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RESEARCH PAPER · Fundamental Research · 2023

Fluorination strategy toward chemical and functional modification

Haotian Qiu, Shilie Pan, Miriding Mutailipu

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Fluorination strategy toward chemical and functional modificationOriginalDiscovery of a new bimetallic borate with strong optical anisotropy activated by π-conjugated [B 2 O 5 ] units3KBa 3 M 2 F 14 Cl (M = Zr, Hf): novel short-wavelength mixed metal halides with the largest second-harmonic generation responses contributed by mixed functional moieties37Pb 2 (SeO 3 )(SiF 6 ): the first selenite fluorosilicate with a wide bandgap and large birefringence achieved through perfluorinated group modification45Tunable Optical Anisotropy in Rare‐Earth Borates with Flexible [BO3] Clusters7M6[Cd2(CO3)2(B12O18)(OH)6] (M = K, Rb): Borate–Carbonates with Two CdCO3 Embedded in a Cyclic Oxoboron Anion10[B3O3F4(OH)]2–: A Versatile Hydroxyfluorooxoborate Heteroanion Producing Compounds with Highly Tunable Optical Anisotropy19Hydrogen bond-derived symmetry transformation in hydroxyborates: Converting the nonlinearity from null to active7Tetrahedra Modification of Phosphates for Optical Anisotropy Enhancement13A Giant Optically Anisotropic Phosphate Driven by Mixed Valence Mercury Units22On the Performance of Second-Order Polarization Propagator Methods in the Calculation of 1JFC and nJFH NMR Spin–Spin Coupling Constants7La 3 (Ga 3 S 3 O 3 )(Si 2 O 7 ): An Oxychalcogenide Demonstrating Ultrawide Optical Bandgap and Favorable Birefringence Propelled by Divergent Anionic Groups6A new ultraviolet-transparent molybdate featuring a layered structure and moderate birefringence0KNa 2 Y 2 B 2 O 6 F 3 : a beryllium free deep-UV nonlinear optical crystal with well-balanced properties2Pb9Si8O22Cl6 and Pb3.07Ca1.93Si3O11: Two Ultraviolet Nonlinear Optical Materials Exhibit a Moderate Second Harmonic Generation Response1Impact of Fluorine in Manganese Citrate Synthesis on Structure and Value-Added Decomposition Products1Breaking the Natural Tendency of Deep‐UV Polyborate Anion Clusters to Inducing Strong Optical Anisotropy13Hydrogen‐Bonded Assembly of Functional Units for Constructing Linear and Nonlinear Optical Crystals10La2Zn3(SeO3)6: A UV Selenite Crystal with Second-Harmonic Generation and Large Birefringence13Non-equivalent terminating roles of hydroxyl and fluorine in hydroxy/fluorooxo-borate optical functional materials2Symmetry Breaking via Anion-Molecule Synergy: Fluorine and Crystalline Water Directed Construction of Noncentrosymmetric Sr(IO2F2)2·2H2O0Achieving the birefringence-bandgap trade-off: Hydrogen-bond engineered biuret-cyanurate14Extending the Chemistry of Scheelite‐type Oxides with Borates7Extending the Chemistry of Scheelite‐type Oxides with Borates2A3ZnNO3X4 (A = Rb, NH4, X = Cl, I): Regulating Cations and Halides Yields Birefringent Crystals with Significantly Enhanced Optical Anisotropy5BaZn2(HPO3)3: A New Barium Zincophosphite with Short Ultraviolet Cutoff Edge2K5NaZr4F22(H2O)2: A Hydrated Zirconium Fluoride with a Second-Harmonic Generation Effect and a Short Ultraviolet Cutoff Edge Induced by Cosubstitution with Heterovalent Cations6Discovery of novel fluorine modification of aryloxyacetic acid derivatives as 4-hydroxyphenylpyruvate dioxygenase inhibitors1Borosilicates as deep-ultraviolet transparent nonlinear optical crystals: Structural motifs, performance limits and future directions9[HgX 2 ] Linear Group Enabled Ultraviolet Birefringent Crystal RbHg 5 Br 11 with Strong Optical Anisotropy and Wide Bandgap12Sulfonated Module Aggregation for Ultrahigh Birefringence in Aqueous-Processable Crystals26The nonlinear optical properties and through-space charge-transfer effects of the twist donor-acceptor