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RESEARCH PAPER · Science China Chemistry · 2021

From borophosphate to fluoroborophosphate: a rational design of fluorine-induced birefringence enhancement

Wenyao Zhang, Zhizhong Zhang, Wenqi Jin, Ruonan Zhang, Meng Cheng, Zhihua Yang, Shilie Pan

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From borophosphate to fluoroborophosphate: a rational design of fluorine-induced birefringence enhancementOriginalLarge optical anisotropy-oriented construction of a carbonate-nitrate chloride compound as a potential ultraviolet birefringent material44Li 7 SrScB 12 O 24 and Li 7 Ba 0.6 Ca 0.4 ScB 12 O 24 : two new quaternary rare-earth borates with short UV cutoff edges4Linear unit BN 2 : a novel birefringence-enhanced fundamental module with sp orbital hybridization9Molecular Engineering Design of the First Sr2Be2B2O7-type Fluoride Carbonates AMgLi2(CO3)2F (A=K, Rb) as Deep-Ultraviolet Birefringent Crystal※1Na 2 SrB 16 O 26 : a new borate with independent interpenetrating B–O networks and deep-ultraviolet cutoff edge4Second-Harmonic Generation-Positive Na 2 Ga 2 SiS 6 with a Broad Band Gap and a High Laser Damage Threshold14(NH4)3B11PO19F3: a deep-UV nonlinear optical crystal with unique [B5PO10F]∞ layers142NaBa3[M2B7O16(OH)2]F2 (M = Ge, Si): Two Synthetic F Analogues of Garrelsite with [B7O16(OH)2]13– Polyanions and Deep-Ultraviolet Cutoff Edges8NaB3O4F(OH): A Hydroxyfluorooxoborate with One-Dimensional Chain Featuring Large Birefringence and Short Ultraviolet Cutoff Edge5C 3 N 6 H 7 SO 3 NH 2 : non-π-conjugated tetrahedra decoupling π-conjugated groups achieving large optical anisotropy and wide band gap29Linear π-conjugated units of the D ∞h point group as superior ultraviolet birefringent units1BaB2P2O8F2: A Fluoroborophosphate with [B2P2O8F2]∞ Layers and Deep-Ultraviolet Cutoff Edge4Ba2B9O13F4·BF4: first fluorooxoborate with unprecedented infinite [B18O26F8] tubes and deep-ultraviolet cutoff edge14Target-Oriented Synthesis of Borate Derivatives Featuring Isolated [B3O3] Six-Membered Rings as Structural Features20(C 3 N 6 H 7 )BF 4 ·H 2 O and (C 3 N 6 H 7 )SO 3 CH 3 ·H 2 O with large birefringence induced by coplanar π-conjugated [C 3 N 6 H 7 ] + groups33K 2 MgMoP 2 O 10 and K 3 Mg 2 MoP 3 O 14 : two new molybdophosphates exhibiting different optical anisotropies induced by variable dimensionality of the anion framework4Novel antimony phosphates with enlarged birefringence induced by lone pair cations4Screening Large Birefringent Materials via Halogen Regulation in Ternary d0-Transition Metal Oxyhalides8Theoretical Investigation of Structural, Electronic and Optical Properties of Cs3MoO4(HCO3) with NLO Active Functional Units2Trithionic guanidine: A novel semi-organic short-wave ultraviolet nonlinear optical sulfate with dimeric heteroleptic tetrahedra14Enhancement of Birefringence in π-Conjugated Oxyfluorides Achieved via van der Waals Layered Structural Optimization10Enhanced Birefringence in Phosphates via “Two Steps in One”: d0 Transition Metal Regulation and Fluorination Synergistic Strategy7Achieving the Birefringence Optimization by Methyl Modulation in Organic Nonlinear Optical Crystals15Structural Evolution and Optical Properties of Hydroxyfluorooxoborates MM′2n-1[B3O3F4(OH)]n (M = K, Cs, and Rb; M′ = K, NH4, and Cs; n = 1, 2, and 3)12Deep ultraviolet transparent borophosphates LiAB 2 P 2 O 9 (A = NH 4 , K) and LiNaB 2 P 2 O 8 (OH) 2 ·H 2 O exhibiting a moderate second-harmonic generation response4Li 2 CeRbB 18 O 30 and Li 2 Cs 2 SrB 18 O 30 : promising low-birefringence materials for UV and deep UV zero-order waveplates4M 2 Al 2 Ti(PO 4 ) 4 (M = Rb, Cs): synthesis and optical property investigation of two titanium phosphates with a dissimilar structural configuration2Na 2 PbB 6 O 10 SO 4 and Ca 2.58 Pb 0.42 B 6 O 11 SO 4 : first borate–sulfates featuring 3D porous borate anionic frameworks0Tailoring UV waveplate materials via rational assembly of functional motifs in scandium fluoride phosphate2KTeOPO 4 and NH 4 SnClSO 4 : two new KTiOPO 4 derivatives as birefringent crystals featuring enhanced optical anisotropy0Microstructural evolution and thermal protection mechanism of ceramifiable silicone composites via boron phosphate phase transformation2Study on luminescence recognition of Fe3+, I− and F− by europium and terbium carboxylic acid complexes0Urea revisited: Isopropyl substitution for a balanced nonlinear optical performance0

