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RESEARCH PAPER · Chemistry of Materials · 2021

A3Te(Zn2Ge)Ge2O14 (A = Sr, Ba, and Pb): New Langasite Mid-infrared Nonlinear Optical Materials by Rational Chemical Substitution

Kaichuang Chen, Chensheng Lin, Shengzi Zhang, Guang Peng, Yu Chen, Dan Zhao, Huixin Fan, Shunda Yang, Xin Wen, Min Luo, Zheshuai Lin, Ning Ye

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A3Te(Zn2Ge)Ge2O14 (A = Sr, Ba, and Pb): New Langasite Mid-infrared Nonlinear Optical Materials by Rational Chemical SubstitutionOriginalRational design of a promising oxychalcogenide infrared nonlinear optical crystal60HgTeO2F(OH): A Nonlinear Optical Oxyfluoride Constructed of Active [TeO2F(OH)]2– Pyramids and V-Shaped [HgO2]2– Groups36Balance of Deep-Ultraviolet Transparency and Large Second Harmonic Generation Response in a Silicate Crystal9Crystallographic Insights into the Crystal Structure and Intrinsic Properties of Ca12Al14O33-Type Rb3LiZn2(MoO4)4Single Crystals1Shedding Light on the Structure and Characterization of K2ZnGe2O6: A Phase-Matchable Nonlinear Optical Crystal19Pb5(GeO4)(Ge2O7) and Pb3.32Ca1.68(GeO4)(Ge2O7): Two Nonlinear Optical Germanates Induced by Diverse PbOx Polyhedra17Synthesis and Complete Characterisation of new Oxide Materials by full and Congruent Crystallisation from Glass or the Molten liquid0Birefringence Dispersion Management of Langasite Nonlinear Crystals for the Improvement of Mid-Infrared Amplification10Achieving broadband ultraviolet to mid-infrared transparency in germanate-based nonlinear optical crystals Cs 3 REGe 3 O 9 (RE = Y, Gd)16The first quaternary rare-earth oxythiogermanate with second-harmonic generation and ferromagnetic behavior26Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates51Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates7Elucidating the structure-nonlinear optical property relationship of Te2O4(OH)26Rational Design of a Niobium Tellurite Crystal Nb2Te3O11 Exhibiting Good Overall Infrared NLO Performance by Structural Genetic Engineering17Flexible Anionic Groups‐Activated Structure Dissymmetry for Strong Nonlinearity in Ln 2 Ae 3 M IV 3 S 12 Family15Not Only Garnets…1Rb 8 Nb 10 Ge 6 O 41 : a new niobium-germanate crystal featuring unique one-dimensional [Nb 7 O 30 ] ∞ chains and wide mid-IR transparency2Centrosymmetric CaBaMF8 and Noncentrosymmetric Li2CaMF8 (M = Zr, Hf): Dimension Variation and Nonlinear Optical Activity Resulting from an Isovalent Cation Substitution-Oriented Design17Pentanary Oxythiogermanates Ba3MGe3O2S8 (M = Ca, Zn) Featuring [Ge3O2S8]8– Trimers and {[MGe3O2S8]6–}∞ Chains: Structural Chemistry and Physical Properties4La3Ga5M0.5Sn0.5O14, (M = Ge, Si): Design and Synthesis of Two Langasite Nonlinear Optical Materials with Large Second Harmonic Generation and Birefringence Induced by Distorted (Sn/M)O6 Octahedra4Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances17A Wide Band Gap Germanate with the Largest Second Harmonic Generation Response Created by Hypoxic Strategy22A Wide Band Gap Germanate with the Largest Second Harmonic Generation Response Created by Hypoxic Strategy5Methyl substitution induced noncentrosymmetric alignment: a new thiazolium-based nonlinear optical crystal of HDT-N1S2Enhancement of optical anisotropy from [BF4] units by ligand substitution0A‐Site Doping Enables Stabilization and Migration of Oxygen Vacancies in Langasite Frameworks1A series of langasite-type compounds: size effect regulation for cation occupation and enhanced SHG response1Design of benzoxazolium-based nonlinear optical crystals with large second-order harmonic generation responses0Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates4Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates0K 3 YGe 3 O 9 : A Rare-Earth Germanate Nonlinear Optical Crystal with a Short Ultraviolet Cutoff Edge and Moderate Second-Harmonic Generation Response1A Telluromolybdate Mid-Infrared Nonlinear Optical Crystal with Wide Transparency and Strong Second-Harmonic Generation Response0

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  1. Rational design of a promising oxychalcogenide infrared nonlinear optical crystal

    Chemical Science · 2022-01-01

    Yansong Cheng, Hongping Wu, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  2. HgTeO2F(OH): A Nonlinear Optical Oxyfluoride Constructed of Active [TeO2F(OH)]2– Pyramids and V-Shaped [HgO2]2– Groups

