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RESEARCH PAPER · ACS Applied Materials & Interfaces · 2016

Defect Engineering of Lead-Free Piezoelectrics with High Piezoelectric Properties and Temperature-Stability

Yu Feng, Weili Li, Dan Xu, Yulong Qiao, Yang Yu, Yu Zhao, Weidong Fei

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Defect Engineering of Lead-Free Piezoelectrics with High Piezoelectric Properties and Temperature-StabilityOriginalDiffuse Phase Transitions and Giant Electrostrictive Coefficients in Lead-Free Fe 3+ -Doped 0.5Ba(Zr 0.2 Ti 0.8 )O 3 -0.5(Ba 0.7 Ca 0.3 )TiO 3 Ferroelectric Ceramics234Lead-free BNT-based composite materials: enhanced depolarization temperature and electromechanical behavior55Effect of Phase Transitions on Thermal Depoling in Lead-Free 0.94(Bi0.5Na0.5TiO3)–0.06(BaTiO3) Based Piezoelectrics141Modulating the electric and magnetic properties of BiFeO3 ceramics20Titanium deficiency in tetragonal-structured (Ba,Ca)(Zr,Ti)O 3 piezoelectric ceramics15Exceptionally High Piezoelectric Coefficient and Low Strain Hysteresis in Grain-Oriented (Ba, Ca)(Ti, Zr)O 3 through Integrating Crystallographic Texture and Domain Engineering217Colossal permittivity behavior and its origin in rutile (Mg1/3Ta2/3)xTi1-xO273Enhanced piezoelectricity in A B O 3 ferroelectrics via intrinsic stress-driven flattening of the free-energy profile14Large-size-mismatch co-dopants for colossal permittivity rutile TiO2 ceramics with temperature stability43Low dielectric loss induced by coupling effects of donor-acceptor ions in (Nb+Al) co-doped rutile TiO2 colossal permittivity ceramics45Non-volatile strain realized in the PNZST ceramics by K doping2Dielectric anomalies in stoichiometric Bi.49Er.01Na.5TiO3-K.5Na.5NbO3 ceramics5Room temperature ferroelectricity in donor-acceptor co-doped TiO2 ceramics using doping-engineering52Direct and converse piezoelectric grain-size effects in BaTiO3 ceramics with different Ba/Ti ratios31Intrinsic uniaxial stress induced by co-doping and its influence on piezoelectric performance of PbZr 0.45 Ti 0.55 O 3 ferroelectric5Lattice‐Defect‐Induced Piezo Response in Methylammonium‐Lead‐Iodide Perovskite Based Nanogenerator27Electromechanical response and piezoelectric properties in (Ba0.85Ca0.15)(Zr0.1Ti0.9)O3 piezoceramics using nano-sized AlN modification23High energy storage density at low electric field of ABO3 antiferroelectric films with ionic pair doping100Design for Highly Piezoelectric and Visible/Near‐Infrared Photoresponsive Perovskite Oxides137Systematic tuning of the photo-dielectric effect in Ba(Al1–xZnx)2O4–δ14Ultrahigh energy harvesting properties in textured lead-free piezoelectric composites68Giant electrostrictive effect in lead-free barium titanate-based ceramics via A-site ion-pairs engineering90Pressure Sensor Based on Polyvinylidene Fluoride Nanofibers Directly Written upon Silicon Substrate4The formation and effect of defect dipoles in lead-free piezoelectric ceramics: A review141Modeling dynamic rotation of defect dipoles and poling time dependence of piezoelectric effect in ferroelectrics10Understanding the mechanism of thermal-stable high-performance piezoelectricity76Enhanced electrical properties in donor–acceptor co-doped Ba(Ti0.92Sn0.08)O3 ceramics2Effects of Long- and Short-Range Ferroelectric Order on the Electrocaloric Effect in Relaxor Ferroelectric Ceramics103Electrical conduction and dielectric relaxation mechanisms in the KNN-based ceramics50Perovskite Sr 1– x (Na 0.5 Bi 0.5 ) x Ti 0.99 Mn 0.01 O 3 Thin Films with Defect Dipoles for High Energy-Storage and Electrocaloric Performance66High temperature stability and mechanical quality factor of donor-acceptor co-doped BaTiO3 piezoelectrics59Ba and Mg co-doping to suppress high-temperature dielectric loss in lead-free Na0.5Bi0.5TiO3-based systems37Giant Piezoelectric Properties of ZnO Film Doped with Acceptor-Donor Ionic Pair0High-performance lead-free ferroelectric BZT–BCT and its application in energy fields74Memory Effect in Antiferroelectrics: A Systematic Analysis on Various Electric Hysteresis Loops11Defects and Aliovalent Doping Engineering in Electroceramics353Hole-pinned defect-dipoles induced colossal permittivity in Bi doped SrTiO3 ceramics with Sr deficiency45Giant current performance in lead-free piezoelectrics stem from local structural heterogeneity46Non-contact localized probing of ferroelectric phase transitions in Li+/Er3+:BaTiO3 ceramics using fluorescence abnormalities8Role of A- and B-site