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RESEARCH PAPER · Nature · 2015

Designing switchable polarization and magnetization at room temperature in an oxide

Pranab Mandal, Michael J. Pitcher, Jonathan Alaria, Hongjun Niu, Pavel Borisov, Plamen S. Stamenov, John B. Claridge, Matthew J. Rosseinsky

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Designing switchable polarization and magnetization at room temperature in an oxideOriginalControlling Phase Assemblage in a Complex Multi‐Cation System: Phase‐Pure Room Temperature Multiferroic (1−x)BiTi(1−y)/2FeyMg(1−y)/2O3–xCaTiO320Novel quasi-symmetric solid oxide fuel cells with enhanced electrochemical performance73Recent developments related to multifunctional ferroelectric for room-temperature applications2Composition‐Dependent Microstructures and Properties of La‐, Zn‐, and Cr‐Modified 0.675BiFeO 3 –0.325BaTiO 3 Ceramics16The evolution of multiferroics1469Ferroic phase transitions and switching properties of modified BiFeO3–SrTiO3 multiferroic perovskites12Designing room-temperature multiferroic materials in a single-phase solid-solution film3Atomically engineered ferroic layers yield a room-temperature magnetoelectric multiferroic347Direct visualization of magnetic‐field‐induced magnetoelectric switching in multiferroic aurivillius phase thin films51Non‐Centrosymmetric Molecular Magnets2A Novel Class of Multiferroic Material, Bi4Ti3O12·nBiFeO3 with Localized Magnetic Ordering Evaluated from Their Single Crystals28Room Temperature Magnetically Ordered Polar Corundum GaFeO 3 Displaying Magnetoelectric Coupling46Stomata-like metal peptide coordination polymer10Modified optical and magnetic properties at room-temperature across lead-free morphotropic phase boundary in (1-x)BiTi 3/8 Fe 2/8 Mg 3/8 O 3 –xCaTiO 38Structure Evolution and Multiferroic Properties in Cobalt Doped Bi4NdTi3Fe1-xCoxO15-Bi3NdTi2Fe1-xCoxO12-δ Intergrowth Aurivillius Compounds29Chemistry-Inspired Adaptable Framework Structures368Ferroelectric and magnetic properties in (1− x )BiFeO 3 – x (0.5CaTiO 3 –0.5SmFeO 3 ) ceramics27A Generalizable Multigram Synthesis and Mechanistic Investigation of YMnO3 Nanoplates13Direct atomic scale determination of magnetic ion partition in a room temperature multiferroic material47Polar Magnets in Double Corundum Oxides60Room-Temperature Multiferroics and Thermal Conductivity of 0.85BiFe1–2xTixMgxO3–0.15CaTiO3 Epitaxial Thin Films (x = 0.1 and 0.2)4The structural and multiferroic properties of Bi(1−x)Ce x Fe(1−x)(Mg0.5Ti0.5) x O3 thin films1Crystal structure, impedance, and multiferroic property of SrZrO3 and MnO2 modified 0.725BiFeO3−0.275BaTiO3 ceramics21Enhanced magnetization in morphologically and magnetically distinct BiFeO3 and La0.7Sr0.3MnO3 composites19Room temperature multiferrocity and magnetodielectric properties of ternary (1-x) (0.94Bi0.5Na0.5TiO3-0.06BaTiO3)-xBiFeO3 (0 ≤x≤ 0.9) solid solutions15Effects of Co doping on structural, magnetic, and electrical properties of 0.6BiFeO3-0.4(Bi0.5K0.5)TiO3 solid solution8Multilayer Ceramic Magnetoelectric Composites with Tailored Interfaces for Enhanced Response24Low temperature synthesis route and structural characterization of (Bi 0.5 A 0.5 )(Sc 0.5 Nb 0.5 )O 3 ( A = K + and Na + ) perovskites5Superlattice-like structure and enhanced ferroelectric properties of intergrowth Aurivillius oxides15Discovery of a magnetic conductive interface in PbZr0.2Ti0.8O3 /SrTiO3 heterostructures25Recent advances in luminescent lanthanide based Single-Molecule Magnets301Correlation between Geometrically Induced Oxygen Octahedral Tilts and Multiferroic Behaviors in BiFeO3 Films26Room