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RESEARCH PAPER · Annual Review of Materials Research · 2022

Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective

Nicole A. Benedek, Michael A. Hayward

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Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic PerspectiveOriginalDesign of high polarization low switching barrier hybrid improper ferroelectric perovskite oxide superlattices7Design Principles for Noncentrosymmetric Materials23MnCaTa2O7─A Magnetically Ordered Polar Phase Prepared via Cation Exchange4Persistent and Quasipersistent Spin Textures in Halide Perovskites Induced by Uniaxial Stress11Displacive phase transitions in infinite-layer nickelates from first- and second-principles calculations7Ferroelectric phase transition in a 1T monolayer of MoTe2 : A first-principles study10Emerging ceramic nanosheets: From tailored synthesis to electronic applications1Out-of-plane ferroelectricity and robust magnetoelectricity in quasi-two-dimensional materials15The past 10 years of molecular ferroelectrics: structures, design, and properties173Coherent control of the translational and point group symmetries of crystals with light11Engineering Collinear Magnetization in Hexagonal LuFeO 3 and Magnetoelectric Control of Skyrmions in Hexagonal 2D Epilayers7Piezoelectricity in n = 2 Ruddlesden–Popper Ferroelectric Oxides9Lattice-distortion couplings in antiferroelectric perovskite AgNbO 3 and comparison with PbZrO 35Atomic Layer Engineering of Ferroelectricity in Dion–Jacobson Perovskites12Tunable Schottky barriers and magnetoelectric coupling driven by ferroelectric polarization reversal of MnI3/In2Se3 multiferroic heterostructures31First-principles prediction of a polar half-metallic ferromagnet in a heterostructure based on PbMnO 3 and SrMnO 33Superconductivity-induced improper orders in nonsymmorphic systems10Structural frustration effects by mixed alkali ions in ferroelectric Dion–Jacobson layered perovskites (Cs,Rb)NdNb 2 O 76Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O74Perspective on 2D perovskite ferroelectrics and multiferroics12Hybrid improper ferroelectricity in a Si-compatible CeO2/HfO2 artificial superlattice2Exploring a Route to Induce Ferromagnetism on Sr3sn2o7 by Non-Jahn-Teller-Distorted Mn3+ Cations0Piezoresistivity as a Fingerprint of Ferroaxial Transitions8Thermally Controlled A-site Cation Ordering and Coupled Polarity in Double Perovskite NaLaZr2O62Structural chirality and related properties in periodic inorganic solids: review and perspectives30Dion–Jacobson (n = 2) Layered Perovskites (A′SmTa2O7; A′ = Rb, Cs) As Potential Ferroelectric Materials6Domain Wall Reactions in Multiple-Order Parameter Ferroelectrics11Structural distortions leading to potential polar materials in n $=$ 3 and 4 Dion–Jacobson-layered perovskite series1Structural, magnetic, dielectric and electrical transport properties of CaCu3Ti2FeVO12 quadruple perovskite oxides synthesized at ambient pressure0Structural Distortions and Uniaxial Negative Thermal Expansion in the Polar Dion–Jacobson Oxide RbNdTa 2 O 70Structural Phase Transitions in Layered Perovskite CsFeF4${\rm CsFeF}_{4}$ and Weak Polar Response in CsFeF4${\rm CsFeF}_{4}$/RbFeF4${\rm RbFeF}_{4}$ Superlattice0Cation Exchange as a Route to Introduce Magnetism to Hybrid-Improper Polar Phases0Piezomagnetism-driven magnetoelectric coupling in altermagnetic multiferroic K 3 Cr 2 F 74Design and Theory of Switchable Linear Magnetoelectricity by Ferroelectricity in Type-I Multiferroics6Route-dependent toxicodynamics of 6PPD-quinone in mussels: Mechanical resilience trades off with subcellular injury and metabolic disruption3A-Site Cation Disorder Engineering in Ruddlesden–Popper Layered Perovskite Oxide La 2 (Ba,Sr)In 2 O 7 for Hybrid Improper Ferroelectricity8Exploring a route to induce ferromagnetism on Sr3Sn2O7 by co-doping with non-Jahn-Teller-distorted Mn3+ and La3+ cations1A study focusing on the influence of multiple cationic substitutions in Dion–Jacobson ( n = 2) layered perovskite oxides0Triggered Ferroelectricity in HfO 2 From Hybrid Phonons and Higher‐Order Dynamical Charges5Atomic-Scale Visualization of Competing Polar Orders in Dion–Jacobson Layered Perovskites2Local indirect magnetoelectric coupling at twin walls in CaMnO 302D dielectrics and ferroelectrics: emerging materials, physics and design principles0Why are some special ferroelectrics immune to the depolarization field?0Coherent dipole units and ferroelectric correlations in asymmetric atomic-layer superlattices0Noncentrosymmetric Manganese Bismuth Thiocyanate Perovskites0

