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RESEARCH PAPER · Inorganic Chemistry · 2015

Syntheses, Characterization, and Optical Properties of Centrosymmetric Ba3(BS3)1.5(MS3)0.5 and Noncentrosymmetric Ba3(BQ3)(SbQ3)

Yanyan Li, Bingxuan Li, Ge Zhang, Liujiang Zhou, Hua Lin, Jinni Shen, Chengyi Zhang, Ling Chen, Li‐Ming Wu

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Syntheses, Characterization, and Optical Properties of Centrosymmetric Ba3(BS3)1.5(MS3)0.5 and Noncentrosymmetric Ba3(BQ3)(SbQ3)OriginalChemInform Abstract: Syntheses, Characterization, and Optical Properties of Centrosymmetric Ba3(BS3)1.5(MS3)0.5 and Noncentrosymmetric Ba3(BQ3)(SbQ3).0The effect of indium substitution on the structure and NLO properties of Ba 6 Cs 2 Ga 10 Se 20 Cl 446Hierarchical active factors to band gap and nonlinear optical response in Ag-containing quaternary-chalcogenide compounds9Trigonal Planar [HgSe3]4– Unit: A New Kind of Basic Functional Group in IR Nonlinear Optical Materials with Large Susceptibility and Physicochemical Stability196Syntheses, structures, and properties of sulfides constructed by SbS 4 teeter-totter polyhedra: Ba 3 La 4 Ga 2 Sb 2 S 15 and BaLa 3 GaSb 2 S 1013Recent achievements on middle and far-infrared second-order nonlinear optical materials433A series of pentanary inorganic supramolecular sulfides (A 3 X)[MB 12 (MS 4 ) 3 ] (A = K, Cs; X = Cl, Br, I; M = Ga, In, Gd) featuring B 12 S 12 clusters54Centrosymmetric to noncentrosymmetric structural transformation of new quaternary selenides induced by isolated dimeric [Sn 2 Se 4 ] units: from Ba 8 Ga 2 Sn 7 Se 18 to Ba 10 Ga 2 Sn 9 Se 2210Thioborates: potential nonlinear optical materials with rich structural chemistry51Mid-Infrared Nonlinear Optical Materials Based on Metal Chalcogenides: Structure–Property Relationship338AgGa2PS6: A New Mid‐Infrared Nonlinear Optical Material with a High Laser Damage Threshold and a Large Second Harmonic Generation Response78Noncentrosymmetric quaternary selenide Ba23Ga8Sb2Se38: Synthesis, structure, and optical properties15BaM2As2S6 (M = Cd, Hg): Synthesis, crystal structure, optical and electronic properties16Cation substitution inducing gap changes and covalent interaction flexibility enhancing second harmonic generation responses in d10 metal chalcogenides11A review on the development of infrared nonlinear optical materials with triangular anionic groups38Ba 6 In 6 Zn 4 Se 19 : a high performance infrared nonlinear optical crystal with [InSe 3 ] 3− trigonal planar functional motifs22Inorganic planar π-conjugated groups in nonlinear optical crystals: review and outlook145New quaternary chalcogenide Ba 4 HgAs 2 S 10 originating from the combination of linear [HgS 2 ] 2− and tetrahedral [AsS 4 ] 3− modules8First non-centrosymmetric antimony chalcogenides containing mixed cations of alkali and alkaline-Earth: Ba14Na4Sb11S31Cl3 featuring unique disorded 43 helical chains of [Sb5S18]21–5Ba3[LiSbS2(S2)2Cl2]: The first zero-dimensional (0D) lithium metal thioantimonate featuring molecular anions of [LiSbS2(S2)2Cl2]6–3Ba 2 BS 3 Cl and Ba 5 B 2 S 8 Cl 2 : first alkaline-earth metal thioborate halides with [BS 3 ] units21Facile syntheses of silver thioantimonates exhibiting second-harmonic generation responses and large birefringence18Structural diversities in centrosymmetric La 8 S 4 Cl 8 La 12 S 8 Cl 4 [SbS 3 ] 8 and non-centrosymmetric Ln 12 S 8 Cl 8 [SbS 3 ] 4 (Ln = La and Ce): syntheses, crystal and electronic structures, and optical properties10Ultraviolet nonlinear optical crystals A 3 SrBi(P 2 O 7 ) 2 (A = K, Rb) with large second harmonic generation responses15A Series of Pentanary Salt-Inclusion Chalcogenoborates Containing a B12Q12 (Q = S, Se) Cluster Exhibiting a Kleinman-Forbidden Frequency-Doubling Effect25Inorganic Chalcogenides: From Zero‐Dimensional Clusters to Three‐Dimensional Frameworks5Structure-performance relationship in tri-coordinated nonlinear optical materials toward optimal second harmonic generation and phase matching31LaBS 3 revisited: a promising mid-infrared nonlinear optical material34From Cc to P 6 3 mc : Structural Variation in La 3 S 2 Cl 2 [SbS 3 ] and La 3 OSCl 2 [SbS 3 ] Induced by the Isovalent Anion Substitution22Zn2BS3Br: An Infrared Nonlinear Optical Material with Significant Dual-Property Enhancements Designed through a Template Grafting Strategy20Ca2Ln(BS3)(SiS4) (Ln = La, Ce, and Gd): Mixed Metal Thioborate‐Thiosilicates as Well‐Performed Infrared Nonlinear Optical Materials29Ga-based IR nonlinear optical materials: Synthesis, structures, and properties65Hydrothermally synthesized first acentric apatite (Bi 5 Na 5 )[PO 4 ] 6 Cl 2 with wide Bi–Na isomorphism and doubled c -axis3Evaluation and prospect of Mid-Infrared nonlinear optical materials in f0 rare earth (RE = Sc, Y, La) chalcogenides45Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units66Achieving Phase‐Matching in Nonlinear Optical Materials CsM 2 In 2 S 6 (M = Cd/In, Hg/In) by the Incorporation of Unprecedented Trigonal Planar MS 3 Motifs6Na 2 B 12 Si 6 Se 18 : a novel B 12 -cluster-containing quaternary selenoborate framework material2Looking Back the Nonlinear Optical Crystals in a Functionalized Unit's Perspective109BaSbBS 4 : a record-high-performance birefringent crystal identified by a target-driven closed-loop strategy28Ca 2 La(MS 4 )(BS 3 ) (M = Ge/Si and Sn/Si): high-performance infrared nonlinear optical materials designed using an atomic site co-occupancy strategy9Selenoborates: a latent structure resource for infrared functional crystal materials1Structural diversity and photocurrent responses of multi-component chalcogenidometalates8BaLa4(SiS4)2(BS3)2: Structurally Ordered Thioborate-Thiosilicate Obtained by Adjusting the Cationic Size2Recent progress in structural design strategies of high-birefringence optical crystals55Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs29Diamond-like Ag x Cu 3− x PS 4 ( x = 1 and 2) synthesized by the metal oxide–boron–chalcogen (MOBQ) routine: local high-entropy engineering for balanced infrared nonlinear optical performance1Coordination chemistry of Sb(III)-based optical crystals: from lone-pair-induced distortion to birefringence and second-harmonic generation0

