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RESEARCH PAPER · Journal of Materials Chemistry · 2011

A congruently melting and deep UV nonlinear optical material: Li3Cs2B5O10

Yun Mo Yang, Shilie Pan, Xueling Hou, Chuanyi Wang, Kenneth Reinhard Poeppelmeier, Zhaohui Chen, Hongping Wu, Zhongxiang Zhou

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A congruently melting and deep UV nonlinear optical material: Li3Cs2B5O10OriginalGrowth, thermal and optical properties of a novel nonlinear optical material K 3 B 6 O 10 Cl57A new congruent-melting oxyborate, Pb 4 O(BO 3 ) 2 with optimally aligned BO 3 triangles adopting layered-type arrangement113A new noncentrosymmetric vanadoborate: synthesis, crystal structure and characterization of K2SrVB5O1222A novel deep UV nonlinear optical crystal Ba3B6O11F2, with a new fundamental building block, B6O14 group180K6Li3Sc2B15O30: A new nonlinear optical crystal with a short absorption edge50Li5Rb2B7O14: a new congruently melting compound with two kinds of B–O one-dimensional chains and short UV absorption edge25UV Nonlinear Optical Crystal Ba2[B6O9(OH)4] Featuring Unique Chiral Layers with a New B18O42 Circle Based on BO3 and BO4 Units97Structure, growth and properties of a novel polar material, KSr4B3O921New Borate‐citrate: Synthesis, Structure, and Properties of Sr[B(C6H5O7)2](H2O)4·3H2O3Synthesis, crystal structure and optical properties of a new orthorhombic phase, Na3ZnB5O1014Synthesis, crystal structure and properties of a new congruently melting compound, K3ZnB5O1016K3YB6O12: A new nonlinear optical crystal with a short UV cutoff edge60Synthesis, growth, crystal structure and optical properties of BaBiBO49Synthesis, Crystal Structure, and Properties of a New Lead Barium Borate, Pb1.13Ba7.87B18O3610Na3Cd3B(PO4)4: A New Noncentrosymmetric Borophosphate with Zero-Dimensional Anion Units81M2Cd3B16O28 (M = Rb, Cs): Two Isostructural Alkali Cadmium Borates with a New Type of Borate Layer29A novel UV nonlinear optical crystal material: K21Yb8B45O9024Growth, crystal structure and optical properties of a new layered fluorine beryllium borate, Sr0.23Ca0.77Na2Be2B2O6F25Synthesis, crystal structure and optical properties of a new beryllium borate, CsBe4(BO3)313New Salt-Inclusion Borate, Li3Ca9(BO3)7·2[LiF]: A Promising UV NLO Material with the Coplanar and High Density BO3 Triangles56Ba2Cd(B3O6)2: A Congruent‐Melting Compound with Isolated B3O6 Units8Semiorganic nonlinear optical material: Crystal growth, structure and optical properties of NaB(L-C4H4O5)27Cs2GeB4O9: a New Second-Order Nonlinear-Optical Crystal139Exploration of a new compound in the M–B–O–X (M: alkali metals; X: halogen) system: Preparation, crystal and electronic structures, and optical properties of Na3B6O10Br20Synthesis and Structure of KPbBP 2 O 8 – A Congruent Melting Borophosphate with Nonlinear Optical Properties35Syntheses, crystal structures, and optical properties of Pb6B3O10X (X=F, Cl, Br)16Noncentrosymmetric mixed-cation borate: Crystal growth, structure and optical properties of Cs2Ca[B4O5(OH)4]2·8H2O14Preparation, Structure, and Second‐order Nonlinear Optical Properties of a Borate‐Carboxylic Acid Compound: NH4B[ d‐ (+)‐C4H4O5]2·H2O3Three New Mixed-Alkali- and Alkaline-Earth-Metal Borates: From 1D Chain to 2D Layer to 3D Framework57Synthesis, structures, optical properties and electronic structures of two mixed metal borates MBaB5O9 (M=Na, K)32Noncentrosymmetric Cubic CsCdBO3 with Bichromophore23Pb 4 Zn 2 B 10 O 21 : a congruently melting lead zinc borate with a novel [B 10 O 24 ] anionic group and an interesting [Pb 4 O 12 ] ∞ chain29Ba3M2[B3O6(OH)]2[B4O7(OH)2] (M=Al, Ga): Two Novel UV Nonlinear Optical Metal Borates Containing Two Types of Oxoboron Clusters123Pb3B6O11F2: the first non-centrosymmetric lead borate fluoride with a large second harmonic generation response61Crystal growth and calculation of the electronic band structure and density of states of Li3Cs2B5O1013New type of complex