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RESEARCH PAPER · Chemical Science · 2025

BaSbBS 4 : a record-high-performance birefringent crystal identified by a target-driven closed-loop strategy

Ming‐Zhi Zhang, Yue Zhao, Chun‐Li Hu, Jiang‐Gao Mao

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BaSbBS 4 : a record-high-performance birefringent crystal identified by a target-driven closed-loop strategyOriginalHg[CS(NH 2 ) 2 ] 4 (SiF 6 ): a fluorosilicate crystal with large birefringence achieved via multi-functional group modification6CsICl 2 : A Record-Birefringent Inorganic Crystal with Ultrawide Infrared Transparency Enabled by Linear Interhalogen ICl 2 – Units36Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals27Hydrogen-bond-driven noncentrosymmetric structure formation in π-conjugated (C3H7N6)(IO3): achieving both strong SHG response and wide bandgap5ZnGa(SeO 3 ) 2 F: a UV transparent birefringent crystal explored in M( ii )–IIIA–selenite–F systems2[Cd 4 P 2 ][I 3 ] and [Cd 2 P][CdCl 3 ]: two Millon's phase phosphides exhibiting wide band gaps and large birefringence0[ICl 4 ] − : A large anisotropic planar anion group produces giant birefringence2Achieving giant optical anisotropy in the mid-far infrared region via ideal alignment of dual functional motifs0Optimal three-dimensional [Ag 4 P 2 S 6 ]-framework assembly directed by a threefold roto-inversion axis for enhanced birefringence0Pyrazinamide–IBr: an organic–inorganic hybrid crystal exhibiting giant optical anisotropy0Halogen‐Bond Coupled Halogenated‐π‐Conjugation Enables Giant Birefringence in Hydrogen‐Bonded Organic Frameworks13Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block12Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block4Li 6 Lu(BO 3 ) 3 : A Rare-Earth Borate Crystal Exhibiting Large Birefringence and Broad UV Transparency1The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 115The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 110Lock‐and‐Key Assembly Enables Record Birefringence in Monocyclic π‐Conjugated Crystals via Spatial Confinement of Linear Polyhalide5Lock‐and‐Key Assembly Enables Record Birefringence in Monocyclic π‐Conjugated Crystals via Spatial Confinement of Linear Polyhalide0Bridging Motifs Induced Ordered Arrangement Contributing Large Birefringence for Hg 4 BiQ 2 Cl 5 (Q═S, Se)1Interlayer Electronic Decoupling Unlocks Giant Birefringence in π‐Conjugated Metal‐Organic Frameworks0Ce(2,2′-bipyridyl)3(SCN)3: Lanthanide Coordination- and Hydrogen-Bond-Directed Binary π-Conjugated Assemblies with Synergistic Large Birefringence and Broad Transparency0Halogen-Mediated Dimensionality Reduction in Bismuth Oxychlorides: Trade-off between Birefringence and Band Gap0A Mild Boc Deprotection Using Armstrong’s Acid0Advances in metal selenite nonlinear optical materials: halogens directed structure modulation and property optimization0A Pyrazinamide–Iodic Acid Cocrystal Exhibiting Strong Second Harmonic Generation for Nonlinear Optics0Cation-Modulated Activation of Linear Units in an Ordered Arrangement Achieves the Largest Optical Anisotropy in Wide-Bandgap Metal Chalcogenides0Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals0Coordination chemistry of Sb(III)-based optical crystals: from lone-pair-induced distortion to birefringence and second-harmonic generation0

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28 direct citing papers saved.

  1. Hg[CS(NH 2 ) 2 ] 4 (SiF 6 ): a fluorosilicate crystal with large birefringence achieved via multi-functional group modification

    Dalton Transactions · 2025-01-01

    Pengfei Li, Xinlei Liu, Si-Qi Zhou, Mingchang Wang, Jingjing Wu, Yu‐Wu Zhong, Jiannian Yao

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  2. CsICl 2 : A Record-Birefringent Inorganic Crystal with Ultrawide Infrared Transparency Enabled by Linear Interhalogen ICl 2 – Units

    Journal of the American Chemical Society · 2025-07-21

    Chong‐An Chen, Yang Li, Congcong Jin, Kang Min Ok

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  3. Five-Membered [C 5 O 5 ] 2 – Rings as Birefringence-Active Genes for Ultrabirefringent Crystals

