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RESEARCH PAPER · Chemistry of Materials · 2019

Competing Polar and Antipolar Structures in the Ruddlesden–Popper Layered Perovskite Li2SrNb2O7

Ritesh Uppuluri, Hirofumi Akamatsu, Arnab Sen Gupta, Huaiyu Hugo Wang, Craig M. Brown, Kleyser Agueda Lopez, Nasim Alem, Venkatraman Gopalan, Thomas E. Mallouk

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Competing Polar and Antipolar Structures in the Ruddlesden–Popper Layered Perovskite Li2SrNb2O7OriginalWeak Ferroelectricity in n = 2 Pseudo Ruddlesden–Popper-Type Niobate Li2SrNb2O736Phase Transition from Weak Ferroelectricity to Incipient Ferroelectricity in Li 2 Sr(Nb 1– x Ta x ) 2 O 728Enhanced hybrid improper ferroelectricity in Sr3−xBaxSn2O7 ceramics with a Ruddlesden–Popper (R–P) structure31Room-temperature ferroelectricity in A-site ordered Ruddlesden-Popper Li2CaTa2O7 ceramics21Highly Tunable Ferroelectricity in Hybrid Improper Ferroelectric Sr3Sn2O740Hybrid improper antiferroelectricity—New insights for novel device concepts2Hybrid improper ferroelectricity in A-site cation ordered Li2La2Ti3O10 ceramic with triple-layer Ruddlesden–Popper structure13Coexisting Mechanisms for the Ferroelectric Phase Transition in Li2SrNb2O721Switching between Proper and Hybrid-Improper Polar Structures via Cation Substitution in A2La(TaTi)O7(A = Li, Na)17Cooperative Cluster Jahn-Teller Effect as a Possible Route to Antiferroelectricity23Revealing pressure-driven structural transitions in the hybrid improper ferroelectric Sr 3 Sn 2 O 714Octahedral rotations in Ruddlesden-Popper layered oxides under pressure from first principles11Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides36B-Site octahedral bridge and A-site polyvalent Cu cation related electron hopping in LiCuNb 3 O 9 -based colossal permittivity materials8Hybrid Improper Ferroelectricity in Highly Cleavable Single Crystals of Dion‐Jacobson‐Compound CsBiNb2O76Phase variation of ferroelectric Li2Sr1−xCax(Nb1−xTax)2O7 by selective reinforcement in the (Nb,Ta)-O covalent bonds10Layered Perovskite Lithium Yttrium Titanate as a Low‐Potential and Ultrahigh‐Rate Anode for Lithium‐Ion Batteries46Symmetry of antiferroelectric crystals crystallized in polar point groups1Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective45Multifunctionality of Li2SrNb2O7: Memristivity, Tunable Rectification, Ferroelasticity, and Ferroelectricity24Chemical Trends of Surface Reconstruction and Band Positions of Nonmetallic Perovskite Oxides from First Principles19Hybrid improper ferroelectricity and phase transition behavior of Li2Nd2Ti3O10 ceramics with A-site ordered triple-layer Ruddlesden-Popper structure6Scaling behavior of order parameters for the hybrid improper ferroelectric (Ca,Sr)3Ti2O75Leakage current characteristics of epitaxial Bi5Ti3FeO15 thin films affected by distribution of 90° domain walls with high conductivity2Leakage current characteristics affected by crystallinity and domain wall current of epitaxial Bi5Ti3FeO15 thin films1Out-of-plane ferroelectricity and robust magnetoelectricity in quasi-two-dimensional materials15Competing polar and antipolar phases in n=2 Ruddlesden-Popper niobates and tantalates from first principles6Polymorphism in the Ruddlesden–Popper Nickelate La 3 Ni 2 O 7 : Discovery of a Hidden Phase with Distinctive Layer Stacking123Magnetoelectric coupling in the multiferroic hybrid-improper ferroelectric Ca3Mn1.9Ti0.1O710Accelerating ferroelectric materials discovery through high-throughput first-principles screening and experimental validation3Piezoelectricity in n = 2 Ruddlesden–Popper Ferroelectric Oxides9Theoretical and data-driven approaches to semiconductors and dielectrics: from prediction to experiment2Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O74Recent Progress of Hybrid Improper Ferroelectrics with Ruddlesden-Popper Structure1The role of urban food street stakeholders in sustainable tourism: Case study of Bangkok, Thailand5Electric-Field-Induced Increase in Permittivity in Uniaxial Antiferroelectric K 3 Nb 3 B 2 O 12 Polycrystalline Ceramics0Crystal structures, dielectric properties, and thermal behavior in hybrid improper ferroelectric Li2Sm2Ti3O10 ceramics0Revival of Layered Ferroelectrics in Thin Films2Hybrid improper ferroelectricity and complex phase evolution in Eu2SrSc2O7 ceramics1Antiferroelectric Phase Transition in Titanite-Type Solid Solutions Na(Nb,Ta)GeO50