    Inorganic Chemistry · 2022-01-14

    Ru‐Ling Tang, Mei Yan, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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  3. Balance of Deep-Ultraviolet Transparency and Large Second Harmonic Generation Response in a Silicate Crystal

    Crystal Growth & Design · 2022-04-04

    Zheyao Xiong, Jing Xu, Haotian Tian, Hongyuan Sha, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  4. Crystallographic Insights into the Crystal Structure and Intrinsic Properties of Ca12Al14O33-Type Rb3LiZn2(MoO4)4Single Crystals

    Inorganic Chemistry · 2022-05-23

    Wenli Zhao, Lili Li, Tao Han, Jinmiao Jiao, Yuheng She, Ning Ye, Zhanggui Hu, Yicheng Wu, Conggang Li

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  5. Shedding Light on the Structure and Characterization of K2ZnGe2O6: A Phase-Matchable Nonlinear Optical Crystal

    Inorganic Chemistry · 2022-07-13

    Jinmiao Jiao, Fei Liang, Conggang Li, Tao Han, Wenli Zhao, Yuheng She, Ning Ye, Zhanggui Hu, Yicheng Wu

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  6. Pb5(GeO4)(Ge2O7) and Pb3.32Ca1.68(GeO4)(Ge2O7): Two Nonlinear Optical Germanates Induced by Diverse PbOx Polyhedra

    Inorganic Chemistry · 2022-08-17

    Mei Yan, Ru‐Ling Tang, Gang-Xiang Liu, Lei Huai, Wenlong Liu, Sheng‐Ping Guo

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  7. Synthesis and Complete Characterisation of new Oxide Materials by full and Congruent Crystallisation from Glass or the Molten liquid

    Unknown journal · 2022-11-18

    Haytem Bazzaoui

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  8. Birefringence Dispersion Management of Langasite Nonlinear Crystals for the Improvement of Mid-Infrared Amplification

    Crystal Growth & Design · 2022-12-06

    Yuzhou Wang, Fei Liang, Dazhi Lu, Haohai Yu, Huaijin Zhang

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  9. Achieving broadband ultraviolet to mid-infrared transparency in germanate-based nonlinear optical crystals Cs 3 REGe 3 O 9 (RE = Y, Gd)

    Inorganic Chemistry Frontiers · 2023-01-01

    Jinmiao Jiao, Conggang Li, Yuheng She, Ning Ye, Zhanggui Hu, Yicheng Wu

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  10. The first quaternary rare-earth oxythiogermanate with second-harmonic generation and ferromagnetic behavior

    Chemical Communications · 2023-01-01

    Mei Yang, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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  11. Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates

    Angewandte Chemie International Edition · 2023-01-05

    Kaichuang Chen, Chensheng Lin, Jindong Chen, Guangsai Yang, Haotian Tian, Min Luo, Tao Yan, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Ning Ye, Guang Peng

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  12. Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates

    Angewandte Chemie · 2023-01-05

    Kaichuang Chen, Chensheng Lin, Jindong Chen, Guangsai Yang, Haotian Tian, Min Luo, Tao Yan, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Ning Ye, Guang Peng

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  13. Elucidating the structure-nonlinear optical property relationship of Te2O4(OH)2

    Materials Today Physics · 2023-04-05

    Sunghwan Cho, Sejin Park, Yunseung Kuk, Kang Min Ok

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  14. Rational Design of a Niobium Tellurite Crystal Nb2Te3O11 Exhibiting Good Overall Infrared NLO Performance by Structural Genetic Engineering

    Inorganic Chemistry · 2023-10-12

    Tinghui Zhang, Jinmiao Jiao, Wenli Zhao, Fulei Wang, Fei Liang, Ning Ye, Zhanggui Hu, Yicheng Wu, Conggang Li

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  15. Flexible Anionic Groups‐Activated Structure Dissymmetry for Strong Nonlinearity in Ln 2 Ae 3 M IV 3 S 12 Family

    Small · 2023-10-24

    Jingjing Xu, Yan Xiao, Kui Wu, Bingbing Zhang, Dazhi Lu, Haohai Yu, Huaijin Zhang

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  16. Not Only Garnets…

    Lithosphere · 2023-12-15

    Irina O. Galuskina, Evgeny V. Galuskin, Yevgeny Vapnik

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  17. Rb 8 Nb 10 Ge 6 O 41 : a new niobium-germanate crystal featuring unique one-dimensional [Nb 7 O 30 ] ∞ chains and wide mid-IR transparency

    Dalton Transactions · 2024-01-01

    Jing Chai, Yuheng She, Jinmiao Jiao, Lili Li, Ning Ye, Zhanggui Hu, Yicheng Wu, Conggang Li

