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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2020

Ca 2 B 5 O 9 Cl and Sr 2 B 5 O 9 Cl: Nonlinear Optical Crystals with Deep-Ultraviolet Transparency Windows

Zujian Wang, Jiangang He, Bing Hu, Pai Shan, Zheyao Xiong, Rongbing Su, Chao He, Xiaoming Yang, Xifa Long

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Ca 2 B 5 O 9 Cl and Sr 2 B 5 O 9 Cl: Nonlinear Optical Crystals with Deep-Ultraviolet Transparency WindowsOriginalSynthesis and characterization of three new rare-earth orthoborates: Ba 2 MgY 2 (BO 3 ) 4 , Ba 2 CdY 2 (BO 3 ) 4 , and Ba 2 CdSc(BO 3 ) 310Enhanced nonlinear optical functionality in birefringence and refractive index dispersion of the deep-ultraviolet fluorooxoborates123A review on phase transition and structure-performance relationship of second-order nonlinear optical polymorphs107Nanostructured Borate Halides for Optical Second Harmonic Generation at Surfaces7LiGaF2(IO3)2: A mixed-metal gallium iodate-fluoride with large birefringence and wide band gap39Ba(MoO2F)2(XO3)2 (X = Se and Te): First Cases of Noncentrosymmetric Fluorinated Molybdenum Oxide Selenite/Tellurite Through Unary Substitution for Enlarging Band Gaps and Second Harmonic Generation34Borates: A Rich Source for Optical Materials1089From centrosymmetric to noncentrosymmetric: effect of the cation on the crystal structures and birefringence values of (NH 4 ) n−2 AE(PO 2 F 2 ) n (AE = Mg, Sr and Ba; n = 2, 3 and 4)9First principles study on low valence states photoluminescence in Bi-doped M2B5O9Cl crystals8Enhanced piezoelectric and dielectric properties of Pb(Yb1/2Nb1/2)O3–Pb(Mg1/3Nb2/3)O3–PbTiO3 crystals by combining alternating and direct current poling21Linear and Nonlinear Optical Properties of Centrosymmetric Sb 4 O 5 SO 4 and Noncentrosymmetric Sb 4 O 4 (SO 4 )(OH) 2 Induced by Lone Pair Stereoactivity55Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units102Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units9An Overview on Recent Trends in Deep‐Ultraviolet (DUV) and Ultraviolet (UV) Nonlinear Optical Crystals25From CeF2(SO4)·H2O to Ce(IO3)2(SO4): Defluorinated Homovalent Substitution for Strong Second-Harmonic-Generation Effect and Sufficient Birefringence53Omnidirectional / Unidirectional Antireflection-Switchable Structures Inspired by Dragonfly Wings23Hybrid organic–inorganic triguanidine arsenate dihydrate for ultraviolet nonlinear optical application15Preparation of M2B5O9Cl:Eu2+ (M=Sr, Ca) blue phosphors by a facile low-temperature self-reduction method and their enhanced luminescent properties25Noncentrosymmetric Rare-Earth Borate Fluoride La2B5O9F3: A New Ultraviolet Nonlinear Optical Crystal with Enhanced Linear and Nonlinear Performance48Luminescent inorganic mixed borate phosphors materials for lighting55Growth and characterization of pure and metal ions-doped l-Taurine: a third-order nonlinear optical crystal for photonic applications1From Phosphate Fluoride to Fluorophosphate: Design of Novel Ultraviolet/Deep-Ultraviolet Nonlinear Optical Materials for BePO3F with Optical Property Enhancement34Dual-Ligand-Oriented Design of Noncentrosymmetric Complexes with Nonlinear-Optical Activity11NaK5Zn2(B5O10)2 and β-K3ZnB5O10: Two Zincoborates with Deep-UV Cutoff Edge9CaBO2F: A novel deep-UV structural template with high nonlinear optical performance induced by electron delocalization25Enhancement on the luminescence of Ca2B5O9Cl:Eu2+ by co-doping of Al3+ and Ba2+ ions for full spectrum lighting application2Enhancement of birefringence and refractive index dispersion optimization from iodates to fluorooxoiodates1Rational Design of the First Ammonium Magnesium Borate with Deep-Ultraviolet Cutoff Edge and Moderate Birefringence and Further Investigation into the Nature of Ammonium in the Borate System15Recent Development of Sn II , Sb III ‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence130Recent Development of SnII, SbIII‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence6Pb(OH)I: A lead(II)-based oxyhalide with a large birefringence5The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals21Rational design of chloride ion transport channels in an open borate framework0Syntheses, structures and properties of two new members of the pentaborate family: NaKB 5 O 8 (OH)·H 2 O and KB 5 O 8 ·2H 2 O3Cadmium Hydroxyl Chloride with Balanced Band Gap and Second-Harmonic-Generation Response2La(SO3NH2)2NO3·H2O: synergistic anion engineering of the first rare-earth nitrate sulfamate defying transparency-birefringence-nonlinearity trade-offs in ultraviolet nonlinear optics8Hydrogen bond formation-modulated H2O2 generation under periodic local polarization piezoelectric electric field4Promising UV/DUV nonlinear optical materials with X-membered (X = multiples of 6) rings in anhydrous inorganic borates20Two scandium borate UV NLO crystals designed through chemical element substitution1The Achievement of a Strong Second Harmonic Generation Response and a Large Birefringence in Sulfates4Accelerating the discovery of athermal deep-ultraviolet nonlinear optical crystals via physics-informed herarchical graph learning1The Enhancement of Phase‐Matching Capability by Recombining π‐Conjugated Group in Nonlinear Optical Sulfates1Mechanoluminescent Mixed‐Anion Borate Sr 2 B 5 O 9 Cl:Eu for Dynamic Anticounterfeiting0Local polarization-piezoelectric field promotes water dissociation for efficient fluorinated pollutants defluorination0The First Silver Lead Borate, AgPb[B5O9]0Dissolution of Liquid B2O3 in Molten CaCl2−CaO0

