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RESEARCH PAPER · Advanced Materials · 2015

Morphotropic Phase Boundary in the Pb‐Free (1 − x)BiTi3/8Fe2/8Mg3/8O3–xCaTiO3 System: Tetragonal Polarization and Enhanced Electromechanical Properties

Pranab Mandal, Alicia Maria Manjón-Sanz, Alex J. Corkett, Tim P. Comyn, Karl Dawson, Timothy Stevenson, James Bennett, Leonard F. Henrichs, Andrew J. Bell, Masaki Takata, Masaki Takata, Marco Zanella, Michelle Dolgos, Umut Adem, Xinming Wan, Michael J. Pitcher, Simon Romani, T. Thao Tran, P. Shiv Halasyamani, John B. Claridge, Matthew J. Rosseinsky

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Morphotropic Phase Boundary in the Pb‐Free (1 − x)BiTi3/8Fe2/8Mg3/8O3–xCaTiO3 System: Tetragonal Polarization and Enhanced Electromechanical PropertiesOriginalDesigning switchable polarization and magnetization at room temperature in an oxide138Lead‐Free Metamaterials with Enormous Apparent Piezoelectric Response79High‐Performance Lead‐Free Piezoceramics with High Curie Temperatures577Controlling Phase Assemblage in a Complex Multi‐Cation System: Phase‐Pure Room Temperature Multiferroic (1−x)BiTi(1−y)/2FeyMg(1−y)/2O3–xCaTiO320Structure evolution and piezoelectric properties across the morphotropic phase boundary of Sm-substituted BiFeO3 ceramics58A multiferroic on the brink: Uncovering the nuances of strain-induced transitions in BiFeO3124Defect Engineering of Lead-Free Piezoelectrics with High Piezoelectric Properties and Temperature-Stability113Flexoelectric piezoelectric metamaterials based on the bending of ferroelectric ceramic wafers49Modified optical and magnetic properties at room-temperature across lead-free morphotropic phase boundary in (1-x)BiTi 3/8 Fe 2/8 Mg 3/8 O 3 –xCaTiO 38Ferroelectric and magnetic properties in (1− x )BiFeO 3 – x (0.5CaTiO 3 –0.5SmFeO 3 ) ceramics27Bismuth layered ceramic solid solution with high temperature piezoelectricity endurance and low sintering temperature14Large piezoelectric responses of Bi(Fe,Mg,Ti)O3-BaTiO3 lead-free piezoceramics near the morphotropic phase boundary28Multifield Control of Domains in a Room-Temperature Multiferroic 0.85BiTi0.1Fe0.8Mg0.1O3–0.15CaTiO3 Thin Film22The Polar/Antipolar Phase Boundary of BiMnO3–BiFeO3–PbTiO3: Interplay among Crystal Structure, Point Defects, and Multiferroism19High temperature stability and mechanical quality factor of donor-acceptor co-doped BaTiO3 piezoelectrics59Large-scale multiferroic complex oxide epitaxy with magnetically switched polarization enabled by solution processing31Giant Piezoelectric Properties of ZnO Film Doped with Acceptor-Donor Ionic Pair0Ferroelectric Polymers Exhibiting Negative Longitudinal Piezoelectric Coefficient: Progress and Prospects123Electric-field-controlled magnetism due to field-induced transition of Pna21/R3c in Bi1-xGdxFeO3 ceramics16Enhanced Electromechanical Response and Thermal Stability of 0.93(Na1/2Bi1/2)TiO3‐0.07BaTiO3 Through Aerosol Deposition of Base Metal Electrodes16Giant Piezoelectric Coefficient in Lead-Free BiFe0.975Ti0.025O3–CaTiO3 Solid Solution Thin Films5Large linear electrostrain of acceptor-donor Co-doped ZnO films8First-principles investigation on multiferroic properties of BiFeO3-REMnO3 (RE = Er, Eu, Gd, Ho, La, Tb)8Complex Structural Disorder in a Polar Orthorhombic Perovskite Observed through the Maximum Entropy Method/Rietveld Technique6Flexible room-temperature multiferroic thin film with multifield tunable coupling properties11Dielectric, ferroelectric and magnetic properties of Bi(Mg,M)O3-modified (M=Hf, Ta) BiFeO3–BaTiO3 ceramics6Emerging Halide Perovskite Ferroelectrics161Synthesis and Characterization of a New Ferroelectric with Low Lead Content, a High Curie Temperature, and a High Piezoelectric Response50.78BiTi0.1Fe0.8Mg0.1O3-0.22CaTiO3 Nanoscale-Thick Thin Films for Doping-Enhanced Electric Applications1Fundamentals, advances and perspectives of piezocatalysis: A marriage of solid-state physics and catalytic chemistry214Separation of K+ and Bi3+ displacements in a Pb-free, monoclinic piezoelectric at the morphotropic phase boundary3Polymorphic Nanodomain Enhancing Multiferroic Properties of Epitaxial (1-x)BiTi0.1Fe0.8Mg0.1O3-(x)CaTiO3 Thin Films0Understanding the effect of rare-earth doping in ABO3 ferroelectrics on capacitive energy storage13A Lamella Chirality-Induced Heterostructure Crystal in Biodegradable Poly(lactic Acid) Reminiscent of a Morphotropic Phase Boundary4Mixed-phase epitaxial doped bismuth ferrite thin film fabrication and its application in memristors0Atomic-scale mechanism unlocks thermal-stable high-κ performance in HfO2 via coherent interfaces3

