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RESEARCH PAPER · Advanced Materials · 2022

Emerging Halide Perovskite Ferroelectrics

Weilin Zheng, Xiucai Wang, Xin Zhang, Bing Chen, Hao Suo, Zhifeng Xing, Yanze Wang, Hanlin Wei, Jiangkun Chen, Yang Guo, Feng Wang

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Emerging Halide Perovskite FerroelectricsOriginalPeripheral substituent regulation of bias structured azulene-based hole transport materials for perovskite solar cells7Inversion of Molecular Chirality Associated with Ferroelectric Switching in a High-Temperature Two-Dimensional Perovskite Ferroelectric88Ferroelectric, Dielectric and Electromechanical Performance of Ba0.92Ca0.08Ti0.95Zr0.05O3 Ceramics with an Enhanced Curie Temperature12Regulation of Quantum Wells Width Distribution in Quasi‐2D Perovskite Films for High‐Performance Photodetectors37An efficient way of harvesting mechanoluminescent light: Flexible pressure sensor application6Direct Observation of the Anisotropic Transport Behavior of Li+ in Graphite Anodes and Thermal Runaway Induced by the Interlayer Polarization14Structure-Related Evolution of Magnetic Order in Anisidinium Tetrachlorocuprates(II)4Regulating 3D Phase in Quasi‐2D Perovskite Films for High‐Performance and Stable Photodetectors17Introducing a Structural Phase Transition in a 1D Perovskite via Cation’s Terminal Group Lengthening5Stabilizing Metal Halide Perovskites for Solar Fuel Production: Challenges, Solutions, and Future Prospects44A Self‐Powered UV Photodetector With Ultrahigh Responsivity Based on 2D Perovskite Ferroelectric Films With Mixed Spacer Cations64Interfacial Pyro‐Phototronic Effect: A Universal Approach for Enhancement of Self‐Powered Photodetection Based on Perovskites with Centrosymmetry38Large Enhancement of Polarization in a Layered Hybrid Perovskite Ferroelectric Semiconductor via Molecular Engineering29Metal-free chiral molecular ferroelectric photovoltaics13Regulation of electrical properties via ferroelectric polarization for high performance Sb2Te3 thermoelectric thin films15Unusual Phase Behaviour for Organo-Halide Perovskite Nanoparticles Synthesized via Reverse Micelle Templating5Trilinear coupling in lead-free halide superlattice CsSnI3/CsSiI3 : A first-principles study0Methylammonium-Based Quasi-Two-Dimensional Perovskite Single Crystals for Highly Sensitive X-ray Detection and Imaging22Tuning Structure and Excitonic Properties of 2D Ruddlesden–Popper Germanium, Tin, and Lead Iodide Perovskites via Interplay between Cations60Dielectric Engineering of 2D Organic–Inorganic Hybrid Perovskites68Ferroelectricity and Thermochromism in a 2D Dion‐Jacobson Organic–Inorganic Hybrid Perovskite7Formation of iminium ions during the processing of metal halide perovskites0Pressure-induced giant emission enhancement, large band gap narrowing and rich polymorphism in two-dimensional 1,2,4-triazolium lead bromide perovskite12Self-Powered Photodetector Based on Cs2agbibr6 Perovskite Film with High Detectivity and Pyroelectric Effect0The past 10 years of molecular ferroelectrics: structures, design, and properties173Unraveling the influence of organic cations on tuning electronic structures and spin-splitting in two-dimensional layered organic–inorganic tin-iodine perovskites3Room-Temperature Photoferroelectrics Semiconductor Driven by the Interlayer Confinement Effect20Topological Nodal-Point Superconductivity in Two-Dimensional Ferroelectric Hybrid Perovskites9Structure Directing Forces in Hybrid Layered Double Perovskites Containing Aromatic Organic Cations5Designing Yolk–Shell Nanostructures for Reversible Water-Vapor-Responsive Dual-Mode Switching of Fluorescence and Structural Color38Effect of Low to High Pressure on the Structural, Mechanical, Electrical, and Optical Properties of Inorganic Material Ca3AsBr3: An Ab Initio Investigation12Halide Anions Tuning of Lead‐Free Perovskite‐Type Ferroelectric Semiconductors with Inverse High‐Temperature Symmetry Breaking11Bi-functional Rb4Ag2BiBr9-PVDF composite based Piezoelectric mechanical energy harvester and light assisted self-charging power unit28Bipolar Plasticity in Synaptic Transistors: Utilizing HfSe2 Channel with Direct-Contact HfO2 Gate Dielectrics0Integration of One-Dimensional (1D) Lead-Free Perovskite Microbelts onto Silicon for Ultraviolet–Visible–Near-Infrared (UV-vis-NIR) Heterojunction Photodetectors19Advanced Design of Light‐Assisted Nanogenerators with Multifunctional Perovskites17Chirality Triggered Biferroicity in a 3D Rubidium Based Perovskite27Mn-doped perovskite quantum dots with thermal stability synthesized at room temperature9Spacer Cation Design Motifs for Enhanced Air Stability in Lead-Free 2D Tin Halide Perovskites42Molecularly thin, two-dimensional all-organic perovskites52Efficient Charge Transport in Inverted Perovskite Solar Cells via 2D/3D Ferroelectric Heterojunction25A Lead‐Free Ferroelectric 2D Dion–Jacobson Tin Iodide Perovskite35Highly Stable MOF‐Type Lead Halide Luminescent Ferroelectrics26Highly Stable MOF‐Type Lead Halide Luminescent Ferroelectrics7Ferroic Characteristics of Metal‐Halide Perovskites0Passivation of 1D@3D perovskite ferroelectric film with hydrophobic molecules for ferro-pyro-phototronic effect-based self-driven photodetector1Broadband Flexible Photodetectors Based on CdS x Se 1– x /PbI 2 Heterojunctions31Pyroelectric effect in high detectivity self-powered photodetector based on Cs2AgBiBr66X‐ray‐ultraviolet–visible‐near‐infrared photoresponses realized in a lead‐free hybrid perovskite ferroelectric through light‐induced ferro‐pyro‐phototronic effect26Piezoelectricity in chalcogenide perovskites27Ferroelectricity induced by lone pair electron effect in halide perovskite monolayers5Experimental Observation of the Fully Ferroelectric–Fully Ferroelastic Effect in Multiferroic Hybrid Perovskites90First principles study on electronic structure and optical property of O-doped lead-free perovskite CsSnCl32Ultrahigh energy harvesting ability of PVDF incorporated with 2D halide perovskite nanosheets via interface effect28Single Crystal Ruddlesden–Popper and Dion–Jacobson Metal Halide Perovskites for Visible Light Photodetectors: Present Status and Future Perspectives26On the thermal expansion of the tetragonal phase of MAPbI 3 and MAPbBr 34Controlling Electronic-Ionic Kinetics via Size Engineering in CsPbBr3 Perovskite Nanocrystals0Emerging Hybrid Metal Halide Glasses for Sensing and Displays14Ferroelectricity in Ultrathin Halide Perovskites2Hysteresis related to ion migration rather than ferroelectric polarization in MAPbI32Prediction of Physical Properties of Double Halides Using Machine Learning Methods2A Z/E isomeric cation designed organic-inorganic cadmium chloride ferroelectric with broadband white-light emission29Highly efficient tunable mid-infrared luminescence achieved by crystal field modulation of CsPb1-xHoxBr3 halide perovskite AlF3-based fluoride glass22D and quasi-2D hybrid halide perovskite single crystals: From fundamentals to functionalized photodetectors15Evidence of multiferroic behavior in sintered BaTiO3 obtained from high-energy ball-milled powders11Phosphonium Cation-Based Ferroelectric 1D Halide Perovskite-Like Semiconductor for Mechanical Energy Harvesting9Light-regulated pyro-phototronic effects in a perovskite Cs 2 SnI 6 -reinforced ferroelectric polymer hybrid nanostructure7Exploring Rashba spin-splitting and optoelectronic properties in lead-free 2D chiral hybrid perovskite (R-/S-/racemic-NEA)2SnI4 materials6Two-dimensional ferroelectricity in all-inorganic halide perovskite monolayer Cs 2 Pb X 4 ( X = F , Cl, Br, I)4Perspective on 2D perovskite ferroelectrics and multiferroics12Study on pressure-induced band gap modulation and physical properties of direct band gap Ca3NX3 (X = Cl, Br) for optoelectronic and thermoelectric applications33A review on photocatalytic methane conversion systems: from fundamental mechanisms to the emerging role of ferroelectric materials30Dynamic control of halide perovskite structures for tailored ferroelectric and second-order nonlinear optical functionalities39Enhanced charge separation and prolonged carrier lifetime in mixed Sn–Ge halide perovskite enabled by spontaneous symmetry breaking and moderate disorder2Growth of copper oxide at V2O5/Cu interface and its impact on the performance of piezoresistive pressure sensors using V2O5 films1Memcapacitors in neuromorphic architectures: the mechanisms, challenges, and applications10High-temperature self-powered X-ray detection in a bilayered hybrid ferroelectric halide perovskite9Self‐Powered Filterless Narrowband UV Photodetection Triggered by Asymmetric Charge Carrier Generation in a Wide‐Bandgap Halide Perovskite