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  1. Synthesis and characterization of three new rare-earth orthoborates: Ba 2 MgY 2 (BO 3 ) 4 , Ba 2 CdY 2 (BO 3 ) 4 , and Ba 2 CdSc(BO 3 ) 3

    Dalton Transactions · 2020-01-01

    Runqing Liu, Hongping Wu, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  2. Enhanced nonlinear optical functionality in birefringence and refractive index dispersion of the deep-ultraviolet fluorooxoborates

    Science China Materials · 2020-03-20

    Zhihua Yang, Abudukadi Tudi, Bing‐Hua Lei, Shilie Pan

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  3. A review on phase transition and structure-performance relationship of second-order nonlinear optical polymorphs

    Coordination Chemistry Reviews · 2020-05-25

    Kui Wu, Ya Feng Yang, Lihua Gao

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  4. Nanostructured Borate Halides for Optical Second Harmonic Generation at Surfaces

    European Journal of Inorganic Chemistry · 2020-06-09

    Deming Tan, Benjamin Kirbus, Lukas M. Eng, Michael Ruck

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  5. LiGaF2(IO3)2: A mixed-metal gallium iodate-fluoride with large birefringence and wide band gap

    Science China Materials · 2020-07-22

    Jin Chen, Chun‐Li Hu, Jiang‐Gao Mao

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  6. Ba(MoO2F)2(XO3)2 (X = Se and Te): First Cases of Noncentrosymmetric Fluorinated Molybdenum Oxide Selenite/Tellurite Through Unary Substitution for Enlarging Band Gaps and Second Harmonic Generation

    ACS Applied Materials & Interfaces · 2020-10-22

    Lin Lin, Xingxing Jiang, Chao Wu, Longhua Li, Zheshuai Lin, Zhipeng Huang, Mark Graeme Humphrey, Chi Zhang

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  7. Borates: A Rich Source for Optical Materials

    Chemical Reviews · 2020-12-14

    Miriding Mutailipu, Kenneth Reinhard Poeppelmeier, Shilie Pan

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  8. From centrosymmetric to noncentrosymmetric: effect of the cation on the crystal structures and birefringence values of (NH 4 ) n−2 AE(PO 2 F 2 ) n (AE = Mg, Sr and Ba; n = 2, 3 and 4)

