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RESEARCH PAPER · Science · 2024

Polyolefin waste to light olefins with ethylene and base-metal heterogeneous catalysts

Richard J. Conk, Jules F. Stahler, Jake X. Shi, Ji Yang, Natalie G. Lefton, John N. Brunn, Alexis T. Bell, John F. Hartwig

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Polyolefin waste to light olefins with ethylene and base-metal heterogeneous catalystsOriginalThe Plastic Problem in Research Laboratories: A Call for Sustainability0Cheap catalysts close the loop on plastics production0Close-loop chemical recycling unlocked via waste polyolefins-ethylene co-metathesis2Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Influence of ball milling parameters on the mechano-chemical conversion of polyolefins35Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100Depolymerization by transition metal complexes: strategic approaches to convert polymeric waste into feedstocks3Upcycling of waste plastics: strategies, status-quo, and prospects3An efficient strategy for simultaneous gold deposition and obtention of hierarchical Au/TS-1 applied to liquid-phase propylene epoxidation0Base-Metal Heterogeneous Catalysts for Upgrading Plastics to Light Olefins3Can mixed plastics be recycled and upcycled without separation?11Influence of functional additives, fillers, and pigments on thermal and catalytic pyrolysis of polyethylene for waste plastic upcycling61Upgrading of waste polyolefins with non-noble metal catalysts21Robust, Reprocessable and Scalable Ethylene Acrylic Acid Copolymer (EAA) Derived Vitrimer Based on Dual Cross-linked Networks2Emerging Plastic Recycling Strategies Based on Photothermal Conversion15Anionic Surfactants from Reactive Separation of Hydrocarbons Derived from Polyethylene Upcycling8Solar refinery: a disruptive strategy for upcycling plastic wastes3Toward a Circular Economy of Heteroatom Containing Plastics: A Focus on Heterogeneous Catalysis in Recycling21Boosting Degradation of Polyethylene at Room Temperature4Sustainable Diesel from Rapeseed Oil Esters by Sequential Semi‐Hydrogenation, Double Bond Isomerization, and Metathesis5Advances and Challenges in Low‐Temperature Upcycling of Waste Polyolefins via Tandem Catalysis25Versatile C─H Alkylation and Alkylidenation via Catalytic Alkylidene Transfer of Enones2Versatile C─H Alkylation and Alkylidenation via Catalytic Alkylidene Transfer of Enones0Upgrading polyolefin plastics: experiences from petroleum refining and distinct characteristics19The role of the Pt-group dehydrogenation catalyst in alkane metathesis for polyolefin deconstruction9Mannich‐Type Polymers: A Versatile Platform for Water‐Degradable, Malleable, and Environmentally Responsive Networks0Mannich‐Type Polymers: A Versatile Platform for Water‐Degradable, Malleable, and Environmentally Responsive Networks0Zeolites in the epoch of catalytic recycling plastic waste: Toward circular economy and sustainability20The Plastic Problem in Research Laboratories: A Call for Sustainability5Selective conversion of polyolefin waste to light olefins by tandem catalytic cracking and isomerizing ethenolysis2Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth5Iron(III)‐Catalyzed C─H Hydroxylation of Low‐Density Polyethylene Coupled with Short Chain Branching Growth2Advances in reaction coupling technologies for efficient conversion of low-carbon molecules1Co-recycling of plastics and other waste materials70A Broad-Spectrum Catalyst for Aliphatic Polymer Breakdown4Methanolysis of mixed plastics catalyzed by ionic liquid: PET depolymerization and recycling of PP/PE8Methanol‐Facilitated Cascaded Polyolefin Upcycling Enabling the Efficient Generation of High‐Value C 9+ Alkylaromatics7Methanol‐Facilitated Cascaded Polyolefin Upcycling Enabling