complexes4Organic π-conjugated units as versatile building blocks for high-performance birefringent crystals6Ionic liquid-derived fluorine doped high entropy metal oxides as efficient electrocatalysts for sulfion valorization0Ba 3 (MoO 2 F 3 )PO 4 F 2 : Rational Design and Synthesis of an Alkaline-Earth Phosphate Fluoride as a Birefringent Crystal1Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion17Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion2Ba2CrIO3F6: a magnetic alkaline-earth chromium fluoroiodate with ferromagnetic exchange interactions1Bandgap tuning through the substitution of alkali metal cations in A 2 AlCuF 6 (A = K, Rb, and Cs) for optoelectronic and renewable energy applications2Broadband infrared-transparent crystals enabled by heterologous isomorphic substitution0From centrosymmetric (C 4 H 8 N 5 )(SbF 4 ) to polar (C 4 H 7 N 4 O)(SbF 4 ): a new UV nonlinear optical material achieved by functional group modulation8K 7 MgY 2 (B 5 O 10 ) 3 : a novel ultraviolet nonlinear optical crystal based on the [B 5 O 10 ] functional unit2Solving the long-standing hygroscopicity and thermal stability issues of the nonlinear optical crystal α-LiIO 3 via homogeneous cation exchange0Te–Se replacement induced structural transition and enhanced band gaps in Cd 5 Se 4 O 12 Cl 2 and Cd 5 Se 4 O 12 Br 21UV and X-ray excited luminescence from m -terphenyl crystals grown by the vertical Bridgman technique0孤对电子效应羟基硼酸盐非线性光学研究进展（特邀）0Confinement-assembled ultraviolet nonlinear optical crystal from pyridine-expanded π-systems with exhibiting strong SHG and birefringence18Synthesis and Characterization of Poly(Fluoro-Aryl-Thiazole) Copolymers: Thermal, Spectroscopic Properties, and Application in Thorium and Aluminum Ions Detection from Aqueous Solutions0KHg 4 Ga 5 S 12 : A Diamond-like Tetrahedral Chalcogenide Exhibiting Giant Phase-Matching Second Harmonic Generation6Ba 5 Zn 4 (B 3 O 6 ) 2 (B 12 O 24 ): A Borate with Edge-Sharing [BO 4 ] Tetrahedral Connection by Introducing Zn into β-BaB 2 O 42Density-Compensated Polarizability Anisotropy for Record Birefringence in Short-Wavelength Ultraviolet Inorganic Crystals11Conformational Editing Drives Covalent Hybridization for Nonlinear Optical Crystals2Rational design of a quasi-0D tungsten tellurite nonlinear optical crystal with exceptionally balanced properties1Dimensionality Engineering of Fluorozirconium Phosphates for Deep-UV-Transparent Crystals with Enhanced Second-Harmonic Generation and Birefringence10K 3 Mg 2 [K 6 MgCl 3 ][Ga 20 S 36 ]: A Diamond-like Framework Based on Mixed-Type Supertetrahedra for Excellent Nonlinear Optical Property1Engineering Cooperative Acid Sites in Hydroxyapatite via Surface Fluorination for Selective Conversion of Glucose to 5‐Hydroxymethylfurfural1Hydrogen- and Fluorine-Functionalized Germagraphene Quantum Dots: DFT Studies and Implications for Anticancer Drug Delivery0A simple and facile regioselective aliphatic fluorination of acetophenone derivatives0Research advances in rare-earth nonlinear optical crystalline materials in 20250Kinetic Trapping of Pressure‐Induced Symmetry Breaking in Hybrid Metal Halides via Fluorine‐Mediated Molecular Locking0Kinetic Trapping of Pressure‐Induced Symmetry Breaking in Hybrid Metal Halides via Fluorine‐Mediated Molecular Locking0Rational Design of a Strong Nonlinear Optical Crystal With Ultrawide Bandgap via Fine‐Tuning of Channel Structures0Proton-transfer-induced supramolecular assembly of 4-Aminopyridinium hydrogen maleate: Synthesis, structure-property correlation toward nonlinear optical (NLO) applications0The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals1The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals0Fluorooxoborate crystal NH4B4O6F: a high-performance candidate for practical vacuum ultraviolet nonlinear optics0

