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RESEARCH PAPER · Chemistry of Materials · 2017

Theory and Neutrons Combine To Reveal a Family of Layered Perovskites without Inversion Symmetry

Tong Zhu, Toby Cohen, Alexandra S. Gibbs, Weiguo Zhang, P. Shiv Halasyamani, Michael A. Hayward, Nicole A. Benedek

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Theory and Neutrons Combine To Reveal a Family of Layered Perovskites without Inversion SymmetryOriginalNanoarchitectonics in dielectric/ferroelectric layered perovskites: from bulk 3D systems to 2D nanosheets62Insights into the polymorphism of Bi 2 W 2 O 9 : single crystal growth and a complete survey of the variable-temperature thermal and dielectric properties11Soft chemistry of ion-exchangeable layered metal oxides183Ferroelectric Sr 3 Zr 2 O 7 : Competition between Hybrid Improper Ferroelectric and Antiferroelectric Mechanisms132Hybrid Improper Ferroelectricity in (Sr,Ca) 3 Sn 2 O 7 and Beyond: Universal Relationship between Ferroelectric Transition Temperature and Tolerance Factor in n = 2 Ruddlesden–Popper Phases123Cation Exchange as a Mechanism To Engineer Polarity in Layered Perovskites33Negative thermal expansion in high pressure layered perovskite Ca 2 GeO 410Abrupt Structural Transformation in Asymmetric ABPO4F (A = K, Rb, Cs)21A -site cation size effect on oxygen octahedral rotations in acentric Ruddlesden-Popper alkali rare-earth titanates11Competing Polar and Antipolar Structures in the Ruddlesden–Popper Layered Perovskite Li2SrNb2O740Synthesis and thermal stability studies of mixed A-site Dion-Jacobson triple-layered perovskites,A′LaNaNb3O10 (A′ = H, Li, Na, K, Rb, CuCl)6Complex Structural Phase Transitions of the Hybrid Improper Polar Dion–Jacobson Oxides RbNdM 2 O 7 and CsNdM 2 O 7 (M = Nb, Ta)35Cooperative interactions govern the fermiology of the polar metal Ca3Ru2O722Cooperative interactions govern the fermiology of the polar metal Ca3Ru2O717Synergistic Influence of d0 (Nb5+) and d10 (Cd2+) Cations in Stabilizing Noncentrosymmetric Dion–Jacobson Layered Perovskites, A′Cd2Nb3O10 (A′ = Rb, Cs)12Ferroelectricity of Dion–Jacobson layered perovskites CsNdNb 2 O 7 and RbNdNb 2 O 720Polar Structures of KNdNb2O7and KNdTa2O710Phase transitions in RbPrNb2O7, a layer structured ferroelectric with a high Curie point26Tuning between Proper and Hybrid-Improper Mechanisms for Polar Behavior in Cs Ln 2Ti2NbO10 Dion-Jacobson Phases22Structural and thermal properties of La-containing Dion – Jacobson homologous series12Ce( iv )-centered charge-neutral perovskite layers topochemically derived from anionic [CeTa 2 O 7 ] − layers9The influence of the 6s 2 configuration of Bi 3+ on the structures of A′BiNb 2 O 7 (A′ = Rb, Na, Li) layered perovskite oxides10Switching between Proper and Hybrid-Improper Polar Structures via Cation Substitution in A2La(TaTi)O7(A = Li, Na)17Layered Double Perovskites75Doping-Enabled Reconfigurable Strongly Correlated Phase in a Quasi-2D Perovskite1Directed synthesis of a hybrid improper magnetoelectric multiferroic material25Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides36Point defect induced incommensurate dipole moments in the KCa2Nb3O10 Dion-Jacobson layered perovskite4The crystal and defect structures of polar KBiNb 2 O 71Designing new polar materials1Lone-Pair-Induced Intra- and Interlayer Polarizations in Sillén-Aurivillius Layered Perovskite Bi4NbO8Br23Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective45Interplay between Oxygen Octahedral Rotation and Deformation in the Acentric ARTiO4 Series toward Negative Thermal Expansion19Second Harmonic Generation in the Polar A′SmNb2O7 (A′ = Rb, Cs) Dion–Jacobson Layered Perovskites11Unleashing the Potential of Strain-Engineered Ferroelectric Oxynitrides for Optimal Photovoltaic Performance2MnCaTa2O7─A Magnetically Ordered Polar Phase Prepared via Cation Exchange4Two-dimensional perovskite NdNb2O7 for high-performance UV photodetectors by a general exfoliation and assembly strategy28Atomic Layer Engineering of Ferroelectricity in Dion–Jacobson Perovskites12“Hexagonal” Perovskites: From Stacking Sequence to Space Group Symmetry and New Opportunities14Synthesis, Structure, and Properties of Dion–Jacobson Double‐Layered Perovskites A′SmNb2O7 (A′=Rb, K, Na, Li, H)4Structural frustration effects by mixed alkali ions in ferroelectric Dion–Jacobson layered perovskites (Cs,Rb)NdNb 2 O 76Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O74Dion–Jacobson (n = 2) Layered Perovskites (A′SmTa2O7; A′ = Rb, Cs) As Potential Ferroelectric Materials6Structural Distortions and Uniaxial Negative Thermal Expansion in the Polar Dion–Jacobson Oxide RbNdTa 2 O 70Enhanced energy storage performance and fatigue resistance in Aurivillius-type CaBi2Nb2O9 thin films via La modification0A study focusing on the influence of multiple cationic substitutions in Dion–Jacobson ( n = 2) layered perovskite oxides0Atomic-Scale Visualization of Competing Polar Orders in Dion–Jacobson Layered Perovskites2