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  1. Design of high polarization low switching barrier hybrid improper ferroelectric perovskite oxide superlattices

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  2. Design Principles for Noncentrosymmetric Materials

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  3. MnCaTa2O7─A Magnetically Ordered Polar Phase Prepared via Cation Exchange

    Chemistry of Materials · 2023-09-09

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  4. Persistent and Quasipersistent Spin Textures in Halide Perovskites Induced by Uniaxial Stress

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  5. Displacive phase transitions in infinite-layer nickelates from first- and second-principles calculations

    Physical review. B./Physical review. B · 2023-10-12

    Yajun Zhang, Jingtong Zhang, Jiahang Li, P. S. Sahoo, Xu He, Jie Wang, Philippe Ghosez

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  6. Ferroelectric phase transition in a 1T monolayer of MoTe2 : A first-principles study

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  7. Emerging ceramic nanosheets: From tailored synthesis to electronic applications

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  8. Out-of-plane ferroelectricity and robust magnetoelectricity in quasi-two-dimensional materials

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    Xue‐Zeng Lu, Hui-Min Zhang, Ying Zhou, Tong Zhu, Hongjun Xiang, Shuai Dong, Hiroshi Kageyama, James M. Rondinelli

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  9. The past 10 years of molecular ferroelectrics: structures, design, and properties

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  10. Coherent control of the translational and point group symmetries of crystals with light

    Physical review. B./Physical review. B · 2024-01-25

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  11. Engineering Collinear Magnetization in Hexagonal LuFeO 3 and Magnetoelectric Control of Skyrmions in Hexagonal 2D Epilayers

    Advanced Functional Materials · 2024-07-11

    M. J. Swamynadhan, Andrew O’Hara, Saurabh Ghosh, Sokrates T. Pantelides

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  12. Piezoelectricity in n = 2 Ruddlesden–Popper Ferroelectric Oxides

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  13. Lattice-distortion couplings in antiferroelectric perovskite AgNbO 3 and comparison with PbZrO 3

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  14. Atomic Layer Engineering of Ferroelectricity in Dion–Jacobson Perovskites

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    Shu Morita, Daisuke Urushihara, Keita Nishibashi, Makoto Kobayashi, Eisuke Yamamoto, Toru Asaka, Hiroshi Nakajima, Shigeo Mori, Minoru Osada

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  15. Tunable Schottky barriers and magnetoelectric coupling driven by ferroelectric polarization reversal of MnI3/In2Se3 multiferroic heterostructures

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  16. First-principles prediction of a polar half-metallic ferromagnet in a heterostructure based on PbMnO 3 and SrMnO 3

    Physical review. B./Physical review. B · 2024-11-12

    Arpita Paul, Umesh Vasudeo Waghmare

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  17. Superconductivity-induced improper orders in nonsymmorphic systems

    Physical review. B./Physical review. B · 2024-11-18

    András Szabó, Aline Ramires

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  18. Structural frustration effects by mixed alkali ions in ferroelectric Dion–Jacobson layered perovskites (Cs,Rb)NdNb 2 O 7

