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RESEARCH PAPER · Advanced Materials · 2021

Tailoring of White Luminescence in a NaLi 3 SiO 4 :Eu 2+ Phosphor Containing Broad‐Band Defect‐Induced Charge‐Transfer Emission

Ming Zhao, Zhiyu Yang, Lixin Ning, Zhiguo Xia

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Tailoring of White Luminescence in a NaLi 3 SiO 4 :Eu 2+ Phosphor Containing Broad‐Band Defect‐Induced Charge‐Transfer EmissionOriginalA solid-solution modulation strategy in trivalent bismuth-doped gallate phosphors for single substrate tunable emission5Defect engineering in trivalent ion doped ceria through vanadium assisted charge compensation: insight using photoluminescence, positron annihilation and electron spin resonance spectroscopy22Enhancing the near-infrared photocatalytic activity and upconversion luminescence of BiOCl:Yb 3+ –Er 3+ nanosheets with polypyrrole in situ modification24Narrowband ultraviolet-B persistent luminescence from (Y,Gd) 3 Ga 5 O 12 :Bi 3+ phosphors for optical tagging application28Bismuth activated blue phosphor with high absorption efficiency for white LEDs55Chasing Down the Eu2+ Ions: The Delicate Structure−Property Relationships in the Ultra‐Narrow Band Phosphor K1.6Na2.1Li0.3[Li3SiO4]4:Eu2+35Achievement of high-efficiency sunlight-like emission in Rb2CaP2O7: Ce3+, Eu2+ phosphors16Double perovskite microcrystals-based white light-emitting diodes without reabsorption of multiphase phosphors13Tailoring Luminescent Properties of SrS:Ce by Modulating Defects: Sr-Deficiency and Na+ Doping1Composition and Antithermal Quenching of Noninteger Stoichiometric Eu2+-Doped Na-β-Alumina with Cyan Emission for Near-UV WLEDs37Design of efficient color-tunable long persistent luminescence phosphor BaGa 2 O 4 :Pr 3+ and its performance enhancement via a trap-induced strategy56Unveiling White Light Emission of a One-Dimensional Cu(I)-Based Organometallic Halide toward Single-Phase Light-Emitting Diode Applications39Site occupancy and luminescence of Ce3+-doped NaK2Li[Li3SiO4]4: A first-principles study3(INVITED)Broadband emission of Lu2SrAl4SiO12:Eu2+ phosphor for full-spectrum lighting6A full visible LED enabled by a broadband yellow emission nepheline phosphor derived from a europium doped SOD zeolite16A novel red-emitting phosphor K 2 MgGeO 4 :Eu 3+ for WLEDs: zero-thermal quenching induced by heterovalent substitution27A novel red-emitting phosphor with an unusual concentration quenching effect for near-UV-based WLEDs40A single-component white-light-emitting fluorescent material with high color rendering index based on resonance energy transfer11Antimony -doped indium-based halide single crystals enabling white-light emission47Broad luminescence tuning in Mn 2+ -doped Rb 2 Zn 3 (P 2 O 7 ) 2 via doping level control based on multiple synergies10Compensation effect of electron traps for enhanced fluorescence intensity ratio thermometry performance22Dual-Site Occupancy Induced Blue Emission in Both Eu2+ and Ce3+ Doped Naba3si2o7f0Enhanced Photoluminescence in Cd xZn (1-x)S Solid Solution Through Defect Activation Strategy to Suppress the Non-Radiative Recombination0Enhanced Photoluminescence in Cd xZn (1-x)S y Solid Solution Through Defect Activation Strategy to Suppress the Non-Radiative Recombination0Enhancing the luminescence performance of Ca 2− x Sr x BO 3 Cl:Eu 2+ ,Dy 3+ by substitution of Sr 2+ for Ca 2+9Eu 2+ -activated MgAl 2 Si 4 O 6 N 4 : a novel oxonitridoalumosilicate blue phosphor for white LEDs6Locally-ordered A-site vacancy assisted photoluminescence enhancement in simply rare-earth doped perovskite oxide13NASICON-type Na 3.6 Lu 1.8− x (PO 4 ) 3 : x Eu 3+ phosphors: structure and luminescence7Self-reduction-induced BaMgP 2 O 7 :Eu 2+/3+ : a multi-stimuli-responsive phosphor for X-ray detection, anti-counterfeiting and optical thermometry36The explanation of abnormal thermal quenching of the charge transfer band based on thermally coupled levels and applications as temperature sensing probes21Eu2+‐Doped Layered Double Borate Phosphor with Ultrawide Near‐Infrared Spectral Distribution in Response to Ultraviolet–Blue Light Excitation110How to Obtain Anti‐Thermal‐Quenching Inorganic Luminescent Materials for Light‐Emitting Diode Applications252High-performance narrow-band green-emitting phosphor enabled by substituting Na with Rb6Near-UV excited green-emission enhancement by efficient energy transfer in Na1.8Mg0.9Si1.1O4:Ce3+,Tb3+ phosphor for solid-state lighting applications13Simultaneous Spectral Tuning and Thermal Stability Adjustment in Ca8ZnGa(1–x)Lax(PO4)7:Eu2+ Phosphors23Microscopic Mechanism of the Heat‐Induced Blueshift in Phosphors and a Logarithmic Energy Dependence on the Nearest Dopant–Vacancy Distance24Microscopic Mechanism of the Heat‐Induced Blueshift in Phosphors and a Logarithmic Energy Dependence on the Nearest Dopant–Vacancy Distance1Tailoring the Luminescent Properties of SrS:Ce3+ by Sr-Deficiency and Na+ Doping15Adjustable luminescence properties of Eu3+ and Bi3+ codoped Ca3Zn3Te2O12 phosphor30Carbon dots embedded in lead-free luminescent metal halide crystals toward single-component white emitters32Deep-level trap formation in Si-substituted Sr2SnO4:Sm3+ for rewritable optical information storage27Time-resolved and temperature-dependent spectroscopy for blue luminescence of monoclinic YSiO2N:Ce3+ phosphor11Role of the Rigid Host Structure in Narrow-Band Green Emission of Eu2+ in Rb2Na2(Li3SiO4)4: Insights into Electron–Phonon Coupling15Novel Orange-Emitting Phosphor Ba2LuGaO5:Bi3+ with High Efficiency and Thermal Robustness Induced by D-Band Emission23Multiple Strategies to Approach High-Efficiency Luminescence Controllable in Blue/Cyan/Green-Emitting Bi 3+ -Activated Phosphors30Evolutionary Generation of Phosphor Materials and Their Progress in Future Applications for Light-Emitting Diodes563Resistance to aggregation-caused quenching: chitosan-based solid carbon dots for white light-emitting diode and 3D printing85Modulating the emission spectrum of Ca2La8(SiO4)6O2:Eu(2+,3+) phosphor through Mn2+ ion doping3Influence of Mn2+ doping on the emission spectrum of Sr2La8(SiO4)6O2:Eu(2+,3+) phosphor8Towards single broadband white emission in Rb0.5K1.5CaPO4(F, Cl): Eu2+ via selective site occupancy engineering for solid-state lighting applications42High-Efficiency Continuous-Luminescence-Controllable Performance and Antithermal Quenching in Bi 3+ -Activated Phosphors35Ultra‐Broadband Green‐Emitting Phosphors without Cyan Gap Based on Double‐Heterovalent Substitution Strategy for Full‐Spectrum WLED Lighting89Mechanochemical Fabrication of a Mn4+-Activated Inorganic Rb2KTiOF5 Perovskite Red Phosphor for White Light-Emitting Diodes3Synthesis and photoluminescence properties of a novel green‐emitting LiYGeO4:Tb3+ long afterglow phosphor9Luminescence properties, tunable emission and energy transfer of Ca9MgLi(PO4)7:Bi3+/Eu3+ phosphor19Shining Transparent Displays with Stable Narrow‐Band Blue‐Emitting Phosphor in Layered Film50Accurately Controlling the Occupation of Eu2+ in Cs(K, Na)3(Li3SiO4)4 to Achieve Narrow-Band Green Emission for Wide Color Gamut Displays29Synthesis, adjustable-color emission and energy transfer of Ba2MgSi2O7:Sm3+, Bi3+ phosphors76Recent progress in Ce 3+ /Eu 2+ -activated LEDs and persistent phosphors: focusing on the local structure