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  1. Large optical anisotropy-oriented construction of a carbonate-nitrate chloride compound as a potential ultraviolet birefringent material

    Chemical Science · 2022-01-01

    Meng Cheng, Wenqi Jin, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  2. Li 7 SrScB 12 O 24 and Li 7 Ba 0.6 Ca 0.4 ScB 12 O 24 : two new quaternary rare-earth borates with short UV cutoff edges

    New Journal of Chemistry · 2022-01-01

    Jianbang Chen, Jie Zhang, Aixin Zhu, Xuchu Huang

    Read original paper ↗ ·

  3. Linear unit BN 2 : a novel birefringence-enhanced fundamental module with sp orbital hybridization

    RSC Advances · 2022-01-01

    Jianbang Chen, Mengfan Wu, Jie Zhang, Xuchu Huang

    Read original paper ↗ ·

  4. Molecular Engineering Design of the First Sr2Be2B2O7-type Fluoride Carbonates AMgLi2(CO3)2F (A=K, Rb) as Deep-Ultraviolet Birefringent Crystal※

    化学学报 · 2022-01-01

    Yunxia Song, Fei Liang, Haotian Tian, Yan Wu, Min Luo

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  5. Na 2 SrB 16 O 26 : a new borate with independent interpenetrating B–O networks and deep-ultraviolet cutoff edge

    Dalton Transactions · 2022-01-01

    Zhikang Chen, Kewang Zhang, Bei Zhang, Jun Zhang

    Read original paper ↗ ·

  6. Second-Harmonic Generation-Positive Na 2 Ga 2 SiS 6 with a Broad Band Gap and a High Laser Damage Threshold

    Inorganic Chemistry · 2022-05-05

    Wenlong Xie, Yihan Yun, Lihan Deng, Guangmao Li, Shilie Pan

    Read original paper ↗ ·

  7. (NH4)3B11PO19F3: a deep-UV nonlinear optical crystal with unique [B5PO10F]∞ layers

    National Science Review · 2022-06-10

    Bingliang Cheng, Zi‐Jian Li, Yu Chu, Abudukadi Tudi, Miriding Mutailipu, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  8. NaBa3[M2B7O16(OH)2]F2 (M = Ge, Si): Two Synthetic F Analogues of Garrelsite with [B7O16(OH)2]13– Polyanions and Deep-Ultraviolet Cutoff Edges

    Inorganic Chemistry · 2022-07-05

    Weijie Xie, Chun‐Li Hu, Zhi Gang Fang, Ming‐Yang Cao, Yuan Hua Lin, Jiang‐Gao Mao

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  9. NaB3O4F(OH): A Hydroxyfluorooxoborate with One-Dimensional Chain Featuring Large Birefringence and Short Ultraviolet Cutoff Edge

