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RESEARCH PAPER · Advanced Materials · 2015

High‐Performance Lead‐Free Piezoceramics with High Curie Temperatures

Myang Hwan Lee, Da Jeong Kim, Jin Su Park, Sang Wook Kim, Tae Kwon Song, Myong‐Ho Kim, Won‐Jeong Kim, D. Do, Il‐Kyoung Jeong

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High‐Performance Lead‐Free Piezoceramics with High Curie TemperaturesOriginalBi nonstoichiometry and composition engineering in (1 − x)Bi 1+y FeO 3+3y/2 − xBaTiO 3 ceramics62Enhanced piezoelectricity in (1 − x)Bi 1.05 Fe 1−y A y O 3 –xBaTiO 3 lead-free ceramics: site engineering and wide phase boundary region77Lead-free piezoceramics – Where to move on?456Superior Piezoelectric Properties in Potassium–Sodium Niobate Lead‐Free Ceramics739Piezoelectric response of BiFeO3 ceramics at elevated temperatures53Multiferroic bismuth ferrite-based materials for multifunctional applications: Ceramic bulks, thin films and nanostructures631Temperature dependent, large electromechanical strain in Nd-doped BiFeO3-BaTiO3 lead-free ceramics225Effect of cooling rate on phase transitions and ferroelectric properties in 0.75BiFeO3-0.25BaTiO3 ceramics58A correlation between piezoelectric response and crystallographic structural parameter observed in lead-free (1-x)(Bi0.5Na0.5)TiO3–xSrTiO3 piezoelectrics79Poling engineering of (K,Na)NbO 3 -based lead-free piezoceramics with orthorhombic–tetragonal coexisting phases87Electric‐field induced phase transition and fatigue behaviors of (Bi 0.5+ x /2 Na 0.5‐ x /2 ) 0.94 Ba 0.06 Ti 1‐ x F e x O 3 ferroelectrics61The structural origin of enhanced piezoelectric performance and stability in lead free ceramics503Electrospun polyetherimide electret nonwoven for bi-functional smart face mask150Crucial role of octahedral untilting R 3 m / P 4 mm morphotropic phase boundary in highly piezoelectric perovskite oxide52Enhanced electromechanical properties of (1-x)BiFeO3–BaTiO3–xLiNbO3 ceramics by quenching process58Temperature dependence of the dielectric and piezoelectric properties of xBiFeO3–(1 − x)BaTiO3 ceramics near the morphotropic phase boundary55Revealing the role of heat treatment in enhancement of electrical properties of lead-free piezoelectric ceramics64A novel ((Bi0.5Na0.5)0.94Ba0.06)1- (K0.5Nd0.5) TiO3 lead-free relaxor ferroelectric ceramic with large electrostrains at wide temperature ranges54Structural and electrical characteristics of potential candidate lead-free BiFeO3-BaTiO3 piezoelectric ceramics124Piezoelectric, ferroelectric and ferromagnetic properties of (1−x)BiFeO3–xBaTiO3 lead-free ceramics near morphotropic phase boundary70Chemical heterogeneity and approaches to its control in BiFeO 3 –BaTiO 3 lead-free ferroelectrics110Large strain and temperature-insensitive piezoelectric effect in high-temperature piezoelectric ceramics64Bismuth ferrite-based lead-free ceramics and multilayers with high recoverable energy density396Enhanced insulating and piezoelectric properties of 0.7BiFeO 3 –0.3BaTiO 3 lead-free ceramics by optimizing calcination temperature: analysis of Bi 3+ volatilization and phase structures110Optimisation of functional properties in lead-free BiFeO 3 –BaTiO 3 ceramics through La 3+ substitution strategy149Practical high strain with superior temperature stability in lead-free piezoceramics through domain engineering63Temperature independence of piezoelectric properties for high-performance BiFeO 3 –BaTiO 3 lead-free piezoelectric ceramics up to 300 °C47Requirements for the transfer of lead-free piezoceramics into application286Large electric‐field‐induced strain and enhanced piezoelectric constant in CuO‐modified BiFeO 3 ‐BaTiO 3 ceramics49High-performance piezoelectric (K,Na,Li)(Nb,Ta,Sb)O3 single crystals by oxygen annealing51Enhanced piezoelectric properties by reducing leakage current in Co modified 0.7BiFeO3-0.3BaTiO3 ceramics62Evidence for two spin-glass transitions with magnetoelastic and magnetoelectric couplings in the multiferroic (Bi1−xBax)(Fe1−xTix)O3 system58High-Performance Piezoelectric Crystals, Ceramics, and Films249Large strain of