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RESEARCH PAPER · Chemistry of Materials · 2016

A Deep-Ultraviolet Nonlinear Optical Crystal: Strontium Beryllium Borate Fluoride with Planar Be(O/F)3 Groups

Na Yu, Shichao Wang, Ning Ye, Fei Liang, Zheshuai Lin, Min Luo, Kenneth Reinhard Poeppelmeier

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A Deep-Ultraviolet Nonlinear Optical Crystal: Strontium Beryllium Borate Fluoride with Planar Be(O/F)3 GroupsOriginalChemInform Abstract: A Deep‐Ultraviolet Nonlinear Optical Crystal: Strontium Beryllium Borate Fluoride with Planar Be(O/F)3 Groups.0SrNO3(OH)·H2O: A new member in strontium nitrate hydrate family with an ultraviolet cut-off edge7BaBe2BO3F3: A KBBF-Type Deep-Ultraviolet Nonlinear Optical Material with Reinforced [Be2BO3F2]∞ Layers and Short Phase-Matching Wavelength80Syntheses, crystal structures and characterization of three alkaline metal borates7Facile Syntheses of Ba2[B4O7(OH)2] and Na[B5O7(OH)2](H2O) Borate Salts Exhibiting Nonlinear Optical Activity in the Ultraviolet50Comparative Interrelationship of the Structural, Nonlinear-Optical and Other Acentric Properties for Oxide, Borate and Carbonate Crystals16Structure Determination and Luminescent Property Studies of the Single Crystal Na3Sm(BO3)212Deep-Ultraviolet Nonlinear-Optical Material K3Sr3Li2Al4B6O20F: Addressing the Structural Instability Problem in KBe2BO3F2105A new mixed alkali metal borate: LiCs[B5O8(OH)]·H2O11MBaYB 6 O 12 (M = Rb, Cs): two new rare-earth borates with large birefringence and short ultraviolet cutoff edges42Nature of the Color of Borates with “Anti-Zeolite” Structure19SrB 5 O 7 F 3 Functionalized with [B 5 O 9 F 3 ] 6− Chromophores: Accelerating the Rational Design of Deep‐Ultraviolet Nonlinear Optical Materials738SrB5O7F3 Functionalized with [B5O9F3]6− Chromophores: Accelerating the Rational Design of Deep‐Ultraviolet Nonlinear Optical Materials116Recent advances in ultraviolet and deep-ultraviolet second-order nonlinear optical crystals256Deep‐Ultraviolet Nonlinear Optical Crystal Cs2Al2(B3O6)2O: A Benign Member of the Sr2Be2(BO3)2O Family with [Al2(B3O6)2O]2− Double Layers70From Sr2Nb2O7to CaxSr2–xNb2O7: An Effective Enhancement of Nonlinear Optical Activity by a Simple Way of Cation Substituting11Bi2ZnOB2O6: a polar material capable of photocatalytic degradation of Rhodamine B15Second-order nonlinear optical crystals with mixed anions251Mg 3 B 7 O 13 Cl: A New Quasi‐Phase Matching Crystal in the Deep‐Ultraviolet Region56Na4Yb(CO3)3F: A New UV Nonlinear Optical Material with a Large Second Harmonic Generation Response8Investigation on the growth, optical, mechanical and dielectric properties of an inorganic potassium pentaborate dihydrate (KB5H4O10.2H2O) single crystal12Experimental characterization and first principles calculations of linear and nonlinear optical properties of two orthophosphates A 3 Al 2 (PO 4 ) 3 (A = Rb, K)37Li 4 Na 2 CsB 7 O 14 : a new edge-sharing [BO 4 ] 5− tetrahedra containing borate with high