    Journal of the American Chemical Society · 2025-09-16

    Jiachen Lu, Yang Li, Kang Min Ok

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  4. Hydrogen-bond-driven noncentrosymmetric structure formation in π-conjugated (C3H7N6)(IO3): achieving both strong SHG response and wide bandgap

    Science China Chemistry · 2025-10-21

    Yu-Wei Kang, Chun‐Li Hu, Jiang‐Gao Mao

    Read original paper ↗ ·

  5. ZnGa(SeO 3 ) 2 F: a UV transparent birefringent crystal explored in M( ii )–IIIA–selenite–F systems

    Inorganic Chemistry Frontiers · 2025-12-20

    Tian-Tian He, C Hu, Ya-Ping Gong, Jiang‐Gao Mao, Fang Kong

    Read original paper ↗ ·

  6. [Cd 4 P 2 ][I 3 ] and [Cd 2 P][CdCl 3 ]: two Millon's phase phosphides exhibiting wide band gaps and large birefringence

    Dalton Transactions · 2026-01-01

    Fupeng Wang, Guang Peng, Ning Ye, Jindong Chen

    Read original paper ↗ ·

  7. [ICl 4 ] − : A large anisotropic planar anion group produces giant birefringence

    Chemical Communications · 2026-01-01

    Yi-Chen Liu, Ming‐Zhi Zhang, Chun‐Li Hu, Jiang‐Gao Mao

    Read original paper ↗ ·

  8. Achieving giant optical anisotropy in the mid-far infrared region via ideal alignment of dual functional motifs

    Inorganic Chemistry Frontiers · 2026-01-01

    Yi-Wen Shan, Ming‐Zhi Zhang, C Hu, Jiang‐Gao Mao

    Read original paper ↗ ·

  9. Optimal three-dimensional [Ag 4 P 2 S 6 ]-framework assembly directed by a threefold roto-inversion axis for enhanced birefringence

    Inorganic Chemistry Frontiers · 2026-01-01

    MF Zhang, C Hu, Jiang‐Gao Mao

    Read original paper ↗ ·

  10. Pyrazinamide–IBr: an organic–inorganic hybrid crystal exhibiting giant optical anisotropy

    Dalton Transactions · 2026-01-01

    Meng-Fan Duan, Jiang‐Gao Mao, Bing‐Ping Yang

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  11. Halogen‐Bond Coupled Halogenated‐π‐Conjugation Enables Giant Birefringence in Hydrogen‐Bonded Organic Frameworks

    Advanced Science · 2026-01-14

    Miao‐Bin Xu, Yun‐Xia Hu, Ming‐Chang Wang, Jia‐jia Li, Jia‐Min Lian, Jin Chen, Ke‐Zhao Du

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  12. Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block

    Angewandte Chemie International Edition · 2026-01-27

    Kaijie Xie, Zhiyong Bai, Weiqi Huang, Ji Qi, Tingjuan Lin, Muhammad Zeeshan, Yanqiang Li, Yang Zhou, Junhua Luo, Sangen Zhao

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  13. Unveiling the Superior Birefringence Property of a Record‐Birefringent Crystal with Unique Building Block

    Angewandte Chemie · 2026-01-27

    Kaijie Xie, Zhiyong Bai, Weiqi Huang, Ji Qi, Tingjuan Lin, Muhammad Zeeshan, Yanqiang Li, Yang Zhou, Junhua Luo, Sangen Zhao

    Read original paper ↗ ·

  14. Li 6 Lu(BO 3 ) 3 : A Rare-Earth Borate Crystal Exhibiting Large Birefringence and Broad UV Transparency

    Inorganic Chemistry · 2026-02-05

    Mingyue Gu, Xianchao Zhu, Zhanggui Hu, Yicheng Wu, Yongmin Guo

    Read original paper ↗ ·

  15. The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 11

    Angewandte Chemie International Edition · 2026-04-25

    Hongshan Wang, Miriding Mutailipu, Shilie Pan, Junjie Li

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  16. The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 11

    Angewandte Chemie · 2026-04-26

    Hongshan Wang, Miriding Mutailipu, Shilie Pan, Junjie Li

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  17. Lock‐and‐Key Assembly Enables Record Birefringence in Monocyclic π‐Conjugated Crystals via Spatial Confinement of Linear Polyhalide

