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RESEARCH PAPER · Chemistry of Materials · 2020

Complex Structural Phase Transitions of the Hybrid Improper Polar Dion–Jacobson Oxides RbNdM 2 O 7 and CsNdM 2 O 7 (M = Nb, Ta)

Tong Zhu, Alexandra S. Gibbs, Nicole A. Benedek, Michael A. Hayward

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Complex Structural Phase Transitions of the Hybrid Improper Polar Dion–Jacobson Oxides RbNdM 2 O 7 and CsNdM 2 O 7 (M = Nb, Ta)OriginalFerroelectricity of Dion–Jacobson layered perovskites CsNdNb 2 O 7 and RbNdNb 2 O 720Polar Structures of KNdNb2O7and KNdTa2O710Tuning between Proper and Hybrid-Improper Mechanisms for Polar Behavior in Cs Ln 2Ti2NbO10 Dion-Jacobson Phases22Structural and thermal properties of La-containing Dion – Jacobson homologous series12Ce( iv )-centered charge-neutral perovskite layers topochemically derived from anionic [CeTa 2 O 7 ] − layers9The influence of the 6s 2 configuration of Bi 3+ on the structures of A′BiNb 2 O 7 (A′ = Rb, Na, Li) layered perovskite oxides10Switching between Proper and Hybrid-Improper Polar Structures via Cation Substitution in A2La(TaTi)O7(A = Li, Na)17Directed synthesis of a hybrid improper magnetoelectric multiferroic material25Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides36Hybrid improper dipolar density wave in NaLaCoWO$_6$0Point defect induced incommensurate dipole moments in the KCa2Nb3O10 Dion-Jacobson layered perovskite4The crystal and defect structures of polar KBiNb 2 O 72Designing new polar materials1Hybrid improper dipolar density wave in NaLaCoWO61Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective45Local atomic structure distortions in the Dion-Jacobson ferroelectric CsBiNb2O71Single-Ion Behavior in New 2-D and 3-D Gadolinium 4f7 Materials: CsGd(SO4)2 and Cs[Gd(H2O)3(SO4)2]·H2O10Cerium(III) Niobate Layered Perovskites: Abnormal Optical Absorption Modulations by Tuning of B-Site Composition and Perovskite Layer Charge Control5Second Harmonic Generation in the Polar A′SmNb2O7 (A′ = Rb, Cs) Dion–Jacobson Layered Perovskites11Chemical Trends of Surface Reconstruction and Band Positions of Nonmetallic Perovskite Oxides from First Principles19Two-dimensional perovskite NdNb2O7 for high-performance UV photodetectors by a general exfoliation and assembly strategy28Out-of-plane ferroelectricity and robust magnetoelectricity in quasi-two-dimensional materials15Structural frustration effects by mixed alkali ions in ferroelectric Dion–Jacobson layered perovskites (Cs,Rb)NdNb 2 O 76Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O74Structural chemistry of the n = 3 Dion–Jacobson phases: controlling polarity and band gap3Dion–Jacobson (n = 2) Layered Perovskites (A′SmTa2O7; A′ = Rb, Cs) As Potential Ferroelectric Materials6Structural Distortions and Uniaxial Negative Thermal Expansion in the Polar Dion–Jacobson Oxide RbNdTa 2 O 70Temperature-induced structural phase transitions in inorganic compounds: symmetry and information-entropy analysis1A study focusing on the influence of multiple cationic substitutions in Dion–Jacobson ( n = 2) layered perovskite oxides0Atomic-Scale Visualization of Competing Polar Orders in Dion–Jacobson Layered Perovskites22D dielectrics and ferroelectrics: emerging materials, physics and design principles0Redox-Neutral Interstitial Hydride Incorporation in Ruddlesden–Popper Oxides0Record‐Low Coercive Field and Stable Curie Temperature in Bulk Hybrid Improper Ferroelectrics via Synergistic A / B ‐Site Co‐Substitution0Hybrid improper ferroelectricity and enhanced Curie temperature in co-substituted La2SrSc2O7-based ceramics0

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  1. Ferroelectricity of Dion–Jacobson layered perovskites CsNdNb 2 O 7 and RbNdNb 2 O 7

    Japanese Journal of Applied Physics · 2020-08-07

    Sota Asaki, Hirofumi Akamatsu, George Hasegawa, Tomohiro Abe, Yuki Nakahira, Suguru Yoshida, Chikako Moriyoshi, Katsuro Hayashi

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  2. Polar Structures of KNdNb2O7and KNdTa2O7

    Chemistry of Materials · 2020-08-25

    Subhadip Mallick, Alexandra S. Gibbs, Weiguo Zhang, P. Shiv Halasyamani, Nicole A. Benedek, Michael A. Hayward

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  3. Tuning between Proper and Hybrid-Improper Mechanisms for Polar Behavior in Cs Ln 2Ti2NbO10 Dion-Jacobson Phases

