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RESEARCH PAPER · Chemistry of Materials · 2016

Directed Lifting of Inversion Symmetry in Ruddlesden–Popper Oxide–Fluorides: Toward Ferroelectric and Multiferroic Behavior

Ronghuan Zhang, Mark S. Senn, Michael A. Hayward

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Directed Lifting of Inversion Symmetry in Ruddlesden–Popper Oxide–Fluorides: Toward Ferroelectric and Multiferroic BehaviorOriginalSynthesis and μ-Raman scattering of Ruddlesden-Popper ceramics Sr3Ti2O7, SrLa2Al2O7 and Sr2LaAlTiO720Structural Modification of the Cation-Ordered Ruddlesden–Popper Phase YSr2Mn2O7 by Cation Exchange and Anion Insertion19Topotactic Reduction toward a Noncentrosymmetric Deficient Perovskite Tb0.50Ca0.50Mn0.96O2.37 with Ordered Mn Vacancies and Piezoelectric Behavior8Soft chemistry of ion-exchangeable layered metal oxides183Structural Diversity from Anion Order in Heteroanionic Materials53Topochemical Fluorination of La2NiO4+d: Unprecedented Ordering of Oxide and Fluoride Ions in La2NiO3F257Ferroelectric Sr 3 Zr 2 O 7 : Competition between Hybrid Improper Ferroelectric and Antiferroelectric Mechanisms132Sr3Ir2O7F2 : Topochemical conversion of a relativistic Mott state into a spin-orbit driven band insulator3Hybrid Improper Ferroelectricity in (Sr,Ca) 3 Sn 2 O 7 and Beyond: Universal Relationship between Ferroelectric Transition Temperature and Tolerance Factor in n = 2 Ruddlesden–Popper Phases123Negative thermal expansion in high pressure layered perovskite Ca 2 GeO 410Heteroanionic Materials by Design: Progress Toward Targeted Properties236Competing Polar and Antipolar Structures in the Ruddlesden–Popper Layered Perovskite Li2SrNb2O740Predicting the Structure Stability of Layered Heteroanionic Materials Exhibiting Anion Order16Preparation of the noncentrosymmetric ferrimagnetic phase La0.9Ba0.1Mn0.96O2.43 by topochemical reduction0Bi2W2O9 : A potentially antiferroelectric Aurivillius phase14High cycle life all-solid-state fluoride ion battery with La2NiO4+d high voltage cathode76Synergistic Influence of d0 (Nb5+) and d10 (Cd2+) Cations in Stabilizing Noncentrosymmetric Dion–Jacobson Layered Perovskites, A′Cd2Nb3O10 (A′ = Rb, Cs)12Synthesis of NaMoO3F and Na5W3O9F5 with Morphological Controllability in Non-Aqueous Solvents15Unraveling the Suppression of Oxygen Octahedra Rotations in A3B2O7 Ruddlesden-Popper Compounds: Engineering Multiferroicity and Beyond53Electrochemical Reduction and Oxidation of Ruddlesden–Popper-Type La 2 NiO 3 F 2 within Fluoride-Ion Batteries38Interplay between Oxo and Fluoro in Vanadium Oxyfluorides for Centrosymmetric and Non-Centrosymmetric Structure Formation4Ferroelectricity and multiferroicity in anti–Ruddlesden–Popper structures23Studies on the structure, optical, ac conduction mechanism by OLPT model and impedance spectroscopy of La-doped Ba2SnO4 Ruddlesden Popper Oxide6Spin and Orbital Effects on Asymmetric Exchange Interaction in Polar Magnets: M(IO3)2 (M = Cu, Mn)0Structure, Magnetism, and Thermal Stability of La2NiO2.5F3: A Ruddlesden–Popper Oxyfluoride Crystallizing in Space Group P42/nnm24Influence of La doping on structure, AC conductivity and impedance spectroscopy of Ba2SnO4 