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RESEARCH PAPER · Coordination Chemistry Reviews · 2021

A comprehensive survey on nonlinear optical phosphates: Role of multicoordinate groups

Junhui Dang, Dajiang Mei, Yuandong Wu, Zheshuai Lin

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A comprehensive survey on nonlinear optical phosphates: Role of multicoordinate groupsOriginalM 6 PS 5 X (M = Ag, Cu; X = Cl, Br) chalcohalides exhibiting strong nonlinear optical responses and high laser damage resistances9Periodic B- and N-doped phenalenyl π-aggregates: unexpected nonlinear optical properties by tuning pancake π–π bonding6UV Solar‐Blind‐Region Phase‐Matchable Optical Nonlinearity and Anisotropy in a π‐Conjugated Cation‐Containing Phosphate196UV Solar‐Blind‐Region Phase‐Matchable Optical Nonlinearity and Anisotropy in a π‐Conjugated Cation‐Containing Phosphate28High-Performance Second-Harmonic-Generation (SHG) Materials: New Developments and New Strategies323Structure-performance relationship in tri-coordinated nonlinear optical materials toward optimal second harmonic generation and phase matching31KCs2[Pb2Br5(HCOO)2]: A Polar 3D Lead‐Bromide Framework Exhibiting Strong Second‐Harmonic Generation Response10Recent advances in nonlinear optical rare earth structures63Complex coordinated functional groups: A great genes for nonlinear optical materials64Phase transition of Mg3(PO4)2 polymorphs at high-temperature: In-situ synchrotron X-ray diffraction and Raman spectroscopic study10AZn 2 (BO 3 )Si 2 O 5 (A = Rb, Cs): first examples of KBe 2 BO 3 F 2 structure type in the borosilicate family exhibiting a deep-ultraviolet cutoff edge25(C 3 N 6 H 7 ) 2 SiF 6 ·H 2 O: an ultraviolet birefringent crystal exceeding the intrinsic energy gap of an organic reagent38Ba 4 Ag 5 (IO 3 ) 6 (I 3 O 8 ) 3 (I 4 O 11 ) 2 : a nonlinear optical crystal containing two types of polyiodate anions16Hexameric poly-fluoroberyllophosphate Na 4 Be 2 PO 4 F 5 with moderate birefringence and deep-ultraviolet transmission as a potential zero-order-waveplate crystal17Li 3 [Al(PO 4 ) 2 (H 2 O) 1.5 ] and Na[AlP 2 O 7 ]: from 2D layered polar to 3D centrosymmetric framework structures8Li 7 SrScB 12 O 24 and Li 7 Ba 0.6 Ca 0.4 ScB 12 O 24 : two new quaternary rare-earth borates with short UV cutoff edges4Nain(C2o4)(Hpo4)(H2o)5: An Ultraviolet Transparent Nonlinear Optical Oxalate-Phosphate with Large Birefringence0Synergistic effect of 2 [V 2 P 2 O 14 ] ∞ layers and hydrogen bonds inducing large birefringence in M(VO) 2 (PO 4 ) 2 ·4H 2 O (M = Ca, Sr, Ba) systems4Polymorphism, polytypism and modular aspect of compounds with the general formula A 2 M 3(TO4)4 (A = Na, Rb, Cs, Ca; M = Mg, Mn, Fe3+, Cu2+; T = S6+, P5+): order–disorder, topological description and DFT calculations11SrZnSnSe4: A quaternary selenide with large second harmonic generation and birefringence39Driving Nonlinear Optical Activity with Dipolar 2-Aminopyrimidinium Cations in (C4H6N3)+(H2PO3)−115CsY(SO4)2·4H2O: A Deep-Ultraviolet Birefringent Crystal Induced by an Edge-Sharing Connection26A deep ultraviolet transparent birefringent monofluorophosphate: Cd2.5(NH4)2(PO3F)3Cl ⋅ 2H2O4Cooperative Enhancement of Second Harmonic Generation in an Organic–Inorganic Hybrid Antimony Halide63AgGaSe2-Inspired Nonlinear Optical Materials: Tetrel Selenides of Alkali Metals and Mercury34AgGaGeSe4: An Infrared Nonlinear Quaternary Selenide with Good Performance6A comprehensive review on metal chalcogenides with three-dimensional frameworks for infrared nonlinear optical applications114Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials28Organic–Inorganic Hybrid Antimony(III) Halides for Second Harmonic Generation34High-peak-power picosecond deep-UV laser sources16Novel structural transformation in K3ReP2S8 thiophosphates originating from the rare-earth (Re) cation sizes induced local coordination asymmetry25Phosphites: A Nonlinear Optical Materials System with a Wide Band Gap and Moderate Second-Harmonic Generation Effect27New lead-iodide formates with a strong second-harmonic generation response and suitable birefringence obtained by the substitution strategy8Oxychalcogenides: A Promising Class of Materials for Nonlinear Optical Crystals with Mixed‐Anion Groups35[Sr 4 Cl 2 ][Si 3 S 9 ]: Ultrawide-bandgap salt-inclusion