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  1. Nanoarchitectonics in dielectric/ferroelectric layered perovskites: from bulk 3D systems to 2D nanosheets

    Dalton Transactions · 2017-11-22

    Minoru Osada, Takayoshi Sasaki

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  2. Insights into the polymorphism of Bi 2 W 2 O 9 : single crystal growth and a complete survey of the variable-temperature thermal and dielectric properties

    CrystEngComm · 2018-01-01

    Xiangxin Tian, Zeliang Gao, Feifei Chen, Qian Wu, Conggang Li, Weiqun Lu, Youxuan Sun, Xutang Tao

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  3. Soft chemistry of ion-exchangeable layered metal oxides

    Chemical Society Reviews · 2018-01-01

    Ritesh Uppuluri, Arnab Sen Gupta, Alyssa S. Rosas, Thomas E. Mallouk

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  4. Ferroelectric Sr 3 Zr 2 O 7 : Competition between Hybrid Improper Ferroelectric and Antiferroelectric Mechanisms

    Advanced Functional Materials · 2018-05-28

    Suguru Yoshida, Koji Fujita, Hirofumi Akamatsu, Olivier Hernandez, Arnab Sen Gupta, Forrest G. Brown, Haricharan Padmanabhan, Alexandra S. Gibbs, Toshihiro Kuge, Ryosuke Tsuji, Shunsuke Murai, James M. Rondinelli, Venkatraman Gopalan, Katsuhisa Tanaka

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  5. Hybrid Improper Ferroelectricity in (Sr,Ca) 3 Sn 2 O 7 and Beyond: Universal Relationship between Ferroelectric Transition Temperature and Tolerance Factor in n = 2 Ruddlesden–Popper Phases

    Journal of the American Chemical Society · 2018-10-23

    Suguru Yoshida, Hirofumi Akamatsu, Ryosuke Tsuji, Olivier Hernandez, Haricharan Padmanabhan, Arnab Sen Gupta, Alexandra S. Gibbs, Ko Mibu, Shunsuke Murai, James M. Rondinelli, Venkatraman Gopalan, Katsuhisa Tanaka, Koji Fujita

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  6. Cation Exchange as a Mechanism To Engineer Polarity in Layered Perovskites

    Chemistry of Materials · 2018-11-26

    Tong Zhu, Guru Khalsa, Dana M. Havas, Alexandra S. Gibbs, Weiguo Zhang, P. Shiv Halasyamani, Nicole A. Benedek, Michael A. Hayward

