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RESEARCH PAPER · Advanced Materials · 2015

Lead‐Free Metamaterials with Enormous Apparent Piezoelectric Response

Wanfeng Zhou, Pan Chen, Qi Pan, Xiaotong Zhang, Baojin Chu

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Lead‐Free Metamaterials with Enormous Apparent Piezoelectric ResponseOriginalSymmetry breaking in hexagonal and cubic polymorphs of BaTiO334Strong Electromechanical Response in Lead Zirconate Titanate Metamaterials20Morphotropic NaNbO3-BaTiO3-CaZrO3 lead-free ceramics with temperature-insensitive piezoelectric properties55Flexoelectric piezoelectric metamaterials based on the bending of ferroelectric ceramic wafers49Sodium bismuth titanate-based lead-free RAINBOW piezoelectric devices15Pyro-paraelectric effect in ferroelectric materials: A device perspective for transcending Curie limitation8Steerable sound transport in a 3D acoustic network1Analysis of high temperature reduction process of Na0.5Bi0.5TiO3-based ceramics9Energy harvesting by exploiting the enhanced flexoelectric-like response of reduced (Na 0.5 Bi 0.5 ) 0.92 Ba 0.08 TiO 3 ceramics29Gradient doped polymer nanowire for moistelectric nanogenerator136Growth, microstructure, energy–storage and dielectric performances of chemical–solution NBT–based thin films: Effect of sodium nonstoichimometry17Flexoelectricity in dielectrics: Materials, structures and characterizations65Poling-free energy harvesters based on robust self-poled ferroelectric fibers47Large Flexoelectriclike Response from the Spontaneously Polarized Surfaces in Ferroelectric Ceramics75An electro-mechanical behavior enhancement method: geometric design with flexoelectricity15Magnetoelectric response from the enhanced ferromagnetism and flexoelectric response in reduced BiFeO3–based ceramics34Controllable anisotropic characteristics in solid solution ferroelectrics12Converse flexoelectricity with relative permittivity gradient33The surface mechanism for the flexoelectric response in sodium bismuth titanate‐based ferroelectric ceramics20Large Thermal–Electrical Response and Rectifying Conduction Behavior in Asymmetrically Reduced Ferroelectric Ceramics25High performance piezotronic devices based on non-uniform strain27Apparent piezoelectric response from the bending of non-poled PVDF12Flexoelectric materials and their related applications: A focused review212A flexoelectric spherical microshell model incorporating the strain gradient effect10Flexoelectricity in solids: Progress, challenges, and perspectives419Flexoelectricity in ferroelectric materials27Investigations on the electrical properties, domain structure, and local piezoelectric response in 0.3Pb(In1/2Nb1/2)–0.4Pb(Mg1/3Nb2/3)–0.3PbTiO3 single crystal4Piezoelectricity and flexoelectricity of sodium bismuth titanate-based ceramics19Bipolar and unipolar fatigue property in Bi0.5Na0.5TiO3–Bi0.5K0·5TiO3–SrTiO3 lead-free piezoelectric ceramics6Designing electromechanical metamaterial with full nonzero piezoelectric coefficients94Large Piezoelectricity in Ternary Lead‐Free Single Crystals121Recent advances in self-actuation and self-sensing materials: State of the art and future perspectives35Flexoelectric response of (1-x)BaTiO3-xSrTiO3 ceramics19Increased effective piezoelectric response of structurally modulated P(VDF-TrFE) film devices for effective energy harvesters29Composition gradient (1-x)Ba(Zr0.2Ti0.8)O3-x(Ba0.7Ca0.3)TiO3 film with improved dielectric, piezoelectric and ferroelectric temperature stability8Improving strain in single crystal by composition-gradients design26A 3D-printed molecular ferroelectric metamaterial43Mathematical and computational modeling of flexoelectricity at mesoscopic and atomistic scales5Flexoelectric Thin-Film Photodetectors89Effect of reduction produced defects on the dielectric relaxation and electrical conduction of Na0.5Bi0.5TiO3-based ceramics5Flexoelectric response of ferroelectric ceramics with reduced surface layer effect15Metamaterial mechanical antenna for very low frequency wireless communication111Comprehensive Review on Flexoelectric Energy Harvesting Technology: Mechanisms, Device Configurations, and Potential Applications74Multichannel Piezo‐Ultrasound Implant with Hybrid Waterborne Acoustic Metastructure for Selective Wireless Energy Transfer at Megahertz Frequencies52Gas sensing properties of asymmetrically reduced Na1/2Bi1/2TiO3–based ceramics0A gravity-driven sintering method to fabricate geometrically complex compact piezoceramics38Self-cleaning performance of in-situ ultrasound generated by quartz-based piezoelectric membrane25Piezoelectricity in nominally centrosymmetric phases43A co-effective strategy to improve the energy storage performance and the electrocaloric effect of ceramic: Using strain-modified calcined powders as sintering precursor5Flexoelectricity in periodically poled lithium niobate by PFM12Flexoelectric or Flexoelectric-Like Effect in Ceramics0Additive manufacturing: pushing the boundaries of piezoelectric materials10Effect of composition gradient on domain structure and piezoelectric properties in Mn-doped KNN single crystals4Effects of residual stress caused by abrasion on the flexoelectric response of BaTiO3 ceramics1Flexoelectric Effect1Speech Communication System Based on Piezoelectric Electret Mechanical Antenna9Powering internet-of-things from ambient energy: a review58Flexoelectric Effect of Ferroelectric Materials and Its Applications34Microstructure enhancement of macroscopic flexoelectric behavior of THV/Al composites7Kirigami–Origami‐Inspired Lead‐Free Piezoelectric Ceramics32Ultra-large electromechanical deformation in lead-free piezoceramics at reduced thickness53Advancements and Prospects of Flexoelectricity54Enhancement of electromechanical response in curved antiferroelectric AgNbO3 ceramics by flexoelectric effect2Compositional heterogeneity enhancing the flexoelectric response of BaTiO3 -based ceramics5Advancements of Flexoelectric Materials and Their Implementations in Flexoelectric Devices78Tailorable piezoelectric and flexoelectric output of a polymer-particle composite3Improving the piezoelectric response of Ba0.85Ca0.15Zr0.10Ti0.90O3 ferroelectric ceramics via the asymmetric-shape-induced flexoelectric effect4Flexoelectric metamaterials design based on anti-trichiral structure8Nonlinear analytical buckling analysis of composite cylindrical shells under magneto‐electro‐mechanical coupling: The role of flexoelectric and flexomagnetic effects0Semiconductive flexoelectric piezoelectric metamaterials with strong electromechanical response6Metastructure strategies for d33 enhancement beyond intrinsic limits in 3D-printed BaTiO3 metamaterials1Ultrahigh electric field-induced strain in lead-free ceramics via novel texture engineering technique0Synergistic effect of Nb2O5/Y2O3 doping and gradient structure on the dielectric and flexoelectric properties of BST ceramics1Large flexoelectric-like response of SrTiO3 ceramics sintered in the reducing atmosphere0High flexoelectric-like response in spark plasma sintering BaTiO3 ceramics0Pyroelectric Energy Conversion Based on PVDF‐Based Ferroelectric Polymers: Device Design and Applications0Flexoelectricity in Photoconversion: Fundamentals, Materials, and Outlooks2Ultrahigh electric field-induced strain in lead-free ceramics via texture engineering technique0Inverse thickness dependence of electrical performances in Na0.5Bi0.5TiO3-based ceramics0