    Journal of Materials Chemistry C · 2024-11-25

    Zhen‐Tao Lu, Sota Asaki, Suguru Yoshida, Chikako Moriyoshi, George Hasegawa, Koji Fujita, Venkatraman Gopalan, Katsuro Hayashi, Hirofumi Akamatsu

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  19. Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O7

    Inorganic Chemistry · 2024-11-27

    Zhen‐Tao Lu, Kai Nishioka, Yang Zhang, Koji Fujita, Katsuro Hayashi, Hirofumi Akamatsu

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  20. Perspective on 2D perovskite ferroelectrics and multiferroics

    Applied Physics Letters · 2024-12-02

    Junting Zhang, Yu Xie, Ke Ji, Xiaofan Shen

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  21. Hybrid improper ferroelectricity in a Si-compatible CeO2/HfO2 artificial superlattice

    npj Computational Materials · 2024-12-19

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  22. Exploring a Route to Induce Ferromagnetism on Sr3sn2o7 by Non-Jahn-Teller-Distorted Mn3+ Cations

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  23. Piezoresistivity as a Fingerprint of Ferroaxial Transitions

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  24. Thermally Controlled A-site Cation Ordering and Coupled Polarity in Double Perovskite NaLaZr2O6

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  25. Structural chirality and related properties in periodic inorganic solids: review and perspectives

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  26. Dion–Jacobson (n = 2) Layered Perovskites (A′SmTa2O7; A′ = Rb, Cs) As Potential Ferroelectric Materials

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  27. Domain Wall Reactions in Multiple-Order Parameter Ferroelectrics

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  28. Structural distortions leading to potential polar materials in n $$=$$ 3 and 4 Dion–Jacobson-layered perovskite series

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  29. Structural, magnetic, dielectric and electrical transport properties of CaCu3Ti2FeVO12 quadruple perovskite oxides synthesized at ambient pressure

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  30. Structural Distortions and Uniaxial Negative Thermal Expansion in the Polar Dion–Jacobson Oxide RbNdTa 2 O 7

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  31. Structural Phase Transitions in Layered Perovskite CsFeF4${\rm CsFeF}_{4}$ and Weak Polar Response in CsFeF4${\rm CsFeF}_{4}$/RbFeF4${\rm RbFeF}_{4}$ Superlattice

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  32. Cation Exchange as a Route to Introduce Magnetism to Hybrid-Improper Polar Phases

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  33. Piezomagnetism-driven magnetoelectric coupling in altermagnetic multiferroic K 3 Cr 2 F 7

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  34. Design and Theory of Switchable Linear Magnetoelectricity by Ferroelectricity in Type-I Multiferroics

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  35. Route-dependent toxicodynamics of 6PPD-quinone in mussels: Mechanical resilience trades off with subcellular injury and metabolic disruption

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  36. A-Site Cation Disorder Engineering in Ruddlesden–Popper Layered Perovskite Oxide La 2 (Ba,Sr)In 2 O 7 for Hybrid Improper Ferroelectricity

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  37. Exploring a route to induce ferromagnetism on Sr3Sn2O7 by co-doping with non-Jahn-Teller-distorted Mn3+ and La3+ cations

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  38. A study focusing on the influence of multiple cationic substitutions in Dion–Jacobson ( n = 2) layered perovskite oxides

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  39. Triggered Ferroelectricity in HfO 2 From Hybrid Phonons and Higher‐Order Dynamical Charges

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  40. Atomic-Scale Visualization of Competing Polar Orders in Dion–Jacobson Layered Perovskites

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  41. Local indirect magnetoelectric coupling at twin walls in CaMnO 3

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  43. Why are some special ferroelectrics immune to the depolarization field?

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  44. Coherent dipole units and ferroelectric correlations in asymmetric atomic-layer superlattices

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  45. Noncentrosymmetric Manganese Bismuth Thiocyanate Perovskites

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