    Angewandte Chemie International Edition · 2026-05-26

    Yun‐Xia Hu, Huai Yu Wu, Jia‐jia Li, Ming‐Chang Wang, Jia‐Min Lian, Jin Yu Luo, Yiru Fu, Zi‐Yan Chen, Yang‐Hang Guo, Jin Chen, Ke‐Zhao Du

    Read original paper ↗ ·

  18. Lock‐and‐Key Assembly Enables Record Birefringence in Monocyclic π‐Conjugated Crystals via Spatial Confinement of Linear Polyhalide

    Angewandte Chemie · 2026-05-26

    Yun‐Xia Hu, Huai Yu Wu, Jia‐jia Li, Ming‐Chang Wang, Jia‐Min Lian, Jin Yu Luo, Yiru Fu, Zi‐Yan Chen, Yang‐Hang Guo, Jin Chen, Ke‐Zhao Du

    Read original paper ↗ ·

  19. Bridging Motifs Induced Ordered Arrangement Contributing Large Birefringence for Hg 4 BiQ 2 Cl 5 (Q═S, Se)

    Small · 2026-06-02

    Zhen‐Cheng Wu, Chang‐Hong Li, Yu‐Xuan Zhang, Mao‐Yin Ran, Sheng‐Ping Guo

    Read original paper ↗ ·

  20. Interlayer Electronic Decoupling Unlocks Giant Birefringence in π‐Conjugated Metal‐Organic Frameworks

    Advanced Materials · 2026-06-18

    Jia-Xiang Zhang, Xinyan Wu, Weishan Li, Haolin Zhong, Jinkun Guo, Qingsheng Zeng, Mao‐Yin Ran, Ze‐Fan Yao, Yu‐Qing Zheng, Qingqing Ji, Jin‐Hu Dou

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  21. Ce(2,2′-bipyridyl)3(SCN)3: Lanthanide Coordination- and Hydrogen-Bond-Directed Binary π-Conjugated Assemblies with Synergistic Large Birefringence and Broad Transparency

    Inorganic Chemistry · 2026-07-24

    Quan-Wei Zhang, Zi-Han Tian, Ming-Xing Wu, Chenyuan Ma, Xing-Yu Bi, Zhi Gang Fang, Meihong Duan

    Read original paper ↗ ·

  22. Halogen-Mediated Dimensionality Reduction in Bismuth Oxychlorides: Trade-off between Birefringence and Band Gap

    Journal of Molecular Structure · 2026-08-03

    Huaiqiang Xun, Shumei Cao, Qingyue Cui, Yi Feng, Rui Wu, Chunmei Huang, Leyan Nian

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  23. A Mild Boc Deprotection Using Armstrong’s Acid

    The Journal of Organic Chemistry · 2026-08-12

    Bijan Mirabi, Byung Joo Lee, Annie R. Hooper

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  24. Advances in metal selenite nonlinear optical materials: halogens directed structure modulation and property optimization

    Coordination Chemistry Reviews · 2026-08-14

    Dan-Dan Zhou, Tian-Tian He, Chun‐Li Hu, Jiang‐Gao Mao, Fang Kong

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  25. A Pyrazinamide–Iodic Acid Cocrystal Exhibiting Strong Second Harmonic Generation for Nonlinear Optics

    Advanced Optical Materials · 2026-08-31

    M. Duan, Chun‐Li Hu, Jiang‐Gao Mao, Bing‐Ping Yang

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  26. Cation-Modulated Activation of Linear Units in an Ordered Arrangement Achieves the Largest Optical Anisotropy in Wide-Bandgap Metal Chalcogenides

    Chemistry of Materials · 2026-09-09

    Wen‐Dong Yao, Xiao Huang, Qiu-Yang Du, Xu‐Bin Ni, Wenlong Liu, Sheng‐Ping Guo

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  27. Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals

    Laser & Photonics Review · 2026-09-24

    Bo Zhang, Weiqi Huang, Yang Chi, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  28. Coordination chemistry of Sb(III)-based optical crystals: from lone-pair-induced distortion to birefringence and second-harmonic generation

    Coordination Chemistry Reviews · 2026-10-06

    Liyi Zhang, Pei Liu, Liling Cao, Ling Huang, Xuehua Dong, Guohong Zou

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