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  1. Weak Ferroelectricity in n = 2 Pseudo Ruddlesden–Popper-Type Niobate Li2SrNb2O7

    Chemistry of Materials · 2019-07-26

    Takayuki Nagai, Hirokazu Shirakuni, Akitoshi Nakano, Hiroshi Sawa, Hiroki Moriwake, Ichiro Terasaki, Hiroki Taniguchi

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  2. Phase Transition from Weak Ferroelectricity to Incipient Ferroelectricity in Li 2 Sr(Nb 1– x Ta x ) 2 O 7

    Chemistry of Materials · 2020-01-06

    Takayuki Nagai, Yasuhide Mochizuki, Hirokazu Shirakuni, Akitoshi Nakano, Fumiyasu Oba, Ichiro Terasaki, Hiroki Taniguchi

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  3. Enhanced hybrid improper ferroelectricity in Sr3−xBaxSn2O7 ceramics with a Ruddlesden–Popper (R–P) structure

    Applied Physics Letters · 2020-01-27

    Bu Hang Chen, Tulai Sun, Xiao Qiang Liu, Xiao Li Zhu, He Tian, Xiang Ming Chen

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  4. Room-temperature ferroelectricity in A-site ordered Ruddlesden-Popper Li2CaTa2O7 ceramics

    Journal of Materiomics · 2020-05-03

    B.H. Zhang, Zhiming Hu, B.H. Chen, Xiao Qiang Liu, X.M. Chen

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  5. Highly Tunable Ferroelectricity in Hybrid Improper Ferroelectric Sr3Sn2O7

    Advanced Functional Materials · 2020-08-19

    Xianghan Xu, Yazhong Wang, Fei‐Ting Huang, Kai Du, Elizabeth Nowadnick, Sang‐Wook Cheong

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  6. Hybrid improper antiferroelectricity—New insights for novel device concepts

    MRS Advances · 2020-12-01

    Xue‐Zeng Lu, James M. Rondinelli

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  7. Hybrid improper ferroelectricity in A-site cation ordered Li2La2Ti3O10 ceramic with triple-layer Ruddlesden–Popper structure

    Applied Physics Letters · 2021-02-01

    Bi Hui Zhang, Diming Xu, Bu Hang Chen, Xiao Qiang Liu, James Hester, Xiang Ming Chen

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  8. Coexisting Mechanisms for the Ferroelectric Phase Transition in Li2SrNb2O7

    Chemistry of Materials · 2021-02-09

    Yasuhide Mochizuki, Takayuki Nagai, Hirokazu Shirakuni, Akitoshi Nakano, Fumiyasu Oba, Ichiro Terasaki, Hiroki Taniguchi

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  9. Switching between Proper and Hybrid-Improper Polar Structures via Cation Substitution in A2La(TaTi)O7(A = Li, Na)

    Chemistry of Materials · 2021-03-31

    Subhadip Mallick, Andrew Dominic Fortes, Weiguo Zhang, P. Shiv Halasyamani, Michael A. Hayward

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  10. Cooperative Cluster Jahn-Teller Effect as a Possible Route to Antiferroelectricity

    Physical Review Letters · 2021-05-04

    K. Geirhos, Jan Langmann, L. Prodan, Alexander A. Tsirlin, Aleksandr Missiul, Georg Eickerling, Anton Jesche, V. Tsurkan, P. Lunkenheimer, Wolfgang Scherer, I. Kézsmárki

