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RESEARCH PAPER · Inorganic Chemistry Frontiers · 2019

Fluoroborophosphates: a family of potential deep ultraviolet NLO materials

Baolin Wu, Chun‐Li Hu, Ru‐Ling Tang, Fei‐Fei Mao, Jianghe Feng, Jiang‐Gao Mao

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Fluoroborophosphates: a family of potential deep ultraviolet NLO materialsOriginalBa 3 Ca 4 (BO 3 ) 3 (SiO 4 )Cl: a new non-centrosymmetric complex alkaline-earth metal borosilicate chloride with a deep-ultraviolet cut-off edge19From centrosymmetric to noncentrosymmetric: cation-directed structural evolution in X 3 ZnB 5 O 10 (X = Na, K, Rb) and Cs 12 Zn 4 (B 5 O 10 ) 4 crystals26Hybridization-activated new deep ultraviolet transparent nonlinear optical material Ba 11 [Al(PO 4 ) 4 ](P 2 O 7 )(PO 4 ) 3 with balanced overall performance and parsimony-forbidden structure23Pb 2 Cd(SeO 3 ) 2 X 2 (X = Cl and Br): two halogenated selenites with phase matchable second harmonic generation27Designing Three Fluorooxoborates with a Wide Transmittance Window by Anionic Group Substitution15Cation Modulation on the Crystal Structure and Band Gap of Fluorooxoborates A3B3O3F6 (A = Alkali and Mixed Alkali Metal)17Designing excellent mid-infrared nonlinear optical materials with fluorooxo-functional group of d0 transition metal oxyfluorides63K 4 (PO 2 F 2 ) 2 (S 2 O 7 ): first fluorooxophosphorsulfate with mixed-anion [S 2 O 7 ] 2− and [PO 2 F 2 ] − groups14Three non-centrosymmetric bismuth phosphates, Li 2 ABi(PO 4 ) 2 (A = K, Rb, and Cs): effects of cations on the crystal structure and SHG response23Cs3B3O3F6 with a Deep-Ultraviolet Cutoff Edge and a Suitable Birefringence as the Potential Zero-Order Waveplate Material31Y 2 (Te 4 O 10 )(SO 4 ): a new sulfate tellurite with a unique Te 4 O 10 polyanion and large birefringence36From centrosymmetric to noncentrosymmetric: effect of the cation on the crystal structures and birefringence values of (NH 4 ) n−2 AE(PO 2 F 2 ) n (AE = Mg, Sr and Ba; n = 2, 3 and 4)9M(B(SeO 3 ) 3 )H 2 O (M = Al, Ga): the first boroselenites with a unique sandwich like double-layer structure9Pb 2 TiFO(SeO 3 ) 2 Br: a new polar compound with the strongest second harmonic generation in the selenite bromide family29Recent advances of oxyfluorides for nonlinear optical applications69Insights into varying dimension structures for deep-UV optical crystals NaBa2Al(P2O7)2 and NaBaAl(PO4)2 constructed separately from unique [Al(P2O7)2] chains and [Al(PO4)2] layers6From borophosphate to fluoroborophosphate: a rational design of fluorine-induced birefringence enhancement33Tetrafluoroborate-Monofluorophosphate (NH4)3[PO3F][BF4]: First Member of Oxyfluoride with B–F and P–F Bonds16H{[Na(H2O)3]6F}(PO4)2 ⋅ 2(H2O): A New Polycation‐Type Phosphate with Deep Ultraviolet Transparency0Ca-cluster-constructed deep-ultraviolet nonlinear-optical crystal Na2Ca17Al2(PO4)14 with strong NLO response11Complex coordinated functional groups: A great genes for nonlinear optical materials64Guanidinium Fluorooxoborates as Efficient Metal-free Short-Wavelength Nonlinear Optical Crystals140Recent Development of Non-π-Conjugated Deep Ultraviolet Nonlinear Optical Materials106Cd 4 REO(BO 3 ) 3 (RE = Sm, Eu, Tb): three new cadmium–rare earth oxyborates with both good NLO and luminescence properties6The effect of Sr doping on the electronic structure and electromagnetic properties of LaCo 0.9 Fe 0.1 O 3 perovskites13Variable dimensionality of the anion framework in four new borophosphates and fluoroborophosphates with short cutoff edges13Noncentrosymmetric Rare-Earth Borate Fluoride La2B5O9F3: A New Ultraviolet Nonlinear Optical Crystal with Enhanced Linear and Nonlinear Performance48Negative Second Harmonic Response of Sn4+in the Fresnoite Oxysulfide Ba2SnSSi2O720(NH4)3B11PO19F3: a deep-UV nonlinear optical crystal with unique [B5PO10F]∞ layers142Synthesis, structure, characterization, and electronic structure calculation of a new molecule-inclusion strontium gallate Sr6(Ga12O24)·Bi2O32KMB 4 O 6 F 3 (M = Co, Fe): two-dimensional magnetic fluorooxoborates with triangular lattices directed by triangular BO 3 units16BaB2P2O8F2: A Fluoroborophosphate with [B2P2O8F2]∞ Layers and Deep-Ultraviolet Cutoff Edge4Recent progress of newly developed functional building units and corresponding nonlinear optical materials14Deep-ultraviolet (DUV) nonlinear optical (NLO) crystals: An application in photonic technologies29Fluorination strategy toward chemical and functional modification65A nonlinear optical crystal with deep-ultraviolet transparency and appropriate birefringence achieved using π-conjugated confined [B 3 O 3 F 4 (OH)] 2−14KPO2(NHCONH2)2: A Promising Deep-Ultraviolet Nonlinear Optical Phosphate Containing Polar [PO2(NHCONH2)2]− Tetrahedra15CdF(C 6 H 4 NO 2 )(H 2 O): a UV nonlinear optical material with unprecedented SHG and birefringence via π-conjugated rings and a unique “Warren truss structure”11Four noncentrosymmetric molybdophosphates discovered by a chemical substitution strategy4Selenoborates: a latent structure resource for infrared functional crystal materials1Chiral-Unit-Oriented Design of Non-π-Conjugated Noncentrosymmetric Phosphates with Short Absorption Edges4Asymmetry-driven organic–inorganic hybrid strategy for constructing structures with exceptional organofunctionalized B–O units2Borophosphate-based second-order nonlinear optical materials: Advances in structural diversity and optical performance0

