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RESEARCH PAPER · Physical Chemistry Chemical Physics · 2016

Experimental and theoretical studies on the linear and nonlinear optical properties of lead phosphate crystals LiPbPO 4

Guopeng Han, Qiong Liu, Ying Wang, Xin Su, Zhihua Yang, Shilie Pan

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Experimental and theoretical studies on the linear and nonlinear optical properties of lead phosphate crystals LiPbPO 4OriginalA promising lead-free fluoride carbonate SHG material designed from a theoretical perspective16Structure comparison and optical properties of Na 7 Mg 4.5 (P 2 O 7 ) 4 : a sodium magnesium phosphate with isolated P 2 O 7 units16Syntheses, structures and properties of metal phosphates Pb 2 Mg(PO 4 ) 2 , Pb 4 Zn 8 (PO 4 ) 8 and α-BaZn 2 (PO 4 ) 28Structure–property relationship of metastable monoclinic potassium niobate (KNbO 3 ) nanowires during phase transitions8Syntheses, Structures, and Characterization of Quaternary Tellurites, Li3MTe4O11 (M = Al, Ga, and Fe)13Large electro-optic response of bulk ferroelectric crystals enhanced by piezoelectric resonance in the high frequency range12Bonding Scheme and Optical Properties in BiM2O2(PO4) (M=Cd, Mg, Zn); Experimental and Theoretical Analysis9Electric–elastic properties of a novel high-quality CdTeMoO 6 piezoelectric crystal12K 2 TeP 2 O 8 : a new telluro-phosphate with a pentagonal Te–P–O layer structure26Syntheses, Crystal Structures and Luminescent Properties of Two New Heterometallic Phosphates: Sn 2 Ge(PO 4 ) 2 (OH) 2 and Sn 2 Mn(PO 4 ) 27A Series of Rare-Earth Borates K 7 MRE 2 B 15 O 30 (M = Zn, Cd, Pb; RE = Sc, Y, Gd, Lu) with Large Second Harmonic Generation Responses103Recent advances in ultraviolet and deep-ultraviolet second-order nonlinear optical crystals257Crystal structures and theoretical studies of polyphosphate LiZnP3O9 for nonlinear optical applications18Influence of Cr 3+ doping on the enhanced dielectric and nonlinear optical features of pyroelectric Pb 5 Ge 3 O 11 single crystals16Syntheses, crystal structures and optical properties of two one-dimensional germanophosphates: HRb3Ge2(HPO4)6 and CsGe(HPO4)2(OH)2Experimental characterization and first principles calculations of linear and nonlinear optical properties of two orthophosphates A 3 Al 2 (PO 4 ) 3 (A = Rb, K)36A 2 Bi 2 (SO 4 ) 2 Cl 4 (A = NH 4 , K, Rb): achieving a subtle balance of the large second harmonic generation effect and sufficient birefringence in sulfate nonlinear optical materials98Investigation into the optimized growth, anisotropic properties and theoretical calculations of the polar material Cs 2 TeW 3 O 128Modulation of perovskite-related frameworks induced by alkaline earth metals in phosphate fluorides A 2 MPO 4 F (A = K, Rb; M = Ba, Ca)8Structural insights into three phosphates with distinct polyanionic configurations20Two new tin( iv )-containing phosphate fluorides with two types of Sn( iv )–P–O–F frameworks and short cutoff edges0Bismuth vanadate single crystal particles modified with tungsten for efficient photoeletrochemical water oxidation15Investigating Cationic Distribution, Defect Structure and Phosphor Characteristics of Na 2 Sm 2 Ca 6 (PO 4 ) 6 F 27Rational Design and Synthesis of a Deep-Ultraviolet Nonlinear Optical Fluorinated Orthophosphate: BaZn(PO4)F16Synthesis, characterization, and theoretical analysis of three new nonlinear optical materials K7MRE2B15O30 (M= Ca and Ba, RE= La and Bi)28RbB 11 O 16 (OH) 2 : First Hydroxyl Rubidium Borate with the B‐O 2D Layer Featuring Large Birefringence in the Rb‐B‐O‐H System5LiGaP 2 O 7 : A Potential UV Nonlinear-Optical Crystal14Highly Polarizable Hg2+ Induced a Strong Second Harmonic Generation Signal and Large Birefringence in LiHgPO4265Synthesis, characterization and theoretical calculation of a noncentrosymmetric compound, Cs0.92B0.92Si5.08O122LiCsPbP2O7: A new alkali metal lead pyrophosphate featuring two dimensional [LiP2O7]∞ layer2Na 3 Sc 2 (PO 4 ) 2 F 3 : rational design and synthesis of an alkali rare-earth phosphate fluoride as an ultraviolet nonlinear optical crystal with an enlarged birefringence49Te 3 O 3 (PO 4 ) 2 : a phosphate crystal with large birefringence activated by the highly distorted [TeO 5 ] group and antiparallel [PO 4 ] pseudo-layer33Three non-centrosymmetric bismuth phosphates, Li 2 ABi(PO 4 ) 2 (A = K, Rb, and Cs): effects of cations on the crystal structure and SHG response23The first rare-earth lead phosphates Pb3AP3O12 (A=Sc, Gd) with remarkable SHG