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  11. Revealing pressure-driven structural transitions in the hybrid improper ferroelectric Sr 3 Sn 2 O 7

    Physical review. B./Physical review. B · 2021-08-12

    Kevin A. Smith, Sriram Poyyapakkam Ramkumar, Nathan C. Harms, Amanda Clune, Xianghan Xu, Sang‐Wook Cheong, Zhenxian Liu, Elizabeth Nowadnick, Janice L. Musfeldt

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  12. Octahedral rotations in Ruddlesden-Popper layered oxides under pressure from first principles

    Physical review. B./Physical review. B · 2021-10-12

    Sriram Poyyapakkam Ramkumar, Elizabeth Nowadnick

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  13. Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides

    Journal of Physics D Applied Physics · 2021-10-22

    Bi Hui Zhang, Xiao Qiang Liu, Xiang Ming Chen

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  14. B-Site octahedral bridge and A-site polyvalent Cu cation related electron hopping in LiCuNb 3 O 9 -based colossal permittivity materials

    Journal of Materials Chemistry C · 2021-12-03

    Dandan Gao, Jiyang Xie, Jian Wang, Wanbiao Hu

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  15. Hybrid Improper Ferroelectricity in Highly Cleavable Single Crystals of Dion‐Jacobson‐Compound CsBiNb2O7

    Advanced Electronic Materials · 2021-12-29

    Xiaochen Fang, Rongwei Hu, Yazhong Wang, Fei‐Ting Huang, Sang‐Wook Cheong

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  16. Phase variation of ferroelectric Li2Sr1−xCax(Nb1−xTax)2O7 by selective reinforcement in the (Nb,Ta)-O covalent bonds

    Physical Review Materials · 2022-04-25

    Akitoshi Nakano, Hirokazu Shirakuni, Takayuki Nagai, Yasuhide Mochizuki, Fumiyasu Oba, Hiroko Yokota, Shogo Kawaguchi, Ichiro Terasaki, Hiroki Taniguchi

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  17. Layered Perovskite Lithium Yttrium Titanate as a Low‐Potential and Ultrahigh‐Rate Anode for Lithium‐Ion Batteries

    Advanced Energy Materials · 2022-06-11

    Yun Zhang, Jun Huang, Nagahiro Saito, Xiaolong Yang, Zhengxi Zhang, Li Yang, Shin‐ichi Hirano

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  18. Symmetry of antiferroelectric crystals crystallized in polar point groups

    IUCrJ · 2022-06-27

    Pai Shan, Xifa Long

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  19. Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective

    Annual Review of Materials Research · 2022-07-01

    Nicole A. Benedek, Michael A. Hayward

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  20. Multifunctionality of Li2SrNb2O7: Memristivity, Tunable Rectification, Ferroelasticity, and Ferroelectricity

    Advanced Materials · 2022-09-04

    Xianghan Xu, Fei‐Ting Huang, Kai Du, Sang‐Wook Cheong

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  21. Chemical Trends of Surface Reconstruction and Band Positions of Nonmetallic Perovskite Oxides from First Principles

    Chemistry of Materials · 2023-02-21

    Yasuhide Mochizuki, Ha‐Jun Sung, Tomoya Gake, Fumiyasu Oba

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  22. Hybrid improper ferroelectricity and phase transition behavior of Li2Nd2Ti3O10 ceramics with A-site ordered triple-layer Ruddlesden-Popper structure

    Journal of Materiomics · 2023-05-29

    Bi Hui Zhang, Diming Xu, Rui Ze Guo, Lu Liu, Xiao Qiang Liu, Xiang Ming Chen

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  23. Scaling behavior of order parameters for the hybrid improper ferroelectric (Ca,Sr)3Ti2O7

    Physical review. B./Physical review. B · 2023-06-08

    Jing Kong, Alicia Maria Manjón-Sanz, Jue Liu, Frederick P. Marlton, Tsz Wing Lo, Dangyuan Lei, Mads R. V. Jørgensen, Abhijit Pramanick

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  24. Leakage current characteristics of epitaxial Bi5Ti3FeO15 thin films affected by distribution of 90° domain walls with high conductivity