and the electronic structure137Sr2BN2Cl:Eu2+-Based Narrow-Band Blue-Emitting Phosphor: A Potential Color Converter for Illumination and Displays10Improved Energy Transfer in Mn-Doped Cs3Cu2I5 Microcrystals Induced by Localized Lattice Distortion37Enhanced Photoluminescence in Cd x Zn 1– x S Solid Solution by Suppressing Non-Radiative Recombination for White Light-Emitting Diodes8Robust single molecular white fluorescence facilitated by blocking aggregate growth in Densely-Woven solid polymeric network5Highly efficient and tunable broadband UV excitable Ba9Lu2Si6O24:Eu2+, Mn2+ single-phase white-light-emitting phosphors21Cyan-rich sunlight-like spectra from Mn 2+ -doped CsCd(Cl 1− y Br y ) 3 perovskites with dual tunable emissions and high stability2Dynamic readout of optical information based on the color-tunable emitting electron-trapping material BaAl 12 O 19 :Eu 2+ toward high security level optical data storage and anticounterfeiting27Energy transfer and tunable emission in BaSrGd 4 O 8 :Bi 3+ ,Eu 3+ phosphors for warm WLED9High performance of broad excitation and narrow emission green phosphor NaAl 11 O 17 :Eu 2+ , Mn 2+ for backlight displays20Probing into the conduction band and type of carriers/traps on red/orange persistent phosphors in vacancy & solid-solution induced (Sr/Ba) 1− x Ca x Ge 4− y O 9 :Mn 2+3Single-component full-color emitting Ca 6 Y 2 Na 2 (PO 4 ) 6 F 2 :Eu 2+ ,Tb 3+ ,Mn 2+ phosphors with superior performance: color-tunable and energy transfer study4To achieve tunable-color emission in a novel tri-doped phosphate sulfate phosphor: Tb 3+ as the energy transfer bridge1White-light emitting multi-lanthanide terephthalate thin films by atomic/molecular layer deposition13Achievement of full-visible-spectrum lighting in Bi3+-activated strontium gallates via lattice site occupancy engineering toward WLEDs applications32Apatite oxynitride phosphor (Mg,Y)5Si3(O,N)13:Ce 3+ ,Mn 2+ : A single‐phased host with solar‐like and efficient emission5Local Structure and Self‐Defect Evolution under Nonstoichiometric Effect Unlock Zero‐Thermal‐Quenching15Regulating Eu 2+ Multisite Occupation through Structural Disorder toward Broadband Near-Infrared Emission91Preparation of novel KAlSiO4: Ce3+ broadband cyan-emitting phosphors via partial cation substitution for applications in white-light LEDs20Facile Synthesis of Highly Efficient and Thermally Stable BaAl 4 Sb 2 O 12 :Eu 2+ Phosphor in Air72Eu 2+ -Doped Ca 4 Y 3 Si 7 O 15 N 5 Phosphor with High Thermal Stability and Pressure Sensitivity for Dual-Functional Applications in W-LEDs and Pressure Sensors32Chemical Group Substitution Enables Highly Efficient Mn4+ Luminescence in Heterovalent Systems27Site‐Engineering for Controlling Multiple‐Excitation and Emission in Eu2+‐Activated CaSrSiO4 Phosphors in Marine Fisheries21Strategic Tuning of Photophysical Response in the Polyhedral Framework of the Garnet Structure toward White Light-Emitting Devices with Enhanced Color Rendering20Broadband Emission Origin in Metal Halide Perovskites: Are Self‐Trapped Excitons or Ions?198Near‐Infrared Persistent Phosphor‐Mediated Smart Sensing Light‐Emitting Diodes for Advanced Driver Assistance Systems11Deep‐Red Ca3Al2Ge3O12:Eu3+ Garnet Phosphor with Near‐Unity Internal Quantum Efficiency and High Thermal Stability for Plant Growth Application67Bright Warm White Emission of Nd 0.9 Yb 0.1 AlO 3 Nanocrystals under High Power Density Infrared Excitation2Synthesis of Eu3+-Doped NaGd9Si6O26 Sub-Microcrystals from a NaGdF4@SiO2 Structure2Advances in aliovalent substitution strategy for the design and synthesis of nonlinear optical materials: d0 transition metal/gallium iodates and