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RESEARCH PAPER · Coordination Chemistry Reviews · 2025

Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairs

Hong Chen, Xin‐Tao Wu, Hua Lin

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Structure-property relationships in IR nonlinear optical chalcogenides with stereochemically active lone pairsOriginalMaximizing the second-harmonic generation response via coordination-induced localization of nonbonding electrons12Synthesis, Crystal Growth, Linear, and Nonlinear Optical Properties of Water-Grown Giant Optical Anisotropic Thiocyanates ABi(SCN) 4 (A = Rb, Cs)3A 2 Sb 2 SO 4 F 6 (A = NH 4 + , Na + ): two sulfate fluoride crystals exhibiting enhanced birefringence driven by stereochemically active antimony( iii )1Ba 4 Al 4 SnS 12 : balancing bandgap and nonlinear optical performance in thioaluminate via multifunctional group engineering0Charge-order-induced directional enhancement of non-diagonal second-order nonlinear optical tensor components2Na 2 SnSO 4 F 2 : an ultraviolet-transparent sulfate crystal with large birefringence driven by stereochemically active tin( ii )1Tailoring linear and nonlinear optical properties of 2D Sc 2 C MXenes via surface termination modulation0van der Waals layered CuInP 2 S 6 as infrared nonlinear optical material1高性能硫属化物红外非线性光学材料构效关系（特邀）0Discovery of Noncentrosymmetric Sr 3 As 2 S 7 and Sr 3 As 2 Se 2.5 S 4.5 Featuring As 3+ /As 5+ Coordination and Their Strong Nonlinear Optical Response2Polar Antiperovskite Oxides: Promising Mid-Infrared Nonlinear Optical Materials with Strong Second-Harmonic Generation2Measurement and analysis of point patterns in materials science: methods, applications, and prospects1Electronegativity Adaption Approach for Solar‐Blind UV Birefringent Crystals With Ultrawide Bandgaps2Electronegativity Adaption Approach for Solar‐Blind UV Birefringent Crystals With Ultrawide Bandgaps1The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 115The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 110Heterovalent Coexistence‐Driven Symmetry Breaking and Dimensional Evolution: Designing Polar Heart‐Shaped Channels for Exceptional MFIR Nonlinear Optics5Defect Diamond‐Like d 10 Metal Indium Selenium With Strong Second‐Harmonic Generation and Enhanced Laser‐Induced Damage Threshold2Noncentrosymmetric monomeric nickel(II) complexes with second-harmonic generation and high iodine capture capacity0From KBa 4 Ge 3 S 10 Cl to ABa 3 EuGe 3 S 11 (A = Na, K) Synthesized by Reactive Flux Assisted Metal Oxide-Boron-Chalcogen (MOBQ) Method: Effect of Cation/Anion Cosubstitution on Crystal Structure and Nonlinear Optical Properties0Salt-Inclusion Rare-Earth Chalcogenides: Exploring Infrared Nonlinear Optical Crystals via a Guest-Framework Modulation Strategy0Hierarchical Ordering Decouples the SHG–Birefringence–LIDT Trade‐Off in a Single‐Phase Mid‐Infrared Nonlinear Optical Crystal0Hierarchical Ordering Decouples the SHG–Birefringence–LIDT Trade‐Off in a Single‐Phase Mid‐Infrared Nonlinear Optical Crystal0Halogen-Mediated Dimensionality Reduction in Bismuth Oxychlorides: Trade-off between Birefringence and Band Gap0Chiral dinuclear EuIII enantiomeric pairs: simultaneously showing photoluminescences, circularly polarized luminescences, second- and third-harmonic generations with enhanced performances0From AgGaSe2 to MIIGa2Se4 (MII = Zn, Cd): Heterovalent Substitution Creates Ordered Vacancies for Balanced IR-NLO Performance0Directing Cluster Nuclearity in Semiconducting Lead Thioborates Built from Adamantane and Superadamantane Boron–Sulfur Clusters0Mixed‐Valence Engineering in Ge 2+ Chalcogenides: Structural Modulation for Balanced Infrared Nonlinear Optics0Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals0

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  1. Maximizing the second-harmonic generation response via coordination-induced localization of nonbonding electrons

    Chemical Science · 2025-11-17

    Jia-Xiang Zhang, A-Lan Xu, Yang Chi, Xin-Tao Wu, Hua Lin, Qi‐Long Zhu

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  2. Synthesis, Crystal Growth, Linear, and Nonlinear Optical Properties of Water-Grown Giant Optical Anisotropic Thiocyanates ABi(SCN) 4 (A = Rb, Cs)

