic properties

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  28. Cd7SiAs6, a Nonchalcopyrite Arsenide with a Strong Nonlinear-Optical Response

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  29. Add a Pinch of Tetrel: The Transformation of a Centrosymmetric Metal into a Nonsymmorphic and Chiral Semiconductor

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  30. Perovskite Quantum Dot‐Ta 2 NiSe 5 Mixed‐Dimensional Van Der Waals Heterostructures for High‐Performance Near‐Infrared Photodetection

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  31. Pnictides: An emerging class of infrared nonlinear optical material candidates

    Journal of Alloys and Compounds · 2021-12-22

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  32. A DFT Study for Analyzing Opto-electronic Behavior of ZnCN2

    Lecture notes in electrical engineering · 2022-01-01

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  33. Broad transparency and wide band gap achieved in a magnetic infrared nonlinear optical chalcogenide by suppressing d–d transitions

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  34. Optimized Bridgman growth and quality improvement of LiInSe2 crystal by annealing in Li2Se vapor atmosphere

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  35. Balance of Deep-Ultraviolet Transparency and Large Second Harmonic Generation Response in a Silicate Crystal

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  36. Shedding Light on the Structure and Characterization of K2ZnGe2O6: A Phase-Matchable Nonlinear Optical Crystal

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  37. The Coming Age of Pnictide and Chalcogenide Ternary Crystals in the Terahertz Frequency Regime

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  38. Trade-Off for Better Balanced Nonlinear Optical Performance with Disordered Si in ZnGeP2

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  39. AIn 3 Si 4 P 9 (A = Ca, Sr): quaternary phosphides with double-helix structures exhibiting high laser-induced damage thresholds

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  40. Recent Advances in Infrared Nonlinear Optical Crystal

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  41. A new stable polymorph of Li 2 TeMo 3 O 12 with wide mid-infrared transparency and a large Raman response

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  42. Atomic structures and carrier dynamics of defects in a ZnGeP2 crystal

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  43. Nitrides: a promising class of nonlinear optical material candidates

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  44. Cs4Zn5P6S18I2: the Largest Birefringence in Chalcohalide Achieved by Highly Polarizable Nonlinear Optical Functional Motifs

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  45. Excellent Nonlinear Optical M[M4Cl][Ga11S20] (M = A/Ba, A = K, Rb) Achieved by Unusual Cationic Substitution Strategy

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  46. K4ZnV5O15Cl: A Congruent‐Melting Mid‐Infrared Nonlinear Optical Crystal Combined with Strong Second‐Harmonic Generation and High Laser‐Induced Damage Threshold

    Advanced Optical Materials · 2023-12-12

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  47. “Three‐in‐One”: A New Hg‐Based Selenide Hg 7 P 2 Se 12 Exhibiting Wide Infrared Transparency Range and Strong Nonlinear Optical Effect

    Advanced Functional Materials · 2023-12-28

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  48. Direct Band Gap Semiconductors with Two‐ and Three‐Dimensional Triel‐Phosphide Frameworks (Triel=Al, Ga, In)

    Chemistry - A European Journal · 2023-12-31

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  49. Structural strategy for advancing nonlinear optical effects in 1D-[MX 2 ] ∞ chains: internal distortion and atomic types

    RSC Advances · 2024-01-01

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  50. FeSi4P4 and CoSi3P3: Hidden Gems of Ternary Tetrel Pnictides with Outstanding Nonlinear Optical Properties

    Chemistry of Materials · 2024-09-03

    Ernesto Soto, Shannon Lee, Andrew P. Porter, Gayatri Viswanathan, Georgiy Akopov, Nethmi W. Hewage, Kui Wu, Victor Trinquet, Guillaume Brunin, Geoffroy Hautier, Gian‐Marco Rignanese, Aaron J. Rossini, Kirill A. Kovnir

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