    Dalton Transactions · 2021-01-01

    Wenyao Zhang, Wenqi Jin, Meng Cheng, Ruonan Zhang, Zhihua Yang, Shilie Pan

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  9. First principles study on low valence states photoluminescence in Bi-doped M2B5O9Cl crystals

    Journal of Alloys and Compounds · 2021-01-11

    Qiaoling Chen, Bibo Lou, Weiguo Jing, Min Yu Yin, Yau Yuen Yeung, Liangbi Su, Chang‐Kui Duan

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  10. Enhanced piezoelectric and dielectric properties of Pb(Yb1/2Nb1/2)O3–Pb(Mg1/3Nb2/3)O3–PbTiO3 crystals by combining alternating and direct current poling

    Journal of Applied Physics · 2021-03-22

    Canhuang Hong, Zujian Wang, Bin Su, Lin Guo, Xiaoming Yang, Xifa Long, Chao He

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  11. Linear and Nonlinear Optical Properties of Centrosymmetric Sb 4 O 5 SO 4 and Noncentrosymmetric Sb 4 O 4 (SO 4 )(OH) 2 Induced by Lone Pair Stereoactivity

    Inorganic Chemistry · 2021-07-21

    Qi Wei, Kui Wang, Chao He, Li Wei, Xiaofei Li, Shuo Zhang, Xing‐Tao An, Jinhua Li, Guo‐Ming Wang

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  12. Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units

    Angewandte Chemie International Edition · 2021-10-09

    Zi‐Jian Li, Wenqi Jin, Fangfang Zhang, Zilong Chen, Zhihua Yang, Shilie Pan

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  13. Achieving Short‐Wavelength Phase‐Matching Second Harmonic Generation in Boron‐Rich Borosulfate with Planar [BO3] Units

    Angewandte Chemie · 2021-10-09

    Zi‐Jian Li, Wenqi Jin, Fangfang Zhang, Zilong Chen, Zhihua Yang, Shilie Pan

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  14. An Overview on Recent Trends in Deep‐Ultraviolet (DUV) and Ultraviolet (UV) Nonlinear Optical Crystals

    ChemistrySelect · 2021-10-18

    Sekar Anand, M. Usha Rani, S. Kalainathan

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  15. From CeF2(SO4)·H2O to Ce(IO3)2(SO4): Defluorinated Homovalent Substitution for Strong Second-Harmonic-Generation Effect and Sufficient Birefringence

    Chemistry of Materials · 2021-11-22

    Tianhui Wu, Xingxing Jiang, Yiran Zhang, Zujian Wang, Hongyuan Sha, Chao Wu, Zheshuai Lin, Zhipeng Huang, Xifa Long, Mark Graeme Humphrey, Chi Zhang

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  16. Omnidirectional / Unidirectional Antireflection-Switchable Structures Inspired by Dragonfly Wings

    Journal of Colloid and Interface Science · 2021-12-08

    Ruyu Chen, Chung-Jui Lai, You-Jie Chen, Meixuan Wu, Hongta Yang

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  17. Hybrid organic–inorganic triguanidine arsenate dihydrate for ultraviolet nonlinear optical application

    Dalton Transactions · 2021-12-15

    Dongmei Wang, Zhuangzhuang Wei, Zhiyong Bai, Lehui Liu, Zhoubin Lin, Lizhen Zhang

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  18. Preparation of M2B5O9Cl:Eu2+ (M=Sr, Ca) blue phosphors by a facile low-temperature self-reduction method and their enhanced luminescent properties

    Journal of Rare Earths · 2022-02-17

    Pan Liang, Lianqing Li, Tong Shen, Lian Wenli, Zhi‐Hong Liu

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  19. Noncentrosymmetric Rare-Earth Borate Fluoride La2B5O9F3: A New Ultraviolet Nonlinear Optical Crystal with Enhanced Linear and Nonlinear Performance

    ACS Applied Materials & Interfaces · 2022-04-13

    Xuping Shi, Abudukadi Tudi, Meng Cheng, Fangfang Zhang, Zhihua Yang, Shujuan Han, Shilie Pan

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  20. Luminescent inorganic mixed borate phosphors materials for lighting

    Luminescence · 2022-06-07

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  21. Growth and characterization of pure and metal ions-doped l-Taurine: a third-order nonlinear optical crystal for photonic applications

