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RESEARCH PAPER · Advanced Science · 2020

Ferroelectric Polymers Exhibiting Negative Longitudinal Piezoelectric Coefficient: Progress and Prospects

Yang Liu, Qing Wang

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Ferroelectric Polymers Exhibiting Negative Longitudinal Piezoelectric Coefficient: Progress and ProspectsOriginalPiezofibers to smart textiles: a review on recent advances and future outlook for wearable technology205Polymer dielectrics exhibiting an anomalously improved dielectric constant simultaneously achieved high energy density and efficiency enabled by CdSe/Cd 1−x Zn x S quantum dots40Observation of a Negative Thermal Hysteresis in Relaxor Ferroelectric Polymers34Toward bioimplantable and biocompatible flexible energy harvesters using piezoelectric ceramic materials37Tailoring Artificial Mode to Enable Cofired Integration of Shear‐type Piezoelectric Devices19A large piezoelectric response in highly-aligned electrospun poly(vinylidene fluoride/trifluoroethylene) nanofiber webs for wearable energy harvesting11Self‐Healing of Electrical Damage in Polymers113Effect of Cationic Substitution of Metal Species in Poly(vinylidene difluoride) (C2H2F2) by Ab Initio Calculations3Exploring the anion chemical space of Ln 2 OF 2−x Cl x H 2 (Ln = Y, La, Gd): a model of electroelastic material with high mechanical sensitivity and energy harvesting2Origins of Electrostriction in Poly(vinylidene fluoride)-Based Ferroelectric Polymers64Ultrafast Electric Field-Induced Phase Transition in Bulk Bi0.5Na0.5TiO3 under High-Intensity Terahertz Irradiation9E-Textile Technology Review–From Materials to Application121Enhanced piezoelectricity from highly polarizable oriented amorphous fractions in biaxially oriented poly(vinylidene fluoride) with pure β crystals253Emerging Opportunities for 2D Semiconductor/Ferroelectric Transistor‐Structure Devices154Coupling of interface effects and porous microstructures in translucent piezoelectric composites for enhanced energy harvesting and sensing81Polarization‐ and Electrode‐Optimized Polyvinylidene Fluoride Films for Harsh Environmental Piezoelectric Nanogenerator Applications44Properties and Applications of Flexible Poly(Vinylidene Fluoride)-Based Piezoelectric Materials101Biomedical Implants with Charge‐Transfer Monitoring and Regulating Abilities49Polymer‐/Ceramic‐based Dielectric Composites for Energy Storage and Conversion201Enhancing Electrostrictive Actuation via Strong Electrostatic Repulsion among Field-Induced Nanodomains in a Relaxor Ferroelectric Poly(vinylidene fluoride-co-trifluoroethylene-co-chlorotrifluoroethylene) Random Terpolymer27Study on flexible large-area Poly(vinylidene fluoride)-based piezoelectric films prepared by extrusion-casting process for sensors and microactuators22Molecular Ferroelectric‐Based Flexible Sensors Exhibiting Supersensitivity and Multimodal Capability for Detection75Electrostriction-enhanced giant piezoelectricity via relaxor-like secondary crystals in extended-chain ferroelectric polymers68Effect of Dipole Mobility in Secondary Crystals on Piezoelectricity of a Poly(vinylidene fluoride-co-trifluoroethylene) 52/48 mol % Random Copolymer with an Extended-Chain Crystal Structure25Discovery of amantadine formate: Toward achieving ultrahigh pyroelectric performances in organics15Flexible cyanoethyl cellulose-based nanocomposites with superior energy storage capability18Introduction and Literature Review1Piezoelectric nanogenerators for personalized healthcare434Hybrid fibrous (PVDF-BaTiO 3 )/ PA-11 piezoelectric patch as an energy harvester for pacemakers37Ferroelectric Polymer Nanofibers Reminiscent of Morphotropic Phase Boundary Behavior for Improved Piezoelectric Energy Harvesting69Dielectric micro-capacitance for enhancing piezoelectricity via aligning MXene sheets in composites81Enhanced Piezoelectricity in Poly(vinylidene fluoride-co-trifluoroethylene-co-chlorotrifluoroethylene) Random Terpolymers with Mixed Ferroelectric Phases39Porous cellulose composite aerogel films with super piezoelectric properties for energy harvesting94Porosity manipulation to boost piezoelectric output via supercritical carbon dioxide foaming and surface modification16Sponge-like piezoelectric micro- and nanofiber structures for mechanical energy harvesting43Enhanced piezoelectricity in polyvinyl chloride film plasticized by diethyl adipate17In-situ electrostatic field regulating the recrystallization behavior of P(VDF-TrFE) films with high β-phase content and enhanced piezoelectric properties towards flexible wireless biosensing device applications53A pyrotoroidic transition in ferroelectric polymer10Enhancement and Function of the Piezoelectric Effect in Polymer Nanofibers42Novel chitosan-acetyl isatin polymer derivatives: synthesis, characterization, and applications in bone tissue