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RESEARCH PAPER · Inorganic Chemistry · 2016

Strong Nonlinear-Optical Response in the Pyrophosphate CsLiCdP2O7 with a Short Cutoff Edge

Yaoguo Shen, Sangen Zhao, Bingqing Zhao, Chengmin Ji, Lina Li, Zhihua Sun, Maochun Hong, Junhua Luo

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Strong Nonlinear-Optical Response in the Pyrophosphate CsLiCdP2O7 with a Short Cutoff EdgeOriginalAlkali earth MO x ( x = 6, 7, 9, 12) polyhedra tuned cadmium selenites with different dimensions and diverse SeO 3 2− coordinations1Two deep-ultraviolet nonlinear optical alkaline-earth metal borates based on different types of oxoboron clusters56M4Mg4(P2O7)3 (M = K, Rb): Structural Engineering of Pyrophosphates for Nonlinear Optical Applications238Non-Centrosymmetric RbNaMgP 2 O 7 with Unprecedented Thermo-Induced Enhancement of Second Harmonic Generation239Recent advances in ultraviolet and deep-ultraviolet second-order nonlinear optical crystals257Crystal structures and theoretical studies of polyphosphate LiZnP3O9 for nonlinear optical applications18MIMIIP3O9 (MI = Rb, MII = Cd, Mg, Ca; MI = Cs, MII = Pb, Sr; MI = K, MII = Mg): Cation Substitution Application in Cyclophosphate Family and Nonlinear Optical Properties35Non-centrosymmetric BaNaP3O9 with a short deep-ultraviolet cutoff edge14ALiZnP2O7 (A = Rb, Cs): Two Mixed Alkali Zinc Pyrophosphates Featuring a [Li2Zn2P4O20]14– Anionic Skeleton34Czochralski Growth and Characterization of a Novel Nonlinear Optical Crystal Te2P2O923A Langbeinite-Type Yttrium Phosphate LiCs2Y2(PO4)336Experimental characterization and first principles calculations of linear and nonlinear optical properties of two orthophosphates A 3 Al 2 (PO 4 ) 3 (A = Rb, K)36Syntheses, structures, anomalous phase transition and optical properties of two new polymorphic α- and β-LiMoPO 611Proton Conduction in Organically Templated 3D Open-Framework Vanadium–Nickel Pyrophosphate19RbB 11 O 16 (OH) 2 : First Hydroxyl Rubidium Borate with the B‐O 2D Layer Featuring Large Birefringence in the Rb‐B‐O‐H System5LiGaP 2 O 7 : A Potential UV Nonlinear-Optical Crystal14Highly Polarizable Hg2+ Induced a Strong Second Harmonic Generation Signal and Large Birefringence in LiHgPO4265Syntheses, crystal structures, and characterizations of three new pyrophosphates CsNaZnP2O7, RbNaZnP2O7, and RbLiMgP2O710LiMII(IO3)3 (MII=Zn and Cd): Two Promising Nonlinear Optical Crystals Derived from a Tunable Structure Model of α‐LiIO398LiMII(IO3)3 (MII=Zn and Cd): Two Promising Nonlinear Optical Crystals Derived from a Tunable Structure Model of α‐LiIO337Synthesis, electrical and dye adsorption properties of KZnFe(PO4)2 zeolite type structure14Structural Origin of Thermally Induced Second Harmonic Generation Enhancement in RbNaMgP2O721Synthesis, characterization, and properties of two new phosphate crystals MZnAl(PO4)2 (M = Na, K) with 3D framework tunnel structures14Syntheses, structures and characterization of non-centrosymmetric Rb 2 Zn 3 (P 2 O 7 ) 2 and centrosymmetric Cs 2 M 3 (P 2 O 7 ) 2 (M = Zn and Mg)26Tellurium–oxygen group enhanced birefringence in tellurium phosphates: a first-principles investigation4Three diphosphates, α-Li 2 Na 2 P 2 O 7 , Li 8 Pb 3 Ba(P 2 O 7 ) 4 and Li 7 Rb(P 2 O 7 ) 2 : influences of co-substitution on the crystal structure9Ultraviolet nonlinear optical crystal: (NH4)ZnPO47Effects of P2O7 clusters arrangement on second harmonic generation responses of pyrophosphates14The first rare-earth lead phosphates Pb3AP3O12 (A=Sc, Gd) with remarkable SHG enhancement8Noncentrosymmetric Orthophosphate YM3(PO4)3 (M = Sr, Ba) Crystals: Single Crystal Growth, Structure, and Properties34Alignment of Polar Moieties Leading to Strong Second Harmonic Response in KCsMoP2O951Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials137Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials29Formation of complete solid-solution and luminescence-evolution of cyclophosphates KMg(PO3)3 – KMn(PO3)315Sb6O7(SO4)2: A Promising Ultraviolet Nonlinear Optical Material with an Enhanced Second‐Harmonic‐Generation Response