thiosilicate nonlinear optical material with unprecedented tri-polymerized [Si 3 S 9 ] clusters21Co-substitution design: a new glaserite-type rare-earth phosphate K 2 RbSc(PO 4 ) 2 with high structural tolerance6Deep-ultraviolet nonlinear-optical crystal BaNa2[PO3(OH)]2 with large birefringence and strong second-harmonic-generation response8Enhancing birefringence of non-π-conjugated sulfate systems through rare-earth metal-centered polyhedra10From BPS 4 to AB 3 P 2 S 10 (A = Na, K): cations inducing dimension reduction and bandgap enlargement7Toward Large Second-Harmonic Generation and Deep-UV Transparency in Strongly Electropositive Transition Metal Sulfates112Machine Learning Regression Model for Predicting the Formation Energy of Nonlinear Optical Crystals5Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization133Excellent Static and dynamic hyperpolarizabilities of TM@C6O6Li6 (TM = Sc, Ti, V, Cr and Mn) complexes to prove their NLO applications19Recent advances of inorganic phosphates with UV/DUV cutoff edge and large second harmonic response7First, second and third order NLO response of alkaline earth metals doped C6O6Li6 organometallic complexes14Four New Sb‐based Orthophosphates: Cation Regulation to Investigate Diversified Structural Architecture1Optimal Design of Mid-Infrared Nonlinear-Optical Crystals: From SrZnSnSe 4 to SrZnSiSe 422Nonlinear optical properties of gold nanoparticles containing borate glasses at spectral region of surface plasmon resonance10From Centrosymmetry to Noncentrosymmetry: Precise Structural Regulation and Characterization on ZnHPO3·2H2O Polymorphs13From Monofluorophosphates A2PO3F to Difluorophosphates APO2F2 (A = alkali metal): Design of a Potential Deep-Ultraviolet Nonlinear Optical Materials System with a Shortened Phase-Matching Wavelength41The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals21Giant NLO response and deep ultraviolet transparency of dual (alkali/alkaline earth) metals doped C6O6Li6 electrides11Deep-ultraviolet (DUV) nonlinear optical (NLO) crystals: An application in photonic technologies29Na 6 Mg 3 P 4 S 16 and RbMg 2 PS 4 Cl 2 : two Mg-based thiophosphates with ultrawide bandgaps resulting from [MgS 6 ] and [MgS x Cl 6− x ] octahedra4A Sharp Improvement of Sulfate's Birefringence Induced by the Synergistic Effect of Heteroleptic and Dimeric Strategies14Ga-based IR nonlinear optical materials: Synthesis, structures, and properties65Halide-driven polarity tuning and optimized SHG-bandgap balance in (C 4 H 11 N 2 )ZnX 3 (X = Cl, Br, I)34Rare-earth-based chalcogenides and their derivatives: an encouraging IR nonlinear optical material candidate70RbSb(SO 4 )(H 2 PO 2 )F: a short-wave UV antimony( iii ) oxysalt with mixed-anions demonstrating enhanced birefringence11Understanding the second and third order nonlinear optical responses of M@b 66/64 Al 12 N 12 : a comprehensive DFT and TD-DFT study29Toward the ultraviolet (UV) or deep-UV nonlinear optical crystals: The combination of π-conjugated planar [XY3] and tetrahedral [XY4]80Guanidinium Vanadate [C(NH2)3]3VO4·2H2O Revealing Enhanced Second-Harmonic Generation and Wide Band Gaps131D Tin(II)‐Based Chiral Hybrid Perovskite Single Crystals with Extremely Distorted Inorganic Chains for Second Harmonic Generation38Electron transfer-mediated synergistic nonlinear optical response in the Agn@C18 (n = 4–6) complexes: A DFT study on the electronic structures and optical characteristics7Centrosymmetric CaBaMF8 and Noncentrosymmetric Li2CaMF8 (M = Zr, Hf): Dimension Variation and Nonlinear Optical Activity Resulting from an Isovalent Cation Substitution-Oriented Design17From Cd(SCN) 2 (CH 4 N 2 S) 2 to Cd(SCN) 2 (C 4 H 6 N 2 ) 2 : Controlling Sulfur Content in Thiocyanate Systems Significantly Improves the Overall Performance of UV Nonlinear Optical Materials9From Cd(SCN) 2 (CH 4 N 2 S) 2 to Cd(SCN) 2 (C 4 H 6 N 2 ) 2 : Controlling Sulfur Content in Thiocyanate Systems Significantly Improves the Overall Performance of UV Nonlinear Optical Materials50(C8H6BrN2O)NO3: A Hybrid Nonlinear Optical Crystal With an Appropriate Birefringence12A Universal Design Strategy Achieving Large Birefringence and Short Phase‐Matching Capability of Optical Materials via Dissimilating Non‐π‐Conjugated Units6Remarkable Second Harmonic Generation Response in (C 5 H 