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RESEARCH PAPER · Dalton Transactions · 2020

Salt-inclusion chalcogenides: an emerging class of IR nonlinear optical materials

Qing-Gang Yue, Wenbo Wei, Hong Chen, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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Salt-inclusion chalcogenides: an emerging class of IR nonlinear optical materialsOriginalA new type of novel salt-inclusion chalcogenide with ultralow thermal conductivity14[GaF(H 2 O)][IO 3 F]: a promising NLO material obtained by anisotropic polycation substitution42A 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks53Aliovalent-cation-substitution-induced structure transformation: a new path toward high-performance IR nonlinear optical materials47Ba 2 BS 3 Cl and Ba 5 B 2 S 8 Cl 2 : first alkaline-earth metal thioborate halides with [BS 3 ] units21Ba 2 Ge 2 Te 5 : a ternary NLO-active telluride with unusual one-dimensional helical chains and giant second harmonic-generation tensors31Recent progress in oxychalcogenides as IR nonlinear optical materials79A Series of Pentanary Salt-Inclusion Chalcogenoborates Containing a B12Q12 (Q = S, Se) Cluster Exhibiting a Kleinman-Forbidden Frequency-Doubling Effect25Quaternary Chalcohalides CdSnSX2 (X = Cl or Br) with Neutral Layers: Syntheses, Structures, and Photocatalytic Properties18AXHg3P2S8 (A = Rb, Cs; X = Cl, Br): New Excellent Infrared Nonlinear Optical Materials with Mixed‐Anion Chalcohalide Groups of Trigonal Planar [HgS2X]3− and Tetrahedral [HgS3X]5−58AZn4Ga5Se12 (A = K, Rb, or Cs): Infrared Nonlinear Optical Materials with Simultaneous Large Second Harmonic Generation Responses and High Laser-Induced Damage Thresholds34Highly Distorted [HgS 4 ] Motif-Driven Structural Symmetry Degradation and Strengthened Second-Harmonic Generation Response in the Defect Diamond-Like Chalcogenide Hg 3 P 2 S 847Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials184The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks36Superior Infrared Nonlinear Optical Performance Achieved by Synergetic Functional Motif and Vacancy Site Modulations48Synthesis and Characterization of New-Type Ionic Cocrystals with Cyanuric Acid and Alkali Halides: AX·(H3C3N3O3)2 (A = Rb, Cs; X = Cl, Br)6Phase Matchability Transformation in the Infrared Nonlinear Optical Materials with Diamond‐Like Frameworks63[ASr 4 Cl][Ge 3 S 10 ] (A = Na, K) and [KBa 4 Cl][Ge 3 S 10 ]: new salt-inclusion infrared nonlinear optical crystals with zero-dimensional [Ge 3 S 9 ] clusters32Achieving a strong second harmonic generation response and a wide band gap in a Hg-based material41The exploration of new infrared nonlinear optical crystals based on the polymorphism of BaGa 4 S 731A new salt-inclusion chalcogenide exhibiting distinctive [Cd11In9S26]3− host framework and decent nonlinear optical performances16Quaternary Noncentrosymmetric Rare-Earth Sulfides Ba4RE2Cd3S10 (RE = Sm, Gd, or Tb): A Joint Experimental and Theoretical Investigation17From Cc to P 6 3 mc : Structural Variation in La 3 S 2 Cl 2 [SbS 3 ] and La 3 OSCl 2 [SbS 3 ] Induced by the Isovalent Anion Substitution22A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications115Recent