anisotropic thermal expansion52A 2 Bi 2 (SO 4 ) 2 Cl 4 (A = NH 4 , K, Rb): achieving a subtle balance of the large second harmonic generation effect and sufficient birefringence in sulfate nonlinear optical materials99Sn 2 B 7 O 12 F with a 2∞[B 14 O 24 ] 6− layer constructed from the unprecedented [B 7 O 16 ] 11− fundamental building block18BeO6 Trigonal Prism with Ultralong Be–O Bonds Observed in a Deep Ultraviolet Optical Crystal Li13BeBe6B9O2712Synthesis and enhanced photocatalytic activity of {1 0 1¯ 0} faceted hexagonal YBO37Ca 2 B 5 O 9 Cl and Sr 2 B 5 O 9 Cl: Nonlinear Optical Crystals with Deep-Ultraviolet Transparency Windows46Synthesis, Crystal Structure, and Characterization of a Noncentrosymmetric Sulfate Cs2Ca2(SO4)320Compressibility of hingganite-(Y): high-pressure single crystal X-ray diffraction study6A 3 BBi(P 2 O 7 ) 2 (A = Rb, Cs; B = Pb, Ba): Isovalent Cation Substitution to Sustain Large Second-Harmonic Generation Responses106Sn3B8O15: A Ternary Tin(II) Borate with Flexible [B8O18]12– Fundamental Building Block Formed by [B7O16]11– and [BO3]3– Groups10Computationally assisted multistage design and prediction driving the discovery of deep-ultraviolet nonlinear optical materials41Recent advances of oxyfluorides for nonlinear optical applications69Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application168Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application18LiB2O3F: A Beryllium-Free Deep-Ultraviolet Nonlinear Optical Material Designed Based on a Boron-Rich Strategy62Sr2Pb(BeB5O10)(BO3): An Excellent Ultraviolet Nonlinear-Optical Beryllium Borate by the Pb-Modified Construction of a Conjugated System and Lone-Pair Effect14Na4B8O9F10: A Deep‐Ultraviolet Transparent Nonlinear Optical Fluorooxoborate with Unexpected Short Phase‐Matching Wavelength Induced by Optimized Chromatic Dispersion133Na4B8O9F10: A Deep‐Ultraviolet Transparent Nonlinear Optical Fluorooxoborate with Unexpected Short Phase‐Matching Wavelength Induced by Optimized Chromatic Dispersion13A bidentate-anionic-group strategy for enhancing electron–phonon coupling and vibronic fluorescence in rare-earth crystals2Deep-ultraviolet nonlinear optical crystals: concept development and materials discovery181LiNaB6O9F2: A Promising UV NLO Crystal Having Fluorine‐Directed Optimal Performances and Double Interpenetrating 3[B6O9F2]∞ Networks33Recent Development of Sn II , Sb III ‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence129Recent Development of SnII, SbIII‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence6Target-Oriented Synthesis of Borate Derivatives Featuring Isolated [B3O3] Six-Membered Rings as Structural Features20(Ga 1− x Al x ) 4 B 2 O 9 : controlled surface acid–base properties and catalytic behavior towards the Strecker reaction1Toward the ultraviolet (UV) or deep-UV nonlinear optical crystals: The combination of π-conjugated planar [XY3] and tetrahedral [XY4]80Research on Nonlinear Optical Materials Based on BO 3 and BO 4 Hydroxy Tetraborates4