enhancement8Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials137Two Pyrophosphates with Large Birefringences and Second‐Harmonic Responses as Ultraviolet Nonlinear Optical Materials29Crystal growth, structural characteristics and electronic structure of Ba1-xPbxFe12O19 (x = 0.23–0.80) hexaferrites27Ba3Sb2(PO4)4 and Cd3Sb2(PO4)4(H2O)2: Two New Antimonous Phosphates with Distinct [Sb(PO4)2] Structure Types and Enhanced Birefringence37Phosphates branching effect on the structure, linear and NLO properties of linear phosphazenes56A comprehensive survey on nonlinear optical phosphates: Role of multicoordinate groups106[C(NH2)3]3PO4·2H2O: A new metal-free ultraviolet nonlinear optical phosphate with large birefringence and second-harmonic generation response70Struvite-type AMgPO4·6H2O (A = NH4, K): Two Natural Deep-Ultraviolet Transparent Nonlinear Optical Crystals13Effects of rare-earth doping and reduction processes in LiCaPO4 compound: A computer simulation study6Cd 2 (IO 3 )(PO 4 ) and Cd 1.62 Mg 0.38 (IO 3 )(PO 4 ): metal iodate-phosphates with large SHG responses and wide band gaps28PO(CH 2 CH 2 CF 3 ) 3 : an organic ultraviolet nonlinear optical material without any anionic group3Structural and spectral investigation of a near-UV-converted LiSrP3O9:Dy3+ phosphor for white light-emitting diodes16CsY(SO4)2·4H2O: A Deep-Ultraviolet Birefringent Crystal Induced by an Edge-Sharing Connection26Lone Pair-Driven Enhancement of Birefringence in Polar Alkali Metal Antimony Phosphates46RbLiZn5(PO4)4 and BaLiZn3(PO4)3: two new zinc orthophosphates with all tetrahedra-based anion frameworks11Structure and optical property evolution in PbM(PO 4 )X (M = Zn, Sn; X = halogen): SHG effect and birefringence21A Rare‐Earth Selenite with Unexpectedly Well‐Balanced Ultraviolet Nonlinear Optical Functionality, Sc(HSeO 3 ) 331Controlling the Nonlinear Optical Behavior and Structural Transformation with A‐Site Cation in α‐AZnPO4 (A = Li, K)20Nanosecond nonlinear optical and gamma radiation shielding behavior of Eu2O3 doped lanthanum containing heavy metal borate glasses: a comparative investigation8Tunable, efficient, ultrafast broadband nonlinear optical properties of TiO2–loaded complex phosphate glasses15Nonlinear refractive index enhancement of Nd3+ ions loaded borate glasses in the near–infrared region by silver nanoparticles8Li2.9Cs1.1(SO4)2: An Ultraviolet Transparent Sulfate as a Nonlinear Optical Crystal16Enhanced nonlinear optical absorption and optical limiting performance of nanoparticles embedded lanthanum alkali borate glasses bearing holmium ions at off–resonant spectral excitation5Two van der Waals Layered Antimony(III) Phosphites as UV Optical Materials11A novel phosphate with Co II square planar coordination, BaCo 0.5 Fe(PO 4 ) 2 : structural and magnetic features3Novel antimony phosphates with enlarged birefringence induced by lone pair cations4Novel polar oxides with exceptional pyroelectric performance: doping-induced polar transition in Ba 6 Pb 3.2 (PO 4 ) 6 Cl 21Syntheses, structures and characterization of noncentrosymmetric MZnPO 4 (M = K, NH 4 )4The effect of co-substitution of heterovalent ions Ga 3+ and Sb 5+ on nonlinear optical properties of phosphate crystals0The electronic structures and optical properties induced by spin-orbit-coupling in LiPbPO4 compound6Structure and optical properties of alkali rare-earth double phosphates of M3RE(PO4)2 (M = K, Rb; RE = Y, La, and Lu)4MgPO2F3: An Ultraviolet Nonlinear Optical System with an Extremely Short Phase-Matching Wavelength Achieved by Introducing Dual-Type Fluorine via Structure Prediction1Functional assembly and modification of nonlinear optical fundamental motifs in phosphates271D Bi ribbon/[PO 4 ] synergy-driven bismuth phosphates for ultraviolet nonlinear optical crystals with large SHG and birefringence0A 3 Sc(PO 4 ) 2 (A = Li, Na): rare earth cations effectively regulate phosphate structures for enhanced birefringence4Exploring hybrid phosphate compound C2H6NO+@H2PO4−: crystallography, optics, and bioactivity0Tuning the Anionic Configuration in ASc2(P2O7)2 (A = Ba, Pb) through A-Site Cationic Coordination Engineering0Na2(C6H4NO3)2·H2O: A promising ultraviolet nonlinear optical crystal with strong second-harmonic generation effect and large birefringence1Sn 4+ /Sn 2+ Aliovalent Substitution: A Strategy for Local Structure Engineering to Enhance Birefringence and Trigger Structural Symmetry Transition0Blue–Green Emitting Phosphor Ba 2 LiAlSi 2 O 8 :Eu 2 + for Phosphor-Converted Light-Emitting Diodes via Single-Particle Diagnosis in a Quasi-Quaternary System0