alkali and alkaline earth metal borates with isolated (B12O24)12− anionic group35Ba4(BO3)3(SiO4)·Ba3X (X = Cl, Br): new salt-inclusion borosilicate halides as potential deep UV nonlinear optical materials58p–(p,π*) interaction mechanism revealing and accordingly designed new member in deep-ultraviolet NLO borates Li n M n−1 B 2n−1 O 4n−2 (M = Cs/Rb, n = 3, 4, 6)52Bulk growth and nonlinear optical properties of thulium calcium oxyborate single crystals29Synthesis, crystal structure, and optical properties of a new lead barium borate, PbBa 2 (B 3 O 6 ) 217The interaction between cations and anionic groups inducing SHG enhancement in a series of apatite-like crystals: A first-principles study23Effect of Halogen (Cl, Br) on the Symmetry of Flexible Perovskite-Related Framework37Zn 4 B 3 O 9 C 2 H 8 N 2 : an organic–inorganic hybrid borate with a novel graphene-like layer8Synthese, Struktur und Frequenzverdopplungseffekt von Calciumcyanurat19Synthesis, Structure, and Frequency‐Doubling Effect of Calcium Cyanurate137Synthesis, crystal structure, and properties of an interesting elliptical vanadoborate housing crystal: [Ni(en)2]6[(VO)12O6B18O39(OH)3]·5H2O12Na3Ba2(B3O6)2F: Next Generation of Deep-Ultraviolet Birefringent Materials190Second-harmonic generation (SHG) and photoluminescence properties of noncentrosymmetric (NCS) layered perovskite solid solutions, CsBi 1−x Eu x Nb 2 O 7 (x = 0, 0.1, and 0.2)30Growth, linear–non-linear optical, fluorescence, thermal and electrical studies of glycine-doped bis-thiourea cadmium formate crystal for electro-optic device applications35Synthesis and Characterization of Mid-Infrared Transparency Compounds: Acentric BaHgS2 and Centric Ba8Hg4S5Se752Two New Crystals in LimCsnBm+nO2(m+n) (m + n = 5, 7; m > n) Series: Noncentrosymmetric Li5Cs2B7O14 and Centrosymmetric Li4CsB5O1016RbMgCO3F: A New Beryllium-Free Deep-Ultraviolet Nonlinear Optical Material342Li 3 AlSiO 5 : the first aluminosilicate as a potential deep-ultraviolet nonlinear optical crystal with the quaternary diamond-like structure55Alkali metal–alkaline earth metal borate crystal LiBa 3 (OH)(B 9 O 16 )[B(OH) 4 ] as a new deep-UV nonlinear optical material34Nonlinear optical (NLO) properties and temperature-dependent photoluminescence in activator-doped noncentrosymmetric (NCS) bismuth tellurite solid solutions, Bi2−Ln TeO5 (Ln = Ce and Eu)8Synthesis, crystal structure and optical properties of a new nocentrosymmetric borate: Ba7(BO3)3F55Top-Seeded Solution Crystal Growth, Morphology, Optical and Thermal Properties of Ba3(ZnB5O10)PO442Crystal Growth and Associated Properties of a Nonlinear Optical Crystal—Ba2Zn(BO3)226Deep Ultraviolet Nonlinear Optical Materials647Synthesis, crystal structure and characterizations of a new red phosphor K 3 EuB 6 O 1229Synthesis and characterization of inorganic nonlinear optical material: Potassium sodium hydroxide borate hydrate (KSB) single crystal10Growth, dielectric and nonlinear optical properties of Li3Cs2B5O10 single crystals0Mixed-Metal Carbonate Fluorides as Deep-Ultraviolet Nonlinear Optical Materials258Synthesis, Crystal Structure, and Nonlinear Optical Properties of a New Alkali and Alkaline Earth Metal Carbonate RbNa5Ca5(CO3)810Solvent-controlled syntheses of mixed-alkali-metal borates exhibiting UV nonlinear optical properties23Syntheses, crystal structures and characterization of three alkaline metal borates7Beryllium‐Free β‐Rb2Al2B2O7 as a Possible Deep‐Ultraviolet Nonlinear Optical Material Replacement for KBe2BO3F2185Beryllium‐Free β‐Rb2Al2B2O7 as a Possible Deep‐Ultraviolet Nonlinear Optical Material Replacement for KBe2BO3F278Synthesis, second-harmonic generations (SHG), and photoluminescence (PL) properties of Ca 4 Bi 6-x Ln x O 13 (Ln=La and Eu) solid solutions3Three Mixed-Alkaline Borates: Na2M2B20O32 (M = Rb, Cs) with Two Interpenetrating Three-Dimensional B-O Networks and Li4Cs4B40O64 with Fundamental Building Block B40O7730Insight on the growth and property studies of inorganic hydrated borate (Na6 [B4O5 (OH)4]3. 