selenites70A stress-charged non-Newtonian-fluid persistent luminescent material0Developing a new persistent luminescence material by introducing cation defects8Photoluminescence of Mn2+ in the Borosulfate Zn[B2(SO4)4] : Mn2+—A Tool to Detect Weak Coordination Behavior of Ligands18Photolumineszenz von Mn2+ in dem Borosulfat Zn[B2(SO4)4] : Mn2+ – Eine Möglichkeit zum Nachweis schwach koordinierender Liganden0A novel broad-band red K2MgSiO4:Eu2+ phosphor and defect-induced tunable emission from red to yellow20Physicochemical Characterization of the Hybrid Molybdate–Tungstate Materials for Solid-State Lighting14Moderate Trap Engineering for Enhanced Thermal Stability and High Efficiency in a Bi3+-Doped Phosphor45Broadband emission characteristics and WLED application of self-activated YMZn3AlO7 (M=Ca, Sr, Ba) phosphors5Superior temperature sensitive luminescent properties of BaY2Al2Ga2GeO12:Bi3+8High-Quantum-Efficiency Blue Phosphors with Superior Thermal Stability Derived from Eu3+-Doped Faujasite Y Zeolite11Pressure tailoring electron-phonon coupling toward enhanced yellow photoluminescence quantum yield and piezochromism54Assembling Two Self‐Trapped Exciton Emissions in 0D Metal Halides with Near‐Unity Quantum Yield and Zero Thermal‐Quenching Photoluminescence44Ce3+-Doped Li2Ca5Gd(BO3)5 Phosphors with Multiple Luminescent Centers and High Pressure Sensitivity under Near UV Excitation9Facile and effective synthesis strategy for terbium‐doped hydroxyapatite toward photoelectric devices and flexible functional fibers12A novel extra-broadband visible-emitting garnet phosphor for efficient single-component pc-WLEDs6A theoretical spectroscopy study of the photoluminescence properties of narrow band Eu 2+ -doped phosphors containing multiple candidate doping centers. Prediction of an unprecedented narrow band red phosphor10Cation vacancy-boosted BaZnB 4 O 8 : x Eu 3+ phosphors with high quantum yield and thermal stability for pc-WLEDs17Enhancement of 4 T 2 → 4 A 2 with temperature via energy transfer of the optical thermometer Mg 5 Al 7 O 16 :Cr 3+6Identifying Organic–Inorganic Interaction Sites Toward Emission Enhancement in Non-Hydrogen-Bonded Hybrid Perovskite via Pressure Engineering22Multimodal dynamic luminescence of self-activated Na 2 CaGe 2 O 6 phosphor via defect manipulation2Narrow-band green phosphor RbK 2 Na(Li 3 SiO 4 ) 4 :Eu 2+ with excellent thermal stability and high efficiency for wide color gamut displays8Preparation of a novel violet-excitable Na 3 YSi 2 O 7 :Eu 2+ green phosphor via salt-flux assistance and its luminescence properties15Progress of Ce 3+ /Eu 2+ doped phosphors for violet chip based full-spectra lighting42Structure, luminescence properties, and valence-induced spectral behavior of a bismuth-activated garnet phosphor9Unlocking color-tunable emission of Eu 2+ -activated phosphors through doping-free exploration of hidden sites3Efficient blue mechanoluminescence in Eu2+-Activated Sr5(PO4)3Cl for advanced anticounterfeiting with mildew-resistant behavior12Thermally Stable Red-Emitting Ca18K3Sc(PO4)14:Mn2+ Phosphor and Enhanced Luminescence by Energy Transfer Between Ce3+-Eu2+-Mn2+22Zero-thermal-quenching broadband yellow-emitting Bi3+-activated phosphors based on metal to metal charge transfer27A new yellowish‐green‐emitting phosphor: Eu 2+ ‐doped Ba 3 YAl 2 O 7.55Optical Information Transmission and Multimode Fluorescence Anticounterfeiting of Ca2–xMgxGe7O16:Mn2+18High‐Efficiency Cyan–Green‐Emitting Y 3 Sc 2 Ga 3 O 12 :Ce Phosphor for Microcrystals and Ultrathin Phosphor‐Glass Composite for Light‐Emitting Diode26Luminescent structure evolution triggered white emission in α-Mg2Al4Si5O18:Eu2+ through Eu2+ occupancy induced by Al3+ content / B3+-P5+ double substitution8Discrete Trap-Enabled Dynamic Multimode Luminescence in Chloro-Apatite Phosphors for Advanced Anticounterfeiting1Defect Regulation Strategy of Porous Persistent Phosphors for Multiple and Dynamic Information Encryption13Europium Ions Self‐Reduction Benefiting from AlO4/Si(Al)O4 Network Structure for Multimode Optical Thermometry Manometry27Achieving Ultra‐Broadband Sunlight‐Like Emission in Single‐Phase Phosphors: The Interplay of Structure and Luminescence44Two substitution strategies realize single-phase full-spectrum emission in Ca10Na(PO4)7:Eu2+ phosphors for WLED17Regulating the broadband near-infrared emission of Eu2+-doped Ca3Sc2Si3O12 phosphors through constructing defect for diversified applications56Trivalent terbium host-sensitized orthoniobate green phosphor with high luminescence thermal stability for promising backlighting white light-emitting diodes1A novel white Y2(Ti0.8Hf0.2)2O7: Eu phosphors regulated by HfO2 exhibiting low color shifting for high temperature2Wide Range Near‐Zero Thermal Quenching of Orange–Yellow Phosphor via Impeding Self‐Oxidation of Eu 2+ for Versatile Optoelectronic Applications20Achieving Eu 2+ Luminescence at Trivalent Lattice Site in Rb 3 Y(PO 4 ) 2 :Eu toward Multicolor Emissions by Carbon and Hydrogen Coreduction23Transcription of Customized Circularly Polarized Luminescence from Enantiomeric Metal–Organic Framework to Carbon Dots12Sunlight‐Activated Eu2+‐Doped Red Persistent Luminescence Material for Night‐Vision Signage, Anti‐Counterfeiting and Location Detection30Suppressed concentration quenching and tunable photoluminescence in Eu2+-activated Rb3Y(PO4)2 phosphors for full-spectrum lighting87Absolutely Structural Disorder Boosting Bandwidth toward Full‐Spectrum White Light from Single Occupancy of Activator36Customized Cyan Phosphors for Efficient Full‐Spectrum Illumination and Fingerprint Detection22Design of a High-Performance Near-Infrared Scintillator through Metal-Atom Substitution in Metal Chalcogenide5Copper-Iodide Hybrid Clusters with Partial Distortion Enable High-Performance Full-Visible-Spectrum White-Light-Emitting Diodes33KBaScSi3O9:Eu2+ Glass‐Ceramics as Single‐Phase High‐Power White Emitters49First-principles study of the electronic structure and optical properties of Eu2+ and Mn2+-doped NaLi3SiO4 phosphor2Tunable Single‐Phase White Light Emission from Complex Perovskite Sr 3 CaNb 2 O 9 : Dy 3+ /Eu 3+ Phosphors21Bright electrospun white Y 2 Zr 2 O 7 :Tm 3+ /Dy 3+ nanotubes with excellent thermal quenching resistance and ultralow color shift1Enhanced Luminescence and Anti-Counterfeiting Properties of Strontium Aluminate by Co-Doping Eu2+ and Dy3+0Energy transfer mediated single-component white light emission in a novel Bi3+/Eu3+ co-doped Sr2Ga2GeO7 phosphor for white LEDs20Achievement of an ultra-broadband deep red phosphor K3Ca0.3Y0.7Si2O7:Eu2+ (phase 1) for phytochrome matching plant-lighting12Site occupation engineering induced red-shifted luminescence in (Ca, Sr)Sc2O4:Eu2+ phosphor20Luminescence characterization and performance modulation of CaScBO 4 : Eu 2+ near-infrared phosphors for night vision lighting applications4Double Perovskite Scintillators Enabled by Co‐Doped Trap Regulation for Thermally Enhanced X‐Ray Imaging31Lighting up metal nanoclusters by the H2O-dictated electron relaxation dynamics28Tailoring of Blue‐Cyan Luminescence in Rb 3 Y[(P 1‐ x Si x )O 4 ] 2 :Eu 2+ Phosphor via Si 4+ ‐P 5+ Heterovalent Substitution for Full‐Spectrum Healthy Lighting25Mn 2+ ‐Activated Alkali Lithooxidosilicate Phosphors as Sustainable Alternative White‐Light Emitters10