Ferroelectric18Emerging low-dimensional perovskite photoferroelectrics: From crystallographic microstructure to applications8Advances in Single‐Crystal Films: Synergistic Insights from Perovskites and Organic Molecules for High‐Performance Optoelectronics5Ultraviolet to Near-Infrared Polarization-Sensitive Photodetectors Based on (Phenethylammonium)2PbI4/PdSe2 Nanosheet Heterojunctions6Perovskite quantum dots Revolutionize Lithium-Sulfur battery Performance: Cathode catalytic Breakthrough with CsPbBr314The optoelectronic properties in two-dimensional sliding ferroelectric material XC (X = Ge, Si) under strain2Unveiling Giant Injection/Shift Current Ratio in Hybrid Quasi‐2D Perovskites3First principles analysis of the impact of pressure on the properties of the inorganic Sr3SbBr3 perovskite for energy harvesting13Incipient ferroelectricity in methylammonium lead halide perovskites7Photogalvanic effects in non-centrosymmetric halide perovskites17DFSE: Inverse Design of Ferroelectrics from Spatial Symmetry Breaking Evolution4Research on the multiplication mechanism of single-carrier transport-based multiplication-type organic photodetector4Visible‐Photoactive Ferroelectric Semiconductor Incorporating Aromatic Dynamic Spacer Enables Optoelectronic Synaptic Plasticity9Structural Phase Transition‐Associated Ferroelectricity and Piezoelectric Energy Harvesting in 0D Halogenozincate Hybrid via Cation's Terminal Group Lengthening4Spatially Resolved Observation of Ferroelectric‐to‐Paraelectric Phase Transition in a Two‐Dimensional Halide Perovskite6Rudorffite silver antimony iodide (AgSb2I7) thin films by thermal and microwave-assisted synthesis for self-powered visible light detection1Multiple Ferroelectric Resonance in 2D Organic–Inorganic Halide Perovskite0Phase-pure ferroelectric quantum wells with tunable photoluminescence for multi-state optoelectronic applications6Ferroelectric Domains and Domain Walls in Organic–Inorganic Hybrid Perovskites5Emerging Hydrochromic Metal Halide Perovskites9Exploring the optical and electrical properties of CsSnBr3 for optoelectronic technologies9Multiaxial Aromatic‐Based Photoferroelectric Induced by Synergistic Intermolecular Interactions for Multidirectional Self‐Powered X‐Ray Detection18Multiaxial Aromatic‐Based Photoferroelectric Induced by Synergistic Intermolecular Interactions for Multidirectional Self‐Powered X‐Ray Detection3Achieving Efficient Self‐Driven Full‐Stokes Photodetection in Optically Active Ferroelectric5Achieving Efficient Self‐Driven Full‐Stokes Photodetection in Optically Active Ferroelectric1Alkaline Earth Metal‐Based Hybrid Organic‐Inorganic Perovskite‐Like Ferroelectrics11Alkaline Earth Metal‐Based Hybrid Organic‐Inorganic Perovskite‐Like Ferroelectrics3From Formability to Bandgap: Machine Learning Accelerates the Discovery and Application of Perovskite Materials28Lone pair expression in fluorinated two-dimensional hybrid perovskite enables multiaxial ferroelectricity and nonlinear optical response24The Tuning of Structure Types and Switchable Dielectric Behavior in Pyridine Bromocuprate (II) Complexes1Molecular Engineering of Layered Halide Double Perovskites: Challenges and Opportunities in Optoelectronics and Beyond22Halide Perovskites for Self‐Driven X‐Ray Detection10Self‐Powered Ferroelectric Bi‐Based Perovskite X‐Ray Detector for Radiation Monitoring and Intelligent Imaging Recognition7Supercooled Liquid Phases of Luminescent Zero Dimensional Metal Halide Hybrids4Second‐Harmonic‐Generation Circular‐Dichroism in Chiral Perovskite Single Crystals Enhanced by Self‐Trapped Excitonic State12Surface ferroelectric phase transition triggered by s − p orbital interaction in two-dimensional monolayer perovskites2First-principles insights into band gap engineering and thermophysical properties of La-based perovskite oxides for solar-driven water splitting6Rotational Flexibility in Dication Drives Ambient Temperature Ferroelectricity in an Organic–Inorganic Hybrid Halide2Rotational Flexibility in Dication Drives Ambient Temperature Ferroelectricity in an Organic–Inorganic Hybrid Halide5Self-powered EA4Pb3Br10 ferroelectric perovskite photodetector for single-pixel imaging and encrypted optical communication5Biaxial Ferroelectric Crystals of 2D Metal‐Halide Perovskite Enable Multidirectional Bulk Photovoltaics for Self‐Driven X‐Ray