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  1. Ba 3 Ca 4 (BO 3 ) 3 (SiO 4 )Cl: a new non-centrosymmetric complex alkaline-earth metal borosilicate chloride with a deep-ultraviolet cut-off edge

    Inorganic Chemistry Frontiers · 2019-01-01

    Zixiu Lu, Fangfang Zhang, Abudukadi Tudi, Sujuan Yu, Zhihua Yang, Shilie Pan

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  2. From centrosymmetric to noncentrosymmetric: cation-directed structural evolution in X 3 ZnB 5 O 10 (X = Na, K, Rb) and Cs 12 Zn 4 (B 5 O 10 ) 4 crystals

    Inorganic Chemistry Frontiers · 2019-01-01

    Tuohetijiang Baiheti, Shujuan Han, Abudukadi Tudi, Zhihua Yang, Hualiang Yu, Shilie Pan

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  3. Hybridization-activated new deep ultraviolet transparent nonlinear optical material Ba 11 [Al(PO 4 ) 4 ](P 2 O 7 )(PO 4 ) 3 with balanced overall performance and parsimony-forbidden structure

    Journal of Materials Chemistry C · 2019-01-01

    Zhi Gang Fang, Bing‐Ping Yang, Chun‐Li Hu, Jiang‐Gao Mao

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  4. Pb 2 Cd(SeO 3 ) 2 X 2 (X = Cl and Br): two halogenated selenites with phase matchable second harmonic generation

    Inorganic Chemistry Frontiers · 2019-01-01

    Ya-Ping Gong, Chun‐Li Hu, Yun‐Xiang Ma, Jiang‐Gao Mao, Fang Kong

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  5. Designing Three Fluorooxoborates with a Wide Transmittance Window by Anionic Group Substitution