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  7. Negative thermal expansion in high pressure layered perovskite Ca 2 GeO 4

    Chemical Communications · 2019-01-01

    Wei‐Tin Chen, Chris Ablitt, Nicholas C. Bristowe, Arash A. Mostofi, Takashi Kei SAITO, Yuichi Shimakawa, Mark S. Senn

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  8. Abrupt Structural Transformation in Asymmetric ABPO4F (A = K, Rb, Cs)

    Inorganic Chemistry · 2019-01-17

    Qingran Ding, Sangen Zhao, Lina Li, Yaoguo Shen, Pai Shan, Zhenyue Wu, Xianfeng Li, Yanqiang Li, Shuai Liu, Junhua Luo

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  9. A -site cation size effect on oxygen octahedral rotations in acentric Ruddlesden-Popper alkali rare-earth titanates

    Physical Review Materials · 2019-06-10

    Hirofumi Akamatsu, Koji Fujita, Toshihiro Kuge, Arnab Sen Gupta, James M. Rondinelli, Isao Tanaka, Katsuhisa Tanaka, Venkatraman Gopalan

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  10. Competing Polar and Antipolar Structures in the Ruddlesden–Popper Layered Perovskite Li2SrNb2O7

    Chemistry of Materials · 2019-06-12

    Ritesh Uppuluri, Hirofumi Akamatsu, Arnab Sen Gupta, Huaiyu Hugo Wang, Craig M. Brown, Kleyser Agueda Lopez, Nasim Alem, Venkatraman Gopalan, Thomas E. Mallouk

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  11. Synthesis and thermal stability studies of mixed A-site Dion-Jacobson triple-layered perovskites,A′LaNaNb3O10 (A′ = H, Li, Na, K, Rb, CuCl)

    Journal of Solid State Chemistry · 2020-02-05

    Léa Gustin, Jérôme Lefebvre, Amy P. Tillman, John B. Wiley

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  12. Complex Structural Phase Transitions of the Hybrid Improper Polar Dion–Jacobson Oxides RbNdM 2 O 7 and CsNdM 2 O 7 (M = Nb, Ta)

    Chemistry of Materials · 2020-04-23

    Tong Zhu, Alexandra S. Gibbs, Nicole A. Benedek, Michael A. Hayward

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  13. Cooperative interactions govern the fermiology of the polar metal Ca3Ru2O7

    Physical Review Research · 2020-05-08

    Danilo Puggioni, M. Horio, J. Chang, James M. Rondinelli

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  14. Cooperative interactions govern the fermiology of the polar metal Ca3Ru2O7

    Zurich Open Repository and Archive (University of Zurich) · 2020-05-08

    Danilo Puggioni, Masafumi Horio, J. Chang, James M. Rondinelli

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  15. Synergistic Influence of d0 (Nb5+) and d10 (Cd2+) Cations in Stabilizing Noncentrosymmetric Dion–Jacobson Layered Perovskites, A′Cd2Nb3O10 (A′ = Rb, Cs)

    Inorganic Chemistry · 2020-05-28

    Shalu Atri, Meenakshi Pokhriyal, S. Uma

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  16. Ferroelectricity of Dion–Jacobson layered perovskites CsNdNb 2 O 7 and RbNdNb 2 O 7

    Japanese Journal of Applied Physics · 2020-08-07

    Sota Asaki, Hirofumi Akamatsu, George Hasegawa, Tomohiro Abe, Yuki Nakahira, Suguru Yoshida, Chikako Moriyoshi, Katsuro Hayashi

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  17. Polar Structures of KNdNb2O7and KNdTa2O7

    Chemistry of Materials · 2020-08-25

    Subhadip Mallick, Alexandra S. Gibbs, Weiguo Zhang, P. Shiv Halasyamani, Nicole A. Benedek, Michael A. Hayward

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  18. Phase transitions in RbPrNb2O7, a layer structured ferroelectric with a high Curie point

    Acta Materialia · 2020-09-22

    Zhongna Yan, Dou Zhang, Xuefan Zhou, Man Zhang, Yajun Yue, Ludan Zhang, Guoliang Xue, Hang Luo, Isaac Abrahams, Haixue Yan