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  1. ChemInform Abstract: Syntheses, Characterization, and Optical Properties of Centrosymmetric Ba3(BS3)1.5(MS3)0.5 and Noncentrosymmetric Ba3(BQ3)(SbQ3).

    ChemInform · 2015-07-01

    Yan‐Yan Li, Bingxuan Li, Ge Zhang, Liujiang Zhou, Hua Lin, Jinni Shen, Cheng‐Yi Zhang, Ling Chen, Li‐Ming Wu

    Read original paper ↗ ·

  2. The effect of indium substitution on the structure and NLO properties of Ba 6 Cs 2 Ga 10 Se 20 Cl 4

    Inorganic Chemistry Frontiers · 2016-01-01

    Yanyan Li, Pengfei Liu, Hua Lin, Meitian Wang, Ling Chen

    Read original paper ↗ ·

  3. Hierarchical active factors to band gap and nonlinear optical response in Ag-containing quaternary-chalcogenide compounds

    Journal of Solid State Chemistry · 2016-04-08

    Junben Huang, Mamatrishat Mamat, Shilie Pan, Zhihua Yang

    Read original paper ↗ ·

  4. Trigonal Planar [HgSe3]4– Unit: A New Kind of Basic Functional Group in IR Nonlinear Optical Materials with Large Susceptibility and Physicochemical Stability

    Journal of the American Chemical Society · 2016-05-03

    Chao Li, Wenlong Yin, Pifu Gong, Xiaoshuang Li, Molin Zhou, Arthur Mar, Zheshuai Lin, Jiyong Yao, Yicheng Wu, Chuangtian Chen

