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RESEARCH PAPER · Inorganic Chemistry Frontiers · 2017

A series of pentanary inorganic supramolecular sulfides (A 3 X)[MB 12 (MS 4 ) 3 ] (A = K, Cs; X = Cl, Br, I; M = Ga, In, Gd) featuring B 12 S 12 clusters

Zongdong Sun, Yang Chi, Huaiguo Xue, Sheng‐Ping Guo

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A series of pentanary inorganic supramolecular sulfides (A 3 X)[MB 12 (MS 4 ) 3 ] (A = K, Cs; X = Cl, Br, I; M = Ga, In, Gd) featuring B 12 S 12 clustersOriginalNa 6 Zn 3 MIII2Q 9 (M III = Ga, In; Q = S, Se): four new supertetrahedron-layered chalcogenides with unprecedented vertex-sharing T 3 -clusters and desirable photoluminescence performances31The first investigation of europium silicate melilite for second-order nonlinear optical application: experimental and theoretical studies29SnI 4 ⋅(S 8 ) 2 : A Novel Adduct‐Type Infrared Second‐Order Nonlinear Optical Crystal184SnI4⋅(S8)2: A Novel Adduct‐Type Infrared Second‐Order Nonlinear Optical Crystal45K 3 Bi 2 Cl 5 O 2 (SO 4 ) 2 : A Novel Pentanary Chloride Oxide Sulfate4Adduct-Type IR Nonlinear-Optical Crystal SbI 3 ·(S 8 ) 3 with a Large Second-Harmonic Generation and a High Laser-Induced Damage Threshold59Second-order nonlinear optical properties of CuGa In1-Se2 (x = 0.54): Experimental and theoretical investigations4An unprecedented pentanary chalcohalide with Mn atoms in two chemical environments: unique bonding characteristics and magnetic properties29Combined experimental and theoretical investigations of Ba 3 GaS 4 I: interesting structural transformation originated from halogen substitution16Transition Metal Free Monoclinic Eu8In17.33S34 and Its Anisotropic Photoelectronic Responses25Mixed-Anion Inorganic Compounds: A Favorable Candidate for Infrared Nonlinear Optical Materials140Partial Congener Substitution Induced Centrosymmetric to Noncentrosymmetric Transformation Witnessed by K3Ga3(Ge7–xMx)Se20 (M = Si, Sn) and Their Nonlinear Optical Properties51Rational design of infrared nonlinear optical chalcogenides by chemical substitution287Salt-inclusion chalcogenides: an emerging class of IR nonlinear optical materials54(Na0.60Ba0.70)Ga2Se4: An Infrared Nonlinear Optical Crystal Designed using AgGaSe2 as the Template38Hexagonal In2Se3: A Defect Wurtzite-Type Infrared Nonlinear Optical Material with Moderate Birefringence Contributed by Unique InSe5 Unit75KInSi1.32Sn0.68Se6: An Infrared Nonlinear Optical Material Containing Three Types of Tetrahedral Units19Second-order nonlinear optical-active selenide borate Zn8Se2(BO2)12: Experimental and theoretical analysis9Salt-Inclusion Chalcogenide [Ba4Cl2][ZnGa4S10]: Rational Design of an IR Nonlinear Optical Material with Superior Comprehensive Performance Derived from AgGaS2134Recent Achievements in Lone-Pair Cation-Based Infrared Second-Order Nonlinear Optical Materials95Synergism of multiple functional chromophores significantly enhancing the birefringence in layered non-centrosymmetric chalcohalides20From thiophosphate to chalcohalide: mixed-anion AgS x Cl y ligands concurrently enhancing nonlinear optical effects and laser-damage threshold10M 6 PS 5 X (M = Ag, Cu; X = Cl, Br) chalcohalides exhibiting strong nonlinear optical responses and high laser damage resistances9A Series of Pentanary Salt-Inclusion Chalcogenoborates Containing a B12Q12 (Q = S, Se) Cluster Exhibiting a Kleinman-Forbidden Frequency-Doubling Effect25Ternary rare-earth sulfides RE3GaS6 (RE = Ho, Er): Crystal chemistry, second-order nonlinear optical properties