    Inorganic Chemistry · 2022-08-18

    Yu Dang, Dongdong Chu, Zhihua Yang, Hongsheng Shi, Shilie Pan

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  10. C 3 N 6 H 7 SO 3 NH 2 : non-π-conjugated tetrahedra decoupling π-conjugated groups achieving large optical anisotropy and wide band gap

    Materials Chemistry Frontiers · 2023-01-01

    Danyang Dou, Qi Shi, Yunjie Bai, Cheng Chen, Bingbing Zhang, Ying Wang

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  11. Linear π-conjugated units of the D ∞h point group as superior ultraviolet birefringent units

    Physical Chemistry Chemical Physics · 2023-01-01

    Rong Yang, Abudukadi Tudi, Yu Dang, Kewang Zhang, Hongsheng Shi

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  12. BaB2P2O8F2: A Fluoroborophosphate with [B2P2O8F2]∞ Layers and Deep-Ultraviolet Cutoff Edge

    Inorganic Chemistry · 2023-01-04

    Jinbin Fan, Mengfan Wu, Bingliang Cheng, Jian Wei Han

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  13. Ba2B9O13F4·BF4: first fluorooxoborate with unprecedented infinite [B18O26F8] tubes and deep-ultraviolet cutoff edge

    Science China Chemistry · 2023-02-23

    Huan Pei, Xuefei Wang, Jie Zhang, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  14. Target-Oriented Synthesis of Borate Derivatives Featuring Isolated [B3O3] Six-Membered Rings as Structural Features

    Inorganic Chemistry · 2023-05-31

    Meng Cheng, Congcong Jin, Wenqi Jin, Xueling Hou

    Read original paper ↗ ·

  15. (C 3 N 6 H 7 )BF 4 ·H 2 O and (C 3 N 6 H 7 )SO 3 CH 3 ·H 2 O with large birefringence induced by coplanar π-conjugated [C 3 N 6 H 7 ] + groups

    Inorganic Chemistry Frontiers · 2024-01-01

    Hangwei Jia, Die Xu, Zi‐Jian Li, Muhammad Sharjeel Arif, Yansheng Jiang, Xueling Hou

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  16. K 2 MgMoP 2 O 10 and K 3 Mg 2 MoP 3 O 14 : two new molybdophosphates exhibiting different optical anisotropies induced by variable dimensionality of the anion framework

    Dalton Transactions · 2024-01-01

    Zhixia Gao, Qiuyuan Feng, Juanjuan Lu, Hong Lei Du

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  17. Novel antimony phosphates with enlarged birefringence induced by lone pair cations

    Dalton Transactions · 2024-01-01

    Mei Hu, Jialong Wang, Nuerbiye Tuerhong, Zhiyuan Zhang, Qun Jing, Zhaohui Chen, Yonglei Yang, Ming‐Hsien Lee

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  18. Screening Large Birefringent Materials via Halogen Regulation in Ternary d0-Transition Metal Oxyhalides

    The Journal of Physical Chemistry C · 2024-01-14

    Xueting Pan, Junben Huang, Yineng Huang

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  19. Theoretical Investigation of Structural, Electronic and Optical Properties of Cs3MoO4(HCO3) with NLO Active Functional Units

    European Journal of Inorganic Chemistry · 2024-03-06

    Jinyu Hu, Yinsheng Huang, Hui Zhu, Huiyan Zhao, Chao He, Xihu Wang

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  20. Trithionic guanidine: A novel semi-organic short-wave ultraviolet nonlinear optical sulfate with dimeric heteroleptic tetrahedra

    Chinese Chemical Letters · 2024-03-08

    Hongyuan Sha, Dongling Yang, Yanran Shang, Zujian Wang, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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  21. Enhancement of Birefringence in π-Conjugated Oxyfluorides Achieved via van der Waals Layered Structural Optimization

    Crystal Growth & Design · 2024-04-01

    Wenyao Zhang, Zichen Li, Xudong Leng, Qun Jing, Qiao Wen

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  22. Enhanced Birefringence in Phosphates via “Two Steps in One”: d0 Transition Metal Regulation and Fluorination Synergistic Strategy