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  1. ChemInform Abstract: A Deep‐Ultraviolet Nonlinear Optical Crystal: Strontium Beryllium Borate Fluoride with Planar Be(O/F)3 Groups.

    ChemInform · 2016-09-01

    Na Yu, Shichao Wang, Ning Ye, Fei Liang, Zheshuai Lin, Min Luo, Kenneth Reinhard Poeppelmeier

    Read original paper ↗ ·

  2. SrNO3(OH)·H2O: A new member in strontium nitrate hydrate family with an ultraviolet cut-off edge

    Journal of Alloys and Compounds · 2016-11-03

    Lili Liu, Yun Mo Yang, Linping Li, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  3. BaBe2BO3F3: A KBBF-Type Deep-Ultraviolet Nonlinear Optical Material with Reinforced [Be2BO3F2]∞ Layers and Short Phase-Matching Wavelength

    Chemistry of Materials · 2016-12-05

    Shu Hai Guo, Xingxing Jiang, Lijuan Liu, Mingjun Xia, Zhi Gang Fang, Xiaoyang Wang, Zheshuai Lin, Chuangtian Chen

    Read original paper ↗ ·

  4. Syntheses, crystal structures and characterization of three alkaline metal borates

    CrystEngComm · 2017-01-01

    Sambasivam Sangaraju, Lili Liu, Yun Mo Yang, Guopeng Han, Beenish Bashir, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  5. Facile Syntheses of Ba2[B4O7(OH)2] and Na[B5O7(OH)2](H2O) Borate Salts Exhibiting Nonlinear Optical Activity in the Ultraviolet

    Inorganic Chemistry · 2017-01-11

    Chao Wu, Longhua Li, Jun‐Ling Song, Gang Yang, Mark Graeme Humphrey, Chi Zhang

    Read original paper ↗ ·

  6. Comparative Interrelationship of the Structural, Nonlinear-Optical and Other Acentric Properties for Oxide, Borate and Carbonate Crystals

    Crystals · 2017-04-12

    Boris I. Kidyarov

    Read original paper ↗ ·

  7. Structure Determination and Luminescent Property Studies of the Single Crystal Na3Sm(BO3)2

    Crystals · 2017-05-05

    Dan Zhao, Fa‐Xue Ma, Cong-Kui Nie, Jian Wang, Lei Zhang, Yun-Chang Fan

    Read original paper ↗ ·

  8. Deep-Ultraviolet Nonlinear-Optical Material K3Sr3Li2Al4B6O20F: Addressing the Structural Instability Problem in KBe2BO3F2

    Inorganic Chemistry · 2017-07-25

    Hongping Wu, Hongwei Yu, Shilie Pan, P. Shiv Halasyamani

    Read original paper ↗ ·

  9. A new mixed alkali metal borate: LiCs[B5O8(OH)]·H2O

    Inorganic Chemistry Communications · 2017-09-14

    Chong‐An Chen, Qi Wei, Guo‐Yu Yang

    Read original paper ↗ ·

  10. MBaYB 6 O 12 (M = Rb, Cs): two new rare-earth borates with large birefringence and short ultraviolet cutoff edges

    Dalton Transactions · 2017-11-30

    Xinglong Chen, Fangfang Zhang, Yunjing Shi, Yanzhou Sun, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  11. Nature of the Color of Borates with “Anti-Zeolite” Structure

    Inorganic Chemistry · 2018-02-19

    Tatyana B. Bekker, V. P. Solntsev, Sergey V. Rashchenko, Alexander Yèlisseyev, А. В. Давыдов, Alexander A. Kragzhda, Alexander E. Kokh, Artem B. Kuznetsov, So-Hyun Park

    Read original paper ↗ ·

  12. SrB 5 O 7 F 3 Functionalized with [B 5 O 9 F 3 ] 6− Chromophores: Accelerating the Rational Design of Deep‐Ultraviolet Nonlinear Optical Materials

    Angewandte Chemie International Edition · 2018-03-02

    Miriding Mutailipu, Min Zhang, Bingbing Zhang, Liying Wang, Zhihua Yang, Xin Hua Zhou, Shilie Pan

    Read original paper ↗ ·

  13. SrB5O7F3 Functionalized with [B5O9F3]6− Chromophores: Accelerating the Rational Design of Deep‐Ultraviolet Nonlinear Optical Materials

    Angewandte Chemie · 2018-03-02

    Miriding Mutailipu, Min Zhang, Bingbing Zhang, Liying Wang, Zhihua Yang, Xin Hua Zhou, Shilie Pan