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  1. Discovery of a new bimetallic borate with strong optical anisotropy activated by π-conjugated [B 2 O 5 ] units

    Dalton Transactions · 2024-01-01

    Meihui Chen, Wei Wei, Jiawei Zhao, Donghai An, Yanna Chen

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  2. KBa 3 M 2 F 14 Cl (M = Zr, Hf): novel short-wavelength mixed metal halides with the largest second-harmonic generation responses contributed by mixed functional moieties

    Chemical Science · 2024-01-01

    Mei Yan, Chun‐Li Hu, Ru‐Ling Tang, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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  3. Pb 2 (SeO 3 )(SiF 6 ): the first selenite fluorosilicate with a wide bandgap and large birefringence achieved through perfluorinated group modification

    Chemical Science · 2024-01-01

    Pengfei Li, Chun‐Li Hu, Jiang‐Gao Mao, Fang Kong

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  4. Tunable Optical Anisotropy in Rare‐Earth Borates with Flexible [BO3] Clusters

    Chemistry - A European Journal · 2024-05-02

    Xiangyu Long, Ran An, Yan An Lv, Xueyan Wu, Miriding Mutailipu

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  5. M6[Cd2(CO3)2(B12O18)(OH)6] (M = K, Rb): Borate–Carbonates with Two CdCO3 Embedded in a Cyclic Oxoboron Anion

    Inorganic Chemistry · 2024-05-09

    Weifeng Chen, Mei-Jun Zou, Jinɡjinɡ Li, Yinan Zhang, You‐Zhao Lan, Jian‐Wen Cheng, Guo‐Yu Yang

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  6. [B3O3F4(OH)]2–: A Versatile Hydroxyfluorooxoborate Heteroanion Producing Compounds with Highly Tunable Optical Anisotropy

    Chemistry of Materials · 2024-07-09

    Zeen Li, Congcong Jin, Changyou Liu, Juanjuan Lu, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  7. Hydrogen bond-derived symmetry transformation in hydroxyborates: Converting the nonlinearity from null to active

    Materials Today Chemistry · 2024-08-29

    Ziqi Chen, Changyou Liu, Junjie Li, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  8. Tetrahedra Modification of Phosphates for Optical Anisotropy Enhancement

    Advanced Optical Materials · 2024-08-29

    Haotian Qiu, Ran An, Junjie Li, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  9. A Giant Optically Anisotropic Phosphate Driven by Mixed Valence Mercury Units

    Laser & Photonics Review · 2024-10-24

    Pengfei Li, Chun‐Li Hu, Jiang‐Gao Mao, Fang Kong

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  10. On the Performance of Second-Order Polarization Propagator Methods in the Calculation of 1JFC and nJFH NMR Spin–Spin Coupling Constants

    Journal of Chemical Theory and Computation · 2024-11-29

    Marinella de Giovanetti, Rodrigo Antonio Cormanich, Stephan P. A. Sauer

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  11. La 3 (Ga 3 S 3 O 3 )(Si 2 O 7 ): An Oxychalcogenide Demonstrating Ultrawide Optical Bandgap and Favorable Birefringence Propelled by Divergent Anionic Groups

    ACS Materials Letters · 2024-12-19

    Ming‐Shu Zhang, Shao‐Min Pei, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  12. A new ultraviolet-transparent molybdate featuring a layered structure and moderate birefringence

    New Journal of Chemistry · 2025-01-01

    Shiyu Du, Paipai Zhang, Haozhen Liu, Donghai An, Yanna Chen

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  13. KNa 2 Y 2 B 2 O 6 F 3 : a beryllium free deep-UV nonlinear optical crystal with well-balanced properties