Ruddlesden Popper oxide32Symmetry and the Role of the Anion Sublattice in Aurivillius Oxyfluoride Bi2TiO4F218Spin and Orbital Effects on Asymmetric Exchange Interaction in Polar Magnets: M(IO3)2 (M = Cu and Mn)8Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides36Improvement of electric insulation in dielectric layered perovskite nickelate films via fluorination8Designing new polar materials1Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective45Spin-orbit excitons and electronic configuration of the 5d4 insulator Sr3Ir2O7F26Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics7Polymorphism in the Ruddlesden–Popper Nickelate La 3 Ni 2 O 7 : Discovery of a Hidden Phase with Distinctive Layer Stacking123La 2 SrSc 2 O 7 : A -Site Cation Disorder Induces Ferroelectricity in Ruddlesden–Popper Layered Perovskite Oxide29“Hexagonal” Perovskites: From Stacking Sequence to Space Group Symmetry and New Opportunities14Interplay between A-site and oxygen-vacancy ordering, and mixed electron/oxide-ion conductivity in n = 1 Ruddlesden–Popper perovskite Sr 2 Nd 2 Zn 2 O 77Possible transformation between half-metallic and metallic states of multiferroic MnGaSSe 2 monolayers0Recent Progress of Hybrid Improper Ferroelectrics with Ruddlesden-Popper Structure1Structure, magnetism and thermal stability of the n = 3 Ruddlesden–Popper oxyfluoride La 4 Ni 3 O 8.4 F 3.54Fluorine as a Key Element in Solid-State Chemistry of Mixed Anions 3d Transition Metal-Based Materials for Electronic Properties and Energy24Energy storage and ferroelectric properties of La‐doped Bi 3 TaTiO 9 thin films affected by La concentration3Atomic-scale observation of geometric reconstruction in a fluorine-intercalated infinite layer nickelate superlattice2Atomic insights into topochemical fluorination and strong octahedral tilt in La2CoO42Controlling the Regioselectivity of Topochemical Reduction Reactions Through Sequential Anion Insertion and Extraction2Controlling the Regioselectivity of Topochemical Reduction Reactions Through Sequential Anion Insertion and Extraction0Gas evolution in Ruddlesden–Popper-type intercalation cathodes in all-solid-state fluoride-ion-batteries: implications on battery performance and synthesis of highly oxidized oxyfluorides5Hybrid improper ferroelectricity and phase transition in La2Sr(Sc1− x In x )2O7 ceramics2Crystal structures, dielectric properties, and phase transition in hybrid improper ferroelectric Li2Sm2Ti3O10 ceramics0Crystal structures, dielectric properties, and thermal behavior in hybrid improper ferroelectric Li2Sm2Ti3O10 ceramics0Synthesis of the Double Infinite-Layer Ni(I) Phase La 3 Ni 2 O 5 F via Sequential Topochemical Reactions2NaI-Mediated Defluorination: A Mild Route to Reduced Ruddlesden–Popper Oxyfluorides Demonstrated on La 2 CoO 3 F 3 as Model System2Redox-Neutral Interstitial Hydride Incorporation in Ruddlesden–Popper Oxides0Cation-driven symmetry breaking in rare-earth borates toward ultraviolet nonlinear optical materials1The distinct displacement of atomic column position induced by crystal symmetry effects in ABF-STEM and iDPC-STEM imaging0Hybrid improper ferroelectricity and enhanced Curie temperature in co-substituted La2SrSc2O7-based ceramics0