    Crystal Growth & Design · 2025-12-30

    Vivian Nguyen, Chu Chu, Monique Sutherlin, Bingbing Zhang, Jian Wang

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  3. A 2 Sb 2 SO 4 F 6 (A = NH 4 + , Na + ): two sulfate fluoride crystals exhibiting enhanced birefringence driven by stereochemically active antimony( iii )

    New Journal of Chemistry · 2026-01-01

    Jia Wang, Wenbin Zhang, Zhihua Yang, Shujuan Han, Shilie Pan

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  4. Ba 4 Al 4 SnS 12 : balancing bandgap and nonlinear optical performance in thioaluminate via multifunctional group engineering

    Dalton Transactions · 2026-01-01

    Jingjing Xu, Xiaowen Wu, Bingbing Zhang, Kui Wu

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  5. Charge-order-induced directional enhancement of non-diagonal second-order nonlinear optical tensor components

    Chemical Communications · 2026-01-01

    马祖驹, Zehui Fang, Zhenlong Xie, Jia-Xiang Zhang, Hua Lin

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  6. Na 2 SnSO 4 F 2 : an ultraviolet-transparent sulfate crystal with large birefringence driven by stereochemically active tin( ii )

    Dalton Transactions · 2026-01-01

    Jia Wang, Wenbin Zhang, X. Ma, Fangfang Zhang, Hong Du, Shujuan Han

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  7. Tailoring linear and nonlinear optical properties of 2D Sc 2 C MXenes via surface termination modulation

    Dalton Transactions · 2026-01-01

    Zehui Fang, Yantong Lu, Ling Ren, Hua Lin, Rongjian Sa, Zuju Ma

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  8. van der Waals layered CuInP 2 S 6 as infrared nonlinear optical material

    Chemical Communications · 2026-01-01

    Zheng-Tao Hu, 马祖驹, Xin‐Tao Wu, Qi‐Long Zhu, Hua Lin

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  9. 高性能硫属化物红外非线性光学材料构效关系（特邀）

    Chinese Journal of Lasers · 2026-01-01

    张成龙 Zhang Chenglong, 王硕 Wang Shuo, Ailijiang Abudurusuli, 黄君本 Huang Junben

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  10. Discovery of Noncentrosymmetric Sr 3 As 2 S 7 and Sr 3 As 2 Se 2.5 S 4.5 Featuring As 3+ /As 5+ Coordination and Their Strong Nonlinear Optical Response

    Chemistry of Materials · 2026-01-27

    Vidyanshu Mishra, Jinseong Kim, Joshua Lim, Manya Rishi, Joon Ik Jang, Abishek K. Iyer

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  11. Polar Antiperovskite Oxides: Promising Mid-Infrared Nonlinear Optical Materials with Strong Second-Harmonic Generation

    Chemistry of Materials · 2026-03-26

    Yunseung Kuk, Kang Min Ok, P. Shiv Halasyamani

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  12. Measurement and analysis of point patterns in materials science: methods, applications, and prospects

    Measurement Science and Technology · 2026-03-31

    Efi-Maria Papia, Alex Kondi, Vassilios Constantoudis

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  13. Electronegativity Adaption Approach for Solar‐Blind UV Birefringent Crystals With Ultrawide Bandgaps

    Angewandte Chemie International Edition · 2026-04-23

    Xinwei Zhou, Zhiyong Bai, Ji Qi, Yuexin Zhang, Weiqi Huang, Yipeng Song, Yong Wang, Chang Liu, Sangen Zhao, Junhua Luo

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  14. Electronegativity Adaption Approach for Solar‐Blind UV Birefringent Crystals With Ultrawide Bandgaps

    Angewandte Chemie · 2026-04-23

    Xinwei Zhou, Zhiyong Bai, Ji Qi, Yuexin Zhang, Weiqi Huang, Yipeng Song, Yong Wang, Chang Liu, Sangen Zhao, Junhua Luo

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  15. The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 11

    Angewandte Chemie International Edition · 2026-04-25

    Hongshan Wang, Miriding Mutailipu, Shilie Pan, Junjie Li

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  16. The Power of Pnictogen Bond: As─As Linkages Drive Wide Bandgap, Strong NLO Response and Large Birefringence in SrGa 3 Si 4 As 11

    Angewandte Chemie · 2026-04-26

    Hongshan Wang, Miriding Mutailipu, Shilie Pan, Junjie Li

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  17. Heterovalent Coexistence‐Driven Symmetry Breaking and Dimensional Evolution: Designing Polar Heart‐Shaped Channels for Exceptional MFIR Nonlinear Optics