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  1. Designing switchable polarization and magnetization at room temperature in an oxide

    Nature · 2015-09-01

    Pranab Mandal, Michael J. Pitcher, Jonathan Alaria, Hongjun Niu, Pavel Borisov, Plamen S. Stamenov, John B. Claridge, Matthew J. Rosseinsky

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  2. Lead‐Free Metamaterials with Enormous Apparent Piezoelectric Response

    Advanced Materials · 2015-09-24

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  3. High‐Performance Lead‐Free Piezoceramics with High Curie Temperatures

    Advanced Materials · 2015-10-07

    Myang Hwan Lee, Da Jeong Kim, Jin Su Park, Sang Wook Kim, Tae Kwon Song, Myong‐Ho Kim, Won‐Jeong Kim, D. Do, Il‐Kyoung Jeong

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  4. Controlling Phase Assemblage in a Complex Multi‐Cation System: Phase‐Pure Room Temperature Multiferroic (1−x)BiTi(1−y)/2FeyMg(1−y)/2O3–xCaTiO3

    Advanced Functional Materials · 2016-02-05

    Pranab Mandal, Michael J. Pitcher, Jonathan Alaria, Hongjun Niu, Marco Zanella, John B. Claridge, Matthew J. Rosseinsky

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  5. Structure evolution and piezoelectric properties across the morphotropic phase boundary of Sm-substituted BiFeO3 ceramics

    Journal of Applied Physics · 2016-02-12

    Xin Shi, Xiao Qiang Liu, Xiang Ming Chen

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  6. A multiferroic on the brink: Uncovering the nuances of strain-induced transitions in BiFeO3

    Applied Physics Reviews · 2016-03-01

    Daniel Sando, Bin Xu, L. Bellaïche, V. Nagarajan

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  7. Defect Engineering of Lead-Free Piezoelectrics with High Piezoelectric Properties and Temperature-Stability

    ACS Applied Materials & Interfaces · 2016-03-24

    Yu Feng, Weili Li, Dan Xu, Yulong Qiao, Yang Yu, Yu Zhao, Weidong Fei

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  8. Flexoelectric piezoelectric metamaterials based on the bending of ferroelectric ceramic wafers

    Applied Physics Letters · 2016-08-15

    Xiaotong Zhang, Jiliang Liu, Mingjin Chu, Baojin Chu

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  9. Modified optical and magnetic properties at room-temperature across lead-free morphotropic phase boundary in (1-x)BiTi 3/8 Fe 2/8 Mg 3/8 O 3 –xCaTiO 3

    Ceramics International · 2017-02-15

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  10. Ferroelectric and magnetic properties in (1− x )BiFeO 3 – x (0.5CaTiO 3 –0.5SmFeO 3 ) ceramics

    Journal of the American Ceramic Society · 2017-05-02

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  11. Bismuth layered ceramic solid solution with high temperature piezoelectricity endurance and low sintering temperature

    Sensors and Actuators A Physical · 2017-05-11

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  12. Large piezoelectric responses of Bi(Fe,Mg,Ti)O3-BaTiO3 lead-free piezoceramics near the morphotropic phase boundary

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    Li‐Feng Zhu, Bo‐Ping Zhang, Shun Li, Gaolei Zhao

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  13. Multifield Control of Domains in a Room-Temperature Multiferroic 0.85BiTi0.1Fe0.8Mg0.1O3–0.15CaTiO3 Thin Film

    ACS Applied Materials & Interfaces · 2018-06-01

    Tingting Jia, Ziran Fan, Junxiang Yao, Cong Liu, Yuhao Li, Junxi Yu, Bi Fu, Hongyang Zhao, Minoru Osada, Ehsan Nasr Esfahani, Yaodong Yang, Yuanxu Wang, Jiangyu Li, Hideo Kimura, Zhenxiang Cheng

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  14. The Polar/Antipolar Phase Boundary of BiMnO3–BiFeO3–PbTiO3: Interplay among Crystal Structure, Point Defects, and Multiferroism

    Advanced Functional Materials · 2018-07-01

    Carmen M. Fernández‐Posada, Alicia Castro, Jean‐Michel Kiat, Florence Porcher, Ovidio Peña-Rodríguez, Ricardo Jiménez, Miguel Algueró, Harvey Amorín

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  15. High temperature stability and mechanical quality factor of donor-acceptor co-doped BaTiO3 piezoelectrics