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  5. Syntheses, structures, and properties of sulfides constructed by SbS 4 teeter-totter polyhedra: Ba 3 La 4 Ga 2 Sb 2 S 15 and BaLa 3 GaSb 2 S 10

    Inorganic Chemistry Frontiers · 2016-11-15

    Ruihuan Duan, Jinni Shen, Chensheng Lin, Pengfei Liu, Hua Lin, Shangxiong Huangfu, Hua‐Jun Zhao, Muhammad Ali Khan, Ling Chen

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  6. Recent achievements on middle and far-infrared second-order nonlinear optical materials

    Coordination Chemistry Reviews · 2016-12-27

    Sheng‐Ping Guo, Yang Chi, Guo‐Cong Guo

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  7. A series of pentanary inorganic supramolecular sulfides (A 3 X)[MB 12 (MS 4 ) 3 ] (A = K, Cs; X = Cl, Br, I; M = Ga, In, Gd) featuring B 12 S 12 clusters

    Inorganic Chemistry Frontiers · 2017-01-01

    Zongdong Sun, Yang Chi, Huaiguo Xue, Sheng‐Ping Guo

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  8. Centrosymmetric to noncentrosymmetric structural transformation of new quaternary selenides induced by isolated dimeric [Sn 2 Se 4 ] units: from Ba 8 Ga 2 Sn 7 Se 18 to Ba 10 Ga 2 Sn 9 Se 22

    RSC Advances · 2017-01-01

    Yanyan Li, Jinqiu Wang, Pengfei Liu, Hua Lin, Ling Chen, Li‐Ming Wu

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  9. Thioborates: potential nonlinear optical materials with rich structural chemistry

    Dalton Transactions · 2017-01-01

    Yu‐Kun Lian, Li‐Ming Wu, Ling Chen

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  10. Mid-Infrared Nonlinear Optical Materials Based on Metal Chalcogenides: Structure–Property Relationship

    Crystal Growth & Design · 2017-03-15

    Fei Liang, Lei Kang, Zheshuai Lin, Yicheng Wu

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  11. AgGa2PS6: A New Mid‐Infrared Nonlinear Optical Material with a High Laser Damage Threshold and a Large Second Harmonic Generation Response

    Chemistry - A European Journal · 2017-07-07

    Jiang‐He Feng, Chun‐Li Hu, Xiang Xu, Bingxuan Li, Mingjian Zhang, Jiang‐Gao Mao

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  12. Noncentrosymmetric quaternary selenide Ba23Ga8Sb2Se38: Synthesis, structure, and optical properties

    Journal of Alloys and Compounds · 2017-09-14

    Wenlong Yin, Molin Zhou, Abishek K. Iyer, Jiyong Yao, Arthur Mar

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  13. BaM2As2S6 (M = Cd, Hg): Synthesis, crystal structure, optical and electronic properties

    Journal of Alloys and Compounds · 2018-05-21

    Yangwu Guo, Fei Liang, Molin Zhou, Zheshuai Lin, Jiyong Yao, Yicheng Wu

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  14. Cation substitution inducing gap changes and covalent interaction flexibility enhancing second harmonic generation responses in d10 metal chalcogenides

    Journal of Alloys and Compounds · 2018-07-30

    Jianian Cheng, Ming‐Hsien Lee, Jun Zhang

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  15. A review on the development of infrared nonlinear optical materials with triangular anionic groups

    Journal of Solid State Chemistry · 2018-11-22

    Yu Chu, Guangmao Li, Xin Su, Kui Wu, Shilie Pan

    Read original paper ↗ ·

  16. Ba 6 In 6 Zn 4 Se 19 : a high performance infrared nonlinear optical crystal with [InSe 3 ] 3− trigonal planar functional motifs

    Journal of Materials Chemistry C · 2020-01-01

    Anyi Zhou, Chensheng Lin, Bingxuan Li, Wen‐Dan Cheng, Zhengxiao Guo, Zhufeng Hou, Fang-Yu Yuan, Guoliang Chai

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  17. Inorganic planar π-conjugated groups in nonlinear optical crystals: review and outlook