temperature insensitive in (1–x)(0.94Bi0.5Na0.5TiO3–0.06BaTiO3) –xSr0.7La0.2TiO3 lead-free ceramics58Enhanced piezoelectric and ferroelectric properties of BiFeO3-BaTiO3 lead-free ceramics by optimizing the sintering temperature and dwell time117High strain (0.4%) Bi(Mg 2/3 Nb 1/3 )O 3 ‐BaTiO 3 ‐BiFeO 3 lead‐free piezoelectric ceramics and multilayers134Optimising dopants and properties in BiMeO3 (Me = Al, Ga, Sc, Y, Mg2/3Nb1/3, Zn2/3Nb1/3, Zn1/2Ti1/2) lead-free BaTiO3-BiFeO3 based ceramics for actuator applications121Lead-free high performance Bi(Zn0.5Ti0.5)O3-modified BiFeO3-BaTiO3 piezoceramics83Large strain of lead-free bismuth ferrite ternary ceramics at elevated temperature69Recent development in lead-free perovskite piezoelectric bulk materials1078High Energy Storage Density and Large Strain in Bi(Zn 2/3 Nb 1/3 )O 3 -Doped BiFeO 3 –BaTiO 3 Ceramics288Lead-free piezoceramics: Status and perspectives262Microscopic Insight into Electric Fatigue Resistance and Thermally Stable Piezoelectric Properties of (K,Na)NbO3-Based Ceramics98Low sintering temperature for lead‐free BiFeO 3 ‐BaTiO 3 ceramics with high piezoelectric performance57Practical High Piezoelectricity in Barium Titanate Ceramics Utilizing Multiphase Convergence with Broad Structural Flexibility280BiFeO3-BaTiO3: A new generation of lead-free electroceramics237Recent progress of ecofriendly perovskite-type dielectric ceramics for energy storage applications121Enhanced piezoelectric, electrocaloric and energy storage properties at high temperature in lead-free Bi0.5(Na1-xKx)0.5TiO3 ceramics47Enhanced Temperature Stability and Defect Mechanism of BNT‐Based Lead‐Free Piezoceramics Investigated by a Quenching Process134Novel bismuth ferrite-based lead-free incipient piezoceramics with high electromechanical response96Quenching-assisted actuation mechanisms in core–shell structured BiFeO 3 –BaTiO 3 piezoceramics55High electrostrain with high Curie temperature in BiFeO3-BaTiO3-based ceramics85Lead-free 0.7BiFeO3-0.3BaTiO3 high-temperature piezoelectric ceramics: Nano-BaTiO3 raw powder leading to a distinct reaction path and enhanced electrical properties54Understanding the mechanism of thermal-stable high-performance piezoelectricity76Processing, piezoelectric and ferroelectric properties of (x)BiFeO3-(1-x)SrTiO3 ceramics50Dielectric, conductivity and ferroelectric properties of lead-free electronic ceramic:0.6Bi(Fe0.98Ga0.02)O3-0.4BaTiO381Enhanced insulating and piezoelectric properties of BiFeO 3 ‐BaTiO 3 ‐Bi 0.5 Na 0.5 TiO 3 ceramics with high Curie temperature70Fabrication of a (K,Na)NbO3-based lead-free 1-3 piezocomposite for high-sensitivity ultrasonic transducers application51Microstructural Origins of High Piezoelectric Performance: A Pathway to Practical Lead‐Free Materials93Enhanced resistance in Bi(Fe1-Sc )O3-0.3BaTiO3 lead-free piezoelectric ceramics: Facile analysis and reduction of oxygen vacancy47Phase structure and energy storage performance for BiFeO3–BaTiO3 based lead-free ferroelectric ceramics134Comparison of multi-valent manganese oxides (Mn4+, Mn3+, and Mn2+) doping in BiFeO3-BaTiO3 piezoelectric ceramics87Electrical conduction mechanisms and effect of atmosphere annealing on the electrical properties of BiFeO3-BaTiO3 ceramics54Thermal Quenching Effects on the Ferroelectric and Piezoelectric Properties of BiFeO3–BaTiO3 Ceramics129Ultrahigh–energy density lead-free dielectric films via polymorphic nanodomain design1149Ultrahigh Performance in Lead-Free Piezoceramics Utilizing a Relaxor Slush Polar State with Multiphase Coexistence522Enhanced piezoelectric properties of 0.7BiFeO3-0.3BaTiO3 lead-free piezoceramics with high Curie temperature by optimizing Bi self-compensation74Thermally stable electrostrain in BiFeO3-BaTiO3-based high temperature lead-free piezoceramics49Excellent thermal stability and aging behaviors in BiFeO 3 ‐BaTiO 3 piezoelectric ceramics with rhombohedral phase105Coexistence of excellent piezoelectric performance and thermal stability in KNN-based lead-free piezoelectric ceramics57Biomedical application of graphene: From drug delivery, tumor