    Chemical Communications · 2025-01-01

    Huijian Zhao, Mengru Liu, Weina Nan, Ning Yang, Conggang Li, Ning Ye, Zhanggui Hu

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  14. Pb9Si8O22Cl6 and Pb3.07Ca1.93Si3O11: Two Ultraviolet Nonlinear Optical Materials Exhibit a Moderate Second Harmonic Generation Response

    Inorganic Chemistry · 2025-01-04

    Meihui Chen, Wei Wei, Jiawei Zhao, Juanjuan Lu, Donghai An, Yanna Chen

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  15. Impact of Fluorine in Manganese Citrate Synthesis on Structure and Value-Added Decomposition Products

    Molecules · 2025-04-16

    Aljaž Škrjanc, Emanuela Trstenjak, Mojca Opresnik, Matej Gabrijelčič, Amalija Golobič, Nataša Zabukovec Logar

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  16. Breaking the Natural Tendency of Deep‐UV Polyborate Anion Clusters to Inducing Strong Optical Anisotropy

    Small · 2025-04-24

    Ziqi Chen, Changyou Liu, Zhi Li, Juanjuan Lu, Junjie Li, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  17. Hydrogen‐Bonded Assembly of Functional Units for Constructing Linear and Nonlinear Optical Crystals

    Advanced Optical Materials · 2025-04-29

    Ziqi Chen, Changyou Liu, Chenxu Li, Juanjuan Lu, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  18. La2Zn3(SeO3)6: A UV Selenite Crystal with Second-Harmonic Generation and Large Birefringence

    Inorganic Chemistry · 2025-05-01

    Pengfei Li, Xiaoxue Wang, Chun‐Li Hu, Jiang‐Gao Mao, Fang Kong

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  19. Non-equivalent terminating roles of hydroxyl and fluorine in hydroxy/fluorooxo-borate optical functional materials

    Science China Chemistry · 2025-06-03

    Huanhuan Cheng, Shilie Pan, Zhihua Yang

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  20. Symmetry Breaking via Anion-Molecule Synergy: Fluorine and Crystalline Water Directed Construction of Noncentrosymmetric Sr(IO2F2)2·2H2O

    Inorganic Chemistry · 2025-06-09

    Peng Jiang, Wenhu Wang, Juhui Cui, Ping Bai, Hongli Wu, Minqiang Gai

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  21. Achieving the birefringence-bandgap trade-off: Hydrogen-bond engineered biuret-cyanurate

    Chinese Journal of Structural Chemistry · 2025-07-29

    Ziqi Chen, Miriding Mutailipu

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  22. Extending the Chemistry of Scheelite‐type Oxides with Borates

    Angewandte Chemie International Edition · 2025-08-12

    Chenhui Hu, Jian Wei Han, Huimin Li, Shujuan Han, Juanjuan Lu, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  23. Extending the Chemistry of Scheelite‐type Oxides with Borates

    Angewandte Chemie · 2025-08-12

    Chenhui Hu, Jian Wei Han, Huimin Li, Shujuan Han, Juanjuan Lu, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  24. A3ZnNO3X4 (A = Rb, NH4, X = Cl, I): Regulating Cations and Halides Yields Birefringent Crystals with Significantly Enhanced Optical Anisotropy

    Inorganic Chemistry · 2025-08-15

    Zhiyuan Zhang, Yabo Wu, Luyong Zhang, Xu Liu, Qiuyuan Feng, Lihan Deng, Jin Li, Shujuan Han

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  25. BaZn2(HPO3)3: A New Barium Zincophosphite with Short Ultraviolet Cutoff Edge

    European Journal of Inorganic Chemistry · 2025-08-27

    Yueling Sun, Anhua Gong

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  26. K5NaZr4F22(H2O)2: A Hydrated Zirconium Fluoride with a Second-Harmonic Generation Effect and a Short Ultraviolet Cutoff Edge Induced by Cosubstitution with Heterovalent Cations