and theoretical investigation18Sn4−δB12Se12[Qx], Q = Se, Te, a B12 Cluster Tunnel Framework Hosting Neutral Chalcogen Chains8Cd3(PO4)(TePO6): A Novel Cadmium Tellurite‐Phosphate featuring a {[TePO6]3−}∞ Chain15Superior Infrared Nonlinear Optical Performance Achieved by Synergetic Functional Motif and Vacancy Site Modulations48AIn 4 S 6 Cl (A = Rb and Cs) and Pb 5 Sn 3 Q 10 Cl 2 (Q = S and Se): quaternary chalcohalides with mixed anionic coordination exhibit photocurrent responses11From oxides to oxysulfides: the mixed-anion GeS 3 O unit induces huge improvement in the nonlinear optical effect and optical anisotropy for potential nonlinear optical materials19KEu 2 In 3 B 12 S 13 : a novel type of thioborate featuring B 12 S 12 cluster and unique In 6 S 6 12-membered ring10KNa 0.78 Eu 0.27 In 3.80 B 12 S 12 : a novel hexanary thioborate featuring a B 12 S 12 cluster and diverse InS x ( x = 4, 5, 6) units9The synthesis and structure–property relation analysis of metal chalcohalide crystals Cs 2 InPS 4 X 2 (X = Cl, Br) with mixed anions6A new salt-inclusion chalcogenide exhibiting distinctive [Cd11In9S26]3− host framework and decent nonlinear optical performances16A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications115Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials28Molecular boron clusters2Syntheses, structures, and characterization of new heteroanionic chalcohalides: Na2Ba17In8Q21F18 (Q = S, Se), KBa2InQ3F2 (Q = S, Se)5Breaking the bottleneck of simultaneously wide band gap and large nonlinear optical coefficient by a “pore reconstruction” strategy in a salt-inclusion chalcogenide26SbI3·3S8: A Novel Promising Inorganic Adducts Crystal for Second Harmonic Generation5Salt-inclusion chalcogenides: Double functional moieties design strategy toward excellent nonlinear optical materials12[K2PbX][Ga7S12] (X = Cl, Br, I): The First Lead‐Containing Cationic Moieties with Ultrahigh Second‐Harmonic Generation and Band Gaps Exceeding the Criterion of 2.33 eV46A series of new rare-earth sulfide borates RE3S3BO3 (RE = Nd, Tb, Dy): Syntheses, structures and optical properties1Excellent Nonlinear Optical M[M4Cl][Ga11S20] (M = A/Ba, A = K, Rb) Achieved by Unusual Cationic Substitution Strategy20Rare-earth-based chalcogenides and their derivatives: an encouraging IR nonlinear optical material candidate70Nonlinear Optical Effects in Europium Melilite Eu2MgSi2O70[Cs14Cl][Tm71Se110]: An unusual salt-inclusion chalcogenide containing different valent Tm centers and ultralow thermal conductivity10Diamond-Like HgIn2Q4 (Q = Se, Te) Synthesized by Flux-Assisted Boron-Chalcogen Method Exhibit Noteworthy Nonlinear Optical Properties Contributed by Three Types of Tetrahedral Motifs9Introduction of Diverse Divalent Main-Group Metal Cations to Tune the Physical Properties of Rare-Earth Thiophosphates7Alkali Metal Substitution-Induced Structural Transformation for RbREP2Se6 (RE = Gd, Tb, Dy) with Second-Harmonic Generation Responses6Doubling Polarizability Anisotropy of The Tetrahedral Motifs to Achieve Phase Matching for Melilite-Type Compound2Ba 10 Zn 7 Ga 6 S 26 : Promising Infrared Nonlinear Optical Crystal Exhibiting a High Laser Damage Threshold0Reactive flux assisted metal oxide–boron–sulfur routine for syntheses of CsRESiS 4 (RE = Sm, Gd–Ho): featuring nonlinear optical activity and wide band gaps5ANb 2 (PS 4 )(S 2 ) 3 (A = K, Rb, Cs): the first Nb-based NLO thiophosphates with [NbS 2 (S 2 ) 3 ] and [Nb 2 PS 6 (S 2 ) 4 ] units exhibiting tri-state structural transformation and high performance6