    The Journal of Physical Chemistry C · 2024-04-22

    Ketian Hou, Changyou Liu, Qiuyuan Feng, Yonglei Yang, Bei Zhang

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  23. Achieving the Birefringence Optimization by Methyl Modulation in Organic Nonlinear Optical Crystals

    Advanced Optical Materials · 2024-09-19

    Dongling Yang, Hongyuan Sha, Zujian Wang, Rongbing Su, Chao He, Bin Su, Xiaoming Yang, Xifa Long

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  24. Structural Evolution and Optical Properties of Hydroxyfluorooxoborates MM′2n-1[B3O3F4(OH)]n (M = K, Cs, and Rb; M′ = K, NH4, and Cs; n = 1, 2, and 3)

    Chemistry of Materials · 2024-11-25

    Huan Pei, Luyong Zhang, Huanhuan Cheng, Shi‐Bin Wang, Zhihua Yang, Fangfang Zhang, Shilie Pan

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  25. Deep ultraviolet transparent borophosphates LiAB 2 P 2 O 9 (A = NH 4 , K) and LiNaB 2 P 2 O 8 (OH) 2 ·H 2 O exhibiting a moderate second-harmonic generation response

    Journal of Materials Chemistry C · 2024-12-23

    Huanhuan Zhao, Chenxu Li, Juanjuan Lu, Zhihua Yang, Jian Wei Han, Shilie Pan

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  26. Li 2 CeRbB 18 O 30 and Li 2 Cs 2 SrB 18 O 30 : promising low-birefringence materials for UV and deep UV zero-order waveplates

    Dalton Transactions · 2025-01-01

    Xiao-Ming Wang, Zhiyuan Zhang, Juanjuan Lu, Feng Zhang, Shilie Pan

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  27. M 2 Al 2 Ti(PO 4 ) 4 (M = Rb, Cs): synthesis and optical property investigation of two titanium phosphates with a dissimilar structural configuration

    New Journal of Chemistry · 2025-01-01

    Tuohetijiang Baiheti, Mairihaba Ababaike, Salamaiti Wumaier, Wang Shutong

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  28. Na 2 PbB 6 O 10 SO 4 and Ca 2.58 Pb 0.42 B 6 O 11 SO 4 : first borate–sulfates featuring 3D porous borate anionic frameworks

    Inorganic Chemistry Frontiers · 2025-01-01

    Huan Pei, Zi‐Jian Li, Shaohuan Liu, Xueling Hou, Fangfang Zhang

    Read original paper ↗ ·

  29. Tailoring UV waveplate materials via rational assembly of functional motifs in scandium fluoride phosphate

    Chemical Communications · 2025-01-01

    Huijian Zhao, Conggang Li, Ning Ye, Zhanggui Hu

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  30. KTeOPO 4 and NH 4 SnClSO 4 : two new KTiOPO 4 derivatives as birefringent crystals featuring enhanced optical anisotropy

    Journal of Materials Chemistry C · 2026-01-01

    Ruo-Nan Zhang, Xuping Shi, Abudukadi Tudi, Wenbin Zhang, Zhihua Yang, Fangfang Zhang, Shilie Pan, Shujuan Han

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  31. Microstructural evolution and thermal protection mechanism of ceramifiable silicone composites via boron phosphate phase transformation

    Polymer Degradation and Stability · 2026-02-10

    Jingyao Xu, Wanting Song, Sujie Hu, Laibin Zhang, Shuilai Qiu

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  32. Study on luminescence recognition of Fe3+, I− and F− by europium and terbium carboxylic acid complexes

    Journal of Molecular Structure · 2026-06-27

    Qiang Zhao, Zhi Shen, Lin-Xi Qin, Meng-ting Fan, Pei-Xuan Zhang, Xin-Yue Zhang

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  33. Urea revisited: Isopropyl substitution for a balanced nonlinear optical performance

    Journal of Molecular Structure · 2026-09-01

    Yang Chi, Ya-Ping Zhao

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