therapy, to theranostics233Less temperature-dependent high dielectric and energy-storage properties of eco-friendly BiFeO3–BaTiO3-based ceramics57Chemical Solution Route for High‐Quality Multiferroic BiFeO3 Thin Films59Strong piezoelectricity of Li2CO3-doped BiFeO3–BaTiO3–Bi(Zn0.5Ti0.5)O3 lead-free piezoelectric ceramics with high Curie temperature and high temperature stability46Enhanced piezoelectric performance of donor La3+-doped BiFeO3–BaTiO3 lead-free piezoceramics58Physical properties of Al doped BiFeO3 obtained by sol-gel route and two-step sintering process43Enhanced electromechanical properties of SrTiO3-BiFeO3-BaTiO3 ceramics via relaxor behavior and phase boundary design57Advances in tuning the “ d 33 ∝ 1/ T d ” bottleneck: simultaneously realizing large d 33 and high T d in Bi 0.5 Na 0.5 TiO 3 -based relaxor ferroelectrics63Emerging new phase boundary in potassium sodium-niobate based ceramics393Fatigue resistant lead-free multilayer ceramic capacitors with ultrahigh energy density171Flexible hybrid piezo/triboelectric energy harvester with high power density workable at elevated temperatures55High-performance lead-free ferroelectric BZT–BCT and its application in energy fields74Improved piezoelectricity in ternary potassium–sodium niobate lead-free ceramics with large strain46Mesoscale origin of dielectric relaxation with superior electrostrictive strain in bismuth ferrite-based ceramics68Nano-domains in lead-free piezoceramics: a review283Progress in lead-free piezoelectric nanofiller materials and related composite nanogenerator devices123Achieving high-energy storage performance in 0.67Bi1Sm FeO3-0.33BaTiO3 lead-free relaxor ferroelectric ceramics118Giant current performance in lead-free piezoelectrics stem from local structural heterogeneity46Perovskite BiFeO3–BaTiO3 Ferroelectrics: Engineering Properties by Domain Evolution and Thermal Depolarization Modification140Structure, Performance, and Application of BiFeO3 Nanomaterials312Large Piezoelectric Response in Hybrid Rare-Earth Double Perovskite Relaxor Ferroelectrics112Perovskite lead-free piezoelectric ceramics287Phase evolution and origin of the high piezoelectric properties in lead-free BiFeO3–BaTiO3 ceramics66Ultrahigh piezoelectricity in lead-free piezoceramics by synergistic design172Origin of large electric-field-induced strain in pseudo-cubic BiFeO3–BaTiO3 ceramics140Phase diagram for Bi-site La-doped BiFeO3BaTiO3 lead-free piezoelectric ceramics56Multifunctional barium titanate ceramics via chemical modification tuning phase structure242Temperature-insensitive piezoelectric properties of lead-free BiFeO3–BaTiO3 ceramics with high Curie temperature68Lead-free BiFeO3 film on glass fiber fabric: Wearable hybrid piezoelectric-triboelectric nanogenerator76Dielectric, ferroelectric, and energy storage properties of Ba(Zn1/3Nb2/3)O3-modfied BiFeO3–BaTiO3 Pb-Free relaxor ferroelectric ceramics56Piezoelectricity in perovskite-type pseudo-cubic ferroelectrics by partial ordering of off-centered cations54Competitive mechanism of temperature-dependent electrical properties in BiFeO3-BaTiO3 ferroelectrics controlled by domain evolution148Progress and challenges of 3D-printing technologies in the manufacturing of piezoceramics48Electroactive nanomaterials in the peripheral nerve regeneration80Expanding the application space for piezoelectric materials44Lead-Free BiFeO3-BaTiO3 Ceramics with High Curie Temperature: Fine Compositional Tuning across the Phase Boundary for High Piezoelectric Charge and Strain Coefficients193Microstructure effects on the energy storage density in BiFeO3-based ferroelectric ceramics44Enhanced electric field induced strain in B-site Sb doped BiFeO3-BaTiO3 lead free ceramics44Influence of sintering method on microstructure, electrical and magnetic properties of BiFeO3–BaTiO3 solid solution ceramics49Role of Bi chemical pressure on electrical properties of BiFeO3–BaTiO3–based ceramics57A Review of a Good Binary Ferroelectric Ceramic: BaTiO3–BiFeO3107Review of lead-free Bi-based dielectric ceramics for energy-storage applications85On the exceptional