    Read original paper ↗ ·

  14. Recent advances in ultraviolet and deep-ultraviolet second-order nonlinear optical crystals

    Coordination Chemistry Reviews · 2018-03-15

    Chao Wu, Gang Yang, Mark Graeme Humphrey, Chi Zhang

    Read original paper ↗ ·

  15. Deep‐Ultraviolet Nonlinear Optical Crystal Cs2Al2(B3O6)2O: A Benign Member of the Sr2Be2(BO3)2O Family with [Al2(B3O6)2O]2− Double Layers

    Chemistry - A European Journal · 2018-04-15

    Zhi Gang Fang, Xingxing Jiang, Meihong Duan, Zhanyu Hou, Changcheng Tang, Mingjun Xia, Lijuan Liu, Zheshuai Lin, Feidi Fan, Lei Bai, Chuangtian Chen

    Read original paper ↗ ·

  16. From Sr2Nb2O7to CaxSr2–xNb2O7: An Effective Enhancement of Nonlinear Optical Activity by a Simple Way of Cation Substituting

    Crystal Growth & Design · 2018-05-25

    Lizhen Zhang, Hui Jun Wu, Yanping Lin, Feifei Yuan, Yisheng Huang, Shijia Sun, Bing Teng, Lingyun Li, Zhoubin Lin

    Read original paper ↗ ·

  17. Bi2ZnOB2O6: a polar material capable of photocatalytic degradation of Rhodamine B

    Journal of Materials Science Materials in Electronics · 2018-06-25

    Jian Liu, Wenwu Zhao, Bo Wang, Hui Yan

    Read original paper ↗ ·

  18. Second-order nonlinear optical crystals with mixed anions

    Coordination Chemistry Reviews · 2018-08-06

    Yu Pan, Sheng‐Ping Guo, Bin‐Wen Liu, Huaiguo Xue, Guo‐Cong Guo

    Read original paper ↗ ·

  19. Mg 3 B 7 O 13 Cl: A New Quasi‐Phase Matching Crystal in the Deep‐Ultraviolet Region

    Advanced Functional Materials · 2018-08-24

    Zujian Wang, Huimin Qiao, Rongbing Su, Bing Hu, Xiaoming Yang, Chao He, Xifa Long

    Read original paper ↗ ·

  20. Na4Yb(CO3)3F: A New UV Nonlinear Optical Material with a Large Second Harmonic Generation Response

    Crystals · 2018-09-30

    Qiaoling Chen, Min Luo, Chensheng Lin

    Read original paper ↗ ·

  21. Investigation on the growth, optical, mechanical and dielectric properties of an inorganic potassium pentaborate dihydrate (KB5H4O10.2H2O) single crystal

    Materials Chemistry and Physics · 2018-10-25

    Ramki Chakaravarthy, R. Ezhil Vizhi

    Read original paper ↗ ·

  22. Experimental characterization and first principles calculations of linear and nonlinear optical properties of two orthophosphates A 3 Al 2 (PO 4 ) 3 (A = Rb, K)

    Inorganic Chemistry Frontiers · 2018-12-20

    Ming Wen, Hongping Wu, Shichao Cheng, Jun Sun, Zhihua Yang, Xiaohong Wu, Shilie Pan

    Read original paper ↗ ·

  23. Li 4 Na 2 CsB 7 O 14 : a new edge-sharing [BO 4 ] 5− tetrahedra containing borate with high anisotropic thermal expansion

    Chemical Communications · 2018-12-26

    Miriding Mutailipu, Min Zhang, Hao Li, Xiao Fan, Zhihua Yang, Shifeng Jin, Gang Wang, Shilie Pan

    Read original paper ↗ ·

  24. A 2 Bi 2 (SO 4 ) 2 Cl 4 (A = NH 4 , K, Rb): achieving a subtle balance of the large second harmonic generation effect and sufficient birefringence in sulfate nonlinear optical materials

    Journal of Materials Chemistry C · 2019-01-01

    Kaichuang Chen, Yi Jin Yang, Guang Peng, Shunda Yang, Tao Yan, Huixin Fan, Zheshuai Lin, Ning Ye