developments on Bi-based oxychalcogenide materials with thermoelectric and optoelectronic applications: an overview33[Cs6Cl][Ga5GeQ12] (Q = S, Se): two novel porous layered chalcohalides exhibiting two-band emission and ion exchange properties6The Solvothermal Synthesis and Properties of Thioantimonates Rb(1,4-DABH)Sb4S7 and Cs2ZnSb2S5: 1D Anion Chains and 2D Anion Layer2Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials28Two new gallium(III)-thioantimonates TM(tren)GaSbS4 (TM = Mn, Fe): Syntheses, crystal structure and properties9[Ba 4 X][In 19 S 32 ] (X = Cl, Br): two quaternary metal chalcohalides exhibiting remarkable photocurrent responses1[Sr 4 Cl 2 ][Si 3 S 9 ]: Ultrawide-bandgap salt-inclusion thiosilicate nonlinear optical material with unprecedented tri-polymerized [Si 3 S 9 ] clusters21A non-centrosymmetric chalcohalide synthesized through the combination of chemical tailoring with aliovalent substitution12An overview of Mg-based IR nonlinear optical materials23Flux-assisted polytypism in the [Na 2 Cl]GaQ 2 heterolayered salt-inclusion chalcogenide family3Tunable Salt-Inclusion Chalcogenides for Ion Exchange, Photoluminescence, and Scintillation12Salt-inclusion chalcogenides: Double functional moieties design strategy toward excellent nonlinear optical materials12Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization133Na3SiS3F: A Wide Bandgap Fluorothiosilicate with Unique [SiS3F] Unit and High Laser‐Induced Damage Threshold39Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance57[Ba4(S2)][ZnGa4S10]: Design of an Unprecedented Infrared Nonlinear Salt‐Inclusion Chalcogenide with Disulfide‐Bonds36Advances in Chalcogenide Crystal Growth: Flux and Solution Syntheses, and Approaches for Postsynthetic Modifications13Ga-based IR nonlinear optical materials: Synthesis, structures, and properties65Rare-earth-based chalcogenides and their derivatives: an encouraging IR nonlinear optical material candidate70Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units66[Cs14Cl][Tm71Se110]: An unusual salt-inclusion chalcogenide containing different valent Tm centers and ultralow thermal conductivity103Pb 8 O 7 I 2 ·2CsI: the salt-inclusion strategy enriches the structural chemistry in lead oxyhalides1AgGaS2 and Derivatives: Design, Synthesis, and Optical Properties10Synergistic Machine Learning Guided Discovery of ABa 3 (BSe 3 ) 2 X (A = Rb, Cs; X = Cl, Br, I): A Promising Family as Property‐Balanced IR Functional Materials10First-principles study of ABSe₃ (A = Li, Na) Perselenoborates: A Promising Family of Nonlinear Optical Materials1Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs29[Rb 4 Cl][Cd 11 In 9 Se 26 ]: a salt inclusion chalcogenide with a diamond-like framework for infrared nonlinear optics0Circumventing the Eg–SHG trade-off in selenides: Salt-inclusion [X4Br2][MGa4Se10] with concurrent large band gap and strong nonlinear optical response1Heterovalent Coexistence‐Driven Symmetry Breaking and Dimensional Evolution: Designing Polar Heart‐Shaped Channels for Exceptional MFIR Nonlinear Optics5From AgGaSe2 to MIIGa2Se4 (MII = Zn, Cd): Heterovalent Substitution Creates Ordered Vacancies for Balanced IR-NLO Performance0