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  1. Na 6 Zn 3 MIII2Q 9 (M III = Ga, In; Q = S, Se): four new supertetrahedron-layered chalcogenides with unprecedented vertex-sharing T 3 -clusters and desirable photoluminescence performances

    Inorganic Chemistry Frontiers · 2018-01-01

    Ailijiang Abudurusuli, Kui Wu, Yilimiranmu Rouzhahong, Zhihua Yang, Shilie Pan

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  2. The first investigation of europium silicate melilite for second-order nonlinear optical application: experimental and theoretical studies

    Dalton Transactions · 2018-01-01

    Yang Chi, Huaiguo Xue, Sheng‐Ping Guo

    Read original paper ↗ ·

  3. SnI 4 ⋅(S 8 ) 2 : A Novel Adduct‐Type Infrared Second‐Order Nonlinear Optical Crystal

    Angewandte Chemie International Edition · 2018-05-06

    Sheng‐Ping Guo, Yang Chi, Huaiguo Xue

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  4. SnI4⋅(S8)2: A Novel Adduct‐Type Infrared Second‐Order Nonlinear Optical Crystal

    Angewandte Chemie · 2018-05-07

    Sheng‐Ping Guo, Yang Chi, Huaiguo Xue

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  5. K 3 Bi 2 Cl 5 O 2 (SO 4 ) 2 : A Novel Pentanary Chloride Oxide Sulfate

    ChemistrySelect · 2018-07-10

    Zhen‐Tao Lu, Yang Chi, Huaiguo Xue, Sheng‐Ping Guo

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  6. Adduct-Type IR Nonlinear-Optical Crystal SbI 3 ·(S 8 ) 3 with a Large Second-Harmonic Generation and a High Laser-Induced Damage Threshold

    Inorganic Chemistry · 2018-08-23

    Sheng‐Ping Guo, Zongdong Sun, Yang Chi, Huaiguo Xue

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  7. Second-order nonlinear optical properties of CuGa In1-Se2 (x = 0.54): Experimental and theoretical investigations

    Solid State Sciences · 2018-09-07

    Zongdong Sun, Yang Chi, Sheng‐Ping Guo

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  8. An unprecedented pentanary chalcohalide with Mn atoms in two chemical environments: unique bonding characteristics and magnetic properties

    Chemical Communications · 2018-11-28

    Yujun Zheng, Yong‐Fang Shi, Chong‐Bin Tian, Hua Lin, Li‐Ming Wu, Xin‐Tao Wu, Qi‐Long Zhu

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  9. Combined experimental and theoretical investigations of Ba 3 GaS 4 I: interesting structural transformation originated from halogen substitution

    Dalton Transactions · 2019-01-01

    Mengyue Li, Yu‐Xiao Zhang, Hua Lin, Zuju Ma, Xin‐Tao Wu, Qi‐Long Zhu

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  10. Transition Metal Free Monoclinic Eu8In17.33S34 and Its Anisotropic Photoelectronic Responses

    Inorganic Chemistry · 2019-03-01

    Yang Chi, Tengfei Jiang, Huaiguo Xue, Sheng‐Ping Guo

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  11. Mixed-Anion Inorganic Compounds: A Favorable Candidate for Infrared Nonlinear Optical Materials

    Crystal Growth & Design · 2019-06-07

    Yanyan Li, Wenjing Wang, Hui Wang, Hua Lin, Li‐Ming Wu

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  12. Partial Congener Substitution Induced Centrosymmetric to Noncentrosymmetric Transformation Witnessed by K3Ga3(Ge7–xMx)Se20 (M = Si, Sn) and Their Nonlinear Optical Properties