    Chemistry of Materials · 2020-09-22

    Vanessa A. Cascos, Jennifer Roberts-Watts, Chloe Skingle, Igor Levin, Weiguo Zhang, P. Shiv Halasyamani, Martin Christopher. Stennett, Neil Christian Hyatt, Éric Bousquet, Emma E. McCabe

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  4. Structural and thermal properties of La-containing Dion – Jacobson homologous series

    Journal of Solid State Chemistry · 2020-10-26

    Alexander Vladimirovich Knyazev, E.V. Syrov, О. В. Крашенинникова, Vladimir M. Kyashkin, Dmitry N. Titaev, Diana Georgievna Fukina

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  5. Ce( iv )-centered charge-neutral perovskite layers topochemically derived from anionic [CeTa 2 O 7 ] − layers

    Chemical Science · 2021-01-01

    Takuya Hasegawa, Naoki Yamasaki, Yusuke Asakura, Tadaharu Ueda, Shu Yin

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  6. The influence of the 6s 2 configuration of Bi 3+ on the structures of A′BiNb 2 O 7 (A′ = Rb, Na, Li) layered perovskite oxides

    Dalton Transactions · 2021-01-01

    Subhadip Mallick, Guru Khalsa, Jeffrey Z. Kaaret, Weiguo Zhang, Maria Batuk, Alexandra S. Gibbs, Joke Hadermann, P. Shiv Halasyamani, Nicole A. Benedek, Michael A. Hayward

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  7. Switching between Proper and Hybrid-Improper Polar Structures via Cation Substitution in A2La(TaTi)O7(A = Li, Na)

    Chemistry of Materials · 2021-03-31

    Subhadip Mallick, Andrew Dominic Fortes, Weiguo Zhang, P. Shiv Halasyamani, Michael A. Hayward

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  8. Directed synthesis of a hybrid improper magnetoelectric multiferroic material

    Nature Communications · 2021-08-16

    Tong Zhu, Fabio Orlandi, Pascal Manuel, Alexandra S. Gibbs, Weiguo Zhang, P. Shiv Halasyamani, Michael A. Hayward

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  9. Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides

    Journal of Physics D Applied Physics · 2021-10-22

    Bi Hui Zhang, Xiao Qiang Liu, Xiang Ming Chen

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  10. Hybrid improper dipolar density wave in NaLaCoWO$_6$

    arXiv (Cornell University) · 2021-10-28

    Andrea Griesi, Enrico Mugnaioli, Arianna Lanza, Valentina Vit, L. Righi, Mauro Gemmi, Fabio Orlandi

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  11. Point defect induced incommensurate dipole moments in the KCa2Nb3O10 Dion-Jacobson layered perovskite

    Physical review. B./Physical review. B · 2021-12-16

    Jing Kong, Sanjeev K. Nayak, Kevin Co, Sanjib Nayak, Jingkun Wu, Antonio M. Feteira, Kevin A. Beyer, S. P. Alpay, Abhijit Pramanick

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  12. The crystal and defect structures of polar KBiNb 2 O 7

    Dalton Transactions · 2022-01-01

    Subhadip Mallick, Weiguo Zhang, Maria Batuk, Alexandra S. Gibbs, Joke Hadermann, P. Shiv Halasyamani, Michael A. Hayward

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  13. Designing new polar materials

    Elsevier eBooks · 2022-01-28

    Emma E. McCabe

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  14. Hybrid improper dipolar density wave in NaLaCoWO6

    Physical Review Materials · 2022-03-30

    Andrea Griesi, Enrico Mugnaioli, Arianna Lanza, Valentina Vit, L. Righi, Mauro Gemmi, Fabio Orlandi

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  15. Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective

    Annual Review of Materials Research · 2022-07-01

    Nicole A. Benedek, Michael A. Hayward

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  16. Local atomic structure distortions in the Dion-Jacobson ferroelectric CsBiNb2O7

    Physical review. B./Physical review. B · 2022-07-06

    Jing Kong, Sanjeev K. Nayak, Jue Liu, S. P. Alpay, Abhijit Pramanick

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  17. Single-Ion Behavior in New 2-D and 3-D Gadolinium 4f7 Materials: CsGd(SO4)2 and Cs[Gd(H2O)3(SO4)2]·H2O

    ACS Organic & Inorganic Au · 2022-09-04

    Ebube E. Oyeka, T. Thao Tran

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  18. Cerium(III) Niobate Layered Perovskites: Abnormal Optical Absorption Modulations by Tuning of B-Site Composition and Perovskite Layer Charge Control

    Inorganic Chemistry · 2022-12-02

    Takuya Hasegawa, Tadaharu Ueda, Yusuke Asakura, Shu Yin

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  19. Second Harmonic Generation in the Polar A′SmNb2O7 (A′ = Rb, Cs) Dion–Jacobson Layered Perovskites

    Chemistry of Materials · 2023-01-23

    Sachin Pal, R. Nagarajan, S. Uma

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  20. Chemical Trends of Surface Reconstruction and Band Positions of Nonmetallic Perovskite Oxides from First Principles