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  1. A new type of novel salt-inclusion chalcogenide with ultralow thermal conductivity

    Chemical Communications · 2020-01-01

    Hong Chen, Pengfei Liu, Hua Lin, Xin‐Tao Wu

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  2. [GaF(H 2 O)][IO 3 F]: a promising NLO material obtained by anisotropic polycation substitution

    Chemical Science · 2021-01-01

    Q. Huang, Chun‐Li Hu, Bing‐Ping Yang, Zhi Gang Fang, Yuan Hua Lin, Jin Chen, Bingxuan Li, Jiang‐Gao Mao

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  3. A 3 Mn 2 Sb 3 S 8 (A = K and Rb): a new type of multifunctional infrared nonlinear optical material based on unique three-dimensional open frameworks

    Inorganic Chemistry Frontiers · 2021-01-01

    Yu Xiao, Man-Man Chen, Yaying Shen, Pengfei Liu, Hua Lin, Yi Liu

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  4. Aliovalent-cation-substitution-induced structure transformation: a new path toward high-performance IR nonlinear optical materials

    Journal of Materials Chemistry C · 2021-01-01

    Chang Liu, Shenghua Zhou, Yu Xiao, Chao Zhang, Hua Lin, Yi Liu

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  5. Ba 2 BS 3 Cl and Ba 5 B 2 S 8 Cl 2 : first alkaline-earth metal thioborate halides with [BS 3 ] units

    Chemical Communications · 2021-01-01

    Jiazheng Zhou, Yu Chu, Junjie Li, Shilie Pan

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  6. Ba 2 Ge 2 Te 5 : a ternary NLO-active telluride with unusual one-dimensional helical chains and giant second harmonic-generation tensors

    Inorganic Chemistry Frontiers · 2021-01-01

    Mao‐Yin Ran, Zuju Ma, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  7. Recent progress in oxychalcogenides as IR nonlinear optical materials

    Dalton Transactions · 2021-01-01

    Yang-Fang Shi, Wenbo Wei, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  8. A Series of Pentanary Salt-Inclusion Chalcogenoborates Containing a B12Q12 (Q = S, Se) Cluster Exhibiting a Kleinman-Forbidden Frequency-Doubling Effect

    Inorganic Chemistry · 2021-02-09

    Shanshan Han, Wen‐Dong Yao, Su‐Xin Yu, Yueling Sun, Anhua Gong, Sheng‐Ping Guo

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  9. Quaternary Chalcohalides CdSnSX2 (X = Cl or Br) with Neutral Layers: Syntheses, Structures, and Photocatalytic Properties

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    Mao‐Yin Ran, Shenghua Zhou, Wenbo Wei, Bang-Jun Song, Yong‐Fang Shi, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  10. AXHg3P2S8 (A = Rb, Cs; X = Cl, Br): New Excellent Infrared Nonlinear Optical Materials with Mixed‐Anion Chalcohalide Groups of Trigonal Planar [HgS2X]3− and Tetrahedral [HgS3X]5−

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  11. AZn4Ga5Se12 (A = K, Rb, or Cs): Infrared Nonlinear Optical Materials with Simultaneous Large Second Harmonic Generation Responses and High Laser-Induced Damage Thresholds

    Inorganic Chemistry · 2021-06-17

    Man-Man Chen, Shenghua Zhou, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  12. Highly Distorted [HgS 4 ] Motif-Driven Structural Symmetry Degradation and Strengthened Second-Harmonic Generation Response in the Defect Diamond-Like Chalcogenide Hg 3 P 2 S 8

    ACS Applied Materials & Interfaces · 2021-07-28

    Wenhao Xing, Fei Liang, Chunlan Tang, Ece Uykur, Zheshuai Lin, Jiyong Yao, Wenlong Yin, Bin Kang

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  13. Transition-metal-based chalcogenides: A rich source of infrared nonlinear optical materials

    Coordination Chemistry Reviews · 2021-08-26

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  14. The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks

    Chemistry - An Asian Journal · 2021-09-01

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  15. Superior Infrared Nonlinear Optical Performance Achieved by Synergetic Functional Motif and Vacancy Site Modulations

    Chemistry of Materials · 2021-11-03

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  16. Synthesis and Characterization of New-Type Ionic Cocrystals with Cyanuric Acid and Alkali Halides: AX·(H3C3N3O3)2 (A = Rb, Cs; X = Cl, Br)

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  17. Phase Matchability Transformation in the Infrared Nonlinear Optical Materials with Diamond‐Like Frameworks

    Advanced Optical Materials · 2021-12-30

    Man‐Man Chen, Shenghua Zhou, Wenbo Wei, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  18. [ASr 4 Cl][Ge 3 S 10 ] (A = Na, K) and [KBa 4 Cl][Ge 3 S 10 ]: new salt-inclusion infrared nonlinear optical crystals with zero-dimensional [Ge 3 S 9 ] clusters

    Inorganic Chemistry Frontiers · 2022-01-01

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  19. Achieving a strong second harmonic generation response and a wide band gap in a Hg-based material

    Inorganic Chemistry Frontiers · 2022-01-01

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  20. The exploration of new infrared nonlinear optical crystals based on the polymorphism of BaGa 4 S 7