    Inorganic Chemistry Frontiers · 2020-01-01

    Pifu Gong, Xiaomeng Liu, Lei Kang, Zheshuai Lin

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  18. New quaternary chalcogenide Ba 4 HgAs 2 S 10 originating from the combination of linear [HgS 2 ] 2− and tetrahedral [AsS 4 ] 3− modules

    Dalton Transactions · 2020-01-01

    Wenhao Xing, Naizheng Wang, Zhuang Li, Wenhao Liu, Jian Tang, Wenlong Yin, Zheshuai Lin, Bin Kang, Jiyong Yao

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  19. First non-centrosymmetric antimony chalcogenides containing mixed cations of alkali and alkaline-Earth: Ba14Na4Sb11S31Cl3 featuring unique disorded 43 helical chains of [Sb5S18]21–

    Journal of Solid State Chemistry · 2020-06-26

    Hua‐Jun Zhao, Biao Qin

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  20. Ba3[LiSbS2(S2)2Cl2]: The first zero-dimensional (0D) lithium metal thioantimonate featuring molecular anions of [LiSbS2(S2)2Cl2]6–

    Journal of Solid State Chemistry · 2020-11-24

    Hua‐Jun Zhao, Pengfei Liu

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  21. Ba 2 BS 3 Cl and Ba 5 B 2 S 8 Cl 2 : first alkaline-earth metal thioborate halides with [BS 3 ] units

    Chemical Communications · 2021-01-01

    Jiazheng Zhou, Yu Chu, Junjie Li, Shilie Pan

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  22. Facile syntheses of silver thioantimonates exhibiting second-harmonic generation responses and large birefringence

    Dalton Transactions · 2021-01-01

    Gang Yang, Xingxing Jiang, Chao Wu, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  23. Structural diversities in centrosymmetric La 8 S 4 Cl 8 La 12 S 8 Cl 4 [SbS 3 ] 8 and non-centrosymmetric Ln 12 S 8 Cl 8 [SbS 3 ] 4 (Ln = La and Ce): syntheses, crystal and electronic structures, and optical properties

    Dalton Transactions · 2021-01-01

    Hua‐Jun Zhao, Pengfei Liu, Li‐Ming Wu

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  24. Ultraviolet nonlinear optical crystals A 3 SrBi(P 2 O 7 ) 2 (A = K, Rb) with large second harmonic generation responses

    Inorganic Chemistry Frontiers · 2021-01-01

    Shiwei Liu, Bingbing Zhang, Hongping Wu, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  25. A Series of Pentanary Salt-Inclusion Chalcogenoborates Containing a B12Q12 (Q = S, Se) Cluster Exhibiting a Kleinman-Forbidden Frequency-Doubling Effect

    Inorganic Chemistry · 2021-02-09

    Shanshan Han, Wen‐Dong Yao, Su‐Xin Yu, Yueling Sun, Anhua Gong, Sheng‐Ping Guo

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  26. Inorganic Chalcogenides: From Zero‐Dimensional Clusters to Three‐Dimensional Frameworks

    Unknown journal · 2021-04-19

    Hua Lin, Xin‐Tao Wu, Qi‐Long Zhu

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  27. Structure-performance relationship in tri-coordinated nonlinear optical materials toward optimal second harmonic generation and phase matching

    Coordination Chemistry Reviews · 2021-06-08

    Fengjuan Hou, Dajiang Mei, Mingjun Xia, Yuandong Wu

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  28. LaBS 3 revisited: a promising mid-infrared nonlinear optical material

    Journal of Materials Chemistry C · 2022-01-01

    Ya‐Xiang Han, Chun‐Li Hu, Zhi Gang Fang, Qianqian Chen, Bingxuan Li, Yuan Hua Lin, Jiang‐Gao Mao

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  29. From Cc to P 6 3 mc : Structural Variation in La 3 S 2 Cl 2 [SbS 3 ] and La 3 OSCl 2 [SbS 3 ] Induced by the Isovalent Anion Substitution

    Crystal Growth & Design · 2022-01-17

    Hua‐Jun Zhao, Hedi Yang, Pengfei Liu, Hua Lin

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  30. Zn2BS3Br: An Infrared Nonlinear Optical Material with Significant Dual-Property Enhancements Designed through a Template Grafting Strategy

    Chemistry of Materials · 2023-03-15

    Chun‐Li Hu, Ya‐Xiang Han, Zhi Gang Fang, Jiang‐Gao Mao

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  31. Ca2Ln(BS3)(SiS4) (Ln = La, Ce, and Gd): Mixed Metal Thioborate‐Thiosilicates as Well‐Performed Infrared Nonlinear Optical Materials