temperature multiferroic behavior and magnetoelectric coupling in (K,Na)NbO3-based ceramics10Multifield Control of Domains in a Room-Temperature Multiferroic 0.85BiTi0.1Fe0.8Mg0.1O3–0.15CaTiO3 Thin Film22Perspective: Magnetoelectric switching in thin film multiferroic heterostructures63The Polar/Antipolar Phase Boundary of BiMnO3–BiFeO3–PbTiO3: Interplay among Crystal Structure, Point Defects, and Multiferroism19Room Temperature Dielectric Pulse Effect in Organic Mixtures16Magnetoelectricity in La2NiMnO6 and its PVDF impregnated derivative18Ferromagnetic and dielectric properties of lead free KNbO3-CoFe2O4 composites23Room-temperature multiferroic properties of Ba2+ doped 0.7Bi0.5Na0.5TiO3-0.3NiFe2O4 ceramics3Environmentally-friendly magnetoelectric ceramic multilayer composites by water-based tape casting19Design for Highly Piezoelectric and Visible/Near‐Infrared Photoresponsive Perovskite Oxides137Atomic-scale mapping of interface reconstructions in multiferroic heterostructures25All-organic room temperature thermally switchable dielectric system8Ferroelectric Origin and Distortion Modes in Doped BiFeO 3 by Crystallography Approach0Formation of bismuth iron oxide based core–shell structures and their dielectric, ferroelectric and magnetic properties13Tetrahedral chain ordering and low dimensional magnetic lattice in a new brownmillerite Sr 2 ScFeO 52Effects of LNO buffer layers on electrical properties of BFO-PT thin films on stainless steel substrates13Study on the structural and magnetic properties of Fe/Co co-doped Bi4Ti3O12 ceramics28Chemically engineered multiferroic morphotropic phase boundary in BiFeO3-based single phase multiferroics12Electric/magnetic behaviors of Nd/Ti co-doped BiFeO3 ceramics with morphotropic phase boundary35Electric Field Induced Room Temperature Null to High Spin State Switching: A Computational Prediction4Luminescent Schiff-Base Lanthanide Single-Molecule Magnets: The Association Between Optical and Magnetic Properties73Magnetoelectric effect in free-standing multiferroic thin film3Intriguing electric field effect on magnetic spin couplings in dielectron clathrate hydrates5Physics‐Guided Data‐Mining Driven Design of Room‐Temperature Multiferroic Perovskite Oxides5Delicate Balance among Three Ferroic Polymorphic Phases in BiFeO3–BiMnO3–PbTiO31Real-time studies of ferroelectric domain switching: a review102From Synthesis to Applications: Copper Calcium Titanate (CCTO) and its Magnetic and Photocatalytic Properties66A d-Band Electron Correlated Thermoelectric Thermistor Established in Metastable Perovskite Family of Rare-Earth Nickelates36Magnetic-field-induced ferroelectric domain dynamics and in-plane polarization in odd and mixed layered Aurivillius structures4Large-scale multiferroic complex oxide epitaxy with magnetically switched polarization enabled by solution processing31Heterostructures: new opportunities for functional materials159Effect of W/Co co-substitution on structural, microstructural, magnetic and electrical properties of Bi4NdFeTi3O15 aurivillius compound13Multiferroic Properties and Magnetoelectric Coupling of Fe‐Doped (Ba0.7Ca0.3)TiO3‐Ba(Zr0.2Ti0.8)O3 Ceramics10Synthesis, Characterizations and applications of oxides materials based on CaCu3Ti4O120Novel Aurivillius Bi 4 Ti 3−2x Nb x Fe x O 12 phases with increasing magnetic-cation fraction until percolation: a novel approach for room temperature multiferroism18Ferroelectric Polymers Exhibiting Negative Longitudinal Piezoelectric Coefficient: Progress and Prospects123Selection and Optimization of a K0.5Na0.5NbO3-Based Material for Environmentally-Friendly Magnetoelectric Composites12Room