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RESEARCH PAPER · Journal of the American Chemical Society · 2024

Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals

Binzhi Zhao, Zhibin Hu, Yichen Sun, Rehemuhali Hajiayi, Teng Wang, Ning Jiao

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Selective Upcycling of Polyolefins into High-Value Nitrogenated ChemicalsOriginalHydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions19Photochemical upcycling of polymers via visible light-driven C–H bond activation23Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Gradient-temperature control enhances oxi-upcycling of polyethylene plastics to dicarboxylic acids over TS-1 zeolite14A Novel Upcycling Process of Polystyrene Wastes into Benzaldehyde by Catalyst-Free Laser Flash Depolymerization and In-Line Oxidation0Efficient upgrading of polystyrene plastics to nitriles through a catalytic oxidative amination process9Highly adaptable oxidative upcycling of polyolefins to multifunctional chemicals containing oxygen and nitrogen9Sustainable base-mediated chemical upcycling of poly (propylene carbonate) to β-hydroxy sulfides and oxides1Synergistic promoting effect of nickel in bimetallic catalyst for highly efficient ammonolysis of polylactic acid plastic waste into alanine0Synergistic Promoting Effect of Nickel in Bimetallic Catalyst for Highly Efficient Ammonolysis of Polylactic Acid Plastic Waste into Alanine0Upcycling of poly(ethylene terephthalate) waste plastics to terephthalonitrile6Nitrogenative Degradation of Polystyrene Waste44Photo‐Driven Direct Construction of Imidazolidines from Anilines and Paraformaldehyde and Its Application in Polyoxymethylene Plastics Usage2Selective Liquid Chemical Production in Waste Polyolefin Photorefinery by Controlling Reactive Species26Synthesis of Polyamides Bearing Directing Groups and Their Catalytic Depolymerization3Accessing a Carboxyl‐Anhydride Molecular Switch‐Mediated Recyclable PECT Through Upcycling End‐of‐Use PET20Accessing a Carboxyl‐Anhydride Molecular Switch‐Mediated Recyclable PECT Through Upcycling End‐of‐Use PET5Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19Upcycling of Waste Plastics into Value-Added Chemicals6Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes22Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes3Electrochemical Commodity Polymer Up‐ and Re‐Cycling: Toward Sustainable and Circular Plastic Treatment14Synergistic Catalysis for Recycling and Upcycling of Plastics35Nitroarenes as the Visible-Light-Responsive Photocatalysts for the Multimode Aerobic Oxidation6Photocatalytic upcycling of polysulfones at ambient conditions30Divergent Upcycling of Polystyrene into Phenol and Hydroquinone Derivatives by Photocatalysis and Electrocatalysis20Divergent Upcycling of Polystyrene into Phenol and Hydroquinone Derivatives by Photocatalysis and Electrocatalysis5Gradient Modulation of Ansa‐Metallocenes for Syndiotactic Propylene Polymerization: Multi‐Stage Remote Substituent Effects1TsOH-assisted photocatalytic aerobic upcycling of polystyrene waste6Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields6Post-polymerisation oxyfunctionalisation of styrene and butadiene-based (co-)polymers using a homogeneous manganese catalyst2Iron-Catalyzed C–H Amination of Polyethylenes11Bicyclic‐Guanidinium Benzenesulfonate: A Fingerprint Monomer for Self‐Recognizably Recyclable Polyester with Antibacterial Performance1Recent advances in thermal oxidative upcycling strategy of waste plastics under mild conditions2Chemical Upcycling of Polyphenylene Sulfide at Room Temperature6Photocatalytic oxidative cleavage of styrenes using water and chlorides for application in rubber degradation0Recent developments in recycling technologies for polymeric plastics8A Multi‐step Synergistic Strategy for Upgrading Plastic Waste into Circular Economy Feedstocks1Converting natural biopolymers to sustainable bioplastics via structure engineering15Electrochemical depolymerization of polycarbonates under catalyst-free conditions0Recent advances in chemical recycling and upcycling of plastic waste into valuable materials, chemicals, and energy: a comprehensive review18Recent Advances in Earth-Abundant Metal-Catalyzed Oxidative Degradation of Polyolefins0Synergistic Effects of Electricity and Light for Efficient Iron‐Catalyzed Recycling of Polystyrene Waste11Synergistische Effekte von Elektrizität und Licht für ein effizientes eisenkatalysiertes Recycling von Polystyrolabfällen2Catalytic upcycling of waste polystyrene plastics into production of fuels and chemicals: A review4Enhanced degradation of microplastics by laccase under ambient conditions: Analysis of underlying molecular mechanisms7Spent Battery-to-Catalyst: Asymmetric Mn–O Motifs Boost Oxygen Activation for Upgrading Polystyrene to Aromatic Oxygenates0Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling1Stepwise hydrogen spillover–engineered synergistic sites enable near-quantitative conversion of waste PET to p-xylene10Non‐Destructive Recycling of Ultra‐Strong Polyolefin Adhesives from Polymer Mixtures1Photocatalytic C–N Coupling to High-Value Chemicals from Waste Plastic and Biomass Feedstocks4Progress and prospects on oxidative depolymerization and upcycling of waste polystyrene plastics0Recycling of polyolefins using recycled PVC under sunlight7Selective Upcycling of Polycarbonate Waste to Cyclohexanol via RuLa Dual‐Atom Catalysis1Selective Upcycling of Polycarbonate Waste to Cyclohexanol via RuLa Dual‐Atom Catalysis4Solar-Driven Upcycling of Polystyrene Enabled by Elemental Sulfur8Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Pd 1.5 H 2 @PdO Nanoparticles Nanoconfined in Nitrogen‐Doped Carbon for the Aerobic Oxidation Benzaldehydes to Arylnitriles0Upcycling of Vulcanized Rubber via Controlled Backbone Cleavage and Functionalization11Precise Structural Design for Chemically Recyclable Polymers1Upcycling of polyethylene waste to biodegradable polyesters via oxidative conversion1Compressed CO 2 -Assisted Catalytic Hydrocracking of Polyethylene over Ru-Loaded Zeolites0Iron-based single-atom catalysts for selective ammoxidation of C(sp3)–H bonds and oxidative C–C cleavage reactions6A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Solvent‐ and Hydrogen‐Free Upcycling of Polystyrene by Layered Double Oxides0Single‐Atom Iron‐Catalyzed Oxidative Esterification: From Methylarenes to the Upcycling of Polystyrene and Lignin‐Derived Feedstocks0Single‐Atom Iron‐Catalyzed Oxidative Esterification: From Methylarenes to the Upcycling of Polystyrene and Lignin‐Derived Feedstocks2Natural Sunlight‐Driven Synthesis of Conjugated Microporous Polymers via Electron Donor‐Acceptor Complexes for Highly Efficient Catalytic Upcycling of Real‐World Plastic Waste0Natural Sunlight‐Driven Synthesis of Conjugated Microporous Polymers via Electron Donor‐Acceptor Complexes for Highly Efficient Catalytic Upcycling of Real‐World Plastic Waste1Photocracking of Polystyrene into Aromatic Products in CH 2 Cl 21Vacancy engineering of graphitic carbon nitride for selective photocatalytic upcycling of polystyrene: the effects of reactive oxygen species1Photocracking of Polystyrene into Aromatic Products in CH 2 Cl 20Stepwise Hydrodeoxygenation of Mixed Oxygenated Plastics Enables Sequential Production of Jet- and Gasoline-Range Fuels0Selective catalytic degradation of polyethylene by aluminum pyridine-based ionic liquids under mild conditions1Carbon radical-promoted NH bond breaking for biomass-derived amino acids to nitriles on low-coordinated Ni centers04CzIPN-Br as an Effective Photoredox Organocatalyst for Visible-Light Aerobic Upcycling of Waste Polystyrene0Selective Oxidative Upcycling of Polyethylene Pyrolyzed Wax to High‐Performance Surfactants Using Synthesized Co and Mn–Co Stearate Catalysts0Transition metal-doped Zn-Co spinel catalysts for enhanced aromatic nitriles synthesis via catalytic co-pyrolysis of PET and urea0