8H2O) single crystal – An effective third order nonlinear optical (NLO) material for optical limiting application20Synthesis, Characterization and Property of a New UV Nonlinear Optical Crystal KNa5Ca5(CO3)84A Series of Rare-Earth Borates K 7 MRE 2 B 15 O 30 (M = Zn, Cd, Pb; RE = Sc, Y, Gd, Lu) with Large Second Harmonic Generation Responses103Recent advances in ultraviolet and deep-ultraviolet second-order nonlinear optical crystals256Deep-ultraviolet nonlinear optical materials: Development trend and innovative exploration16Structural, elastic, electronic, phonon, dielectric and optical properties of Bi3TeBO9 from first-principles calculations27Investigation on the growth, optical, mechanical and dielectric properties of an inorganic potassium pentaborate dihydrate (KB5H4O10.2H2O) single crystal12Two Lanthanide Borate Chlorides LnB4O6(OH)2Cl (Ln = La, Ce) with Wide Ultraviolet Transmission Windows and Large Second-Harmonic Generation Responses25Ba 3 Ca 4 (BO 3 ) 3 (SiO 4 )Cl: a new non-centrosymmetric complex alkaline-earth metal borosilicate chloride with a deep-ultraviolet cut-off edge19Li2CsB7O10(OH)4: A Deep-Ultraviolet Nonlinear-Optical Mixed-Alkaline Borate Constructed by Unusual Heptaborate Anions98Four new deep ultraviolet borates with isolated B12O24 groups: Synthesis, structure, and optical properties9NaCa5BO3(SiO4)2 with Interesting Isolated [BO3] and [SiO4] Units in Alkali- and Alkaline-Earth-Metal Borosilicates14Synthesis, characterization, and theoretical analysis of three new nonlinear optical materials K7MRE2B15O30 (M= Ca and Ba, RE= La and Bi)28Crystal structure and second harmonic generation in Bi2TeO5: An X-N study from synchrotron and neutron diffraction data8Rb7SrY2(B5O10)3: A Rare-Earth Pentaborate with Moderate Second-Harmonic Response and Interesting Phase-Matching Behavior29Synthesis, crystal structure and optical properties of a new fluoroborate compound: Al7-xLi1+xB4O16+xF1-x (x = 1/3)2K 2.64 Cs 0.36 SiF 7 : a new fluorosilicate with a trans -perovskite structure3Solubilities, densities and refractive indices of the reciprocal quaternary systems (Na+, K+//Cl−, B5O8− - H2O) and (Li+, K+//Cl−, B5O8− - H2O) at 298.15 K and atmospheric pressure9Borates: A Rich Source for Optical Materials1097An antimony( iii ) borate with large birefringence exhibiting unwonted [B 5 O 11 ] fundamental building blocks and dimeric [Sb 2 O 6 ] clusters26Computationally assisted multistage design and prediction driving the discovery of deep-ultraviolet nonlinear optical materials41Second-order nonlinear optical property of the ultraviolet transparent alkali metal-rare earth metal carbonate Na3Y(CO3)3.3H2O5Exploring linear-nonlinear optical, dielectric and microscopic traits of sulphamic acid crystal exploiting Zn2+ for photonic device applications14Preparation, structural, optical and thermal behavior of nonlinear Potassium DL-malato borate hydrate (C8H8BKO10H2O) single crystal5A non–centrosymmetric compound K7Li2Y2B15O30 by introducing more alkali metals into A7MRe2B15O30 family10Rare-Earth Scandium Borate Fluoride with a Deep-Ultraviolet Cutoff Edge12Cd8(BO3)4SiO4: Metal Cation Inducing the Formation of Isolated [BO3] and [SiO4] Units in Borate Silicate15Prediction of ultraviolet optical materials in the K 2 O–B 2 O 3 system1Structural Regulations of Layered Borates: From Centric Layers to Chiral Porous Layers3Modulating Electron Density of Boron–Oxygen Groups in Borate via Metal Electronegativity for Propane Oxidative Dehydrogenation5Noncentrosymmetric Crystal [C10H8NO2]2SiF6·H2O with Large Birefringence12Nucleation kinetics, FTIR, DFT and Hirshfeld surface analysis of sodium hydrogen oxalate hydrate (NaHC2O4∙H2O) single crystal4Promising UV/DUV nonlinear optical materials with X-membered (X = multiples of 6) rings in anhydrous inorganic borates20Synthesis and characterization of mixed carbonate and bicarbonate materials as candidates for deep-UV applications1