the Efficient Generation of High‐Value C 9+ Alkylaromatics0Uncovering strategies for quantifying thermo-kinetics, reaction heat, and synergistic rates of heat transfer-degradation in the chemical upcycling of polyolefins5Photocatalytic upcycling of polysulfones at ambient conditions30Highly selective aerobic oxidation of polystyrene to benzoic acid catalyzed by nitrogen dioxide9Adjustable Upcycling of Polyethylene Terephthalate to Biodegradable Polymer Monomers by Mn‐Catalyzed Solvent Switching Strategy26Adjustable Upcycling of Polyethylene Terephthalate to Biodegradable Polymer Monomers by Mn‐Catalyzed Solvent Switching Strategy0From Polyethylene to Conjugated Polyenes: a Mechanochemical One‐Pot Upcycling Strategy for Selective Functionalization1From Low-Cost Industrial Byproducts to High-Performance Flexible Films and Water-Based Hydrophobic Coatings via Green Processes0Catalytic and selective chemical recycling of post-consumer rubbers into cycloalkenes17Current developments in multifunctional technology for waste plastic chemical recycling and case studies0The Science of Polymer Chemical Recycling Catalysis: Uncovering Kinetic and Thermodynamic Linear Free Energy Relationships30In-line NMR guided orthogonal transformation of real-life plastics63The role of H2 donation in heterogeneous Mo-based olefin metathesis site creation0Mechanistic alteration of polyethylene oxidation via heterogenous catalysis for enhanced fatty di-carboxylic acid yields6Block copolymer molecular design to address practical limitations to recycling polyolefin blends12Waste polyethylene to long-chain unsaturated esters and alcohols via alkene cross-metathesis0Catalysis for the Energy Transition8Enhancing Mechanical Properties and Crystallization Kinetics of Isotactic Polypropylene by Boronic Acid-Cross-Linked Additives3Facile Synthesis of Polyhydroperoxides from Ethylene and Carbon Monoxide10Integrated low-temperature PVC and polyolefin upgrading38Efficient conversion of polyethylene to light olefins by self-confined cracking and reforming22High value olefins from polypropylene by in situ catalytic pyrolysis4Catalytic Depolymerization of Plastics to Valuable Products7Novel nanocomposite enables self-supporting, high-mass-loading carbon cathodes for advanced zinc-ion capacitors1High-Resolution Mapping of the Nordic Plastic Cycle Suggests Capacity Expansion for Both Mechanical and Chemical Recycling1Pyrolysis kinetics, volatile evolution, and backbone degradation mechanisms of typical nitrogen-containing plastics based on TG-FTIR-GC/MS and density functional theory8Closed-loop recycling of polyethylene to ethylene and propylene via a kinetic decoupling–recoupling strategy32The role of catalyst acidity and microstructure on light olefin selectivity in polyethylene deconstruction in short contact time pulse Joule-heated reactors3Mechanistic insights into support-induced catalyst activity and deactivation pathways of Co-Ni-Mo catalyst during biomass pyrolysis-chemical vapor deposition process2Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation1Selective, Oxygen‐Tunable, and Metal‐Free Functionalization of Polyethylene Through Dual‐Mode Nitrosation and Carbonylation7Upcycling of Disposable Face Masks into Water‐Resistant and Flame Retardant Foams3Active Site Dynamics in Molybdenum-Based Silica-Supported Olefin Metathesis Catalysts: Site Renewal and Decay Beyond the Chauvin Cycle5Fractionated degradation and valorization of polypropylene waste into sulfonate surfactants2Decarboxylation-Triggered Polymer Deconstruction11Tuning High-Density Polyethylene Microstructure and Properties from Known Distributions of Dynamic Bonds7Breaking the yield–selectivity trade-off in polystyrene waste valorization via tandem depolymerization and hydrogenolysis18Chemical