Activated by SbIII Lone‐Pair Stereoactivity62Computationally assisted multistage design and prediction driving the discovery of deep-ultraviolet nonlinear optical materials41To improve the key properties of nonlinear optical crystals assembled with tetrahedral functional building units46A comprehensive survey on nonlinear optical phosphates: Role of multicoordinate groups106AZn(PO3)3 (A = K, Rb): Deep-Ultraviolet Nonlinear Optical Phosphates Derived from Synergy of a Unique [ZnO6] Octahedron and a [PO3]∞ Chain25NaSb3O2(SO4)3·H2O: A New Alkali-Metal Antimony(III) Sulfate with a Unique Sb6O20H4 Unit and Moderate Birefringence19Recent Development of Non-π-Conjugated Deep Ultraviolet Nonlinear Optical Materials106Nain(C2o4)(Hpo4)(H2o)5: An Ultraviolet Transparent Nonlinear Optical Oxalate-Phosphate with Large Birefringence0A deep ultraviolet transparent birefringent monofluorophosphate: Cd2.5(NH4)2(PO3F)3Cl ⋅ 2H2O4Crystal growth, structure elucidation and CHARDI/BVS investigations of β-KCoFe(PO4)21First-Principles Calculations of the Structural, Electronic, Optical, and Mechanical Properties of 21 Pyrophosphate Crystals10LiKCuP2O7: Cation substitution application with mixed-alkaline copper-containing pyrophosphate and magnetic properties2Cadmium phosphates with two types of fundamental building units and a wide ultraviolet transparency window1Isomeric Cd(NH4)2(PO3F)2·2H2O: Solution concentration-driven elimination of antiparallel dipole-dipole interaction generating an SHG β phase12Recent advances of inorganic phosphates with UV/DUV cutoff edge and large second harmonic response7Cs2Pb4Br10: A layered perovskite shows large birefringence11Strategy for a Rational Design of Deep-Ultraviolet Nonlinear Optical Materials from Zeolites2Ultrashort Phase‐Matching Wavelength and Strong Second‐Harmonic Generation in Deep‐UV‐Transparent Oxyfluorides by Covalency Reduction33Ultrashort Phase‐Matching Wavelength and Strong Second‐Harmonic Generation in Deep‐UV‐Transparent Oxyfluorides by Covalency Reduction3Approach for quality deep-ultraviolet nonlinear optical crystals via a substitution strategy of channel species in zeolite3Structural characterisation and optical properties of new alkaline earth phosphate CaMg(P 4 O 12 ) and alkaline alumophosphate Cs 3 Al 4 (PO 4 ) 51Predicting structural, electronic, and optical properties of mixed-phase LiMg0.5X0.5PO4 (X = lanthanide) via first-principles study1A2Cd(PO3)4 (A = K, Rb, Cs): Series of cadmium polyphosphates with infinite 1[(PO3)4]ꝏ chains and deep ultraviolet transparency windows2K4Cd3Ge4O13: A Congruent-Melting Germanate Nonlinear Optical Crystal with a Moderate Second-Harmonic Generation Intensity and Broad Transparent Window2Deep‐Ultraviolet Transparent Nonlinear Optical Phosphates: A New Alternative to Conventional Borates9Designing a novel perovskite-type KCd(NH 2 SO 3 ) 3 with deep-ultraviolet transparency and strong second-harmonic generation response2Hydrothermal Synthesis of a Novel 2D‐Layered Vanadium Pyrophosphate With Multi‐Channel and Outstanding Proton Transport Properties1Tuning the Anionic Configuration in ASc2(P2O7)2 (A = Ba, Pb) through A-Site Cationic Coordination Engineering0Growth, structure and optical properties of PbBi3PO8 crystals0Sn 4+ /Sn 2+ Aliovalent Substitution: A Strategy for Local Structure Engineering to Enhance Birefringence and Trigger Structural Symmetry Transition0Enhanced tripling-performance in [C(NH2)3]4P2O7·H2O as UV nonlinear optical material due to π-conjugated cation and hydrogen bonding intervention1Ternary Anion‐Engineered Rare Earth Crystals for Broadband UV Transparency and Enhanced Second‐Harmonic Generation1Dimensionality Engineering of Fluorozirconium Phosphates for Deep-UV-Transparent Crystals with Enhanced Second-Harmonic Generation and Birefringence10Thermally activated sodium-ion transport and optical properties of NaBa(PO3)3 for high-temperature electronics and energy storage applications0Tuning structural symmetry to enhance the linear and nonlinear optical response of NaM(PO3)3 (M= Ba, Cd, Ca) metaphosphates for next-generation deep-UV photonics1