temperature magnetoelectric coupling in a molecular ferroelectric ytterbium(III) complex210Phase transition and fluorescence regulation of BaAl2Si2O8:Eu using Ba source18A photoswitchable polar crystal that exhibits superionic conduction100Room temperature multiferroic properties and polymorphic phase transition-induced noticeable magnetodielectric anomalies in Fe/Co co-doped (K0.52Na0.48)NbO3 ceramics5Electrical Studies on Bi4NdTi3Fe0.7Co0.3O15-Bi3NdTi2Fe0.7Co0.3O12–δ Intergrowth Aurivillius Ceramics5Dielectric Relaxation Mechanism in High-Pressure Synthesized BiCr0.5Mn0.5O35Heterostructured materials: superior properties from hetero-zone interaction1143Enhancement of magnetic and dielectric properties of KNbO3–CoFe2O4 multiferroic composites via thermal treatment16Magnetoelectric Studies of Close-Packed and Hierarchically Ordered CoFe2O4/Pb(Zr0.52Ti0.48)O3/La0.6Sr0.4MnO3/LaNiO3 Multiferroic Thin Films2A Molecular Crystal Shows Multiple Correlated Magnetic and Ferroelectric Switchings22Tunable polarization with enhanced multiferroic response of W/Co co-doped Bi4LaFeTi3O15 Aurivillius ceramics21Enhanced Magnetoelectric Effects in Self-Assembled Hemispherical Close-Packed CoFe2O3-Pb(Zr0.52Ti0.48)O3 Thin Film4Effect of Ca dopant on magnetic and magnetodielectric properties of Y3Fe5O1229Persistence of Ferroelectricity Close to Unit-Cell Thickness in Structurally Disordered Aurivillius Phases21Metallic ferroelectric-ferromagnetic multiferroics in strained EuTiO3−xHx3Orthorhombic BiFeO3 : Theoretical studies on magnetoelectric effects of the multiferroic phase2Magnetoelectric Coupling and Decoupling in Multiferroic Hexagonal YbFeO3 Thin Films0Multiferroic Aurivillius Bi 4 Ti 2− x Mn x Fe 0.5 Nb 0.5 O 12 ( n = 3) compounds with tailored magnetic interactions7Reentrance of spin-driven ferroelectricity through rotational tunneling of ammonium1Role of magnetic ordering in the phase coexistence at the structural instability of the multiferroic BiFeO3–PbTiO32Dielectric and piezoelectric properties of lead-free Na0.5Bi0.5TiO3-SrTiO3-BiFeO3 ternary system5Giant linear magnetoelectric effect at the morphotropic phase boundary of epitaxial Sr0.5Ba0.5MnO3 films11Peculiar magnetism of Bi1−xDyxFeO3 ceramics at the morphotropic phase boundary8Effect of sintering temperature on structural, dielectric, and electrical property studies of Bi4NdTi3FeO15 aurivillius ceramics16Breaking Material Property Trade-offs via Macrodesign of Microstructure100Ferromagnetic, dielectric, and ferroelectric characteristic near the morphotropic phase boundary in (1-x)(0.7BiFeO3-0.3BiNa0.5Ti O3)-x(CaTiO3) solid solution2Room-temperature multiferrocity and magnetodielectric properties of ternary BiFeO3–Bi0.5Na0.5TiO3–CaTiO3 ceramics across the rhombohedral–orthorhombic phase boundary4Enhanced piezoelectric and ferroelectric properties of tetragonal BiFeO3–BaTiO3 ceramics via tailoring sintering temperature and dwell time8Giant Piezoelectric Coefficient in Lead-Free BiFe0.975Ti0.025O3–CaTiO3 Solid Solution Thin Films5Progress in the Development of Single-Phase Magnetoelectric Multiferroic Oxides3Atomic Visualization and Switching of Ferroelectric Order in β‐In2Se3 Films at the Single Layer Limit57Insights on the role of defects on the magnetic and magneto electric coupling effects in nano BiFeO39Ferro-electric and magnetic properties in Bi 5 Ti 3 FeO 15 films by Mn doping4Effect of Co-Substitution of Na0.5bi0.5tio3 and Catio3 on the Structure and Properties of Bifeo3 Ceramics3Charged Domain Wall and Polar Vortex Topologies in a Room-Temperature Magnetoelectric Multiferroic Thin Film30Flexible room-temperature multiferroic thin