    Inorganic Chemistry · 2019-03-04

    Dequan Jiang, Guopeng Han, Ying Wang, Hao Li, Zhihua Yang, Shilie Pan

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  6. Cation Modulation on the Crystal Structure and Band Gap of Fluorooxoborates A3B3O3F6 (A = Alkali and Mixed Alkali Metal)

    Inorganic Chemistry · 2019-09-18

    Wenyao Zhang, Zhonglei Wei, Zhihua Yang, Shilie Pan

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  7. Designing excellent mid-infrared nonlinear optical materials with fluorooxo-functional group of d0 transition metal oxyfluorides

    Science China Materials · 2019-10-24

    Junben Huang, Siru Guo, Zhizhong Zhang, Zhihua Yang, Shilie Pan

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  8. K 4 (PO 2 F 2 ) 2 (S 2 O 7 ): first fluorooxophosphorsulfate with mixed-anion [S 2 O 7 ] 2− and [PO 2 F 2 ] − groups

    Dalton Transactions · 2020-01-01

    Wenyao Zhang, Wenqi Jin, Zhihua Yang, Shilie Pan

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  9. Three non-centrosymmetric bismuth phosphates, Li 2 ABi(PO 4 ) 2 (A = K, Rb, and Cs): effects of cations on the crystal structure and SHG response

    Inorganic Chemistry Frontiers · 2020-01-01

    Ming Wen, Cong Hu, Hongping Wu, Zhihua Yang, Hao Yu, Shilie Pan

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  10. Cs3B3O3F6 with a Deep-Ultraviolet Cutoff Edge and a Suitable Birefringence as the Potential Zero-Order Waveplate Material

    Inorganic Chemistry · 2020-09-11

    Meng Cheng, Wenqi Jin, Zhihua Yang, Shilie Pan

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  11. Y 2 (Te 4 O 10 )(SO 4 ): a new sulfate tellurite with a unique Te 4 O 10 polyanion and large birefringence

    Inorganic Chemistry Frontiers · 2020-10-26

    Pengfei Li, Chun‐Li Hu, Fang Kong, Shao‐Ming Ying, Jiang‐Gao Mao

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  12. From centrosymmetric to noncentrosymmetric: effect of the cation on the crystal structures and birefringence values of (NH 4 ) n−2 AE(PO 2 F 2 ) n (AE = Mg, Sr and Ba; n = 2, 3 and 4)

    Dalton Transactions · 2021-01-01

    Wenyao Zhang, Wenqi Jin, Meng Cheng, Ruonan Zhang, Zhihua Yang, Shilie Pan

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  13. M(B(SeO 3 ) 3 )H 2 O (M = Al, Ga): the first boroselenites with a unique sandwich like double-layer structure

    Dalton Transactions · 2021-01-01

    Ming‐Yang Cao, Chun‐Li Hu, Fang Kong, Zheyao Xiong, Jiang‐Gao Mao

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  14. Pb 2 TiFO(SeO 3 ) 2 Br: a new polar compound with the strongest second harmonic generation in the selenite bromide family

    Journal of Materials Chemistry C · 2021-01-01

    Lili Liu, Bingbing Zhang, P. Shiv Halasyamani, Weiguo Zhang

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  15. Recent advances of oxyfluorides for nonlinear optical applications

    Inorganic Chemistry Frontiers · 2021-01-01

    Shuo Bai, Dan Wang, Hongkun Liu, Ying Wang

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  16. Insights into varying dimension structures for deep-UV optical crystals NaBa2Al(P2O7)2 and NaBaAl(PO4)2 constructed separately from unique [Al(P2O7)2] chains and [Al(PO4)2] layers

    Journal of Solid State Chemistry · 2021-06-15

    Fang Wang, Xiao-Ni Yao, Yao Guo, Yang Liguo, Yi-Gang Chen, Xian‐Ming Zhang

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  17. From borophosphate to fluoroborophosphate: a rational design of fluorine-induced birefringence enhancement

    Science China Chemistry · 2021-08-04

    Wenyao Zhang, Zhizhong Zhang, Wenqi Jin, Ruonan Zhang, Meng Cheng, Zhihua Yang, Shilie Pan