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  18. Centrosymmetric CaBaMF8 and Noncentrosymmetric Li2CaMF8 (M = Zr, Hf): Dimension Variation and Nonlinear Optical Activity Resulting from an Isovalent Cation Substitution-Oriented Design

    Inorganic Chemistry · 2024-03-06

    Mei Yan, Ru‐Ling Tang, Wei Xu, Wenlong Liu, Sheng‐Ping Guo

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  19. Pentanary Oxythiogermanates Ba3MGe3O2S8 (M = Ca, Zn) Featuring [Ge3O2S8]8– Trimers and {[MGe3O2S8]6–}∞ Chains: Structural Chemistry and Physical Properties

    Inorganic Chemistry · 2024-04-12

    Xinxin Fan, Mei Yang, Wen‐Dong Yao, Wenfeng Zhou, Tengfei Jiang, Wenlong Liu, Sheng‐Ping Guo

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  20. La3Ga5M0.5Sn0.5O14, (M = Ge, Si): Design and Synthesis of Two Langasite Nonlinear Optical Materials with Large Second Harmonic Generation and Birefringence Induced by Distorted (Sn/M)O6 Octahedra

    Inorganic Chemistry · 2024-07-25

    Jingxuan Hou, Jiajia Wang, Fei Liang, Shihui Ma, Hongwei Yu, Hongping Wu, Ning Ye, Zhanggui Hu, Yicheng Wu

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  21. Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances

    Small · 2024-12-23

    Junben Huang, Ailijiang Abudurusuli, Zhihua Yang, Shilie Pan

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  22. A Wide Band Gap Germanate with the Largest Second Harmonic Generation Response Created by Hypoxic Strategy

    Angewandte Chemie International Edition · 2025-02-11

    Qi‐Chang Song, Chun‐Li Hu, Fang Kong, Fang Kong, Jiang‐Gao Mao

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  23. A Wide Band Gap Germanate with the Largest Second Harmonic Generation Response Created by Hypoxic Strategy

    Angewandte Chemie · 2025-02-11

    Qi‐Chang Song, Chun‐Li Hu, Fang Kong, Jiang‐Gao Mao

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  24. Methyl substitution induced noncentrosymmetric alignment: a new thiazolium-based nonlinear optical crystal of HDT-N1S

    Journal of Molecular Structure · 2025-05-17

    Bin Li, Xinyuan Zhang, Zhanggui Hu, Ning Ye

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  25. Enhancement of optical anisotropy from [BF4] units by ligand substitution

    Journal of Organometallic Chemistry · 2025-06-20

    Xiaotian Zhang, Chunbo Jiang, Lu Qi, Chao Wu, Chi Zhang

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  26. A‐Site Doping Enables Stabilization and Migration of Oxygen Vacancies in Langasite Frameworks

    Small Structures · 2025-12-31

    Yang Chen, Zhaoji Luo, Xiaohui Li, Cheng Li, Sihao Deng, Lunhua He, Qiang Li, Xianran Xing, Xiaojun Kuang

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  27. A series of langasite-type compounds: size effect regulation for cation occupation and enhanced SHG response

    Inorganic Chemistry Frontiers · 2026-01-01

    Zhi Deng, Nian‐Tzu Suen, Zhen‐Cheng Wu, Huizhi Gao, Sheng‐Ping Guo

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  28. Design of benzoxazolium-based nonlinear optical crystals with large second-order harmonic generation responses

    Chemical Communications · 2026-01-01

    Shaona Wang, Bin Li, Xinyuan Zhang, Zhanggui Hu, Ning Ye

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  29. Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates

    Angewandte Chemie International Edition · 2026-02-17

    Jin Li, Deshuai Xiao, Xinyuan Zhang, Pifu Gong, Zheshuai Lin, Zhanggui Hu, Ning Ye

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  30. Strategic Integration Between Trigonal Architecture Construction and Molecular Polarization Enhancement for Record SHG Effect in Selenates

    Angewandte Chemie · 2026-02-17

    Jin Li, Deshuai Xiao, Xinyuan Zhang, Pifu Gong, Zheshuai Lin, Zhanggui Hu, Ning Ye

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  31. K 3 YGe 3 O 9 : A Rare-Earth Germanate Nonlinear Optical Crystal with a Short Ultraviolet Cutoff Edge and Moderate Second-Harmonic Generation Response

    Inorganic Chemistry · 2026-03-12

    Mingyue Gu, Xianchao Zhu, Zhanggui Hu, Yicheng Wu, Yongmin Guo

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  32. A Telluromolybdate Mid-Infrared Nonlinear Optical Crystal with Wide Transparency and Strong Second-Harmonic Generation Response

    Inorganic Chemistry · 2026-09-16

    Hanyue Zhou, Wenli Zhao, Huijian Zhao, Zelong Liu, Shijie Zhao, Ning Ye, Zhanggui Hu, Conggang Li

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