recycling of polyolefin wastes: recent advances and insights into recycling routes0Electrocatalytic dechlorination of polyvinylidene chloride for tandem dual radical-driven synthesis of β-chloroalcohols0Chemical Upcycling of Polyphenylene Sulfide at Room Temperature6A self-regenerative Sn–W/γ-Al 2 O 3 catalyst for low-carbon and scalable polyolefin upcycling via tandem dehydrogenation–metathesis2Decoupling Acidity from Micropore Confinement in an Amorphous–Crystalline Composite for Selective Polyolefin Waste Cracking14Recent developments in recycling technologies for polymeric plastics8Carbon–carbon bond cleavage for lignin and plastics deconstruction0Direct upcycling of mixed plastic waste into liquid alkanes3Metal-free carbocatalysts for the selective production of ethylbenzene and cumene from mixed plastic waste0Photoreforming of plastic waste into value-added chemicals with hydrogen production4Pyrolysis kinetics and backbone decomposition mechanisms of nylon 6/6: insights from TG-FTIR-GC/MS and density functional theory0Recent Advances in Earth-Abundant Metal-Catalyzed Oxidative Degradation of Polyolefins0Site surgery in single atom catalysis: machine learning assisted precise regulation of coordination environment and decoding of structure-activity relationships4Unsaturated C2 synthons in photocatalysis: Taming and directing acetylene and ethylene in radical reactions2Highly Selective Conversion of Polyethylene Terephthalate into Liquid Fuel via Nb-Assisted Ru Bimetallic Catalyst15Thiol-Regulated Rhodium Nanocatalyst for Electrochemical Reductive Perdeuteration of Alkenes9Synergistic Effects of Electricity and Light for Efficient Iron‐Catalyzed Recycling of Polystyrene Waste11Synergistische Effekte von Elektrizität und Licht für ein effizientes eisenkatalysiertes Recycling von Polystyrolabfällen2Synergistic Alloy and Support Effects in Covalent Organic Framework‐Stabilized AuPd Catalysts for Aerobic 5‐Hydroxymethylfurfural Oxidation to 2,5‐Furandicarboxylic Acid2Current perspective on heterogeneous thermal catalytic approaches for closed-loop polyolefin plastic recycling1Mild‐Condition Upcycling of Polyolefins Enabled by Micropore Confinement in Zeolites3Mild‐Condition Upcycling of Polyolefins Enabled by Micropore Confinement in Zeolites5Non‐Destructive Recycling of Ultra‐Strong Polyolefin Adhesives from Polymer Mixtures1Heterogeneous olefin metathesis promotion using molecular hydrogen0Mechanically Triggered Chemical Recyclable Polyethylene‐Like Materials1Mechanically Triggered Chemical Recyclable Polyethylene‐Like Materials5Recycling of polyolefins using recycled PVC under sunlight7Selective Upcycling of Polycarbonate Waste to Cyclohexanol via RuLa Dual‐Atom Catalysis1Selective Upcycling of Polycarbonate Waste to Cyclohexanol via RuLa Dual‐Atom Catalysis4Balancing polyolefins waste and CO2 upcycling via microwave-stimulated oxygen dynamics1Synergistic bifunctional catalysis and plasma activation for valorizing polypropylene and CO2 to gasoline-range olefins1Thermo-chemical upgrading of waste polyethylene and polypropylene plastics0Upcycling and Redesigning of Polyolefins3Deep and precise polyethylene upgrading via tandem cracking0One-pot co-upcycling of mixed polyolefin waste6Upcycling of Vulcanized Rubber via Controlled Backbone Cleavage and Functionalization11Cleavage Alkylation Coupling with Versatile Amide-Based Eutectic Catalytic Systems0Enhancing carbon nanotubes production from pyrolysis–catalysis of plastic waste through monolithic heating18Interfacial configurational entropy tuning strategy enabling liquid alloys for efficient depolymerization of polyolefin waste2Heterogeneous Transfer Dehydrogenation for Catalytic Upcycling of Polyethylene0Shape-Selective Conversion of High-Density Polyethylene into Benzene