    Inorganic Chemistry · 2025-08-27

    Bing-Wei Miao, Guo-Ren Zhu, Ling Wang, Wenfeng Zhou, Wenlong Liu, Ru‐Ling Tang

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  27. Discovery of novel fluorine modification of aryloxyacetic acid derivatives as 4-hydroxyphenylpyruvate dioxygenase inhibitors

    Journal of Fluorine Chemistry · 2025-08-29

    Hao Huang, Jing Leng, Jie Xu, Lei Zhou, Ming‐Xing Li, Diandian Ni, Zhenzhong Ding, Xiaoyan Gao

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  28. Borosilicates as deep-ultraviolet transparent nonlinear optical crystals: Structural motifs, performance limits and future directions

    Chinese Journal of Structural Chemistry · 2025-09-01

    Yangfeifei Ou, Xiaoliang Zhou, You‐Zhao Lan, Jian‐Wen Cheng

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  29. [HgX 2 ] Linear Group Enabled Ultraviolet Birefringent Crystal RbHg 5 Br 11 with Strong Optical Anisotropy and Wide Bandgap

    Advanced Science · 2025-09-09

    Yingtai Du, Wangfei Che, Yunfei Shi, Juanjuan Lu, Xiaodong Zhou, Ting Liu, Shilie Pan, Junjie Li

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  30. Sulfonated Module Aggregation for Ultrahigh Birefringence in Aqueous-Processable Crystals

    Journal of the American Chemical Society · 2025-10-14

    Congcong Jin, Yang Li, Chong‐An Chen, Jihyun Lee, Chanhee Ko, Soo‐Yeon Lee, Kang Min Ok

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  31. The nonlinear optical properties and through-space charge-transfer effects of the twist donor-acceptor complexes

    Dyes and Pigments · 2025-10-21

    Li Wang, Tongwei Liu, Yanli Liu, Mei‐Shan Wang

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  32. Organic π-conjugated units as versatile building blocks for high-performance birefringent crystals

    Chinese Journal of Structural Chemistry · 2025-11-19

    Zhenchao Bai, Sangen Zhao, Kang Min Ok, Junhua Luo

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  33. Ionic liquid-derived fluorine doped high entropy metal oxides as efficient electrocatalysts for sulfion valorization

    Journal of environmental chemical engineering · 2025-11-20

    Longmei Shi, Anshuang Wu, Shengyun Xu, Jinbiao Liang, Shucan Qin, Jiaming Mao, Yanrong Liu, Yingyi Ma

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  34. Ba 3 (MoO 2 F 3 )PO 4 F 2 : Rational Design and Synthesis of an Alkaline-Earth Phosphate Fluoride as a Birefringent Crystal

    Crystal Growth & Design · 2025-11-26

    Feng Xu, Mengya Qin, Bin Su, Chao He, Shaohua Yu, Yu Li, Rong Guo, Chan Zheng

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  35. Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion

    Angewandte Chemie International Edition · 2025-11-26

    Xiangyu Long, Fuming Li, Haotian Qiu, Xueling Hou, Juanjuan Lu, Junjie Li, Zhihua Yang, Jinhui Cao, Shilie Pan, Miriding Mutailipu

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  36. Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion

    Angewandte Chemie · 2025-11-26

    Xiangyu Long, Fuming Li, Haotian Qiu, Xueling Hou, Juanjuan Lu, Junjie Li, Zhihua Yang, Jinhui Cao, Shilie Pan, Miriding Mutailipu

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  37. Ba2CrIO3F6: a magnetic alkaline-earth chromium fluoroiodate with ferromagnetic exchange interactions

    Journal of Solid State Chemistry · 2025-12-24

    Shuaikun Li, Yanhong Wang, Haibo Li, Hang Liu, Yun Lv, Hongcheng Lu

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  38. Bandgap tuning through the substitution of alkali metal cations in A 2 AlCuF 6 (A = K, Rb, and Cs) for optoelectronic and renewable energy applications

    RSC Advances · 2026-01-01

    Muhammad Yaqoob, Nora Mobark Farhan, Hudabia Murtaza, Quratul Ain, Rawiyah A. Alkahtani, Junaid Munir, Mohammed Sultan Al-Buriahi