temperature stability of ferroelectric Al1-xScxN thin films124Progress and perspectives in dielectric energy storage ceramics394Low sintering temperature, large strain and reduced strain hysteresis of BiFeO3–BaTiO3 ceramics for piezoelectric multilayer actuator applications55Paraelectric Matrix-Tuned Energy Storage in BiFeO3–BaTiO3–SrTiO3 Relaxor Ferroelectrics53Piezoelectric performance of Zr-modified lead-free BiFeO3-BaTiO3 ceramics49High piezoelectric properties in 0.7BiFeO3–0.3BaTiO3 ceramics with MnO and MnO2 addition55Ultrahigh energy harvesting performance in lead-free piezocomposites with intragranular structure43Evolution from Lead‐Based to Lead‐Free Piezoelectrics: Engineering of Lattices, Domains, Boundaries, and Defects Leading to Giant Response227BiFeO3-Based Relaxor Ferroelectrics for Energy Storage: Progress and Prospects53Grain Size Effects in Mn-Modified 0.67BiFeO3–0.33BaTiO3 Ceramics53Effective A-Site Modulation and Crystal Phase Evolution for High Ferro/Piezoelectric Performance in Abo3 Compounds: Yttrium-Doped Bifeo3-Batio357Enhanced Electric Field-Induced Strain Properties in Lead-Free BF-BT-Based Piezoceramics by Local Structure Inhomogeneity53Prospects of Metal‐Free Perovskites for Piezoelectric Applications60Multilayered Piezoelectric Nanogenerator Based on Lead-Free Poly(vinylidene fluoride)-(0.67BiFeO 3 -0.33BaTiO 3 ) Electrospun Nanofiber Mats for Fast Charging of Supercapacitors61Controllable electrical, magnetoelectric and optical properties of BiFeO3 via domain engineering147Ultrahigh piezoelectric strain in lead-free BiFeO3-BaTiO3 ceramics at elevated temperature48High‐Performance Strain of Lead‐Free Relaxor‐Ferroelectric Piezoceramics by the Morphotropic Phase Boundary Modification81Energy storage performance of BiFeO 3 –SrTiO 3 –BaTiO 3 relaxor ferroelectric ceramics48Recent progress in bismuth-based high Curie temperature piezo-/ferroelectric perovskites for electromechanical transduction applications88Ferroelectric BaTiO3 Based Multi‐Effects Coupled Materials and Devices46Boosting the High Performance of BiFeO3-BaTiO3 Lead-Free Piezoelectric Ceramics: One-Step Preparation and Reaction Mechanisms52Ultra-high piezoelectric performance by rational tuning of heterovalent-ion doping in lead-free piezoelectric ceramics103Emerging Halide Perovskite Ferroelectrics161Greatly improved piezoelectricity and thermal stability of (Na, Sm) Co-doped CaBi2Nb2O9 ceramics64Enhancement of Piezoelectricity by Novel Poling Method of the Rare‐Earth Modified BiFeO3–BaTiO3 Lead‐Free Ceramics44Improvement in piezoelectric performance of the lead-free BiFeO3-BaTiO3 ceramics by synergistic approach51Establishing a Relationship between the Piezoelectric Response and Oxygen Vacancies in Lead-Free Piezoelectrics46Tailoring tactics for optimizing microwave absorbing behaviors in ferrite materials70Design and development of a new lead-free BiFeO3-BaTiO3 quenched ceramics for high piezoelectric strain performance54BiAlO 3 ‐modified BiFeO 3 –BaTiO 3 high Curie temperature lead‐free piezoelectric ceramics with enhanced performance53BiFeO3-BaTiO3 ferroelectrics: Decrypting the mechanism of rare earth doping-induced electrical property discrepancy via scaling behavior and multi-level structure85Cold sintering behaviors of barium titanates: Recent progress and impact on microstructure, densification and dielectric-ferroelectric response49Bismuth Ferrite-Based Lead-Free High-Entropy Piezoelectric Ceramics44Temperature stability of perovskite-structured lead-free piezoceramics: Evaluation methods, improvement strategies, and future perspectives56Highly Transparent and Flexible All-Nanofiber-Based Piezocomposite Containing BaTiO3-Embedded P(VDF-TrFE) Nanofibers for Harvesting and Monitoring Human Kinetic Movements47Promising Lead-Free BiFeO3-BaTiO3 Ferroelectric Ceramics: Optimization Strategies and Diverse Device Applications48Ultrahigh thermal stability and piezoelectricity of lead-free KNN-based texture piezoceramics89Ultrahigh piezoelectric performances of (K,Na)NbO3 based ceramics enabled by structural flexibility and grain orientation54