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  19. Tuning between Proper and Hybrid-Improper Mechanisms for Polar Behavior in Cs Ln 2Ti2NbO10 Dion-Jacobson Phases

    Chemistry of Materials · 2020-09-22

    Vanessa A. Cascos, Jennifer Roberts-Watts, Chloe Skingle, Igor Levin, Weiguo Zhang, P. Shiv Halasyamani, Martin Christopher. Stennett, Neil Christian Hyatt, Éric Bousquet, Emma E. McCabe

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  20. Structural and thermal properties of La-containing Dion – Jacobson homologous series

    Journal of Solid State Chemistry · 2020-10-26

    Alexander Vladimirovich Knyazev, E.V. Syrov, О. В. Крашенинникова, Vladimir M. Kyashkin, Dmitry N. Titaev, Diana Georgievna Fukina

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  21. Ce( iv )-centered charge-neutral perovskite layers topochemically derived from anionic [CeTa 2 O 7 ] − layers

    Chemical Science · 2021-01-01

    Takuya Hasegawa, Naoki Yamasaki, Yusuke Asakura, Tadaharu Ueda, Shu Yin

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  22. The influence of the 6s 2 configuration of Bi 3+ on the structures of A′BiNb 2 O 7 (A′ = Rb, Na, Li) layered perovskite oxides

    Dalton Transactions · 2021-01-01

    Subhadip Mallick, Guru Khalsa, Jeffrey Z. Kaaret, Weiguo Zhang, Maria Batuk, Alexandra S. Gibbs, Joke Hadermann, P. Shiv Halasyamani, Nicole A. Benedek, Michael A. Hayward

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  23. Switching between Proper and Hybrid-Improper Polar Structures via Cation Substitution in A2La(TaTi)O7(A = Li, Na)

    Chemistry of Materials · 2021-03-31

    Subhadip Mallick, Andrew Dominic Fortes, Weiguo Zhang, P. Shiv Halasyamani, Michael A. Hayward

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  24. Layered Double Perovskites

    Annual Review of Materials Research · 2021-05-05

    Hayden A. Evans, Lingling Mao, Ram Seshadri, Anthony Kevin Cheetham

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  25. Doping-Enabled Reconfigurable Strongly Correlated Phase in a Quasi-2D Perovskite

    The Journal of Physical Chemistry Letters · 2021-05-24

    Lifu Zhang, Jie Jiang, Yao Cai, Shukai Yao, Bilal Azhar, Zhizhong Chen, Yang Hu, Saloni Pendse, Yuwei Guo, Ru Jia, Zhiting Tian, Chengliang Sun, Peilin Liao, Jian Zhong Shi

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  26. Directed synthesis of a hybrid improper magnetoelectric multiferroic material

    Nature Communications · 2021-08-16

    Tong Zhu, Fabio Orlandi, Pascal Manuel, Alexandra S. Gibbs, Weiguo Zhang, P. Shiv Halasyamani, Michael A. Hayward

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  27. Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides

    Journal of Physics D Applied Physics · 2021-10-22

    Bi Hui Zhang, Xiao Qiang Liu, Xiang Ming Chen

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  28. Point defect induced incommensurate dipole moments in the KCa2Nb3O10 Dion-Jacobson layered perovskite

    Physical review. B./Physical review. B · 2021-12-16

    Jing Kong, Sanjeev K. Nayak, Kevin Co, Sanjib Nayak, Jingkun Wu, Antonio M. Feteira, Kevin A. Beyer, S. P. Alpay, Abhijit Pramanick

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  29. The crystal and defect structures of polar KBiNb 2 O 7

    Dalton Transactions · 2022-01-01

    Subhadip Mallick, Weiguo Zhang, Maria Batuk, Alexandra S. Gibbs, Joke Hadermann, P. Shiv Halasyamani, Michael A. Hayward

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  30. Designing new polar materials

    Elsevier eBooks · 2022-01-28

    Emma E. McCabe

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  31. Lone-Pair-Induced Intra- and Interlayer Polarizations in Sillén-Aurivillius Layered Perovskite Bi4NbO8Br