    Inorganic Chemistry Frontiers · 2022-01-01

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  21. A new salt-inclusion chalcogenide exhibiting distinctive [Cd11In9S26]3− host framework and decent nonlinear optical performances

    Journal of Alloys and Compounds · 2022-01-06

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  22. Quaternary Noncentrosymmetric Rare-Earth Sulfides Ba4RE2Cd3S10 (RE = Sm, Gd, or Tb): A Joint Experimental and Theoretical Investigation

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  23. From Cc to P 6 3 mc : Structural Variation in La 3 S 2 Cl 2 [SbS 3 ] and La 3 OSCl 2 [SbS 3 ] Induced by the Isovalent Anion Substitution

    Crystal Growth & Design · 2022-01-17

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  24. A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications

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  25. Recent developments on Bi-based oxychalcogenide materials with thermoelectric and optoelectronic applications: an overview

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  26. [Cs6Cl][Ga5GeQ12] (Q = S, Se): two novel porous layered chalcohalides exhibiting two-band emission and ion exchange properties

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  27. The Solvothermal Synthesis and Properties of Thioantimonates Rb(1,4-DABH)Sb4S7 and Cs2ZnSb2S5: 1D Anion Chains and 2D Anion Layer

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  28. Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials

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  29. Two new gallium(III)-thioantimonates TM(tren)GaSbS4 (TM = Mn, Fe): Syntheses, crystal structure and properties

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  30. [Ba 4 X][In 19 S 32 ] (X = Cl, Br): two quaternary metal chalcohalides exhibiting remarkable photocurrent responses

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  31. [Sr 4 Cl 2 ][Si 3 S 9 ]: Ultrawide-bandgap salt-inclusion thiosilicate nonlinear optical material with unprecedented tri-polymerized [Si 3 S 9 ] clusters

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  32. A non-centrosymmetric chalcohalide synthesized through the combination of chemical tailoring with aliovalent substitution

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  33. An overview of Mg-based IR nonlinear optical materials

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  34. Flux-assisted polytypism in the [Na 2 Cl]GaQ 2 heterolayered salt-inclusion chalcogenide family

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  35. Tunable Salt-Inclusion Chalcogenides for Ion Exchange, Photoluminescence, and Scintillation

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  36. Salt-inclusion chalcogenides: Double functional moieties design strategy toward excellent nonlinear optical materials

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  37. Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization

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  38. Na3SiS3F: A Wide Bandgap Fluorothiosilicate with Unique [SiS3F] Unit and High Laser‐Induced Damage Threshold

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  39. Recent advances in IR nonlinear optical chalcogenides with well-balanced comprehensive performance

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  40. [Ba4(S2)][ZnGa4S10]: Design of an Unprecedented Infrared Nonlinear Salt‐Inclusion Chalcogenide with Disulfide‐Bonds

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  41. Advances in Chalcogenide Crystal Growth: Flux and Solution Syntheses, and Approaches for Postsynthetic Modifications

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  42. Ga-based IR nonlinear optical materials: Synthesis, structures, and properties

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  43. Rare-earth-based chalcogenides and their derivatives: an encouraging IR nonlinear optical material candidate

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  44. Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units

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  45. [Cs14Cl][Tm71Se110]: An unusual salt-inclusion chalcogenide containing different valent Tm centers and ultralow thermal conductivity

    Chinese Journal of Structural Chemistry · 2024-07-27

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  46. 3Pb 8 O 7 I 2 ·2CsI: the salt-inclusion strategy enriches the structural chemistry in lead oxyhalides

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  47. AgGaS2 and Derivatives: Design, Synthesis, and Optical Properties

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  48. Synergistic Machine Learning Guided Discovery of ABa 3 (BSe 3 ) 2 X (A = Rb, Cs; X = Cl, Br, I): A Promising Family as Property‐Balanced IR Functional Materials

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  49. First-principles study of ABSe₃ (A = Li, Na) Perselenoborates: A Promising Family of Nonlinear Optical Materials

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  50. Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs

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