    Read original paper ↗ ·

  25. Sn 2 B 7 O 12 F with a 2∞[B 14 O 24 ] 6− layer constructed from the unprecedented [B 7 O 16 ] 11− fundamental building block

    Inorganic Chemistry Frontiers · 2019-01-01

    Zixiu Lu, Fangfang Zhang, Abudukadi Tudi, Zhizhong Zhang, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  26. BeO6 Trigonal Prism with Ultralong Be–O Bonds Observed in a Deep Ultraviolet Optical Crystal Li13BeBe6B9O27

    Inorganic Chemistry · 2019-01-22

    Yi-Gang Chen, Meiling Xing, Yao Guo, Zheshuai Lin, Xiujun Fan, Xian‐Ming Zhang

    Read original paper ↗ ·

  27. Synthesis and enhanced photocatalytic activity of {1 0 1¯ 0} faceted hexagonal YBO3

    Chemical Physics Letters · 2019-04-27

    Jian Liu, Wenwu Zhao, Bo Wang, Hui Yu Yan

    Read original paper ↗ ·

  28. Ca 2 B 5 O 9 Cl and Sr 2 B 5 O 9 Cl: Nonlinear Optical Crystals with Deep-Ultraviolet Transparency Windows

    ACS Applied Materials & Interfaces · 2020-01-07

    Zujian Wang, Jiangang He, Bing Hu, Pai Shan, Zheyao Xiong, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

    Read original paper ↗ ·

  29. Synthesis, Crystal Structure, and Characterization of a Noncentrosymmetric Sulfate Cs2Ca2(SO4)3

    European Journal of Inorganic Chemistry · 2020-02-24

    Yaoguo Shen, Xiaoling Xue, Wenyuan Tu, Zhiqun Liu, Renwen Yan, Hong Zhang, Junrong Jia

    Read original paper ↗ ·

  30. Compressibility of hingganite-(Y): high-pressure single crystal X-ray diffraction study

    Physics and Chemistry of Minerals · 2020-04-10

    Liudmila A. Gorelova, Anna Pakhomova, Sergey V. Krivovichev, Anatoly V. Kasatkin, Leonid Dubrovinsky

    Read original paper ↗ ·

  31. A 3 BBi(P 2 O 7 ) 2 (A = Rb, Cs; B = Pb, Ba): Isovalent Cation Substitution to Sustain Large Second-Harmonic Generation Responses

    Chemistry of Materials · 2020-09-28

    Lu Qi, Zhaohui Chen, Xuerui Shi, Xiaodong Zhang, Qun Jing, Na Li, Zhongqi Jiang, Bingbing Zhang, Ming‐Hsien Lee

    Read original paper ↗ ·

  32. Sn3B8O15: A Ternary Tin(II) Borate with Flexible [B8O18]12– Fundamental Building Block Formed by [B7O16]11– and [BO3]3– Groups

    Inorganic Chemistry · 2020-12-29

    Siru Guo, Wen-Bin Zhang, Min Zhang, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  33. Computationally assisted multistage design and prediction driving the discovery of deep-ultraviolet nonlinear optical materials

    Materials Chemistry Frontiers · 2021-01-01

    Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  34. Recent advances of oxyfluorides for nonlinear optical applications

    Inorganic Chemistry Frontiers · 2021-01-01

    Shuo Bai, Dan Wang, Hongkun Liu, Ying Wang

    Read original paper ↗ ·

  35. Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application

    Angewandte Chemie International Edition · 2021-04-19

    Ming Xia, Fuming Li, Miriding Mutailipu, Shujuan Han, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  36. Discovery of First Magnesium Fluorooxoborate with Stable Fluorine Terminated Framework for Deep‐UV Nonlinear Optical Application

    Angewandte Chemie · 2021-04-19

    Ming Xia, Fuming Li, Miriding Mutailipu, Shujuan Han, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  37. LiB2O3F: A Beryllium-Free Deep-Ultraviolet Nonlinear Optical Material Designed Based on a Boron-Rich Strategy