    Inorganic Chemistry · 2019-09-25

    Xiaohui Li, Nian‐Tzu Suen, Yang Chi, Yueling Sun, Anhua Gong, Huaiguo Xue, Sheng‐Ping Guo

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  13. Rational design of infrared nonlinear optical chalcogenides by chemical substitution

    Coordination Chemistry Reviews · 2019-12-21

    Hua Lin, Wenbo Wei, Hong Chen, Xintao Wu, Qi‐Long Zhu

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  14. Salt-inclusion chalcogenides: an emerging class of IR nonlinear optical materials

    Dalton Transactions · 2020-01-01

    Qing-Gang Yue, Wenbo Wei, Hong Chen, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  15. (Na0.60Ba0.70)Ga2Se4: An Infrared Nonlinear Optical Crystal Designed using AgGaSe2 as the Template

    Inorganic Chemistry · 2020-03-03

    Yanan Li, Huaiguo Xue, Sheng‐Ping Guo

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  16. Hexagonal In2Se3: A Defect Wurtzite-Type Infrared Nonlinear Optical Material with Moderate Birefringence Contributed by Unique InSe5 Unit

    ACS Applied Materials & Interfaces · 2020-03-30

    Yang Chi, Zongdong Sun, Qian-Ting Xu, Huaiguo Xue, Sheng‐Ping Guo

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  17. KInSi1.32Sn0.68Se6: An Infrared Nonlinear Optical Material Containing Three Types of Tetrahedral Units

    Inorganic Chemistry · 2020-04-21

    Xiaohui Li, Yi-Ting Chen, Huaiguo Xue, Sheng‐Ping Guo

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  18. Second-order nonlinear optical-active selenide borate Zn8Se2(BO2)12: Experimental and theoretical analysis

    Journal of Solid State Chemistry · 2020-07-18

    Wenfeng Zhou, Xiaohui Li, Wen‐Dong Yao, Huaiguo Xue, Sheng‐Ping Guo

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  19. Salt-Inclusion Chalcogenide [Ba4Cl2][ZnGa4S10]: Rational Design of an IR Nonlinear Optical Material with Superior Comprehensive Performance Derived from AgGaS2

    Chemistry of Materials · 2020-08-14

    Hong Chen, Yanyan Li, Bingxuan Li, Pengfei Liu, Hua Lin, Qi‐Long Zhu, Xintao Wu

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  20. Recent Achievements in Lone-Pair Cation-Based Infrared Second-Order Nonlinear Optical Materials

    Crystal Growth & Design · 2020-12-22

    Mei Yan, Huaiguo Xue, Sheng‐Ping Guo

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  21. Synergism of multiple functional chromophores significantly enhancing the birefringence in layered non-centrosymmetric chalcohalides

    Inorganic Chemistry Frontiers · 2020-12-23

    Junben Huang, Jianian Cheng, Bing‐Hua Lei, Zhonglei Wei, Shilie Pan, Zhihua Yang

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  22. From thiophosphate to chalcohalide: mixed-anion AgS x Cl y ligands concurrently enhancing nonlinear optical effects and laser-damage threshold

    Chemical Communications · 2021-01-01

    Lihua Gao, Yu Chu, Xiaowen Wu, Bingbing Zhang, Kui Wu

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  23. M 6 PS 5 X (M = Ag, Cu; X = Cl, Br) chalcohalides exhibiting strong nonlinear optical responses and high laser damage resistances

    Dalton Transactions · 2021-01-01

    Lihua Gao, Xiaowen Wu, Daqing Yang, Xinyu Tian, Jingjing Xu, Bingbing Zhang, Kui Wu

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  24. A Series of Pentanary Salt-Inclusion Chalcogenoborates Containing a B12Q12 (Q = S, Se) Cluster Exhibiting a Kleinman-Forbidden Frequency-Doubling Effect