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  1. Synthesis and μ-Raman scattering of Ruddlesden-Popper ceramics Sr3Ti2O7, SrLa2Al2O7 and Sr2LaAlTiO7

    Journal of Alloys and Compounds · 2017-07-16

    Anderson Dias, Jéssica Ivone Viegas, Roberto Luiz Moreira

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  2. Structural Modification of the Cation-Ordered Ruddlesden–Popper Phase YSr2Mn2O7 by Cation Exchange and Anion Insertion

    Inorganic Chemistry · 2017-08-04

    Ronghuan Zhang, Alexandra S. Gibbs, Weiguo Zhang, P. Shiv Halasyamani, Michael A. Hayward

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  3. Topotactic Reduction toward a Noncentrosymmetric Deficient Perovskite Tb0.50Ca0.50Mn0.96O2.37 with Ordered Mn Vacancies and Piezoelectric Behavior

    Chemistry of Materials · 2017-10-30

    Hao Zhang, Song Wei Gao, Qinghua Zhang, Jingen Wu, Jie Liang, Cheng Dong, Lin Gu, Shuxiang Dong, Junliang Sun, Fuhui Liao, Jianhua Lin, Ruqiang Zou, Guobao Li

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  4. Soft chemistry of ion-exchangeable layered metal oxides

    Chemical Society Reviews · 2018-01-01

    Ritesh Uppuluri, Arnab Sen Gupta, Alyssa S. Rosas, Thomas E. Mallouk

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  5. Structural Diversity from Anion Order in Heteroanionic Materials

    Chemistry of Materials · 2018-04-30

    Nenian Charles, Richard J. Saballos, James M. Rondinelli

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  6. Topochemical Fluorination of La2NiO4+d: Unprecedented Ordering of Oxide and Fluoride Ions in La2NiO3F2

    Inorganic Chemistry · 2018-05-11

    Kerstin Wissel, Jonas Heldt, Pedro B. Groszewicz, Supratik Dasgupta, Hergen Breitzke, Manuel Donzelli, Aamir Iqbal Waidha, Andrew Dominic Fortes, Jochen Rohrer, Peter Raymond Slater, Gerd Buntkowsky, Oliver Clemens

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  7. Ferroelectric Sr 3 Zr 2 O 7 : Competition between Hybrid Improper Ferroelectric and Antiferroelectric Mechanisms

    Advanced Functional Materials · 2018-05-28

    Suguru Yoshida, Koji Fujita, Hirofumi Akamatsu, Olivier Hernandez, Arnab Sen Gupta, Forrest G. Brown, Haricharan Padmanabhan, Alexandra S. Gibbs, Toshihiro Kuge, Ryosuke Tsuji, Shunsuke Murai, James M. Rondinelli, Venkatraman Gopalan, Katsuhisa Tanaka

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  8. Sr3Ir2O7F2 : Topochemical conversion of a relativistic Mott state into a spin-orbit driven band insulator

    Physical review. B./Physical review. B · 2018-10-16

    Christi Peterson, Michael W. Swift, Zach Porter, Raphaële J. Clément, Guang Xin Wu, Gihyeon Ahn, S. J. Moon, Bryan C. Chakoumakos, Jacob P. C. Ruff, Huibo B. Cao, Chris G. Van de Walle, Stephen D. Wilson

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  9. Hybrid Improper Ferroelectricity in (Sr,Ca) 3 Sn 2 O 7 and Beyond: Universal Relationship between Ferroelectric Transition Temperature and Tolerance Factor in n = 2 Ruddlesden–Popper Phases

    Journal of the American Chemical Society · 2018-10-23

    Suguru Yoshida, Hirofumi Akamatsu, Ryosuke Tsuji, Olivier Hernandez, Haricharan Padmanabhan, Arnab Sen Gupta, Alexandra S. Gibbs, Ko Mibu, Shunsuke Murai, James M. Rondinelli, Venkatraman Gopalan, Katsuhisa Tanaka, Koji Fujita

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  10. Negative thermal expansion in high pressure layered perovskite Ca 2 GeO 4

    Chemical Communications · 2019-01-01

    Wei‐Tin Chen, Chris Ablitt, Nicholas C. Bristowe, Arash A. Mostofi, Takashi Kei SAITO, Yuichi Shimakawa, Mark S. Senn

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  11. Heteroanionic Materials by Design: Progress Toward Targeted Properties

    Advanced Materials · 2019-03-12

    Jaye K. Harada, Nenian Charles, Kenneth Reinhard Poeppelmeier, James M. Rondinelli