engineering11Polyvinylidene Fluoride Copolymers with Grafted Polyethyl Methacrylate Chains: Synthesis and Thermal and Dielectric Properties3Defects in poly(vinylidene fluoride)-based ferroelectric polymers from a molecular perspective44Thermo‐responsive dielectric pulse in poly(vinylidene fluoride)/polyethylene glycol fibrous mats4On the origin of enhanced power output in ferroelectric polymer-based triboelectric nanogenerators: Role of dipole charge versus piezoelectric charge31Temperature-Dependent Rotational Dipole Mobility and Devitrification of the Rigid Amorphous Fraction in Unpoled and Poled Biaxially Oriented Poly(vinylidene fluoride)23Deciphering the peculiar hysteresis loops of 0.05Pb(Mn1/3Sb2/3)O3–0.95Pb(Zr0.52Ti0.48)O3 piezoelectric ceramics16Study on relaxor polymer interface matrix for piezoelectric nanocomposite generators23Atomistic investigation on the mechanical properties and phase transition process of poly (vinylidene flouride)0Origin of the negative longitudinal piezoelectric effect and electric auxetic effect in hexagonal A I B IV C V semiconductors5Flexible Lead-Free Piezoelectric Ba0.94Sr0.06Sn0.09Ti0.91O3/PDMS Composite for Self-Powered Human Motion Monitoring25Defected poly(vinylidene fluoride) with enhanced piezoelectricity via liquid crystal small molecules doping7A Review on PVDF Nanofibers in Textiles for Flexible Piezoelectric Sensors152Effect of Centrifugal Force on Power Output of a Spin-Coated Poly(Vinylidene Fluoride-Trifluoroethylene)-Based Piezoelectric Nanogenerator15Piezoelectric Polymers2Microstructure enhancement of macroscopic flexoelectric behavior of THV/Al composites7Suppressing charge injection and preventing the extension of electrical trees of polymer-based composites through two-dimensional metal–organic frameworks nanosheets17Effect of chemical defects on electrostriction-enhanced piezoelectric property of poly(vinylidene fluoride) via high-power ultrasonication25The past, present, and future of piezoelectric fluoropolymers: Towards efficient and robust wearable nanogenerators32Robotic e-skin for high performance stretchable acceleration sensor via combinations of novel soft and functional polymers23A (Ba0. 94Ca0 .06)(Ti0. 95Zr0 .05) O3 ceramic sheet doping to improve the inverse piezoelectric effect of the poly (vinylidene fluoride‐trifluoroethylene)‐based composite film3Electrostrictive and piezoelectrical properties of chitosan-poly(3-hydroxybutyrate) blend films20Tuning the Electromechanical Response of P(VDF-TrFE)/ZnSnO3-Based Binary Piezoelectric Composites for Biomechanical Energy-Harvesting and Self-Powered Mechanosensing18Ferroelectric Materials for High Energy Density Batteries: Progress and Outlook52A review: Polyacrylonitrile as high-performance piezoelectric materials88New Insight into Nanoscale Identification of the Polar Axis Direction in Organic Ferroelectric Films3Customizing Three-Dimensional Elastic Barium Titanate Sponge for Intelligent Piezoelectric Sensing15Ferroelectric materials for multiphysic energy harvesting0Review of Piezoelectric Properties and Power Output of PVDF and Copolymer-Based Piezoelectric Nanogenerators88Mechanisms of Direct and Converse Piezoelectricity in Ferroelectric Polymers9The past 10 years of molecular ferroelectrics: structures, design, and properties173Origin of different piezoelectric responses in elemental Sb and Bi monolayers17Flutter-Driven Piezoelectric Wind Energy Harvesting System Based on PVDF Nanofiber for Low Power Applications19Porous, Self-Polarized Ferroelectric Polymer Films Exhibiting Behavior Reminiscent of Morphotropic Phase Boundary Induced by Size-Dependent Interface Effect for Self-Powered Sensing34Utilizing Shear Piezoelectricity of Chiral Lead‐Free Metal Halides for Electromechanical Sensing25Investigation on relaxor-ferroelectric behavior of BNBT-KNN ceramics with Ta doping10Challenges and opportunities in piezoelectric polymers: Effect of oriented amorphous fraction in ferroelectric semicrystalline polymers29Multiscale understanding the interfacial layer in poly(vinylidene fluoride)-based ferroelectric polymers2Phase structure deciphering for pure polymers with a giant piezoelectric response26Scalable piezoelectric energy harvesting from PVDF-HFP/BZT-BCT/GO hybrid composite film12Flexible PVDF/BST nanocomposites for mechanical energy harvesting application17Ingenious Structure Engineering to Enhance Piezoelectricity in Poly(vinylidene fluoride) for Biomedical Applications30Screening Vertically Polarized 2D Layered Materials with Giant Negative Longitudinal Piezoelectricity by Comprehensive Calculations and Experimental Characterizations9Poling-Induced Wettability Transition of a Uniaxially Oriented Poly(vinylidene fluoride) Film14Relations structure-propriétés des copolymères piézoélectriques P(VDF-co-TrFE) et de leurs composites à base de céramiques électroactives0Rapid