film with multifield tunable coupling properties11Strong magnetoelectric coupling at an atomic nonmagnetic electromagnetic probe in bismuth ferrite8Enhancement of polarization and magnetization in polycrystalline magnetoelectric composite2Phase evolution and enhanced piezoelectric, multiferroic, and magnetoelectric properties in Cr–Mn co-doped BiFeO3–BaTiO3 system5Coexisting magnetic orders and concomitant Morin-like transition and relaxor behavior in multiferroic Aurivillius Bi4Ti3 − 2xNbxFexO12 compounds4Electrical and magnetic studies on promising Aurivillius intergrowth compound6Time-dependent exchange creates the time-frustrated state of matter0Manganese substitution induced magnetic transformation and magnetoelectricity in SrFe 12 O 199High piezoelectric, dielectric relaxation and semiconductor properties in a one-dimensional organic–inorganic hybrid complex: [2-methyl-1,5-pentanediamine][BiCl 5 ]11Room Temperature Polar and Weak-Ferromagnetic Oxide with Low Dielectric Loss3Achieving High-Temperature Multiferroism by Atomic Architecture4Structural evolution and coexistence of ferroelectricity and antiferromagnetism in Fe, Nb co-doped BaTiO3 ceramics21Domain-wall magnetoelectric coupling in multiferroic hexagonal YbFeO3 films190.78BiTi0.1Fe0.8Mg0.1O3-0.22CaTiO3 Nanoscale-Thick Thin Films for Doping-Enhanced Electric Applications1Effect of ferrite phase addition on Pb-Free multiferroic composite material for energy storage applications6Lattice‐mediated room temperature magnetoelectric effect in (1‐ y )BiFe 1‐ x Cr x O 3 ‐ y BaTi 1‐ x Mn x O 3 solid solutions2Comparative assessment of structural, magnetic and impedance properties of xLaMnO3-(1-x)BiFeO3 solid solutions2Polymorphic Nanodomain Enhancing Multiferroic Properties of Epitaxial (1-x)BiTi0.1Fe0.8Mg0.1O3-(x)CaTiO3 Thin Films0Study on the magnetoelectric effect, ferroelectric and optical investigation of (1− x ) BCT + x NZLFO multiferroic composite6Synthesis and properties of rare-earth high-entropy perovskite10Magnetization response and magnetoelectric coupling of Mn-doped BiFeO3 thin films–microwave-assisted sol–gel approach1Large switchable polarization and piezoelectricity in multiferroic BiFeO3-Bi0.5K0.5TiO3-based single crystals1Synergetic enhancement of electric polarization and magnetization in Fe-doped Pb(Zr0.52Ti0.48)O3 modulated with “magnetoelectric composite” defect-dipoles1Electric properties of Sm doped bismuth ferrite-based thin film and its resistive switching behavior for memristor5Switchable valley-contrasting Berry curvature in two-dimensional valley-semi-half-metals2Evolution of Magnetic Symmetry through the BiFeO3–Ca2Fe4/3W2/3O6 Phase Diagram2Mixed-phase epitaxial doped bismuth ferrite thin film fabrication and its application in memristors0Spin-electronic applications of innovative dilute magnetic compositions: Ferromagnetism at room temperature of Ba0.98Gd0.02Ti0.98X0.02O3 (X = Ru, Mn, Fe)2Room Temperature Giant Magnetoelectric Coupling in {Co III 3 Dy III } Molecular Single Crystal Derived Nanogenerator5Pressure-induced spin reorientation and isostructural phase transition in S m 0.5 Y 0.5 Fe O 31Tunable ferroelectric and magnetic orders coexistence in Sr-doped BaTi0.92Co0.08O3 perovskite for lead-free multifunctional applications0Stress and oxygen vacancy synergy enables high-linearity resistivity modulation in nickelate heterostructures for voltage sensing2Chiral Ni2+/Yb3+ molecular complex with room-temperature magnetic-field driven 180° polarization reversal0Structure evolution, magnetic, electric and optical properties of Er doped BiFe0.97Ti0.03O3 nanoparticles with morphotropic phase boundary0