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  1. Alkali earth MO x ( x = 6, 7, 9, 12) polyhedra tuned cadmium selenites with different dimensions and diverse SeO 3 2− coordinations

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  2. Two deep-ultraviolet nonlinear optical alkaline-earth metal borates based on different types of oxoboron clusters

    Dalton Transactions · 2017-01-01

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  3. M4Mg4(P2O7)3 (M = K, Rb): Structural Engineering of Pyrophosphates for Nonlinear Optical Applications

    Chemistry of Materials · 2017-01-30

    Hongwei Yu, Joshua Young, Hongping Wu, Weiguo Zhang, James M. Rondinelli, P. Shiv Halasyamani

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  4. Non-Centrosymmetric RbNaMgP 2 O 7 with Unprecedented Thermo-Induced Enhancement of Second Harmonic Generation

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  5. Recent advances in ultraviolet and deep-ultraviolet second-order nonlinear optical crystals

    Coordination Chemistry Reviews · 2018-03-15

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  6. Crystal structures and theoretical studies of polyphosphate LiZnP3O9 for nonlinear optical applications

    Journal of Solid State Chemistry · 2018-03-29

    Zhiqing Xie, Xin Su, Hanqin Ding, Hongyi Li

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  7. MIMIIP3O9 (MI = Rb, MII = Cd, Mg, Ca; MI = Cs, MII = Pb, Sr; MI = K, MII = Mg): Cation Substitution Application in Cyclophosphate Family and Nonlinear Optical Properties

    Inorganic Chemistry · 2018-05-30

    Maierhaba Abudoureheman, Xiaobo Pan, Shujuan Han, Yilimiranmu Rouzhahong, Zhihua Yang, Hongping Wu, Shilie Pan

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  8. Non-centrosymmetric BaNaP3O9 with a short deep-ultraviolet cutoff edge

    Journal of Alloys and Compounds · 2018-06-07

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  9. ALiZnP2O7 (A = Rb, Cs): Two Mixed Alkali Zinc Pyrophosphates Featuring a [Li2Zn2P4O20]14– Anionic Skeleton

    Inorganic Chemistry · 2018-08-20

    Zhaohui Chen, Yuan Fang, Wenyao Zhang, Wenqiang Chen, Xuefang Lu, Qun Jing, Ming‐Hsien Lee

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  10. Czochralski Growth and Characterization of a Novel Nonlinear Optical Crystal Te2P2O9

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  11. A Langbeinite-Type Yttrium Phosphate LiCs2Y2(PO4)3

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  12. Experimental characterization and first principles calculations of linear and nonlinear optical properties of two orthophosphates A 3 Al 2 (PO 4 ) 3 (A = Rb, K)

    Inorganic Chemistry Frontiers · 2018-12-20

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  13. Syntheses, structures, anomalous phase transition and optical properties of two new polymorphic α- and β-LiMoPO 6

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  14. Proton Conduction in Organically Templated 3D Open-Framework Vanadium–Nickel Pyrophosphate

    Inorganic Chemistry · 2019-03-14

    Le Zhang, Xinxin Liu, Xuejiao Sun, Juan Jian, Guanghua Li, Hongming Yuan

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  15. RbB 11 O 16 (OH) 2 : First Hydroxyl Rubidium Borate with the B‐O 2D Layer Featuring Large Birefringence in the Rb‐B‐O‐H System

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  16. LiGaP 2 O 7 : A Potential UV Nonlinear-Optical Crystal

    Inorganic Chemistry · 2019-05-10

    Yunfei Li, Fei Liang, Huimin Song, Wang Liu, Zheshuai Lin, Guochun Zhang, Yicheng Wu

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  17. Highly Polarizable Hg2+ Induced a Strong Second Harmonic Generation Signal and Large Birefringence in LiHgPO4

    Journal of the American Chemical Society · 2019-06-16

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  18. Syntheses, crystal structures, and characterizations of three new pyrophosphates CsNaZnP2O7, RbNaZnP2O7, and RbLiMgP2O7