microwave annealing of ferroelectric copolymer films for multifunctional perception4Optimization of electro-strain and ferroelectric properties of P(VDF-TrFE) films under the synergistic effect of PTO nanosheets and in-situ electrostatic field5Giant piezoelectricity in fluoropolymer fiber mats achieved by corona poling in water10High β-Phase Barium Titanium Oxide Nanoparticle/P(VDF-TrFE) Composites for Mechanical Sensing12Significantly Enhanced Piezoelectricity of Poly(Vinylidene Fluoride) via Orienting Nanobound State Ions9Ultrahigh piezoelectric coefficient of poly(vinylidene fluoride) achieved via electric-poling-induced partial γ-β phase transition9Perception and Recognition of Proximity and Contact Processes via Parallel Double‐Transistor Configuration9High-Performance Mechano-Sensitive Piezoelectric Nanogenerator from Post-Treated Nylon-11,11 Textiles for Energy Harvesting and Human Motion Monitoring8Highly biodegradable piezoelectric flexible wearable tactile sensors with amino acid crystals: a paradigm shift towards smart transient electronics34Strain‐Induced Polar Interfaces in Ferroelectric Polymer Nanocomposites10Sign of the piezoelectric response in double-path ferroelectrics9Enhanced electrocaloric effect in relaxor ferroelectric polymers through hot press processing2Morphotropic Phase Boundary in Irradiated Ferroelectric Polymers13Stimuli-responsive smart materials enabled high-performance biosensors for liquid biopsies10Advances in copolymers based on polyvinylidene fluoride (PVDF) and their composites for piezoelectric energy harvesting8Current trends of characterization techniques for PVDF and related composite piezoelectric materials for nanogenerator9Field-Effect Crystal Engineering in Proton–π-Electron Correlated Systems1Enhanced Piezoelectricity in Stretched Relaxor Ferroelectric Polymers Near the Morphotropic Phase Boundary4Scalable solution-processed ferroelectric polymers exhibiting markedly enhanced piezoelectricity10Low-dimensional materials in piezoelectric and triboelectric nanogenerators0Multistackable, Domino‐Overlapped CNT Scaffolds Homogeneously Hybridized with BTO‐P(VDF‐TrFE) for High‐Performance Piezoelectric Nanogenerators2Piezoelectric polymer nanocomposite: Fabricating methods for materials and devices4Structural Manipulation of the Oriented Amorphous Fraction to Improve the Piezoelectricity of Poly(vinylidene fluoride- co -trifluoroethylene) by Thermal Annealing1Giant Reversible Piezoelectricity from Symmetry-Governed Stochastic Dipole Hopping3Poly(vinylidene Fluoride)‐Based Ferroelectric Polymers for Electromechanical Transduction: A Systematic Review of Materials and Actuators5Experimentally confirmed ferroelectricity in organic compounds identified by database mining1A Skin-Adhesive Bimodal Sensing Patch for Decoding Occlusal Dysfunction0Micro-CT assisted finite element analysis and functionalization of dental implants with piezoelectric coatings for improved bio-mechanical and anti-bacterial performance1Direct evidence for electrostriction‐enhanced piezoelectricity in poly(vinylidene fluoride‐ co ‐trifluoroethylene) random copolymers0Incorporating Molybdenum Disulfide Sheets in Polymer‐Ceramic Composites for Piezoelectric Energy Harvesting: COMSOL Prediction and Experimental Evaluation0Morphotropic Phase Boundary in Graft Poly(Vinylidene Fluoride‐ co ‐Tetrafluoroethylene) With High Curie Temperature0Self‐Powered Fast Response Flexible Ultraviolet Sensors Based on Reversible Deformed Nanowires for UV Communications Under Sunlight0Bioinspired asymmetric structural synergy for soft robotics: closed-loop piezoelectric harvesting and ionic actuation1Enhanced piezoelectricity and pyroelectricity in poly(vinylidene fluoride-co-tetrafluoroethylene) via hot pressing1Study of Dielectric and Piezoelectric Properties of Reduced Graphene Oxide‐Reinforced Poly (Vinylidene Fluoride‐Co‐Hexafluoropropylene) Based Three Phase Composite Films for Energy Storage and Harvesting Applications0From Flexible to Conformable Pressure Sensors: Mechanisms, Materials, and Biomedical Applications1Piezoelectric materials for surface modification of titanium-based implants: material design, biological mechanisms, and translational challenges0Construction and Evaluation of P(VDF-TrFE) Nanofiber-Clustered Surfaces0

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  48. Atomistic investigation on the mechanical properties and phase transition process of poly (vinylidene flouride)

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  49. Origin of the negative longitudinal piezoelectric effect and electric auxetic effect in hexagonal A I B IV C V semiconductors

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  50. Flexible Lead-Free Piezoelectric Ba0.94Sr0.06Sn0.09Ti0.91O3/PDMS Composite for Self-Powered Human Motion Monitoring

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