6 NO) + (CH 3 SO 3 ) − : Unraveling the Role of Hydrogen Bond in Thermal Driven Nonlinear Optical Switch50Remarkable Second Harmonic Generation Response in (C5H6NO)+(CH3SO3)−: Unraveling the Role of Hydrogen Bond in Thermal Driven Nonlinear Optical Switch10Old tree blossoms anew: Research progress on the structures and optical properties of ultraviolet selenites56Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units66Ag 2 GeS 3 : A Diamond‐Like Chalcogenide as an IR Nonlinear Optical Material with Outstanding Second‐Harmonic Generation Response28A2Cd(PO3)4 (A = K, Rb, Cs): Series of cadmium polyphosphates with infinite 1[(PO3)4]ꝏ chains and deep ultraviolet transparency windows2Exploration of the structure, electronic and optical properties of AB 2(PO3)5 polyphosphates: a first-principle approach3Structure and optical properties of alkali rare-earth double phosphates of M3RE(PO4)2 (M = K, Rb; RE = Y, La, and Lu)4A Giant Optically Anisotropic Phosphate Driven by Mixed Valence Mercury Units22SbO(OH)2(IO3): The First Polar Sb5+‐Iodate with a Strong Second‐Harmonic Generation Response and a Wide Bandgap8Recent progress in nonlinear optical molybdenum/tungsten tellurites: Structures, crystal growth and characterizations34Functional assembly and modification of nonlinear optical fundamental motifs in phosphates27A 3 Sc(PO 4 ) 2 (A = Li, Na): rare earth cations effectively regulate phosphate structures for enhanced birefringence4A review of recent developments in rare earth-doped nanophosphors for emerging technological applications78Hg 2 (HTe 2 O 5 )(PO 4 ): a novel phosphate crystal with enhanced birefringence enabled by the synergistic modification of multiple functional groups12Two mixed P–O anionic phosphates with a distinctive structural transformation and deep ultraviolet cutoff edge0Na3Y2F3P2O8 and K4Y3F5P4O14: [YOF] Polyhedra Inducing Birefringence Enhancement in Non-π-Conjugated Phosphate Systems3Structural and Vibrational Properties of Calcium, Strontium, Barium, and Lead Borophosphates from First Principles2Three Deep-UV Phosphate Optical Materials with Interesting Structural Evolution0Resonant Second-Harmonic Generation in a Hybrid Manganese Bromide: [3-Quinuclidinone]2MnBr43Correlation between structure and optical properties of mixed zinc nickelorthophosphate nanoparticles synthesis by coprecipitation route0Maximizing the second-harmonic generation response via coordination-induced localization of nonbonding electrons12(C 4 H 8 N 5 )(PhPHO 2 )·H 2 O: a polar ionic cocrystal with strong second-harmonic generation and high birefringence0Achieving record-high birefringence in a 3D fluorozincoborate via coplanar alignment of π-conjugated [BO 3 ] units0Charge-order-induced directional enhancement of non-diagonal second-order nonlinear optical tensor components2Crystal structures and optical properties of cesium zinc phosphites with distinct layered frameworks0Experimental and theoretical investigation on N-(Naphthalen-5-yl)-N-phenyl benzamide organic single crystal toward its NLO applications3Suppressing antiparallel dipole alignment: A molecular engineering strategy toward sem-organic UV NLO crystals0Two hydrated ionic cocrystals of phenylphosphonate exhibiting second-harmonic generation and proton conductivity0Theoretical investigation of spectroscopic, electronic, molecular docking, static and frequency dependent nonlinear optical response on 2-(4-hydroxyphenyl)-4,5-diphenyl-1 H-imidazole1Strong Optical Nonlinearity in Polar Hypophosphites via Chiral Cation Assembly1Accelerated Discovery of Fluorophosphates as Deep‐Ultraviolet Nonlinear Optical Materials in the Y–P–O–F System: Unveiling New Composition‐Structure‐Property Rules1Metal–organic framework-based second-order nonlinear optical materials: From structural design to functional applications0A Strategy for Enhancing the Optical Anisotropy of Phosphates via Tetrahedral Unit Modification0From AgGaSe2 to MIIGa2Se4 (MII = Zn, Cd): Heterovalent Substitution Creates Ordered Vacancies for Balanced IR-NLO Performance0Potential Deep Ultraviolet Phosphate With Y‐Based: 1 [(PO 3 ) 4 ] ∞ Chains AYP 4 O 12 (A = K, NH 4 ) and the First [P 3 O 10 ] Anionic Framework KLiYP 3 O 100Borophosphate-based second-order nonlinear optical materials: Advances in structural diversity and optical performance0