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  1. Hydrogen-free upcycling of polyethylene waste to methylated aromatics over Ni/ZSM-5 under mild conditions

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  2. Photochemical upcycling of polymers via visible light-driven C–H bond activation

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  3. Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions

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  4. Gradient-temperature control enhances oxi-upcycling of polyethylene plastics to dicarboxylic acids over TS-1 zeolite

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  5. A Novel Upcycling Process of Polystyrene Wastes into Benzaldehyde by Catalyst-Free Laser Flash Depolymerization and In-Line Oxidation

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  6. Efficient upgrading of polystyrene plastics to nitriles through a catalytic oxidative amination process

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  7. Highly adaptable oxidative upcycling of polyolefins to multifunctional chemicals containing oxygen and nitrogen

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  8. Sustainable base-mediated chemical upcycling of poly (propylene carbonate) to β-hydroxy sulfides and oxides

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  9. Synergistic promoting effect of nickel in bimetallic catalyst for highly efficient ammonolysis of polylactic acid plastic waste into alanine

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  10. Synergistic Promoting Effect of Nickel in Bimetallic Catalyst for Highly Efficient Ammonolysis of Polylactic Acid Plastic Waste into Alanine

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  11. Upcycling of poly(ethylene terephthalate) waste plastics to terephthalonitrile

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  14. Selective Liquid Chemical Production in Waste Polyolefin Photorefinery by Controlling Reactive Species

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  16. Accessing a Carboxyl‐Anhydride Molecular Switch‐Mediated Recyclable PECT Through Upcycling End‐of‐Use PET

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  19. Upcycling of Waste Plastics into Value-Added Chemicals

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  20. Synergistic Co‐Recycling: Selective Oxidation of Polyethylene to Dicarboxylic Acids over Spent LiCoO 2 Cathodes

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  49. Stepwise hydrogen spillover–engineered synergistic sites enable near-quantitative conversion of waste PET to p-xylene

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  50. Non‐Destructive Recycling of Ultra‐Strong Polyolefin Adhesives from Polymer Mixtures

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