    Solid State Sciences · 2019-07-22

    Huimin Song, Shengzi Zhang, Yunfei Li, Wang Liu, Zheshuai Lin, Jiyong Yao, Guochun Zhang

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  19. LiMII(IO3)3 (MII=Zn and Cd): Two Promising Nonlinear Optical Crystals Derived from a Tunable Structure Model of α‐LiIO3

    Angewandte Chemie International Edition · 2019-09-20

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  20. LiMII(IO3)3 (MII=Zn and Cd): Two Promising Nonlinear Optical Crystals Derived from a Tunable Structure Model of α‐LiIO3

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  21. Synthesis, electrical and dye adsorption properties of KZnFe(PO4)2 zeolite type structure

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  22. Structural Origin of Thermally Induced Second Harmonic Generation Enhancement in RbNaMgP2O7

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  23. Synthesis, characterization, and properties of two new phosphate crystals MZnAl(PO4)2 (M = Na, K) with 3D framework tunnel structures

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  24. Syntheses, structures and characterization of non-centrosymmetric Rb 2 Zn 3 (P 2 O 7 ) 2 and centrosymmetric Cs 2 M 3 (P 2 O 7 ) 2 (M = Zn and Mg)

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  25. Tellurium–oxygen group enhanced birefringence in tellurium phosphates: a first-principles investigation

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  26. Three diphosphates, α-Li 2 Na 2 P 2 O 7 , Li 8 Pb 3 Ba(P 2 O 7 ) 4 and Li 7 Rb(P 2 O 7 ) 2 : influences of co-substitution on the crystal structure

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  27. Ultraviolet nonlinear optical crystal: (NH4)ZnPO4

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  28. Effects of P2O7 clusters arrangement on second harmonic generation responses of pyrophosphates

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  29. The first rare-earth lead phosphates Pb3AP3O12 (A=Sc, Gd) with remarkable SHG enhancement

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  30. Noncentrosymmetric Orthophosphate YM3(PO4)3 (M = Sr, Ba) Crystals: Single Crystal Growth, Structure, and Properties

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  31. Alignment of Polar Moieties Leading to Strong Second Harmonic Response in KCsMoP2O9

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  32. Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials

    Angewandte Chemie International Edition · 2020-06-19

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  33. Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials

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  34. Formation of complete solid-solution and luminescence-evolution of cyclophosphates KMg(PO3)3 – KMn(PO3)3

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  35. Sb6O7(SO4)2: A Promising Ultraviolet Nonlinear Optical Material with an Enhanced Second‐Harmonic‐Generation Response Activated by SbIII Lone‐Pair Stereoactivity

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  36. Computationally assisted multistage design and prediction driving the discovery of deep-ultraviolet nonlinear optical materials

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  37. To improve the key properties of nonlinear optical crystals assembled with tetrahedral functional building units

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  38. A comprehensive survey on nonlinear optical phosphates: Role of multicoordinate groups

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  39. AZn(PO3)3 (A = K, Rb): Deep-Ultraviolet Nonlinear Optical Phosphates Derived from Synergy of a Unique [ZnO6] Octahedron and a [PO3]∞ Chain

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  40. NaSb3O2(SO4)3·H2O: A New Alkali-Metal Antimony(III) Sulfate with a Unique Sb6O20H4 Unit and Moderate Birefringence

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  41. Recent Development of Non-π-Conjugated Deep Ultraviolet Nonlinear Optical Materials

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  42. Nain(C2o4)(Hpo4)(H2o)5: An Ultraviolet Transparent Nonlinear Optical Oxalate-Phosphate with Large Birefringence

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  43. A deep ultraviolet transparent birefringent monofluorophosphate: Cd2.5(NH4)2(PO3F)3Cl ⋅ 2H2O

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  44. Crystal growth, structure elucidation and CHARDI/BVS investigations of β-KCoFe(PO4)2

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  45. First-Principles Calculations of the Structural, Electronic, Optical, and Mechanical Properties of 21 Pyrophosphate Crystals

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  46. LiKCuP2O7: Cation substitution application with mixed-alkaline copper-containing pyrophosphate and magnetic properties

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  47. Cadmium phosphates with two types of fundamental building units and a wide ultraviolet transparency window

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  48. Isomeric Cd(NH4)2(PO3F)2·2H2O: Solution concentration-driven elimination of antiparallel dipole-dipole interaction generating an SHG β phase

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  49. Recent advances of inorganic phosphates with UV/DUV cutoff edge and large second harmonic response

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