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RESEARCH PAPER · Inorganic Chemistry Frontiers · 2022

(C 3 N 6 H 7 ) 2 SiF 6 ·H 2 O: an ultraviolet birefringent crystal exceeding the intrinsic energy gap of an organic reagent

Yaoguo Shen, Yingwu Zhou, Xiaoling Xue, Hualiang Yu, Sangen Zhao, Junhua Luo

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(C 3 N 6 H 7 ) 2 SiF 6 ·H 2 O: an ultraviolet birefringent crystal exceeding the intrinsic energy gap of an organic reagentOriginalC 10 H 10 ClNO 3 : exploration of birefringent crystals in an isoquinoline system20C 10 H 6 NO 2 Cd(NO 3 )·2H 2 O: a birefringent crystal with an enlarged band-gap derived from covalent edge-sharing connection4C 3 N 6 H 7 SO 3 NH 2 : non-π-conjugated tetrahedra decoupling π-conjugated groups achieving large optical anisotropy and wide band gap29Design and synthesis of anisotropic crystals with π -conjugated rings toward giant birefringence36Two UV optical crystals with strong optical anisotropy, large band gaps and an α-BBO type structure7β-(C 3 H 7 N 6 ) 2 Cl 2 ·H 2 O and (C 3 H 7 N 6 )F·H 2 O: two UV birefringent crystals induced by uniformly aligned structural groups35Naphthalene-Like Unit That Induces Strong Optical Anisotropy in C10H8NO2Br and C10H8NO2Br·H2O12C14H10BrNO2: A Birefringent Crystal with an Expanded π-Conjugated Group13Cs2Pb4Br10: A layered perovskite shows large birefringence11Designing Sulfate Crystals with Strong Optical Anisotropy through π‐Conjugated Tailoring51Designing Sulfate Crystals with Strong Optical Anisotropy through π‐Conjugated Tailoring11(C 3 N 6 H 7 )BF 4 ·H 2 O and (C 3 N 6 H 7 )SO 3 CH 3 ·H 2 O with large birefringence induced by coplanar π-conjugated [C 3 N 6 H 7 ] + groups33Crystal clear: unveiling giant birefringence in organic–inorganic cocrystals33Pb 2 (SeO 3 )(SiF 6 ): the first selenite fluorosilicate with a wide bandgap and large birefringence achieved through perfluorinated group modification45Research progress in optical materials with cationic organic planar π-conjugated groups containing CN bonds34Exceptional Optical Anisotropy Enhancement Achieved Through Dual‐Ions Cosubstitution Strategy in Novel Hybrid Bismuth Halides23C9H7NBrX (X = Cl, Br, NO3): Three Excellent Birefringent Crystals with Distinct Optical Anisotropy Regulated by Anions34Noncentrosymmetric Crystal [C10H8NO2]2SiF6·H2O with Large Birefringence12[C8H6BrN2O]Cl and [C8H6IN2O]Cl: Two birefringent crystals with π-conjugated quinazoline groups2[C3H7N6]3[B3O5(OH)2] and [C3H8N6]4[B12O19(OH)6]: Two Melamine Borates with Large Birefringence13(C 5 N 2 H 7 )IO 2 F 2 and (C 3 N 6 H 8 )(IO 2 F 2 ) 2 : two new organic–inorganic hybrid fluoroiodate birefringent crystals7(C 7 H 3 NO 4 ) 2 Sb 2 F 2 ·2H 2 O: a pyridine-based compound shows large optical anisotropy4[C(NH 2 ) 3 ] 2 [C 2 H 5 (C 2 O 4 )]Cl: rational design of a metal-free UV birefringent crystal through the synergistic assembly of three distinct motifs5Greatly enhancing birefringence of fluorosilicates through the synergetic effect of functional units13Recent progress in structural design strategies of high-birefringence optical crystals54[CON3H6BF4]: An Efficient Metal‐Free Borate with Optimized Birefringence Achieved by Structural Design Strategy15[C( NH2 )3] 2SiF6 : Design of Deep Ultraviolet Crystals with Large Birefringence Based on a Fluorination‐Oriented Strategy13Four Benzoguanamine-Based Birefringent Crystals with Excellent Optical Anisotropy5Anion-Ordered [B3O5(OH)2] Induced by Crystal Water with Deep Ultraviolet Transparency and Large Birefringence in Boron-Rich Borophosphates4Enhancing Birefringence via a Planar‐Conformation‐Locking Strategy3Na6(SO4)2SiF6: A Stable Sulfate Fluosilicate with Wide Deep-Ultraviolet Transparency Window and Strong Second-Harmonic Generation Response4Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion17Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion2Hydrogen‐Bond‐Driven Metal‐Free Crystal (C 6 H 7 N 2 O)(NH 2 SO 3 ) with Giant Birefringence and Solar‐Blind Ultraviolet Transmission0Achieving Ultra‐High Optical Anisotropy via Structural Regulation and Coplanar Engineering of Extended π‐Conjugated [H 2–x C 3 N 3 S 3 ] (x = 1, 2) Groups3Cationic‐Dual‐Modulated Linear and V‐Shaped Birefringent‐Active Unit Generates Remarkable Birefringence6Dual-tuning birefringence in hybrid crystals via Cd/Zn metal center and organic ligand isomerism0Strategically designed deep-ultraviolet optical crystals with balanced properties by small heteroatom substitution1