excess doping on the improvement of the piezoelectric properties of BaTiO3 lead-free piezoceramics6Electrostrain Enhancement at Tricritical Point for BaTi1−xHfxO3 Ceramics19Multifunctional barium titanate ceramics via chemical modification tuning phase structure242Oxygen vacancy enhanced ferroelectricity in BTO:SRO nanocomposite films34Enhanced piezoelectric properties of 0.49Pb(Ni,Nb)O3–0.51Pb(Hf,Ti)O3 ceramics by ion pair doping5Porosity Modulated High-Performance Piezoelectric Nanogenerator Based on Organic/Inorganic Nanomaterials for Self-Powered Structural Health Monitoring81Confinement Aided Simultanous Water Cleaning and Energy Harvesting Using Atomically Thin Wurtzite (Wurtzene)11Investigation of the piezoelectric and anti-reduction properties of (Ba, Ca) (Ti, Sn, Hf) textured ceramics prepared under low oxygen partial pressure conditions at low sintering temperatures18Hardening effect in lead-free piezoelectric ceramics58Fluorescence-based quantitative characterization of structural phase transitions in Li+/Er3+:BaTiO3 ferroelectric ceramics6Manipulating temperature stability in KNN-based ceramics via defect design46Modulation on the electrical and optical properties of Na and Rh co-doped Ruddlesden-Popper layered Ca3Ti2O77Boron doped SiC thin film on Silicon synthesized from polycarbosilane: a new lead free material for applications in piezosensors1Large linear electrostrain of acceptor-donor Co-doped ZnO films8Evolution from Lead‐Based to Lead‐Free Piezoelectrics: Engineering of Lattices, Domains, Boundaries, and Defects Leading to Giant Response227Synergistic enhancement of piezoelectricity and thermal stability in AlN-doped Bi0.5Na0.5TiO3-based ceramics32Combined merits of high dielectric breakdown strength and low sintering temperature acquired in MgO-based dielectric ceramics: from theoretical prediction to experimental validation8Ultrahigh energy harvesting properties in temperature-insensitive eco-friendly high-performance KNN-based textured ceramics113High d33 Lead-Free Piezoceramics: A Review64Local symmetry breaking and magnetic properties of acceptor-donor codoped Ca3Mn2O7 hybrid improper ferroelectrics1Ultrahigh strain in textured BCZT-based lead-free ceramics with CuO sintering agent33Engineering the Defects and Microstructures in Ferroelectrics for Enhanced/Novel Properties: An Emerging Way to Cope with Energy Crisis and Environmental Pollution144Ion-Pair Engineering-Induced High Piezoelectricity in Bi 4 Ti 3 O 12 -Based High-Temperature Piezoceramics74High-electromechanical performance for high-power piezoelectric applications: Fundamental, progress, and perspective224Defect engineering of BiOX (X = Cl, Br, I) based photocatalysts for energy and environmental applications: Current progress and future perspectives227A correlative study between the microstructure and electrical properties of lead-free piezoceramics (1-x)BHT-xYLG driven by the synergistic action of multiple factors11Vacancy-assisted ferroelectric domain growth in BaTiO3 under an applied electric field: A molecular dynamics study10“Comments on: [High temperature stability and mechanical quality factor of donor-acceptor co-doped BaTiO3 piezoelectrics]”1Temperature and frequency dependent defect dipole kinematics in "hard" piezoelectric ceramics13Colossal permittivity of (Tm+Nb) co-doped rutile-TiO2 ceramics with ultralow dielectric loss and excellent thermal stability41Broad-temperature-span and improved piezoelectric/dielectric properties in potassium sodium niobate-based ceramics through diffusion phase transition16Porous (K0.5Na0.5)0.94Li0.06NbO3-polydimethylsiloxane piezoelectric composites harvesting mechanical energy for efficient decomposition of dye wastewater55Effect of a lattice distortion strategy on the phase transition and properties in KNN‐based ceramics19Abnormal piezoelectric properties of acceptor doped 0.75BF-0.25BT lead-free ceramics for application in atomizer18Correlation between structural, luminescence, and dielectric properties of novel Sm3+ and trioxotungsten-doped NBBT ceramic system for multifunctional device applications3Enhanced hydrogen production of acidified ruddlesden–popper type perovskite oxides in water and seawater by coupled piezo-photocatalysis41A facile strategy for concurrently promoting piezoelectric properties and thermal depolarization in unmodified BNT–BT piezoceramics: reasonable sintering temperature to regulate oxygen vacancy12Greatly improved piezoelectricity and thermal stability of (Na, Sm) Co-doped