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  1. Controlling Phase Assemblage in a Complex Multi‐Cation System: Phase‐Pure Room Temperature Multiferroic (1−x)BiTi(1−y)/2FeyMg(1−y)/2O3–xCaTiO3

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  2. Novel quasi-symmetric solid oxide fuel cells with enhanced electrochemical performance

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  3. Recent developments related to multifunctional ferroelectric for room-temperature applications

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  4. Composition‐Dependent Microstructures and Properties of La‐, Zn‐, and Cr‐Modified 0.675BiFeO 3 –0.325BaTiO 3 Ceramics

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  5. The evolution of multiferroics

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  6. Ferroic phase transitions and switching properties of modified BiFeO3–SrTiO3 multiferroic perovskites

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  7. Designing room-temperature multiferroic materials in a single-phase solid-solution film

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  8. Atomically engineered ferroic layers yield a room-temperature magnetoelectric multiferroic

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  9. Direct visualization of magnetic‐field‐induced magnetoelectric switching in multiferroic aurivillius phase thin films

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  10. Non‐Centrosymmetric Molecular Magnets

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  11. A Novel Class of Multiferroic Material, Bi4Ti3O12·nBiFeO3 with Localized Magnetic Ordering Evaluated from Their Single Crystals

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  12. Room Temperature Magnetically Ordered Polar Corundum GaFeO 3 Displaying Magnetoelectric Coupling

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  13. Stomata-like metal peptide coordination polymer

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  14. Modified optical and magnetic properties at room-temperature across lead-free morphotropic phase boundary in (1-x)BiTi 3/8 Fe 2/8 Mg 3/8 O 3 –xCaTiO 3

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  15. Structure Evolution and Multiferroic Properties in Cobalt Doped Bi4NdTi3Fe1-xCoxO15-Bi3NdTi2Fe1-xCoxO12-δ Intergrowth Aurivillius Compounds

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  16. Chemistry-Inspired Adaptable Framework Structures

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  17. Ferroelectric and magnetic properties in (1− x )BiFeO 3 – x (0.5CaTiO 3 –0.5SmFeO 3 ) ceramics

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  18. A Generalizable Multigram Synthesis and Mechanistic Investigation of YMnO3 Nanoplates

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  19. Direct atomic scale determination of magnetic ion partition in a room temperature multiferroic material

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  21. Room-Temperature Multiferroics and Thermal Conductivity of 0.85BiFe1–2xTixMgxO3–0.15CaTiO3 Epitaxial Thin Films (x = 0.1 and 0.2)

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  22. The structural and multiferroic properties of Bi(1−x)Ce x Fe(1−x)(Mg0.5Ti0.5) x O3 thin films

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  23. Crystal structure, impedance, and multiferroic property of SrZrO3 and MnO2 modified 0.725BiFeO3−0.275BaTiO3 ceramics

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  24. Enhanced magnetization in morphologically and magnetically distinct BiFeO3 and La0.7Sr0.3MnO3 composites

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  25. Room temperature multiferrocity and magnetodielectric properties of ternary (1-x) (0.94Bi0.5Na0.5TiO3-0.06BaTiO3)-xBiFeO3 (0 ≤x≤ 0.9) solid solutions