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  34. Near-UV excited green-emission enhancement by efficient energy transfer in Na1.8Mg0.9Si1.1O4:Ce3+,Tb3+ phosphor for solid-state lighting applications

    Optics & Laser Technology · 2022-02-08

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  35. Simultaneous Spectral Tuning and Thermal Stability Adjustment in Ca8ZnGa(1–x)Lax(PO4)7:Eu2+ Phosphors

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  36. Microscopic Mechanism of the Heat‐Induced Blueshift in Phosphors and a Logarithmic Energy Dependence on the Nearest Dopant–Vacancy Distance

    Angewandte Chemie International Edition · 2022-02-14

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  37. Microscopic Mechanism of the Heat‐Induced Blueshift in Phosphors and a Logarithmic Energy Dependence on the Nearest Dopant–Vacancy Distance

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  38. Tailoring the Luminescent Properties of SrS:Ce3+ by Sr-Deficiency and Na+ Doping

    Inorganic Chemistry · 2022-02-15

    Shuqin Chang, Jipeng Fu, Xuan Sun, Guangcan Bai, Guoquan Liu, Kaina Wang, Ligang Xu, Qi Wei, Thomas Meier, Mingxue Tang

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  39. Adjustable luminescence properties of Eu3+ and Bi3+ codoped Ca3Zn3Te2O12 phosphor

    Materials Research Bulletin · 2022-04-10

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  40. Carbon dots embedded in lead-free luminescent metal halide crystals toward single-component white emitters

    Science China Materials · 2022-04-18

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  41. Deep-level trap formation in Si-substituted Sr2SnO4:Sm3+ for rewritable optical information storage

    Materials Today Chemistry · 2022-04-22

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  42. Time-resolved and temperature-dependent spectroscopy for blue luminescence of monoclinic YSiO2N:Ce3+ phosphor

    Journal of Luminescence · 2022-05-01

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  43. Role of the Rigid Host Structure in Narrow-Band Green Emission of Eu2+ in Rb2Na2(Li3SiO4)4: Insights into Electron–Phonon Coupling

    Inorganic Chemistry · 2022-05-03

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  44. Novel Orange-Emitting Phosphor Ba2LuGaO5:Bi3+ with High Efficiency and Thermal Robustness Induced by D-Band Emission

    The Journal of Physical Chemistry C · 2022-05-19

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  45. Multiple Strategies to Approach High-Efficiency Luminescence Controllable in Blue/Cyan/Green-Emitting Bi 3+ -Activated Phosphors

    The Journal of Physical Chemistry C · 2022-05-20

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  46. Evolutionary Generation of Phosphor Materials and Their Progress in Future Applications for Light-Emitting Diodes

    Chemical Reviews · 2022-05-22

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  47. Resistance to aggregation-caused quenching: chitosan-based solid carbon dots for white light-emitting diode and 3D printing

    Advanced Composites and Hybrid Materials · 2022-06-07

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  48. Modulating the emission spectrum of Ca2La8(SiO4)6O2:Eu(2+,3+) phosphor through Mn2+ ion doping

    Chemical Papers · 2022-06-08

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  49. Influence of Mn2+ doping on the emission spectrum of Sr2La8(SiO4)6O2:Eu(2+,3+) phosphor

    Inorganic Chemistry Communications · 2022-06-09

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  50. Towards single broadband white emission in Rb0.5K1.5CaPO4(F, Cl): Eu2+ via selective site occupancy engineering for solid-state lighting applications

    Chemical Engineering Journal · 2022-06-27

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