with Zeolite-Encapsulated Subnanometer Pt Catalysts6Electrochemically mediated disproportionation for selective formaldehyde upcycling in acid2Selective Upcycling of Waste Polyethylene into Propane Facilitated by the Undulation Confinement Effect in Zeolite Channels5Direct Polymer-on-Polymer Grafting of Polyolefins under Visible Light2Site-selective dehydrogenation and protonation synergy for efficient polyolefin upcycling into aromatics0Chemical recycling via precision depolymerization: fundamentals, design principles, and emerging frontiers for circular polymer systems3Adaptive Brønsted Acidity From Heterolytic Dihydrogen Activation Enables Polyethylene Hydrogenolysis Over Pd‐Encapsulated Na‐Zeolites2Adaptive Brønsted Acidity From Heterolytic Dihydrogen Activation Enables Polyethylene Hydrogenolysis Over Pd‐Encapsulated Na‐Zeolites1Phosphorus-modified plate-like ZSM-5 for oriented regulation of product distribution in catalytic plastic cracking0Atomic-Scale Mapping of Atomically Dispersed Light-Element Species in Oxide Nanomaterials by Solid-State NMR0A Panoramic View on Plastic Waste Recycling and Upcycling: Heterogeneous Catalytic Strategies for Diverse Plastics and Multiple Pathways6Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Atomically precise catalysts design toward efficient waste plastic hydrogenolysis2A Review on Catalyst Chemical Recycling Technologies for Production of Light Gaseous Compounds from Polyolefin Waste1Liquid alloy-driven ambient upcycling of fluoropolymer waste1Light‐Driven Coupled Upcycling of Polyethylene and CO 2 to Aromatics over Zeolite–Ni/CeO 2 Composite Catalysts0Quantitative Polyethylene Upcycling to Liquid Olefins over Ru-Containing Layered Zeolites0Encounter-State Over-Anchoring Governs Productive PETase Binding on PET Surfaces0Unrecyclable Polyethylene as a Catalytic Metal Support for Organic Reactions0Chlorine Radical Mediated Tandem Dehydrogenation–Oxidation for Upcycling Polyolefins to Functional Wax at Low Temperature in Air0Chlorine Radical Mediated Tandem Dehydrogenation–Oxidation for Upcycling Polyolefins to Functional Wax at Low Temperature in Air0From Polyolefin Plastics Back to Olefins: Chemical Recycling and Circular Economy0Toward Full-Range Recycling of Disposable Diapers0Bridging barriers: Integrated process intensification and catalytic strategies for valorizing waste polyolefin plastics to hydrocarbon products0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Ambient‐Pressure Polyolefin Upcycling With Earth‐Abundant Catalyst0Efficient solar-driven interfacial steam-hydropower co-generation by high-quality carbon nanotube from discarded polyolefin separator0Atomically dispersed cerium enabling mild polyolefin hydrocracking to simple gas streams0Covalent‐Organic Framework‐Manipulated Multi‐Reactant Activation Enables Polystyrene Electrodegradation in Tandem With Over‐Oxidation Product Upgrading0Covalent‐Organic Framework‐Manipulated Multi‐Reactant Activation Enables Polystyrene Electrodegradation in Tandem With Over‐Oxidation Product Upgrading0Ru Single‐Atom Anchored Zeolite for Selective Upcycling of Polyolefins Into Butanes0Ru Single‐Atom Anchored Zeolite for Selective Upcycling of Polyolefins Into Butanes0Hierarchical Accessibility and Framework‐Al Organization in Ultra‐High‐Silica ZSM‐5 Enable Efficient Cracking of Polyolefin Waste to Light Olefins0Hierarchical Accessibility and Framework‐Al Organization in Ultra‐High‐Silica ZSM‐5 Enable Efficient Cracking of Polyolefin Waste to Light Olefins0Challenges in polyolefin re/upcycling catalysis specific to polymer feedstock0

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  50. The role of H2 donation in heterogeneous Mo-based olefin metathesis site creation

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