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  2. Periodic B- and N-doped phenalenyl π-aggregates: unexpected nonlinear optical properties by tuning pancake π–π bonding

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  3. UV Solar‐Blind‐Region Phase‐Matchable Optical Nonlinearity and Anisotropy in a π‐Conjugated Cation‐Containing Phosphate

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  4. UV Solar‐Blind‐Region Phase‐Matchable Optical Nonlinearity and Anisotropy in a π‐Conjugated Cation‐Containing Phosphate

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  5. High-Performance Second-Harmonic-Generation (SHG) Materials: New Developments and New Strategies

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  6. Structure-performance relationship in tri-coordinated nonlinear optical materials toward optimal second harmonic generation and phase matching

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  7. KCs2[Pb2Br5(HCOO)2]: A Polar 3D Lead‐Bromide Framework Exhibiting Strong Second‐Harmonic Generation Response

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  8. Recent advances in nonlinear optical rare earth structures

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  9. Complex coordinated functional groups: A great genes for nonlinear optical materials

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  10. Phase transition of Mg3(PO4)2 polymorphs at high-temperature: In-situ synchrotron X-ray diffraction and Raman spectroscopic study

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  11. AZn 2 (BO 3 )Si 2 O 5 (A = Rb, Cs): first examples of KBe 2 BO 3 F 2 structure type in the borosilicate family exhibiting a deep-ultraviolet cutoff edge

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  12. (C 3 N 6 H 7 ) 2 SiF 6 ·H 2 O: an ultraviolet birefringent crystal exceeding the intrinsic energy gap of an organic reagent

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  13. Ba 4 Ag 5 (IO 3 ) 6 (I 3 O 8 ) 3 (I 4 O 11 ) 2 : a nonlinear optical crystal containing two types of polyiodate anions

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  14. Hexameric poly-fluoroberyllophosphate Na 4 Be 2 PO 4 F 5 with moderate birefringence and deep-ultraviolet transmission as a potential zero-order-waveplate crystal

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  15. Li 3 [Al(PO 4 ) 2 (H 2 O) 1.5 ] and Na[AlP 2 O 7 ]: from 2D layered polar to 3D centrosymmetric framework structures