    Inorganic Chemistry · 2021-02-09

    Shanshan Han, Wen‐Dong Yao, Su‐Xin Yu, Yueling Sun, Anhua Gong, Sheng‐Ping Guo

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  25. Ternary rare-earth sulfides RE3GaS6 (RE = Ho, Er): Crystal chemistry, second-order nonlinear optical properties and theoretical investigation

    Journal of Alloys and Compounds · 2021-02-15

    Hao-Yu Chen, Yingying Zhang, Yifan Yang, Sheng‐Ping Guo

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  26. Sn4−δB12Se12[Qx], Q = Se, Te, a B12 Cluster Tunnel Framework Hosting Neutral Chalcogen Chains

    Chemistry of Materials · 2021-02-25

    Daniel G. Chica, Ioannis Spanopoulos, Shiqiang Hao, Chris M. Wolverton, Mercouri G. Kanatzidis

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  27. Cd3(PO4)(TePO6): A Novel Cadmium Tellurite‐Phosphate featuring a {[TePO6]3−}∞ Chain

    European Journal of Inorganic Chemistry · 2021-10-12

    Wen‐Dong Yao, Mei Yan, Xiaohui Li, Wenlong Liu, Ru‐Ling Tang

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  28. Superior Infrared Nonlinear Optical Performance Achieved by Synergetic Functional Motif and Vacancy Site Modulations

    Chemistry of Materials · 2021-11-03

    Shao‐Min Pei, Bin‐Wen Liu, Xiao‐Ming Jiang, Ya-Qian Zou, Wen‐Fa Chen, Qiu-Nan Yan, Guo‐Cong Guo

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  29. AIn 4 S 6 Cl (A = Rb and Cs) and Pb 5 Sn 3 Q 10 Cl 2 (Q = S and Se): quaternary chalcohalides with mixed anionic coordination exhibit photocurrent responses

    Dalton Transactions · 2022-01-01

    Lin‐Tao Jiang, Mingze Li, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  30. From oxides to oxysulfides: the mixed-anion GeS 3 O unit induces huge improvement in the nonlinear optical effect and optical anisotropy for potential nonlinear optical materials

    RSC Advances · 2022-01-01

    Xinyu Tian, Xiaodong Zhang, Yan Xiao, Xiaowen Wu, Bingbing Zhang, Daqing Yang, Kui Wu

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  31. KEu 2 In 3 B 12 S 13 : a novel type of thioborate featuring B 12 S 12 cluster and unique In 6 S 6 12-membered ring

    Dalton Transactions · 2022-01-01

    Shanshan Han, Qian-Ting Xu, Wenlong Liu, Sheng‐Ping Guo

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  32. KNa 0.78 Eu 0.27 In 3.80 B 12 S 12 : a novel hexanary thioborate featuring a B 12 S 12 cluster and diverse InS x ( x = 4, 5, 6) units

    Inorganic Chemistry Frontiers · 2022-01-01

    Shanshan Han, Su‐Xin Yu, Wenlong Liu, Sheng‐Ping Guo

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  33. The synthesis and structure–property relation analysis of metal chalcohalide crystals Cs 2 InPS 4 X 2 (X = Cl, Br) with mixed anions

    Dalton Transactions · 2022-01-01

    Chunlan Tang, Wenhao Xing, Naizheng Wang, Jian Tang, Zheshuai Lin, Jieyun Wu, Wenlong Yin, Bin Kang

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  34. A new salt-inclusion chalcogenide exhibiting distinctive [Cd11In9S26]3− host framework and decent nonlinear optical performances

    Journal of Alloys and Compounds · 2022-01-06

    Shao‐Min Pei, Lin‐Tao Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  35. A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications

    Coordination Chemistry Reviews · 2022-07-19

    Hong Chen, Mao‐Yin Ran, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  36. Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials

    European Journal of Inorganic Chemistry · 2022-10-05

    Jun Li, Shanshan Han, Sheng‐Ping Guo

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  37. Molecular boron clusters