    Laser & Photonics Review · 2026-05-14

    B R Zhang, Ping Feng, Sheng‐Hua Zhou, Xin-Tao Wu, Hua Lin, Qi‐Long Zhu

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  18. Defect Diamond‐Like d 10 Metal Indium Selenium With Strong Second‐Harmonic Generation and Enhanced Laser‐Induced Damage Threshold

    Small · 2026-05-17

    Muhammad Zeeshan, Zhiyong Bai, Kaijie Xie, Jin Zhou, Ji Qi, Muhammad Arsalan, Liangmeng Zhu, Weiqi Huang, Junhua Luo, Sangen Zhao

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  19. Noncentrosymmetric monomeric nickel(II) complexes with second-harmonic generation and high iodine capture capacity

    Inorganic Chemistry Communications · 2026-05-25

    Xu-Wen Li, Mingqian Wang, Jun-Yi Huang, Hong‐Bin Luo, Xu-Sheng Gao, Xiao‐Ming Ren

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  20. From KBa 4 Ge 3 S 10 Cl to ABa 3 EuGe 3 S 11 (A = Na, K) Synthesized by Reactive Flux Assisted Metal Oxide-Boron-Chalcogen (MOBQ) Method: Effect of Cation/Anion Cosubstitution on Crystal Structure and Nonlinear Optical Properties

    Inorganic Chemistry · 2026-06-12

    Qiu-Yang Du, Ming-Yang Li, Nan Zhang, Wenfeng Zhou, Ru‐Ling Tang, Sheng‐Ping Guo

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  21. Salt-Inclusion Rare-Earth Chalcogenides: Exploring Infrared Nonlinear Optical Crystals via a Guest-Framework Modulation Strategy

    Inorganic Chemistry · 2026-06-15

    Wen‐Dong Yao, Qiu-Yang Du, Xu‐Bin Ni, Yi-Fan Fu, Zhi-Wei Jiang, Wenfeng Zhou, Sheng‐Ping Guo

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  22. Hierarchical Ordering Decouples the SHG–Birefringence–LIDT Trade‐Off in a Single‐Phase Mid‐Infrared Nonlinear Optical Crystal

    Angewandte Chemie International Edition · 2026-07-24

    Yan Guo, Ming‐Xin Li, Ying Guo, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  23. Hierarchical Ordering Decouples the SHG–Birefringence–LIDT Trade‐Off in a Single‐Phase Mid‐Infrared Nonlinear Optical Crystal

    Angewandte Chemie · 2026-07-24

    Yan Guo, Ming‐Xin Li, Yi Guo, Bin‐Wen Liu, Xiao‐Ming Jiang, Guo‐Cong Guo

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  24. Halogen-Mediated Dimensionality Reduction in Bismuth Oxychlorides: Trade-off between Birefringence and Band Gap

    Journal of Molecular Structure · 2026-08-03

    Huaiqiang Xun, Shumei Cao, Qingyue Cui, Yi Feng, Rui Wu, Chunmei Huang, Leyan Nian

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  25. Chiral dinuclear EuIII enantiomeric pairs: simultaneously showing photoluminescences, circularly polarized luminescences, second- and third-harmonic generations with enhanced performances

    Journal of Molecular Structure · 2026-08-28

    Xiaodi Du, Chunyang Li, Congli Gao, Tao Wu, Xi-Li Li

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  26. From AgGaSe2 to MIIGa2Se4 (MII = Zn, Cd): Heterovalent Substitution Creates Ordered Vacancies for Balanced IR-NLO Performance

    Chinese Journal of Structural Chemistry · 2026-09-01

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  27. Directing Cluster Nuclearity in Semiconducting Lead Thioborates Built from Adamantane and Superadamantane Boron–Sulfur Clusters

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  28. Mixed‐Valence Engineering in Ge 2+ Chalcogenides: Structural Modulation for Balanced Infrared Nonlinear Optics

    Advanced Optical Materials · 2026-09-23

    Chunlan Tang, Aoge Yao, Wenhao Xing, Cihai Hong, Jian Tang, Lei Kang, Jiang Huang, Jieyun Wu, Wenlong Yin, Bin Kang

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  29. Domino‐Effect Amplification via Covalent‐Chain Engineering for Giant Birefringence in NaAsQ 2 (Q = S, Se) Crystals

    Laser & Photonics Review · 2026-09-24

    Bo Zhang, Weiqi Huang, Yang Chi, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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