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  12. Competing Polar and Antipolar Structures in the Ruddlesden–Popper Layered Perovskite Li2SrNb2O7

    Chemistry of Materials · 2019-06-12

    Ritesh Uppuluri, Hirofumi Akamatsu, Arnab Sen Gupta, Huaiyu Hugo Wang, Craig M. Brown, Kleyser Agueda Lopez, Nasim Alem, Venkatraman Gopalan, Thomas E. Mallouk

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  13. Predicting the Structure Stability of Layered Heteroanionic Materials Exhibiting Anion Order

    Inorganic Chemistry · 2019-09-17

    Jaye K. Harada, Kenneth Reinhard Poeppelmeier, James M. Rondinelli

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  14. Preparation of the noncentrosymmetric ferrimagnetic phase La0.9Ba0.1Mn0.96O2.43 by topochemical reduction

    Journal of Solid State Chemistry · 2020-04-05

    Thomas G. Parsons, Joke Hadermann, P. Shiv Halasyamani, Michael A. Hayward

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  15. Bi2W2O9 : A potentially antiferroelectric Aurivillius phase

    Physical review. B./Physical review. B · 2020-04-29

    Hania Djani, Emma E. McCabe, W. Zhang, P. Shiv Halasyamani, Antonio M. Feteira, Jordan Bieder, Éric Bousquet, Philippe Ghosez

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  16. High cycle life all-solid-state fluoride ion battery with La2NiO4+d high voltage cathode

    Communications Materials · 2020-05-15

    Mohammad Ali Nowroozi, Kerstin Wissel, Manuel Donzelli, Niloofar Hosseinpourkahvaz, Sergi Plana‐Ruiz, Ute Kolb, Roland Schoch, Matthias Bauer, Ali Muhammad Malik, Jochen Rohrer, Sergei I. Ivlev, Florian Kraus, Oliver Clemens

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  17. Synergistic Influence of d0 (Nb5+) and d10 (Cd2+) Cations in Stabilizing Noncentrosymmetric Dion–Jacobson Layered Perovskites, A′Cd2Nb3O10 (A′ = Rb, Cs)

    Inorganic Chemistry · 2020-05-28

    Shalu Atri, Meenakshi Pokhriyal, S. Uma

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  18. Synthesis of NaMoO3F and Na5W3O9F5 with Morphological Controllability in Non-Aqueous Solvents

    Inorganic Chemistry · 2020-07-21

    Yusuke Asakura, Tomoyo Akahira, Makoto Kobayashi, Minoru Osada, Shu Yin

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  19. Unraveling the Suppression of Oxygen Octahedra Rotations in A3B2O7 Ruddlesden-Popper Compounds: Engineering Multiferroicity and Beyond

    Physical Review Letters · 2020-10-08

    Yajun Zhang, Jie Wang, Philippe Ghosez

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  20. Electrochemical Reduction and Oxidation of Ruddlesden–Popper-Type La 2 NiO 3 F 2 within Fluoride-Ion Batteries

    Chemistry of Materials · 2021-01-06

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  21. Interplay between Oxo and Fluoro in Vanadium Oxyfluorides for Centrosymmetric and Non-Centrosymmetric Structure Formation

    Molecules · 2021-01-24

    Prashanth Sandineni, Hooman Yaghoobnejad Asl, Weiguo Zhang, P. Shiv Halasyamani, K. Ghosh, Amitava Choudhury

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  22. Ferroelectricity and multiferroicity in anti–Ruddlesden–Popper structures

    Proceedings of the National Academy of Sciences · 2021-04-23

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  23. Studies on the structure, optical, ac conduction mechanism by OLPT model and impedance spectroscopy of La-doped Ba2SnO4 Ruddlesden Popper Oxide