    Elsevier eBooks · 2022-10-12

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  38. Syntheses, structures, and characterization of new heteroanionic chalcohalides: Na2Ba17In8Q21F18 (Q = S, Se), KBa2InQ3F2 (Q = S, Se)

    Journal of Alloys and Compounds · 2022-11-22

    Dong Gao, Xiao Ji, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongping Wu

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  39. Breaking the bottleneck of simultaneously wide band gap and large nonlinear optical coefficient by a “pore reconstruction” strategy in a salt-inclusion chalcogenide

    Materials Horizons · 2023-01-01

    Shao‐Min Pei, Bin‐Wen Liu, Wen‐Fa Chen, Xiao‐Ming Jiang, Guo‐Cong Guo

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  40. SbI3·3S8: A Novel Promising Inorganic Adducts Crystal for Second Harmonic Generation

    Materials · 2023-01-27

    Tushar Kanti Das, Marcin Jesionek, Mirosława Kępińska, M. Nowak, Michalina Kotyczka-Morańska, Maciej Zubko, Jarosław Młyńczak, Krzysztof Kopczyński

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  41. Salt-inclusion chalcogenides: Double functional moieties design strategy toward excellent nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-02-07

    Chao-Hong Xie, Bin‐Wen Liu, Guo‐Cong Guo

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  42. [K2PbX][Ga7S12] (X = Cl, Br, I): The First Lead‐Containing Cationic Moieties with Ultrahigh Second‐Harmonic Generation and Band Gaps Exceeding the Criterion of 2.33 eV

    Advanced Science · 2023-02-27

    Wen‐Fa Chen, Bin‐Wen Liu, Shao‐Min Pei, Xiao‐Ming Jiang, Guo‐Cong Guo

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  43. A series of new rare-earth sulfide borates RE3S3BO3 (RE = Nd, Tb, Dy): Syntheses, structures and optical properties

    Journal of Solid State Chemistry · 2023-08-18

    Yun Xie, Da-Li Chen, Yu-Long Wei, Nan Zhang, Wen‐Dong Yao, Sheng‐Ping Guo

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  44. Excellent Nonlinear Optical M[M4Cl][Ga11S20] (M = A/Ba, A = K, Rb) Achieved by Unusual Cationic Substitution Strategy

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  45. Rare-earth-based chalcogenides and their derivatives: an encouraging IR nonlinear optical material candidate

    Chemical Science · 2024-01-01

    Ping Feng, Jiaxiang Zhang, Mao‐Yin Ran, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  46. Nonlinear Optical Effects in Europium Melilite Eu2MgSi2O7

    physica status solidi (b) · 2024-07-08

    K. M. Tsysar, Д. И. Бажанов, Karine Karlenovna Abgaryan, N. N. Kiselyova

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  47. [Cs14Cl][Tm71Se110]: An unusual salt-inclusion chalcogenide containing different valent Tm centers and ultralow thermal conductivity

    Chinese Journal of Structural Chemistry · 2024-07-27

    Hong Chen, Mao‐Yin Ran, Long-Hua Li, Xin‐Tao Wu, Hua Lin

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  48. Diamond-Like HgIn2Q4 (Q = Se, Te) Synthesized by Flux-Assisted Boron-Chalcogen Method Exhibit Noteworthy Nonlinear Optical Properties Contributed by Three Types of Tetrahedral Motifs

    Inorganic Chemistry · 2025-06-24

    Jian Ping Cheng, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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  49. Introduction of Diverse Divalent Main-Group Metal Cations to Tune the Physical Properties of Rare-Earth Thiophosphates

    Inorganic Chemistry · 2025-07-18

    Zi-Nan Chen, Hai-Ping Xu, Wen‐Dong Yao, Mingyang Li, Chen‐Yi Zhao, Wenlong Liu, Sheng‐Ping Guo

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  50. Alkali Metal Substitution-Induced Structural Transformation for RbREP2Se6 (RE = Gd, Tb, Dy) with Second-Harmonic Generation Responses

    Inorganic Chemistry · 2025-08-08

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