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  4. A novel deep UV nonlinear optical crystal Ba3B6O11F2, with a new fundamental building block, B6O14 group

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  6. Li5Rb2B7O14: a new congruently melting compound with two kinds of B–O one-dimensional chains and short UV absorption edge

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  7. UV Nonlinear Optical Crystal Ba2[B6O9(OH)4] Featuring Unique Chiral Layers with a New B18O42 Circle Based on BO3 and BO4 Units

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  8. Structure, growth and properties of a novel polar material, KSr4B3O9

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  9. New Borate‐citrate: Synthesis, Structure, and Properties of Sr[B(C6H5O7)2](H2O)4·3H2O

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  10. Synthesis, crystal structure and optical properties of a new orthorhombic phase, Na3ZnB5O10

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  11. Synthesis, crystal structure and properties of a new congruently melting compound, K3ZnB5O10

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  12. K3YB6O12: A new nonlinear optical crystal with a short UV cutoff edge

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  13. Synthesis, growth, crystal structure and optical properties of BaBiBO4

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  16. M2Cd3B16O28 (M = Rb, Cs): Two Isostructural Alkali Cadmium Borates with a New Type of Borate Layer

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  17. A novel UV nonlinear optical crystal material: K21Yb8B45O90

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  20. New Salt-Inclusion Borate, Li3Ca9(BO3)7·2[LiF]: A Promising UV NLO Material with the Coplanar and High Density BO3 Triangles

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  21. Ba2Cd(B3O6)2: A Congruent‐Melting Compound with Isolated B3O6 Units

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  30. Synthesis, structures, optical properties and electronic structures of two mixed metal borates MBaB5O9 (M=Na, K)

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  31. Noncentrosymmetric Cubic CsCdBO3 with Bichromophore

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  32. Pb 4 Zn 2 B 10 O 21 : a congruently melting lead zinc borate with a novel [B 10 O 24 ] anionic group and an interesting [Pb 4 O 12 ] ∞ chain

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  33. Ba3M2[B3O6(OH)]2[B4O7(OH)2] (M=Al, Ga): Two Novel UV Nonlinear Optical Metal Borates Containing Two Types of Oxoboron Clusters

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  34. Pb3B6O11F2: the first non-centrosymmetric lead borate fluoride with a large second harmonic generation response

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  35. Crystal growth and calculation of the electronic band structure and density of states of Li3Cs2B5O10

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  36. New type of complex alkali and alkaline earth metal borates with isolated (B12O24)12− anionic group

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  37. Ba4(BO3)3(SiO4)·Ba3X (X = Cl, Br): new salt-inclusion borosilicate halides as potential deep UV nonlinear optical materials

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  38. p–(p,π*) interaction mechanism revealing and accordingly designed new member in deep-ultraviolet NLO borates Li n M n−1 B 2n−1 O 4n−2 (M = Cs/Rb, n = 3, 4, 6)

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  39. Bulk growth and nonlinear optical properties of thulium calcium oxyborate single crystals

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  40. Synthesis, crystal structure, and optical properties of a new lead barium borate, PbBa 2 (B 3 O 6 ) 2

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  41. The interaction between cations and anionic groups inducing SHG enhancement in a series of apatite-like crystals: A first-principles study

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  42. Effect of Halogen (Cl, Br) on the Symmetry of Flexible Perovskite-Related Framework

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  43. Zn 4 B 3 O 9 C 2 H 8 N 2 : an organic–inorganic hybrid borate with a novel graphene-like layer

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  44. Synthese, Struktur und Frequenzverdopplungseffekt von Calciumcyanurat

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  45. Synthesis, Structure, and Frequency‐Doubling Effect of Calcium Cyanurate

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  46. Synthesis, crystal structure, and properties of an interesting elliptical vanadoborate housing crystal: [Ni(en)2]6[(VO)12O6B18O39(OH)3]·5H2O

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  47. Na3Ba2(B3O6)2F: Next Generation of Deep-Ultraviolet Birefringent Materials

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  48. Second-harmonic generation (SHG) and photoluminescence properties of noncentrosymmetric (NCS) layered perovskite solid solutions, CsBi 1−x Eu x Nb 2 O 7 (x = 0, 0.1, and 0.2)

    Journal of Materials Chemistry C · 2015-01-01

    Hyung Gu Kim, Jae Soo Yoo, Kang Min Ok

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