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  26. Effects of Co doping on structural, magnetic, and electrical properties of 0.6BiFeO3-0.4(Bi0.5K0.5)TiO3 solid solution

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  27. Multilayer Ceramic Magnetoelectric Composites with Tailored Interfaces for Enhanced Response

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  28. Low temperature synthesis route and structural characterization of (Bi 0.5 A 0.5 )(Sc 0.5 Nb 0.5 )O 3 ( A = K + and Na + ) perovskites

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  29. Superlattice-like structure and enhanced ferroelectric properties of intergrowth Aurivillius oxides

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  30. Discovery of a magnetic conductive interface in PbZr0.2Ti0.8O3 /SrTiO3 heterostructures

    Nature Communications · 2018-02-09

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  31. Recent advances in luminescent lanthanide based Single-Molecule Magnets

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  32. Correlation between Geometrically Induced Oxygen Octahedral Tilts and Multiferroic Behaviors in BiFeO3 Films

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    Sung Su Lee, Young‐Min Kim, Hyun‐Jae Lee, Okkyun Seo, Hu Young Jeong, Qian He, Albina Y. Borisevich, Boyoun Kang, Owoong Kwon, Seunghun Kang, Yunseok Kim, T. Y. Koo, Jong‐Soo Rhyee, Do Young Noh, Beongki Cho, Ji Hui Seo, Jun Hee Lee, Ji Young Jo

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  33. Room temperature multiferroic behavior and magnetoelectric coupling in (K,Na)NbO3-based ceramics

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    Min Zhou, Xiaomei Lü, Xingyu Xu, Lin Liu, Lin Lei, Shuyu Xiao, Fengzhen Huang, Xiaomin Wang, Jinsong Zhu

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  34. Multifield Control of Domains in a Room-Temperature Multiferroic 0.85BiTi0.1Fe0.8Mg0.1O3–0.15CaTiO3 Thin Film

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    Tingting Jia, Ziran Fan, Junxiang Yao, Cong Liu, Yuhao Li, Junxi Yu, Bi Fu, Hongyang Zhao, Minoru Osada, Ehsan Nasr Esfahani, Yaodong Yang, Yuanxu Wang, Jiangyu Li, Hideo Kimura, Zhenxiang Cheng

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  35. Perspective: Magnetoelectric switching in thin film multiferroic heterostructures

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    Peter Benjamin Meisenheimer, Steve Novakov, Nguyen M. Vu, John T. Heron

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  36. The Polar/Antipolar Phase Boundary of BiMnO3–BiFeO3–PbTiO3: Interplay among Crystal Structure, Point Defects, and Multiferroism

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    Carmen M. Fernández‐Posada, Alicia Castro, Jean‐Michel Kiat, Florence Porcher, O. Peña, Ricardo Jiménez, Miguel Algueró, Harvey Amorín

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  37. Room Temperature Dielectric Pulse Effect in Organic Mixtures

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    Peng Fei Meng, Yulong Wu, Quan Zhang, Guoan Cheng, Xiaoling Wu, Ruiting Zheng

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  38. Magnetoelectricity in La2NiMnO6 and its PVDF impregnated derivative

    Journal of Applied Physics · 2018-07-24

    Sweta Tiwary, Sourav Kuila, M. R. Sahoo, Alok Barik, P. D. Babu, Prakash Nath Vishwakarma

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  39. Ferromagnetic and dielectric properties of lead free KNbO3-CoFe2O4 composites

    Solid State Sciences · 2018-09-26

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  43. Atomic-scale mapping of interface reconstructions in multiferroic heterostructures

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  46. Formation of bismuth iron oxide based core–shell structures and their dielectric, ferroelectric and magnetic properties

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  47. Tetrahedral chain ordering and low dimensional magnetic lattice in a new brownmillerite Sr 2 ScFeO 5

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  48. Effects of LNO buffer layers on electrical properties of BFO-PT thin films on stainless steel substrates

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