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  10. Multiferroic bismuth ferrite-based materials for multifunctional applications: Ceramic bulks, thin films and nanostructures

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  11. Temperature dependent, large electromechanical strain in Nd-doped BiFeO3-BaTiO3 lead-free ceramics

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  31. Crucial role of octahedral untilting R 3 m / P 4 mm morphotropic phase boundary in highly piezoelectric perovskite oxide

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  32. Enhanced electromechanical properties of (1-x)BiFeO3–BaTiO3–xLiNbO3 ceramics by quenching process

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  33. Temperature dependence of the dielectric and piezoelectric properties of xBiFeO3–(1 − x)BaTiO3 ceramics near the morphotropic phase boundary

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  34. Revealing the role of heat treatment in enhancement of electrical properties of lead-free piezoelectric ceramics

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  35. Nonstoichiometric Effects in the Leakage Current and Electrical Properties of Bismuth Ferrite Ceramics

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  36. Large piezoelectric responses of Bi(Fe,Mg,Ti)O3-BaTiO3 lead-free piezoceramics near the morphotropic phase boundary

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  37. A coexistence of multi-relaxor states in 0.5BiFeO3–0.5BaTiO3

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  38. A novel ((Bi0.5Na0.5)0.94Ba0.06)1- (K0.5Nd0.5) TiO3 lead-free relaxor ferroelectric ceramic with large electrostrains at wide temperature ranges

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  39. Structural and electrical characteristics of potential candidate lead-free BiFeO3-BaTiO3 piezoelectric ceramics

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  40. Fabrication of lead-free piezoelectric (Bi0.5Na0.5)TiO3–BaTiO3 ceramics using electrophoretic deposition

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  41. Piezoelectric, ferroelectric and ferromagnetic properties of (1−x)BiFeO3–xBaTiO3 lead-free ceramics near morphotropic phase boundary

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  42. Temperature invariant high dielectric properties over the range 200 °C–500 °C in BiFeO3 based ceramics

    Journal of the European Ceramic Society · 2017-11-24

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  43. Chemical heterogeneity and approaches to its control in BiFeO 3 –BaTiO 3 lead-free ferroelectrics

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  44. Large strain and temperature-insensitive piezoelectric effect in high-temperature piezoelectric ceramics

    Journal of Materials Chemistry C · 2017-12-20

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  45. Application of Lead-Free Piezoelectric Materials

    Springer eBooks · 2018-01-01

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  46. Bismuth ferrite-based lead-free ceramics and multilayers with high recoverable energy density

    Journal of Materials Chemistry A · 2018-01-01

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  47. Bismuth Ferrite-Based Piezoelectric Materials

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  48. Enhanced insulating and piezoelectric properties of 0.7BiFeO 3 –0.3BaTiO 3 lead-free ceramics by optimizing calcination temperature: analysis of Bi 3+ volatilization and phase structures

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  49. Historical Introduction

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  50. Optimisation of functional properties in lead-free BiFeO 3 –BaTiO 3 ceramics through La 3+ substitution strategy

    Journal of Materials Chemistry A · 2018-01-01

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