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  1. C 10 H 10 ClNO 3 : exploration of birefringent crystals in an isoquinoline system

    Inorganic Chemistry Frontiers · 2023-01-01

    Hao Chen, Shaobin Zhang, Bo Wen Chen, Yaoguo Shen, Junhua Luo

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  2. C 10 H 6 NO 2 Cd(NO 3 )·2H 2 O: a birefringent crystal with an enlarged band-gap derived from covalent edge-sharing connection

    Dalton Transactions · 2023-01-01

    Yu Wang, Yaoguo Shen, Weiqi Huang, Sangen Zhao

    Read original paper ↗ ·

  3. C 3 N 6 H 7 SO 3 NH 2 : non-π-conjugated tetrahedra decoupling π-conjugated groups achieving large optical anisotropy and wide band gap

    Materials Chemistry Frontiers · 2023-01-01

    Danyang Dou, Qi Shi, Yunjie Bai, Cheng Chen, Bingbing Zhang, Ying Wang

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  4. Design and synthesis of anisotropic crystals with π -conjugated rings toward giant birefringence

    Materials Chemistry Frontiers · 2023-01-01

    Yunqi Zhao, Liangmeng Zhu, Yanqiang Li, Xiaojun Kuang, Junhua Luo, Sangen Zhao

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  5. Two UV optical crystals with strong optical anisotropy, large band gaps and an α-BBO type structure

    Dalton Transactions · 2023-01-01

    Lehui Liu, Feifei Yuan, Yisheng Huang, Zhoubin Lin, Lizhen Zhang

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  6. β-(C 3 H 7 N 6 ) 2 Cl 2 ·H 2 O and (C 3 H 7 N 6 )F·H 2 O: two UV birefringent crystals induced by uniformly aligned structural groups

    Inorganic Chemistry Frontiers · 2023-01-01

    Yaoguo Shen, Liang Ma, Guofa Dong, Hualiang Yu, Junhua Luo

    Read original paper ↗ ·

  7. Naphthalene-Like Unit That Induces Strong Optical Anisotropy in C10H8NO2Br and C10H8NO2Br·H2O

    Inorganic Chemistry · 2023-05-19

    Yaoguo Shen, Yingwu Zhou, Xiaoling Xue, Guofa Dong

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  8. C14H10BrNO2: A Birefringent Crystal with an Expanded π-Conjugated Group

    Crystal Growth & Design · 2023-08-03

    Yaoguo Shen, Zixiang Chen, Guofa Dong, Junhua Luo

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  9. Cs2Pb4Br10: A layered perovskite shows large birefringence

    Inorganic Chemistry Communications · 2023-08-26

    Bo Chen, Hao Chen, Shaobin Zhang, Yaoguo Shen

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  10. Designing Sulfate Crystals with Strong Optical Anisotropy through π‐Conjugated Tailoring

    Angewandte Chemie International Edition · 2023-10-27

    Zhiyong Bai, Kang Min Ok

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  11. Designing Sulfate Crystals with Strong Optical Anisotropy through π‐Conjugated Tailoring