CaBi2Nb2O9 ceramics64Microscopic structure and migration of 90° ferroelectric domain wall in BaTiO3 determined via molecular dynamics simulations7Outstanding electromechanical performance in piezoelectric ceramics via synergistic effects of defect engineering and domain miniaturization50Design strategies of perovskite energy-storage dielectrics for next-generation capacitors115Stress dependent impedance spectroscopy of niobium based ceramics0Energy Harvesting Using ZnO Nanosheet-Decorated 3D-Printed Fabrics3Defect engineering in barium titanate ferroelectric ceramic showing simultaneous enhancement of piezoelectric coefficient and mechanical quality factor18Tuning Ferroelectric Properties of Barium Titanate by Lateral Strain: A Molecular Dynamics Simulation Study2Ultrahigh strain in PZ-PT-BNT piezoelectric ceramic15Well-balanced performance achieved in PZT piezoceramics via a multiscale regulation strategy28Simultaneous increase in piezoelectric response and Curie point in BaTiO3 based Pb-free piezoceramic24Chemical-Composition Tuning-Enabled Optimization of Structure, Properties, and Performance of Lead-Free (1 – x)BaZr0.05Ti0.95O3–(x)Ba0.92Ca0.08TiO3 Electroceramics5Colossal permittivity and ferroelectric properties regulation of different kinds of doped TiO26Temperature stability of perovskite-structured lead-free piezoceramics: Evaluation methods, improvement strategies, and future perspectives56The influence of thermo-electromechanical coupling on the performance of lead-free BNT-PDMS piezoelectric composites3Cu2+ and W6+ co-doped Na0·5Bi0·5TiO3 solid solution: An effective approach to inhibit oxygen vacancy generation and suppress oxygen ion conduction22Strategy to achieve both enhanced dielectric tunability and reduced dielectric loss in the barium zirconium titanate ceramics12Engineering strategies to enhance the piezoelectric catalytic performance of inorganic fibers in water treatment and energy regeneration14Modifying the high‐temperature dielectric properties of PLZT antiferroelectric ceramics by donor‒acceptor codoping2Computational Study of the Piezoelectric Performance of Barium Titanate Crystals in the Presence of Vacancy Defect: Molecular Dynamics Approach8Deciphering the Effect of Defect Dipoles on the Polarization and Electrostrain Behavior in Perovskite Ferroelectrics46Ultrahigh thermal stability and piezoelectricity of lead-free KNN-based texture piezoceramics89Piezoelectricity in excess of 30 pC N −1 with a high Curie temperature of 950 °C in strongly textured CaBi 2 Nb 2 O 9 ceramics18Defect engineering for arresting aging in donor-acceptor co-doped BaTiO33Simultaneous realization of giant d33, large kp, and high Qm from periodic interface strain generated by co-doping strategy7Enhanced piezoelectric properties and thermal stability in donor-acceptor co-doped BaTiO3 ceramics0High-temperature rolling-mediated functionality in polycrystalline BaTiO34Optimizing electrostrain in textured PNN-PHT piezoceramics through defect engineering4The effect of (In3+, Ta5+) co-dopant on dielectric properties and nonlinear characteristics of Bi2/3Cu3Ti4O12 ceramics2Enhanced electrocaloric effect in ferroelectric ceramics via defect dipole engineering17Large electrostrictive properties via double defect dipole designing in Na0.5Bi0.5TiO3 -based ceramics1Effect of perpendicular defect dipoles on phase transition and electrocaloric effect of BaTiO30High-power piezoelectric properties in manganese-modified PMN-PZT ceramics via defect and phase-boundary engineering0Enhancement of Curie temperature in high-performance textured Al2O3-doped (Ba0.95Ca0.05)(Ti0.94Zr0.05Sn0.01)O3 composite ceramics0Concurrently good piezoelectricity and thermal stability by control of multiple phase boundaries in KNN ceramics0Achieving high d33 and d33* simultaneously through the synergy of internal bias fields and multiphase coexistence in (Bi0.5Na0.5)0.76Sr0.24TiO3 ceramics0Tunable phase transition and electrocaloric effect via A-B-site donor-acceptor co-doping in BaTiO3 ceramics0

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  48. Hardening effect in lead-free piezoelectric ceramics

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  49. Fluorescence-based quantitative characterization of structural phase transitions in Li+/Er3+:BaTiO3 ferroelectric ceramics

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  50. Manipulating temperature stability in KNN-based ceramics via defect design

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