    Inorganic Chemistry · 2022-06-15

    Chengchao Zhong, Yui Ishii, Cédric Tassel, Tong Zhu, Daichi Kato, Kosuke Kurushima, Yukihiro Fujibayashi, Takashi Kei SAITO, T. Ogawa, Akihide Kuwabara, Shigeo Mori, Hiroshi Kageyama

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  32. Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective

    Annual Review of Materials Research · 2022-07-01

    Nicole A. Benedek, Michael A. Hayward

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  33. Interplay between Oxygen Octahedral Rotation and Deformation in the Acentric ARTiO4 Series toward Negative Thermal Expansion

    Chemistry of Materials · 2022-07-11

    Suguru Yoshida, Hirofumi Akamatsu, Alexandra S. Gibbs, Shogo Kawaguchi, Venkatraman Gopalan, Katsuhisa Tanaka, Koji Fujita

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  34. Second Harmonic Generation in the Polar A′SmNb2O7 (A′ = Rb, Cs) Dion–Jacobson Layered Perovskites

    Chemistry of Materials · 2023-01-23

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  35. Unleashing the Potential of Strain-Engineered Ferroelectric Oxynitrides for Optimal Photovoltaic Performance

    The Journal of Physical Chemistry C · 2023-07-28

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  36. MnCaTa2O7─A Magnetically Ordered Polar Phase Prepared via Cation Exchange

    Chemistry of Materials · 2023-09-09

    Subhadip Mallick, Fabio Orlandi, Pascal Manuel, Weiguo Zhang, P. Shiv Halasyamani, Michael A. Hayward

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  37. Two-dimensional perovskite NdNb2O7 for high-performance UV photodetectors by a general exfoliation and assembly strategy

    Nano Energy · 2023-09-16

    Yong Zhang, Jian Yao, Yu Teng, Zheng Zhang, Lin Wang, Xiujun Wang, Yunfei Li, Lixing Kang, Jr‐Hau He, Xiaosheng Fang

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  38. Atomic Layer Engineering of Ferroelectricity in Dion–Jacobson Perovskites

    Journal of the American Chemical Society · 2024-08-26

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  39. “Hexagonal” Perovskites: From Stacking Sequence to Space Group Symmetry and New Opportunities

    Chemistry of Materials · 2024-09-18

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  40. Synthesis, Structure, and Properties of Dion–Jacobson Double‐Layered Perovskites A′SmNb2O7 (A′=Rb, K, Na, Li, H)

    European Journal of Inorganic Chemistry · 2024-10-23

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  41. Structural frustration effects by mixed alkali ions in ferroelectric Dion–Jacobson layered perovskites (Cs,Rb)NdNb 2 O 7

    Journal of Materials Chemistry C · 2024-11-25

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  42. Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O7

    Inorganic Chemistry · 2024-11-27

    Zhen‐Tao Lu, Kai Nishioka, Yang Zhang, Koji Fujita, Katsuro Hayashi, Hirofumi Akamatsu

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  43. Dion–Jacobson (n = 2) Layered Perovskites (A′SmTa2O7; A′ = Rb, Cs) As Potential Ferroelectric Materials

    The Journal of Physical Chemistry C · 2025-03-11

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  44. Structural Distortions and Uniaxial Negative Thermal Expansion in the Polar Dion–Jacobson Oxide RbNdTa 2 O 7

    Chemistry of Materials · 2025-05-15

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  45. Enhanced energy storage performance and fatigue resistance in Aurivillius-type CaBi2Nb2O9 thin films via La modification

    Journal of the Korean Ceramic Society · 2025-12-03

    Yoonho Ahn, Jong Yeog Son

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  46. A study focusing on the influence of multiple cationic substitutions in Dion–Jacobson ( n = 2) layered perovskite oxides

    Dalton Transactions · 2026-01-01

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  47. Atomic-Scale Visualization of Competing Polar Orders in Dion–Jacobson Layered Perovskites

    Chemistry of Materials · 2026-04-21

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