    Angewandte Chemie · 2023-10-27

    Zhiyong Bai, Kang Min Ok

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  12. (C 3 N 6 H 7 )BF 4 ·H 2 O and (C 3 N 6 H 7 )SO 3 CH 3 ·H 2 O with large birefringence induced by coplanar π-conjugated [C 3 N 6 H 7 ] + groups

    Inorganic Chemistry Frontiers · 2024-01-01

    Hangwei Jia, Die Xu, Zi‐Jian Li, Muhammad Sharjeel Arif, Yansheng Jiang, Xueling Hou

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  13. Crystal clear: unveiling giant birefringence in organic–inorganic cocrystals

    Chemical Science · 2024-01-01

    Yang Li, Kang Min Ok

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  14. Pb 2 (SeO 3 )(SiF 6 ): the first selenite fluorosilicate with a wide bandgap and large birefringence achieved through perfluorinated group modification

    Chemical Science · 2024-01-01

    Pengfei Li, Chun‐Li Hu, Jiang‐Gao Mao, Fang Kong

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  15. Research progress in optical materials with cationic organic planar π-conjugated groups containing CN bonds

    Inorganic Chemistry Frontiers · 2024-01-01

    Hangwei Jia, Xueling Hou, Shilie Pan

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  16. Exceptional Optical Anisotropy Enhancement Achieved Through Dual‐Ions Cosubstitution Strategy in Novel Hybrid Bismuth Halides

    Small · 2024-01-17

    Zhiyong Bai, Kang Min Ok

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  17. C9H7NBrX (X = Cl, Br, NO3): Three Excellent Birefringent Crystals with Distinct Optical Anisotropy Regulated by Anions

    Small · 2024-05-10

    Yaoguo Shen, Mingliang Ding, Gang Chen, Yingjie Luo, Sangen Zhao, Junhua Luo

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  18. Noncentrosymmetric Crystal [C10H8NO2]2SiF6·H2O with Large Birefringence

    Inorganic Chemistry · 2024-07-12

    Liqin Liu, Hai‐Lan Huang, Mingliang Ding, Yaoguo Shen

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  19. [C8H6BrN2O]Cl and [C8H6IN2O]Cl: Two birefringent crystals with π-conjugated quinazoline groups

    Inorganic Chemistry Communications · 2024-09-16

    Zhifeng Tang, Hai‐Lan Huang, Yuxin Zhou, Yu Wang, Yaoguo Shen, Renwen Yan, Lin Wu

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  20. [C3H7N6]3[B3O5(OH)2] and [C3H8N6]4[B12O19(OH)6]: Two Melamine Borates with Large Birefringence

    Inorganic Chemistry · 2024-11-18

    Ya-Lan Deng, Chun‐Li Hu, Jiang‐Gao Mao

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  21. (C 5 N 2 H 7 )IO 2 F 2 and (C 3 N 6 H 8 )(IO 2 F 2 ) 2 : two new organic–inorganic hybrid fluoroiodate birefringent crystals

    Dalton Transactions · 2025-01-01

    Si Yuan, Chun‐Li Hu, Jiang‐Gao Mao

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  22. (C 7 H 3 NO 4 ) 2 Sb 2 F 2 ·2H 2 O: a pyridine-based compound shows large optical anisotropy

    Dalton Transactions · 2025-01-01

    Yaoguo Shen, Jiajia Xiong, Yiman Yang, Zhifeng Tang

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  23. [C(NH 2 ) 3 ] 2 [C 2 H 5 (C 2 O 4 )]Cl: rational design of a metal-free UV birefringent crystal through the synergistic assembly of three distinct motifs

    Chemical Communications · 2025-01-01

    Yu-Ming Pan, Xinyou An, Zhi Gang Fang

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  24. Greatly enhancing birefringence of fluorosilicates through the synergetic effect of functional units

    Inorganic Chemistry Frontiers · 2025-01-01

    Liang Ma, Yi‐Lei Lv, Bing-Wei Miao, Guo-Ren Zhu, Wenlong Liu, Sheng‐Ping Guo, Ru‐Ling Tang

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  25. Recent progress in structural design strategies of high-birefringence optical crystals