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  24. Spin and Orbital Effects on Asymmetric Exchange Interaction in Polar Magnets: M(IO3)2 (M = Cu, Mn)

    arXiv (Cornell University) · 2021-08-09

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  25. Structure, Magnetism, and Thermal Stability of La2NiO2.5F3: A Ruddlesden–Popper Oxyfluoride Crystallizing in Space Group P42/nnm

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  26. Influence of La doping on structure, AC conductivity and impedance spectroscopy of Ba2SnO4 Ruddlesden Popper oxide

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  27. Symmetry and the Role of the Anion Sublattice in Aurivillius Oxyfluoride Bi2TiO4F2

    Inorganic Chemistry · 2021-09-01

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  28. Spin and Orbital Effects on Asymmetric Exchange Interaction in Polar Magnets: M(IO3)2 (M = Cu and Mn)

    Inorganic Chemistry · 2021-10-12

    Ebube E. Oyeka, Michal Jerzy Winiarski, Maurice Sorolla, Keith M. Taddei, Allen O. Scheie, T. Thao Tran

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  29. Review of experimental progress of hybrid improper ferroelectricity in layered perovskite oxides

    Journal of Physics D Applied Physics · 2021-10-22

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  30. Improvement of electric insulation in dielectric layered perovskite nickelate films via fluorination

    Journal of Materials Chemistry C · 2021-12-22

    Takuma Nishimura, Tsukasa Katayama, Shishin Mo, Akira Chikamatsu, Tetsuya Hasegawa

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  31. Designing new polar materials

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  32. Hybrid Improper Ferroelectricity: A Theoretical, Computational, and Synthetic Perspective

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  33. Spin-orbit excitons and electronic configuration of the 5d4 insulator Sr3Ir2O7F2

    Physical review. B./Physical review. B · 2022-09-22

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  34. Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics

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  35. Polymorphism in the Ruddlesden–Popper Nickelate La 3 Ni 2 O 7 : Discovery of a Hidden Phase with Distinctive Layer Stacking

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  36. La 2 SrSc 2 O 7 : A -Site Cation Disorder Induces Ferroelectricity in Ruddlesden–Popper Layered Perovskite Oxide

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  37. “Hexagonal” Perovskites: From Stacking Sequence to Space Group Symmetry and New Opportunities

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  38. Interplay between A-site and oxygen-vacancy ordering, and mixed electron/oxide-ion conductivity in n = 1 Ruddlesden–Popper perovskite Sr 2 Nd 2 Zn 2 O 7

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  39. Possible transformation between half-metallic and metallic states of multiferroic MnGaSSe 2 monolayers

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  40. Recent Progress of Hybrid Improper Ferroelectrics with Ruddlesden-Popper Structure

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  41. Structure, magnetism and thermal stability of the n = 3 Ruddlesden–Popper oxyfluoride La 4 Ni 3 O 8.4 F 3.5

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  42. Fluorine as a Key Element in Solid-State Chemistry of Mixed Anions 3d Transition Metal-Based Materials for Electronic Properties and Energy

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  43. Energy storage and ferroelectric properties of La‐doped Bi 3 TaTiO 9 thin films affected by La concentration

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  44. Atomic-scale observation of geometric reconstruction in a fluorine-intercalated infinite layer nickelate superlattice

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  45. Atomic insights into topochemical fluorination and strong octahedral tilt in La2CoO4

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  46. Controlling the Regioselectivity of Topochemical Reduction Reactions Through Sequential Anion Insertion and Extraction

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  47. Controlling the Regioselectivity of Topochemical Reduction Reactions Through Sequential Anion Insertion and Extraction

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  48. Gas evolution in Ruddlesden–Popper-type intercalation cathodes in all-solid-state fluoride-ion-batteries: implications on battery performance and synthesis of highly oxidized oxyfluorides

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  49. Hybrid improper ferroelectricity and phase transition in La2Sr(Sc1− x In x )2O7 ceramics

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  50. Crystal structures, dielectric properties, and phase transition in hybrid improper ferroelectric Li2Sm2Ti3O10 ceramics

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