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  1. A promising lead-free fluoride carbonate SHG material designed from a theoretical perspective

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  2. Structure comparison and optical properties of Na 7 Mg 4.5 (P 2 O 7 ) 4 : a sodium magnesium phosphate with isolated P 2 O 7 units

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  4. Structure–property relationship of metastable monoclinic potassium niobate (KNbO 3 ) nanowires during phase transitions

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  5. Syntheses, Structures, and Characterization of Quaternary Tellurites, Li3MTe4O11 (M = Al, Ga, and Fe)

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  8. Electric–elastic properties of a novel high-quality CdTeMoO 6 piezoelectric crystal

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  9. K 2 TeP 2 O 8 : a new telluro-phosphate with a pentagonal Te–P–O layer structure

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  10. Syntheses, Crystal Structures and Luminescent Properties of Two New Heterometallic Phosphates: Sn 2 Ge(PO 4 ) 2 (OH) 2 and Sn 2 Mn(PO 4 ) 2

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  11. A Series of Rare-Earth Borates K 7 MRE 2 B 15 O 30 (M = Zn, Cd, Pb; RE = Sc, Y, Gd, Lu) with Large Second Harmonic Generation Responses

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  13. Crystal structures and theoretical studies of polyphosphate LiZnP3O9 for nonlinear optical applications

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  14. Influence of Cr 3+ doping on the enhanced dielectric and nonlinear optical features of pyroelectric Pb 5 Ge 3 O 11 single crystals

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  15. Syntheses, crystal structures and optical properties of two one-dimensional germanophosphates: HRb3Ge2(HPO4)6 and CsGe(HPO4)2(OH)

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  16. Experimental characterization and first principles calculations of linear and nonlinear optical properties of two orthophosphates A 3 Al 2 (PO 4 ) 3 (A = Rb, K)

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  17. A 2 Bi 2 (SO 4 ) 2 Cl 4 (A = NH 4 , K, Rb): achieving a subtle balance of the large second harmonic generation effect and sufficient birefringence in sulfate nonlinear optical materials

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  18. Investigation into the optimized growth, anisotropic properties and theoretical calculations of the polar material Cs 2 TeW 3 O 12

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  19. Modulation of perovskite-related frameworks induced by alkaline earth metals in phosphate fluorides A 2 MPO 4 F (A = K, Rb; M = Ba, Ca)

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  20. Structural insights into three phosphates with distinct polyanionic configurations

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  21. Two new tin( iv )-containing phosphate fluorides with two types of Sn( iv )–P–O–F frameworks and short cutoff edges

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  34. The first rare-earth lead phosphates Pb3AP3O12 (A=Sc, Gd) with remarkable SHG enhancement

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