    Coordination Chemistry Reviews · 2025-05-08

    A-Lan Xu, Mao‐Yin Ran, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  26. [CON3H6BF4]: An Efficient Metal‐Free Borate with Optimized Birefringence Achieved by Structural Design Strategy

    Small · 2025-05-23

    Muhammad Arif, Xu Liu, Hangwei Jia, Zhihua Yang, Xueling Hou, Shilie Pan

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  27. [C( NH2 )3] 2SiF6 : Design of Deep Ultraviolet Crystals with Large Birefringence Based on a Fluorination‐Oriented Strategy

    Chinese Journal of Chemistry · 2025-06-24

    Shaohua Liu, Xiaoqin Ma, Xifa Long, Yun Mo Yang

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  28. Four Benzoguanamine-Based Birefringent Crystals with Excellent Optical Anisotropy

    Inorganic Chemistry · 2025-07-19

    Yaoguo Shen, Lingxin Yan, Xin‐Yi Wang, Zhifeng Tang, Liang Ma, Guofa Dong

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  29. Anion-Ordered [B3O5(OH)2] Induced by Crystal Water with Deep Ultraviolet Transparency and Large Birefringence in Boron-Rich Borophosphates

    Chemistry of Materials · 2025-08-20

    Huanhuan Zhao, Chenxu Li, Zhihua Yang, Xueling Hou, Jian Wei Han, Shilie Pan

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  30. Enhancing Birefringence via a Planar‐Conformation‐Locking Strategy

    Laser & Photonics Review · 2025-09-04

    Yaoguo Shen, Jiajia Xiong, Mengqing Wu, M.-R. Li, Yingwu Zhou, Yanjie Zhang

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  31. Na6(SO4)2SiF6: A Stable Sulfate Fluosilicate with Wide Deep-Ultraviolet Transparency Window and Strong Second-Harmonic Generation Response

    Chemistry of Materials · 2025-10-02

    Zilong Geng, Zuju Ma, Ruibiao Fu, Xintao Wu

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  32. Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion

    Angewandte Chemie International Edition · 2025-11-26

    Xiangyu Long, Fuming Li, Haotian Qiu, Xueling Hou, Juanjuan Lu, Junjie Li, Zhihua Yang, Jinhui Cao, Shilie Pan, Miriding Mutailipu

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  33. Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion

    Angewandte Chemie · 2025-11-26

    Xiangyu Long, Fuming Li, Haotian Qiu, Xueling Hou, Juanjuan Lu, Junjie Li, Zhihua Yang, Jinhui Cao, Shilie Pan, Miriding Mutailipu

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  34. Hydrogen‐Bond‐Driven Metal‐Free Crystal (C 6 H 7 N 2 O)(NH 2 SO 3 ) with Giant Birefringence and Solar‐Blind Ultraviolet Transmission

    Advanced Optical Materials · 2025-12-10

    Zhenkai Cen, Z.-Y. Li, Guang Peng, Junbo Gong, Junbo Gong

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  35. Achieving Ultra‐High Optical Anisotropy via Structural Regulation and Coplanar Engineering of Extended π‐Conjugated [H 2–x C 3 N 3 S 3 ] (x = 1, 2) Groups

    Advanced Functional Materials · 2025-12-12

    Muhammad Arif, Xu Liu, Hangwei Jia, Zhihua Yang, Xueling Hou, Shilie Pan

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  36. Cationic‐Dual‐Modulated Linear and V‐Shaped Birefringent‐Active Unit Generates Remarkable Birefringence

    Advanced Optical Materials · 2025-12-29

    Jing‐Jing Zhao, Shu‐Fang Li, Jin K. Chen, Hongbo Huang, Bingbing Zhang, Dong Yan

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  37. Dual-tuning birefringence in hybrid crystals via Cd/Zn metal center and organic ligand isomerism

    Dalton Transactions · 2026-01-01

    Yaoguo Shen, Xinyi Wang, Mengqing Wu, Yiman Yang, Lingxin Yan

    Read original paper ↗ ·

  38. Strategically designed deep-ultraviolet optical crystals with balanced properties by small heteroatom substitution

    Inorganic Chemistry Frontiers · 2026-01-01

    Mei Hu, Zhencheng Wu, Xin Su, Hongheng Chen, Qun Jing, Zhaohui Chen, Ming‐Hsien Lee

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