    Journal of Materials Science Materials in Electronics · 2022-06-11

    Sindhu Tilak, G. Vinitha, H.M. Suresh Kumar

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  22. From Phosphate Fluoride to Fluorophosphate: Design of Novel Ultraviolet/Deep-Ultraviolet Nonlinear Optical Materials for BePO3F with Optical Property Enhancement

    ACS Applied Materials & Interfaces · 2022-08-18

    Mengfan Wu, Junwei Feng, Congwei Xie, Abudukadi Tudi, Dongdong Chu, Juanjuan Lu, Shilie Pan, Zhihua Yang

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  23. Dual-Ligand-Oriented Design of Noncentrosymmetric Complexes with Nonlinear-Optical Activity

    Inorganic Chemistry · 2022-09-30

    Jinhua Li, Xiao‐Fan Jiang, Qi Wei, Zhen‐Zhen Xue, Guo‐Ming Wang, Guo‐Yu Yang

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  24. NaK5Zn2(B5O10)2 and β-K3ZnB5O10: Two Zincoborates with Deep-UV Cutoff Edge

    Inorganic Chemistry · 2022-10-10

    Wenjuan Ma, Jie Zhang, Feng Yu, Bin Dai

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  25. CaBO2F: A novel deep-UV structural template with high nonlinear optical performance induced by electron delocalization

    Science China Materials · 2022-11-09

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  26. Enhancement on the luminescence of Ca2B5O9Cl:Eu2+ by co-doping of Al3+ and Ba2+ ions for full spectrum lighting application

    Optical Materials · 2022-11-28

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  27. Enhancement of birefringence and refractive index dispersion optimization from iodates to fluorooxoiodates

    New Journal of Chemistry · 2023-01-01

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  28. Rational Design of the First Ammonium Magnesium Borate with Deep-Ultraviolet Cutoff Edge and Moderate Birefringence and Further Investigation into the Nature of Ammonium in the Borate System

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  29. Recent Development of Sn II , Sb III ‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence

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  30. Recent Development of SnII, SbIII‐based Birefringent Material: Crystal Chemistry and Investigation of Birefringence

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  31. Pb(OH)I: A lead(II)-based oxyhalide with a large birefringence

    Inorganic Chemistry Communications · 2023-06-25

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  32. The Strategy to Improve the Phase Matching Ability in Tetrahedron‐Based Deep‐Ultraviolet Nonlinear Optical Crystals

    Advanced Optical Materials · 2023-07-09

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  33. Rational design of chloride ion transport channels in an open borate framework

    Journal of Materials Chemistry A · 2024-01-01

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  34. Syntheses, structures and properties of two new members of the pentaborate family: NaKB 5 O 8 (OH)·H 2 O and KB 5 O 8 ·2H 2 O

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  35. Cadmium Hydroxyl Chloride with Balanced Band Gap and Second-Harmonic-Generation Response

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  36. La(SO3NH2)2NO3·H2O: synergistic anion engineering of the first rare-earth nitrate sulfamate defying transparency-birefringence-nonlinearity trade-offs in ultraviolet nonlinear optics

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  37. Hydrogen bond formation-modulated H2O2 generation under periodic local polarization piezoelectric electric field

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  38. Promising UV/DUV nonlinear optical materials with X-membered (X = multiples of 6) rings in anhydrous inorganic borates

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  39. Two scandium borate UV NLO crystals designed through chemical element substitution

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  40. The Achievement of a Strong Second Harmonic Generation Response and a Large Birefringence in Sulfates

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  41. Accelerating the discovery of athermal deep-ultraviolet nonlinear optical crystals via physics-informed herarchical graph learning

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  42. The Enhancement of Phase‐Matching Capability by Recombining π‐Conjugated Group in Nonlinear Optical Sulfates

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  43. Mechanoluminescent Mixed‐Anion Borate Sr 2 B 5 O 9 Cl:Eu for Dynamic Anticounterfeiting

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  44. Local polarization-piezoelectric field promotes water dissociation for efficient fluorinated pollutants defluorination

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  45. The First Silver Lead Borate, AgPb[B5O9]

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  46. Dissolution of Liquid B2O3 in Molten CaCl2−CaO

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