    Small · 2023-09-19

    Ya‐Xiang Han, Chun‐Li Hu, Jiang‐Gao Mao

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  32. Ga-based IR nonlinear optical materials: Synthesis, structures, and properties

    Coordination Chemistry Reviews · 2023-12-21

    Jiaxiang Zhang, Ping Feng, Mao‐Yin Ran, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  33. Hydrothermally synthesized first acentric apatite (Bi 5 Na 5 )[PO 4 ] 6 Cl 2 with wide Bi–Na isomorphism and doubled c -axis

    New Journal of Chemistry · 2024-01-01

    Elena L. Belokoneva, Anatoly S. Volkov, Olga V. Dimitrova, Sergey Yu. Stefanovich, Nadezhda B. Govorko

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  34. Evaluation and prospect of Mid-Infrared nonlinear optical materials in f0 rare earth (RE = Sc, Y, La) chalcogenides

    Coordination Chemistry Reviews · 2024-03-22

    Linfeng Dong, Shengzi Zhang, Pifu Gong, Lei Kang, Zheshuai Lin

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  35. Recent advances and future perspectives on rare-earth-based nonlinear optical materials with π-conjugated [XO3] (X = B, C, N) units

    Coordination Chemistry Reviews · 2024-07-03

    Bo Zhang, Mao‐Yin Ran, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  36. Achieving Phase‐Matching in Nonlinear Optical Materials CsM 2 In 2 S 6 (M = Cd/In, Hg/In) by the Incorporation of Unprecedented Trigonal Planar MS 3 Motifs

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    Lin‐Tao Jiang, Yi‐Bing Huang, Shao‐Min Pei, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  37. Na 2 B 12 Si 6 Se 18 : a novel B 12 -cluster-containing quaternary selenoborate framework material

    Dalton Transactions · 2024-12-09

    Gopabandhu Panigrahi, Hunter B. Tisdale, Gregory W. Morrison, Hans‐Conrad zur Loye

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  38. Looking Back the Nonlinear Optical Crystals in a Functionalized Unit's Perspective

    Advanced Functional Materials · 2024-12-15

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  39. BaSbBS 4 : a record-high-performance birefringent crystal identified by a target-driven closed-loop strategy

    Chemical Science · 2025-01-01

    Ming‐Zhi Zhang, Yue Zhao, Chun‐Li Hu, Jiang‐Gao Mao

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  40. Ca 2 La(MS 4 )(BS 3 ) (M = Ge/Si and Sn/Si): high-performance infrared nonlinear optical materials designed using an atomic site co-occupancy strategy

    Inorganic Chemistry Frontiers · 2025-01-01

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  41. Selenoborates: a latent structure resource for infrared functional crystal materials

    Inorganic Chemistry Frontiers · 2025-01-01

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  42. Structural diversity and photocurrent responses of multi-component chalcogenidometalates

    Inorganic Chemistry Frontiers · 2025-01-01

    Chang Liu, Wen-Jing Tian, Mao‐Yin Ran, Pan Gao, Panpan Jing, Yi Liu, Hua Lin

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  43. BaLa4(SiS4)2(BS3)2: Structurally Ordered Thioborate-Thiosilicate Obtained by Adjusting the Cationic Size

    Inorganic Chemistry · 2025-03-19

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  44. Recent progress in structural design strategies of high-birefringence optical crystals

    Coordination Chemistry Reviews · 2025-05-08

    A-Lan Xu, Mao‐Yin Ran, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  45. Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs

    Coordination Chemistry Reviews · 2025-09-03

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  46. Diamond-like Ag x Cu 3− x PS 4 ( x = 1 and 2) synthesized by the metal oxide–boron–chalcogen (MOBQ) routine: local high-entropy engineering for balanced infrared nonlinear optical performance

    Inorganic Chemistry Frontiers · 2026-01-01

    Ao Guo, Rong-Ling Zhu, Zi-Nan Chen, Zhi Deng, Zong-Ze Li, Shao-Peng Gui, Mao‐Yin Ran, Sheng‐Ping Guo

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  47. Coordination chemistry of Sb(III)-based optical crystals: from lone-pair-induced distortion to birefringence and second-harmonic generation

    Coordination Chemistry Reviews · 2026-10-06

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