Detection0Theoretical investigation of noncentrosymmetric Ruddlesden-Popper germanium perovskites Cs 2 Ge X 4 ( X = Cl , Br, and I) for second harmonic generation0Antimony Compounds as Potential Ferroelectric Materials1Optoelectronic and photovoltaic applications of layered halide perovskites Cs3X2Cl9 (X = Mo, Tc, Ru and Rh): A-first principle study2Ferroelectric Transistors: from Materials Innovation to Intelligent Electronic Systems13Origin of ferroelectricity in germanium-based inorganic halide perovskites2Ferroelectric‐Configured In‐Sensor Dynamic Computing with 2D Perovskites for Dim Object Recognition11Programmable piezoelectric domains and amplified d33 in 2D perovskites A2PbBr4 enabled by chain-length directed polar order0Boosting the piezoresponse in ferroelectric polymer via perovskite nanorod incorporation0Empirical equations to estimate tetragonal to cubic phase transitions in lead iodide perovskites1Ferroelectric high entropy oxides0Realizing Surface Acoustic Wave Device Based on 2D Ruddlesden‐Popper Perovskite: Exploring Acoustic and Acoustoelectric Characteristics0Interface‐Engineered TiO 2 Interlayer for Reliable Hafnia‐Based MFMIS FeFETs1Compositing halide perovskites for multifunctionalities beyond optoelectronics1Unveiling the Role of Halide Variation in Ba 3 BiX 3 (X = I, Br, Cl, and F) Perovskites Through First Principle DFT Approach: Tuning the Physical Properties2A Wide-Bandgap Molecular Ferroelectric Semiconductor with a Two-Step Wide-Temperature Second Harmonic Generation Response: [FMeQ] 2 ZnI 44Structural phase transition, electronic and dielectric properties of the perovskite selenites MSeO3 (M = Mg, Ca, Sr and Ba)0Strain‐Engineered Lattice‐Driven Chirality in CsPbBr 3 Nanorods0Growth and Characterization of Rb 0.146 K 0.854 Ta 0.61 Nb 0.39 O 3 Crystal0Dimensionality Engineering: A Pathway to Ferroelectric Halide Perovskites3Enhancing the Ferroelectricity of MAPbI 3 via Hydroxyl Groups to Boost Photocatalytic Performance1Bright Dual-Phase Organic Luminescence from Zero-Dimensional Lead Halide Hybrids via Sensitized Thermally Activated Delayed Fluorescence for Multifunctional Applications2Evaluation of organic–inorganic hybrid ferroelectric TMCM-GaCl4 synthesized via hand mixing0Analysis of the photoelectric properties and application potential of cesium-based lead-free double perovskites Cs2PtCl6, CsZrI6 and Cs2TeBr60Flexoelectricity in Photoconversion: Fundamentals, Materials, and Outlooks2High-entropy 1D halide perovskite piezoelectrics found by megalibrary synthesis and rapid nonlinear optical screening0Perspective on Ferroelectric and Nonferroelectric Low‐Dimensional Metal Halide Perovskites for Memristor Technology1Lead‐Free Hybrid Halide Perovskite for Piezoelectric Energy Harvesting0Direct Observation of Noncollinear Ferrielectricity in a Two-Dimensional Hybrid Germanium Perovskite1Enhancing carrier transport in Cs2AgBiBr6 double perovskites through multifunctional ferroelectric polymer doping1Record-high Glass coefficient in the shift current response of a ferroelectric halide perovskite0First‐Principle Analysis of the Structural, Elastic, Electronic, and Optical Properties of Novel AHgF 3 (A = K and Fr) Perovskite0Multistage Fluorination in a Metal‐Free Perovskite Ferroelectric Enables Multidirectional Self‐Powered X‐Ray Detection0

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  37. Chirality Triggered Biferroicity in a 3D Rubidium Based Perovskite

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  39. Spacer Cation Design Motifs for Enhanced Air Stability in Lead-Free 2D Tin Halide Perovskites

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  46. Passivation of 1D@3D perovskite ferroelectric film with hydrophobic molecules for ferro-pyro-phototronic effect-based self-driven photodetector

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  47. Broadband Flexible Photodetectors Based on CdS x Se 1– x /PbI 2 Heterojunctions

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  48. Pyroelectric effect in high detectivity self-powered photodetector based on Cs2AgBiBr6

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  49. X‐ray‐ultraviolet–visible‐near‐infrared photoresponses realized in a lead‐free hybrid perovskite ferroelectric through light‐induced ferro‐pyro‐phototronic effect

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