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  18. Tetrafluoroborate-Monofluorophosphate (NH4)3[PO3F][BF4]: First Member of Oxyfluoride with B–F and P–F Bonds

    ACS Organic & Inorganic Au · 2021-08-04

    Haotian Qiu, Wenbing Cai, Zhihua Yang, Yanli Liu, Miriding Mutailipu, Shilie Pan

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  19. H{[Na(H2O)3]6F}(PO4)2 ⋅ 2(H2O): A New Polycation‐Type Phosphate with Deep Ultraviolet Transparency

    European Journal of Inorganic Chemistry · 2021-10-26

    Xu-Kui Yang, Yuting Liu, Yuxin Li, Peixin Ma, Tixian Zeng, Meihong Duan, Zhi Gang Fang, Da-Bin Qin

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  20. Ca-cluster-constructed deep-ultraviolet nonlinear-optical crystal Na2Ca17Al2(PO4)14 with strong NLO response

    Journal of Alloys and Compounds · 2021-11-30

    Yi-Gang Chen, Xiaoxiu Yu, Yao Guo, Yuanbin Xue, Xiaohui Hao, Xiao-Ni Yao, Xian‐Ming Zhang

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  21. Complex coordinated functional groups: A great genes for nonlinear optical materials

    Chinese Chemical Letters · 2021-12-03

    Weikang Wang, Dajiang Mei, Shaoguo Wen, Jian Wang, Yuandong Wu

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  22. Guanidinium Fluorooxoborates as Efficient Metal-free Short-Wavelength Nonlinear Optical Crystals

    Chemistry of Materials · 2021-12-24

    Congcong Jin, Hao Zeng, Feng Zhang, Haotian Qiu, Zhihua Yang, Miriding Mutailipu, Shilie Pan

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  23. Recent Development of Non-π-Conjugated Deep Ultraviolet Nonlinear Optical Materials

    Chemistry of Materials · 2021-12-29

    Weiqi Huang, Sangen Zhao, Junhua Luo

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  24. Cd 4 REO(BO 3 ) 3 (RE = Sm, Eu, Tb): three new cadmium–rare earth oxyborates with both good NLO and luminescence properties

    CrystEngComm · 2022-01-01

    Ming‐Yang Cao, Chun‐Li Hu, Peng-Fei Chen, Qian Wang, Bingxuan Li, Yuan Hua Lin, Jiang‐Gao Mao

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  25. The effect of Sr doping on the electronic structure and electromagnetic properties of LaCo 0.9 Fe 0.1 O 3 perovskites

    Inorganic Chemistry Frontiers · 2022-01-01

    Fan Wang, Yue Wu, Yue Zhao, Ming Zhou, Shaolong Tang, Guangbin Ji

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  26. Variable dimensionality of the anion framework in four new borophosphates and fluoroborophosphates with short cutoff edges

    Dalton Transactions · 2022-01-01

    Ruonan Zhang, Siru Guo, Xuping Wang, Rong Yang, Zhen Chen, Wenyao Zhang, Fangfang Zhang, Zhiyong Guo, Shujuan Han, Zhihua Yang

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  27. Noncentrosymmetric Rare-Earth Borate Fluoride La2B5O9F3: A New Ultraviolet Nonlinear Optical Crystal with Enhanced Linear and Nonlinear Performance

    ACS Applied Materials & Interfaces · 2022-04-13

    Xuping Shi, Abudukadi Tudi, Meng Cheng, Fangfang Zhang, Zhihua Yang, Shujuan Han, Shilie Pan

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  28. Negative Second Harmonic Response of Sn4+in the Fresnoite Oxysulfide Ba2SnSSi2O7

    Chemistry of Materials · 2022-05-05

    Batoul Almoussawi, Wen‐Dong Yao, Sheng‐Ping Guo, Myung‐Hwan Whangbo, Valérie Dupray, Simon Clevers, Shuiquan Deng, Houria Kabbour

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  29. (NH4)3B11PO19F3: a deep-UV nonlinear optical crystal with unique [B5PO10F]∞ layers