    Chemistry of Materials · 2021-06-14

    Chun‐Li Hu, Jin Chen, Zhi Gang Fang, Ru‐Ling Tang, Jiang‐Gao Mao

    Read original paper ↗ ·

  38. Sr2Pb(BeB5O10)(BO3): An Excellent Ultraviolet Nonlinear-Optical Beryllium Borate by the Pb-Modified Construction of a Conjugated System and Lone-Pair Effect

    Inorganic Chemistry · 2021-06-18

    Zhe Dai, Yi-Gang Chen, Yao Guo, Fang Wang, Yuanyu Yang, Xian‐Ming Zhang

    Read original paper ↗ ·

  39. Na4B8O9F10: A Deep‐Ultraviolet Transparent Nonlinear Optical Fluorooxoborate with Unexpected Short Phase‐Matching Wavelength Induced by Optimized Chromatic Dispersion

    Angewandte Chemie International Edition · 2021-12-21

    Huanhuan Cheng, Fuming Li, Zhihua Yang, Shilie Pan

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  40. Na4B8O9F10: A Deep‐Ultraviolet Transparent Nonlinear Optical Fluorooxoborate with Unexpected Short Phase‐Matching Wavelength Induced by Optimized Chromatic Dispersion

    Angewandte Chemie · 2021-12-21

    Huanhuan Cheng, Fuming Li, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  41. A bidentate-anionic-group strategy for enhancing electron–phonon coupling and vibronic fluorescence in rare-earth crystals

    Journal of Materials Chemistry C · 2022-01-01

    Jingcheng Feng, Fangyan Wang, Wang Liu, Fei Liang, Guochun Zhang, Haohai Yu, Huaijin Zhang

    Read original paper ↗ ·

  42. Deep-ultraviolet nonlinear optical crystals: concept development and materials discovery

    Light Science & Applications · 2022-07-01

    Lei Kang, Zheshuai Lin

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  43. LiNaB6O9F2: A Promising UV NLO Crystal Having Fluorine‐Directed Optimal Performances and Double Interpenetrating 3[B6O9F2]∞ Networks

    Advanced Optical Materials · 2022-12-03

    Xiaojing Li, Zilong Chen, Fuming Li, Fangfang Zhang, Zhihua Yang, Shilie Pan

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  44. Recent Development of Sn II , Sb III ‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence

    Angewandte Chemie International Edition · 2023-03-13

    Shujuan Han, Abudukadi Tudi, Wenbin Zhang, Xueling Hou, Zhihua Yang, Shilie Pan

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  45. Recent Development of SnII, SbIII‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence

    Angewandte Chemie · 2023-03-13

    Shujuan Han, Abudukadi Tudi, Wenbin Zhang, Xueling Hou, Zhihua Yang, Shilie Pan

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  46. Target-Oriented Synthesis of Borate Derivatives Featuring Isolated [B3O3] Six-Membered Rings as Structural Features

    Inorganic Chemistry · 2023-05-31

    Meng Cheng, Congcong Jin, Wenqi Jin, Xueling Hou

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  47. (Ga 1− x Al x ) 4 B 2 O 9 : controlled surface acid–base properties and catalytic behavior towards the Strecker reaction

    Dalton Transactions · 2024-01-01

    Weilu Wang, Zhong Fan, Shiji Tang, Yun Wu, Ke Xu, Binbin Luo, Steven L. Suib

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  48. Toward the ultraviolet (UV) or deep-UV nonlinear optical crystals: The combination of π-conjugated planar [XY3] and tetrahedral [XY4]

    Coordination Chemistry Reviews · 2024-02-02

    W. Zhang, Xueling Hou, Shujuan Han, Shilie Pan

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  49. Research on Nonlinear Optical Materials Based on BO 3 and BO 4 Hydroxy Tetraborates

    Advanced Optical Materials · 2025-09-15

    Shuai An, Bailin Chen, Fangfang Zhang, Xueling Hou, Shilie Pan

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