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  1. Symmetry breaking in hexagonal and cubic polymorphs of BaTiO3

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  2. Strong Electromechanical Response in Lead Zirconate Titanate Metamaterials

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  3. Morphotropic NaNbO3-BaTiO3-CaZrO3 lead-free ceramics with temperature-insensitive piezoelectric properties

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  4. Flexoelectric piezoelectric metamaterials based on the bending of ferroelectric ceramic wafers

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  5. Sodium bismuth titanate-based lead-free RAINBOW piezoelectric devices

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  6. Pyro-paraelectric effect in ferroelectric materials: A device perspective for transcending Curie limitation

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  7. Steerable sound transport in a 3D acoustic network

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  8. Analysis of high temperature reduction process of Na0.5Bi0.5TiO3-based ceramics

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  9. Energy harvesting by exploiting the enhanced flexoelectric-like response of reduced (Na 0.5 Bi 0.5 ) 0.92 Ba 0.08 TiO 3 ceramics

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  10. Gradient doped polymer nanowire for moistelectric nanogenerator

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  11. Growth, microstructure, energy–storage and dielectric performances of chemical–solution NBT–based thin films: Effect of sodium nonstoichimometry

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  12. Flexoelectricity in dielectrics: Materials, structures and characterizations

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  13. Poling-free energy harvesters based on robust self-poled ferroelectric fibers

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  14. Large Flexoelectriclike Response from the Spontaneously Polarized Surfaces in Ferroelectric Ceramics

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  15. An electro-mechanical behavior enhancement method: geometric design with flexoelectricity

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  16. Magnetoelectric response from the enhanced ferromagnetism and flexoelectric response in reduced BiFeO3–based ceramics

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  17. Controllable anisotropic characteristics in solid solution ferroelectrics

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  18. Converse flexoelectricity with relative permittivity gradient

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  19. The surface mechanism for the flexoelectric response in sodium bismuth titanate‐based ferroelectric ceramics

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  20. Large Thermal–Electrical Response and Rectifying Conduction Behavior in Asymmetrically Reduced Ferroelectric Ceramics

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  22. Apparent piezoelectric response from the bending of non-poled PVDF

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  23. Flexoelectric materials and their related applications: A focused review

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  24. A flexoelectric spherical microshell model incorporating the strain gradient effect

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  30. Designing electromechanical metamaterial with full nonzero piezoelectric coefficients

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  50. Flexoelectricity in periodically poled lithium niobate by PFM

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