    Journal of Alloys and Compounds · 2023-09-11

    Eunmi Lee, Jong Yeog Son

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  25. Leakage current characteristics affected by crystallinity and domain wall current of epitaxial Bi5Ti3FeO15 thin films

    Journal of Applied Physics · 2023-11-08

    Hyun Wook Shin, Jong Yeog Son

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  26. Out-of-plane ferroelectricity and robust magnetoelectricity in quasi-two-dimensional materials

    Science Advances · 2023-11-22

    Xue‐Zeng Lu, Hui-Min Zhang, Ying Zhou, Tong Zhu, Hongjun Xiang, Shuai Dong, Hiroshi Kageyama, James M. Rondinelli

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  27. Competing polar and antipolar phases in n=2 Ruddlesden-Popper niobates and tantalates from first principles

    Physical Review Materials · 2023-12-07

    Kishwar-E Hasin, Elizabeth Nowadnick

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  28. Polymorphism in the Ruddlesden–Popper Nickelate La 3 Ni 2 O 7 : Discovery of a Hidden Phase with Distinctive Layer Stacking

    Journal of the American Chemical Society · 2024-01-31

    Xinglong Chen, Junjie Zhang, Arashdeep Singh Thind, Shekhar Sharma, Harrison LaBollita, Gordon G. C. Peterson, Hong Zheng, Daniel Phelan, Antía S. Botana, Robert F. Klie, John F. Mitchell

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  29. Magnetoelectric coupling in the multiferroic hybrid-improper ferroelectric Ca3Mn1.9Ti0.1O7

    Physical review. B./Physical review. B · 2024-05-08

    Yannik Zemp, Morgan Trassin, Elzbieta Gradauskaite, Bin Gao, Sang‐Wook Cheong, Th. Lottermoser, M. Fiebig, Mads Christof Weber

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  30. Accelerating ferroelectric materials discovery through high-throughput first-principles screening and experimental validation

    Japanese Journal of Applied Physics · 2024-07-01

    Daisuke Hirai, Tomoki Murata, Sakyo Hirose

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  31. Piezoelectricity in n = 2 Ruddlesden–Popper Ferroelectric Oxides

    Chemistry of Materials · 2024-08-02

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  32. Theoretical and data-driven approaches to semiconductors and dielectrics: from prediction to experiment

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  33. Suppression of Ferroelectric Transitions by Symmetry Trapping in Dion–Jacobson-Layered Perovskites Cs(La,Nd)Nb2O7

    Inorganic Chemistry · 2024-11-27

    Zhen‐Tao Lu, Kai Nishioka, Yang Zhang, Koji Fujita, Katsuro Hayashi, Hirofumi Akamatsu

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  34. Recent Progress of Hybrid Improper Ferroelectrics with Ruddlesden-Popper Structure

    Journal of Inorganic Materials · 2025-01-01

    ZHANG Bihui, Liu Xiaoqiang, Xiangming Chen

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  35. The role of urban food street stakeholders in sustainable tourism: Case study of Bangkok, Thailand

    International Journal of ADVANCED AND APPLIED SCIENCES · 2025-01-01

    Phusit Phukamchanoad

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  36. Electric-Field-Induced Increase in Permittivity in Uniaxial Antiferroelectric K 3 Nb 3 B 2 O 12 Polycrystalline Ceramics

    Inorganic Chemistry · 2025-11-26

    Toshiya Uohashi, Yoshinobu Hirose, Koji Maruyama, Hiroki Takeuchi, Hiroki Taniguchi

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  37. Crystal structures, dielectric properties, and thermal behavior in hybrid improper ferroelectric Li2Sm2Ti3O10 ceramics

    SSRN Electronic Journal · 2026-01-01

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  38. Revival of Layered Ferroelectrics in Thin Films

    Small Science · 2026-01-01

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  39. Hybrid improper ferroelectricity and complex phase evolution in Eu2SrSc2O7 ceramics

    Applied Physics Letters · 2026-07-06

    Cang Huan Ye, Zhe Guo, Zheng Duan Zhang, Xiao Qiang Liu, Z.V. Gareeva, Xiang Ming Chen

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  40. Antiferroelectric Phase Transition in Titanite-Type Solid Solutions Na(Nb,Ta)GeO5

    Inorganic Chemistry · 2026-08-26

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