    National Science Review · 2022-06-10

    Bingliang Cheng, Zi‐Jian Li, Yu Chu, Abudukadi Tudi, Miriding Mutailipu, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  30. Synthesis, structure, characterization, and electronic structure calculation of a new molecule-inclusion strontium gallate Sr6(Ga12O24)·Bi2O3

    Journal of Solid State Chemistry · 2022-10-06

    Lei Huai, Lunan Zhang, Beibei Zhang, Guangan Jia, Wen‐Dong Yao, Wenlong Liu, Ru‐Ling Tang

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  31. KMB 4 O 6 F 3 (M = Co, Fe): two-dimensional magnetic fluorooxoborates with triangular lattices directed by triangular BO 3 units

    Dalton Transactions · 2023-01-01

    Yanhong Wang, Shuang long Li, Yaling Dou, Hui Li, Hongcheng Lu

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  32. BaB2P2O8F2: A Fluoroborophosphate with [B2P2O8F2]∞ Layers and Deep-Ultraviolet Cutoff Edge

    Inorganic Chemistry · 2023-01-04

    Jinbin Fan, Mengfan Wu, Bingliang Cheng, Jian Wei Han

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  33. Recent progress of newly developed functional building units and corresponding nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-05-11

    Wenjing Tan, Chenyang Zhang, Chenyang Zhang, Tingting Huang, Bingbing Zhang

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  34. Deep-ultraviolet (DUV) nonlinear optical (NLO) crystals: An application in photonic technologies

    Optical Materials · 2023-08-23

    Biswajit Dalai, Sarat Kumar Dash

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  35. Fluorination strategy toward chemical and functional modification

    Fundamental Research · 2023-12-19

    Haotian Qiu, Shilie Pan, Miriding Mutailipu

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  36. A nonlinear optical crystal with deep-ultraviolet transparency and appropriate birefringence achieved using π-conjugated confined [B 3 O 3 F 4 (OH)] 2−

    New Journal of Chemistry · 2024-01-01

    Tao Ouyang, Chen Xu, Shanshan Chen, Yanqiang Li, Xiaoying Shang, Zhiyong Bai, Ningtao Jiang, Zhishuo Yan, Junhua Luo, Sangen Zhao

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  37. KPO2(NHCONH2)2: A Promising Deep-Ultraviolet Nonlinear Optical Phosphate Containing Polar [PO2(NHCONH2)2]− Tetrahedra

    Chemistry of Materials · 2024-03-04

    Fuhai Chen, Fuxiang Mo, Hongming Chen, Mei‐Jin Lin, Yong Chen

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  38. CdF(C 6 H 4 NO 2 )(H 2 O): a UV nonlinear optical material with unprecedented SHG and birefringence via π-conjugated rings and a unique “Warren truss structure”

    Inorganic Chemistry Frontiers · 2025-01-01

    Jie Gou, Yaolong Zhu, Xin Su, Can Hui Yang, YunJie Wang, Qingwen Zhu, Yi Xiong, Qi Wu

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  39. Four noncentrosymmetric molybdophosphates discovered by a chemical substitution strategy

    Dalton Transactions · 2025-01-01

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  40. Selenoborates: a latent structure resource for infrared functional crystal materials

    Inorganic Chemistry Frontiers · 2025-01-01

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  41. Chiral-Unit-Oriented Design of Non-π-Conjugated Noncentrosymmetric Phosphates with Short Absorption Edges

    The Journal of Physical Chemistry Letters · 2025-02-17

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  42. Asymmetry-driven organic–inorganic hybrid strategy for constructing structures with exceptional organofunctionalized B–O units

    Inorganic Chemistry Frontiers · 2025-12-20

    Haoran Wang, chenxu li, Xue Bai, Qingyu Liu, Xueling Hou, Min Zhang

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  43. Borophosphate-based second-order nonlinear optical materials: Advances in structural diversity and optical performance

    Coordination Chemistry Reviews · 2026-09-17

    Bo Zhao, Yaozu Li, Danyang Dou, Wenjing Zhang, Huiyi Zhang, Bingbing Zhang, Ying Wang

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