    Acta Materialia · 2019-09-25

    Ruixuan Song, Yu Zhao, Weili Li, Yang Yu, Jie Sheng, Ze Li, Yulei Zhang, Hetian Xia, Weidong Fei

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  16. Large-scale multiferroic complex oxide epitaxy with magnetically switched polarization enabled by solution processing

    National Science Review · 2019-10-08

    Cong Liu, Feng An, Paria Sadat Musavi Gharavi, Qinwen Lu, Junkun Zha, Chao Chen, Liming Wang, Xiaozhi Zhan, Zedong Xu, Yuan Zhang, Ke Qu, Junxiang Yao, Yun Ou, Zhiming Zhao, Xiangli Zhong, Dongwen Zhang, V. Nagarajan, Lang Chen, Tao Zhu, Deyang Chen, Xiaofang Zhai, Peng Dong Gao, Tingting Jia, Shuhong Xie, Gaokuo Zhong, Jiangyu Li

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  17. Giant Piezoelectric Properties of ZnO Film Doped with Acceptor-Donor Ionic Pair

    SSRN Electronic Journal · 2020-01-01

    Chang Gao, Zhao Yú, Weili Li, Yulong Qiao, Zhao Wang, Lü Jing, Jie Sheng, Weidong Fei

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  18. Ferroelectric Polymers Exhibiting Negative Longitudinal Piezoelectric Coefficient: Progress and Prospects

    Advanced Science · 2020-02-05

    Yang Liu, Qing Wang

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  19. Electric-field-controlled magnetism due to field-induced transition of Pna21/R3c in Bi1-xGdxFeO3 ceramics

    Journal of Materiomics · 2021-03-11

    Jing Chen, Nan Su, Xiao Li Zhu, Xiao Qiang Liu, Jinxing Zhang, Xiang Ming Chen

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  20. Enhanced Electromechanical Response and Thermal Stability of 0.93(Na1/2Bi1/2)TiO3‐0.07BaTiO3 Through Aerosol Deposition of Base Metal Electrodes

    Advanced Materials Interfaces · 2021-05-07

    Neamul Hayet Khansur, Udo R. Eckstein, Hana Uršič, Matej Šadl, Martin Brehl, Alexander T. Martin, Kevin Riess, Dominique de Ligny, Kyle Grant Webber

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  21. Giant Piezoelectric Coefficient in Lead-Free BiFe0.975Ti0.025O3–CaTiO3 Solid Solution Thin Films

    Crystal Growth & Design · 2021-09-27

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  22. Large linear electrostrain of acceptor-donor Co-doped ZnO films

    Journal of Material Science and Technology · 2021-10-31

    Chang Gao, Yu Zhao, Weili Li, Yulong Qiao, Zhao Wang, Lü Jing, Jie Sheng, Weidong Fei

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  23. First-principles investigation on multiferroic properties of BiFeO3-REMnO3 (RE = Er, Eu, Gd, Ho, La, Tb)

    Materials Today Communications · 2021-11-09

    Mohamed Ait Tamerd, Majid EL Kassaoui, Brahim Abraime, Adil Marjaoui, M. El Marssi, A. Benyoussef, Abdallah El Kenz, Abdelilah Lahmar

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  24. Complex Structural Disorder in a Polar Orthorhombic Perovskite Observed through the Maximum Entropy Method/Rietveld Technique

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  25. Flexible room-temperature multiferroic thin film with multifield tunable coupling properties

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  26. Dielectric, ferroelectric and magnetic properties of Bi(Mg,M)O3-modified (M=Hf, Ta) BiFeO3–BaTiO3 ceramics

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  27. Emerging Halide Perovskite Ferroelectrics

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  28. Synthesis and Characterization of a New Ferroelectric with Low Lead Content, a High Curie Temperature, and a High Piezoelectric Response

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  29. 0.78BiTi0.1Fe0.8Mg0.1O3-0.22CaTiO3 Nanoscale-Thick Thin Films for Doping-Enhanced Electric Applications

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  30. Fundamentals, advances and perspectives of piezocatalysis: A marriage of solid-state physics and catalytic chemistry

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  31. Separation of K+ and Bi3+ displacements in a Pb-free, monoclinic piezoelectric at the morphotropic phase boundary

    Acta Materialia · 2023-12-13

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  32. Polymorphic Nanodomain Enhancing Multiferroic Properties of Epitaxial (1-x)BiTi0.1Fe0.8Mg0.1O3-(x)CaTiO3 Thin Films

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  33. Understanding the effect of rare-earth doping in ABO3 ferroelectrics on capacitive energy storage

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  34. A Lamella Chirality-Induced Heterostructure Crystal in Biodegradable Poly(lactic Acid) Reminiscent of a Morphotropic Phase Boundary

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  35. Mixed-phase epitaxial doped bismuth ferrite thin film fabrication and its application in memristors

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  36. Atomic-scale mechanism unlocks thermal-stable high-κ performance in HfO2 via coherent interfaces

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