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  39. Broadband infrared-transparent crystals enabled by heterologous isomorphic substitution

    Dalton Transactions · 2026-01-01

    B Yang, Ziqi Chen, Zhenjiang Lu, Juanjuan Lu

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  40. From centrosymmetric (C 4 H 8 N 5 )(SbF 4 ) to polar (C 4 H 7 N 4 O)(SbF 4 ): a new UV nonlinear optical material achieved by functional group modulation

    Chemical Science · 2026-01-01

    Zhixiang Wang, Chun-Li Hu, Chuan‐Fu Sun, Jiang‐Gao Mao, Fang Kong

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  41. K 7 MgY 2 (B 5 O 10 ) 3 : a novel ultraviolet nonlinear optical crystal based on the [B 5 O 10 ] functional unit

    New Journal of Chemistry · 2026-01-01

    Haozhen Liu, Shiyu Du, Paipai Zhang, Jiawei Zhao, Yanna Chen, Donghai An

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  42. Solving the long-standing hygroscopicity and thermal stability issues of the nonlinear optical crystal α-LiIO 3 via homogeneous cation exchange

    Inorganic Chemistry Frontiers · 2026-01-01

    Jiahao Wan, Zhengli Liang, Xiuying Zhang, Hongming Liu, Le Yang, Ping Wang, Lehui Liu, Xingxing Jiang, Zheshuai Lin, Qi Wu

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  43. Te–Se replacement induced structural transition and enhanced band gaps in Cd 5 Se 4 O 12 Cl 2 and Cd 5 Se 4 O 12 Br 2

    Dalton Transactions · 2026-01-01

    Maqsood Iqbal, Jiazheng Zhou, Aqsa Munawar, Juanjuan Lu, Junjie Li

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  44. UV and X-ray excited luminescence from m -terphenyl crystals grown by the vertical Bridgman technique

    Journal of Materials Chemistry C · 2026-01-01

    Praveen Joshwa Ramesh, Rajesh Paulraj, Mohit Tyagi

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  45. 孤对电子效应羟基硼酸盐非线性光学研究进展（特邀）

    Chinese Journal of Lasers · 2026-01-01

    刘开通 Liu Kaitong, 饶远 Rao Yuan, 熊龙耀 Xiong Longyao, 张志忠 Zhang Zhizhong

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  46. Confinement-assembled ultraviolet nonlinear optical crystal from pyridine-expanded π-systems with exhibiting strong SHG and birefringence

    Science China Chemistry · 2026-01-04

    Chunmei Huang, Xuan Pang, Fuming M. Li, Shumei Cao, Shilie Pan, Miriding Mutailipu

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  47. Synthesis and Characterization of Poly(Fluoro-Aryl-Thiazole) Copolymers: Thermal, Spectroscopic Properties, and Application in Thorium and Aluminum Ions Detection from Aqueous Solutions

    Polymer Science Series B · 2026-02-01

    Suha S. Altarawneh, Ahmad Zeidan

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  48. KHg 4 Ga 5 S 12 : A Diamond-like Tetrahedral Chalcogenide Exhibiting Giant Phase-Matching Second Harmonic Generation

    Chemistry of Materials · 2026-02-03

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  49. Ba 5 Zn 4 (B 3 O 6 ) 2 (B 12 O 24 ): A Borate with Edge-Sharing [BO 4 ] Tetrahedral Connection by Introducing Zn into β-BaB 2 O 4

    Inorganic Chemistry · 2026-02-05

    Kaitong Liu, Yuan Rao, Zhaoxue Li, Shihang Zhou, Zhizhong Zhang, Yanhui Zhang

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  50. Density-Compensated Polarizability Anisotropy for Record Birefringence in Short-Wavelength Ultraviolet Inorganic Crystals

    Journal of the American Chemical Society · 2026-03-05

    Chong‐An Chen, Yang Li, Congcong Jin, S. D. Lee, Zhihua Yang, Kang Min Ok

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