    Chemistry of Materials · 2023-02-21

    Yasuhide Mochizuki, Ha‐Jun Sung, Tomoya Gake, Fumiyasu Oba

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  21. Two-dimensional perovskite NdNb2O7 for high-performance UV photodetectors by a general exfoliation and assembly strategy

    Nano Energy · 2023-09-16

    Yong Zhang, Jian Yao, Yu Teng, Zhen Zhang, Lin Wang, Xiujun Wang, Yunfei Li, Lixing Kang, Jr‐Hau He, Xiaosheng Fang

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  22. Out-of-plane ferroelectricity and robust magnetoelectricity in quasi-two-dimensional materials

    Science Advances · 2023-11-22

    Xue‐Zeng Lu, Hui-Min Zhang, Ying Zhou, Tong Zhu, Hongjun Xiang, Shuai Dong, Hiroshi Kageyama, James M. Rondinelli

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  23. Structural frustration effects by mixed alkali ions in ferroelectric Dion–Jacobson layered perovskites (Cs,Rb)NdNb 2 O 7

    Journal of Materials Chemistry C · 2024-11-25

    Zhen‐Tao Lu, Sota Asaki, Suguru Yoshida, Chikako Moriyoshi, George Hasegawa, Koji Fujita, Venkatraman Gopalan, Katsuro Hayashi, Hirofumi Akamatsu

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  24. Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O7

    Inorganic Chemistry · 2024-11-27

    Zhen‐Tao Lu, Kai Nishioka, Yang Zhang, Koji Fujita, Katsuro Hayashi, Hirofumi Akamatsu

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  25. Structural chemistry of the n = 3 Dion–Jacobson phases: controlling polarity and band gap

    Journal of Materials Chemistry A · 2025-01-01

    Areesha Ali, Vanessa A. Cascos, Faith G. Pritchard, Jan R. R. Verlet, Nicole R. Sutherland, Jack Matthew Woolley, James Lloyd‐Hughes, Maxim Avdeev, Andy Beeby, Stewart J. Clark, Emma E. McCabe

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  26. Dion–Jacobson (n = 2) Layered Perovskites (A′SmTa2O7; A′ = Rb, Cs) As Potential Ferroelectric Materials

    The Journal of Physical Chemistry C · 2025-03-11

    Vandana Yadav, Sachin Pal, S. Uma

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  27. Structural Distortions and Uniaxial Negative Thermal Expansion in the Polar Dion–Jacobson Oxide RbNdTa 2 O 7

    Chemistry of Materials · 2025-05-15

    P. Neenu Lekshmi, Da Silva, Pedro Rocha‐Rodrigues, John S. O. Evans, J.H. Belo, Pedro Silva de Sousa, Alicia Maria Manjón-Sanz, A. M. dos Santos, A. M. L. Lopes, João P. Araújo

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  28. Temperature-induced structural phase transitions in inorganic compounds: symmetry and information-entropy analysis

    Progress in Solid State Chemistry · 2025-09-11

    Sergey V. Krivovichev

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  29. A study focusing on the influence of multiple cationic substitutions in Dion–Jacobson ( n = 2) layered perovskite oxides

    Dalton Transactions · 2026-01-01

    Vandana Yadav, S. Uma

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  30. Atomic-Scale Visualization of Competing Polar Orders in Dion–Jacobson Layered Perovskites

    Chemistry of Materials · 2026-04-21

    Shu Morita, Keita Nishibashi, Keito Niwa, Makoto Kobayashi, Eisuke Yamamoto, Rubén Cantón-Vitoria, Daisuke Urushihara, Toru Asaka, Hidetaka Kasai, Shigeo Mori, Minoru Osada

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  31. 2D dielectrics and ferroelectrics: emerging materials, physics and design principles

    Applied Physics Express · 2026-06-11

    Minoru Osada

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  32. Redox-Neutral Interstitial Hydride Incorporation in Ruddlesden–Popper Oxides

    Inorganic Chemistry · 2026-06-23

    Daichi Kato, Shuhei Ueda, Tong Zhu, Hiroki Ubukata, Hikaru Takeuchi, Takashi Honda, Yusuke Nambu, Tatsuya Tsumori, Kotaro Nakai, Cédric Tassel, Itaru Oikawa, Hitoshi Takamura, Teruki Motohashi, Miwa Saito, Yusuke Asai, Ryotaro Aso, Koji Fujita, Hiroshi Kageyama

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  33. Record‐Low Coercive Field and Stable Curie Temperature in Bulk Hybrid Improper Ferroelectrics via Synergistic A / B ‐Site Co‐Substitution

    Advanced Functional Materials · 2026-08-11

    Zhe Guo, Jia Ling Li, Jia Min Lin, Tulai Sun, Yu Huang, Xiao Li Zhu, Xiao Qiang Liu, Xiang Ming Chen

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  34. Hybrid improper ferroelectricity and enhanced Curie temperature in co-substituted La2SrSc2O7-based ceramics

    Journal of Applied Physics · 2026-09-01

    Wei Yi Huang, Zheng Duan Zhang, Zhe Guo, Shu Ya Wu, Xiao Qiang Liu, Xiang Ming Chen

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