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  16. Li 7 SrScB 12 O 24 and Li 7 Ba 0.6 Ca 0.4 ScB 12 O 24 : two new quaternary rare-earth borates with short UV cutoff edges

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  17. Nain(C2o4)(Hpo4)(H2o)5: An Ultraviolet Transparent Nonlinear Optical Oxalate-Phosphate with Large Birefringence

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  19. Polymorphism, polytypism and modular aspect of compounds with the general formula A 2 M 3(TO4)4 (A = Na, Rb, Cs, Ca; M = Mg, Mn, Fe3+, Cu2+; T = S6+, P5+): order–disorder, topological description and DFT calculations

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  23. A deep ultraviolet transparent birefringent monofluorophosphate: Cd2.5(NH4)2(PO3F)3Cl ⋅ 2H2O

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  28. Chalcohalides: A Rising Type of Second‐Order Nonlinear Optical Materials

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  29. Organic–Inorganic Hybrid Antimony(III) Halides for Second Harmonic Generation

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  30. High-peak-power picosecond deep-UV laser sources

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  31. Novel structural transformation in K3ReP2S8 thiophosphates originating from the rare-earth (Re) cation sizes induced local coordination asymmetry

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  32. Phosphites: A Nonlinear Optical Materials System with a Wide Band Gap and Moderate Second-Harmonic Generation Effect

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  33. New lead-iodide formates with a strong second-harmonic generation response and suitable birefringence obtained by the substitution strategy

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  34. Oxychalcogenides: A Promising Class of Materials for Nonlinear Optical Crystals with Mixed‐Anion Groups

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  35. [Sr 4 Cl 2 ][Si 3 S 9 ]: Ultrawide-bandgap salt-inclusion thiosilicate nonlinear optical material with unprecedented tri-polymerized [Si 3 S 9 ] clusters

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  36. Co-substitution design: a new glaserite-type rare-earth phosphate K 2 RbSc(PO 4 ) 2 with high structural tolerance

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  37. Deep-ultraviolet nonlinear-optical crystal BaNa2[PO3(OH)]2 with large birefringence and strong second-harmonic-generation response

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  38. Enhancing birefringence of non-π-conjugated sulfate systems through rare-earth metal-centered polyhedra

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  39. From BPS 4 to AB 3 P 2 S 10 (A = Na, K): cations inducing dimension reduction and bandgap enlargement

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  40. Toward Large Second-Harmonic Generation and Deep-UV Transparency in Strongly Electropositive Transition Metal Sulfates

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  41. Machine Learning Regression Model for Predicting the Formation Energy of Nonlinear Optical Crystals

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  42. Recent progress in the design of IR nonlinear optical materials by partial chemical substitution: Structural evolution and performance optimization

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  43. Excellent Static and dynamic hyperpolarizabilities of TM@C6O6Li6 (TM = Sc, Ti, V, Cr and Mn) complexes to prove their NLO applications

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  44. Recent advances of inorganic phosphates with UV/DUV cutoff edge and large second harmonic response

    Chinese Journal of Structural Chemistry · 2023-02-13

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  45. First, second and third order NLO response of alkaline earth metals doped C6O6Li6 organometallic complexes

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    Naveen Kosar, Sunaina Wajid, Khurshid Ayub, Mazhar Amjad Gilani, Tariq Mahmood

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  46. Four New Sb‐based Orthophosphates: Cation Regulation to Investigate Diversified Structural Architecture

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    Hongyu Huang, Na Li, Ruixin Zhang, Xinmei Wang, Xianmeng He, Lei Wu, Lili Liu, Qun Jing, Zhaohui Chen

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  47. Optimal Design of Mid-Infrared Nonlinear-Optical Crystals: From SrZnSnSe 4 to SrZnSiSe 4

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  48. Nonlinear optical properties of gold nanoparticles containing borate glasses at spectral region of surface plasmon resonance

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    K. Gurushantha, B.N. Swetha, Sangeeta B. Kolavekar, A.G. Pramod, Aljawhara H. Almuqrin, M.I. Sayyed, Gangareddy Jagannath, K. Keshavamurthy

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  49. From Centrosymmetry to Noncentrosymmetry: Precise Structural Regulation and Characterization on ZnHPO3·2H2O Polymorphs

    Inorganic Chemistry · 2023-07-02

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