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RESEARCH PAPER · Angewandte Chemie International Edition · 2024

Remarkable Second Harmonic Generation Response in (C 5 H 6 NO) + (CH 3 SO 3 ) − : Unraveling the Role of Hydrogen Bond in Thermal Driven Nonlinear Optical Switch

Zi‐Peng Zhang, Xin Liu, Rui‐Xi Wang, Shuang Zhao, Wen‐Jie He, Hong‐Yu Chen, Xue‐Bin Deng, Li‐Ming Wu, Zhengyang Zhou, Ling Chen

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Remarkable Second Harmonic Generation Response in (C 5 H 6 NO) + (CH 3 SO 3 ) − : Unraveling the Role of Hydrogen Bond in Thermal Driven Nonlinear Optical SwitchOriginalLooking Back the Nonlinear Optical Crystals in a Functionalized Unit's Perspective109Hg[CS(NH 2 ) 2 ] 4 (SiF 6 ): a fluorosilicate crystal with large birefringence achieved via multi-functional group modification6Highly stable and reversible birefringence switching triggered by thermally stimulated phase transition1Optimizing optical anisotropy in low-dimensional structures via intralayer hydrogen bonding modulation and anionic substitution17Synergistic engineering of ultraviolet metal-free crystals with exceptional birefringence via pyridine-derived dimers14Zwitterionic Glycine-Based Antimony Fluorides with Exceptional Ultraviolet Nonlinear Optical Properties11Inch‐sized K[NH2(CH2COO)2]: a High‐Performance UV Nonlinear Optical Crystal Enabled by Novel Flexible π‐Conjugated Building Units, [NH2(CH2COO)2]−13Regulation of Refractive Index by Halogens in Two-Dimensional Layered Methylsulfonate Halides7(3‐C6H10N2)ZnX4 (X = Cl and Br): Two Excellent UV Nonlinear Optical Crystals Designed by Combination of π‐conjugated and [ZnX4]2− Tetrahedral Units26A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence4A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence19Metal Cation Engineered UV Birefringent Crystals in π‐Conjugated Sulfonates with Record‐High Optical Anisotropy17Sb2(TeO4)(SO4): An Anhydrous Tellurite Sulfate with Large Birefringence and Enhanced Thermal Stability8Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization89Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization13Controllable Synthesis of a Strong Ultraviolet Nonlinear Optical Crystal by Tailoring the Lead Oxychloride Polyhedron3Unravelling the impact of octahedral distortion and non-covalent interactions on the hyperpolarizabilities of Co(II) and Ni(II) coordination complexes with uridine nucleotide11Mathematical Double‐Matrix Switchable Homochiral Ferroelectric18Mathematical Double‐Matrix Switchable Homochiral Ferroelectric6Breaking the Birefringence Barrier in B–O Crystals via B–C π-scaffolding38Synthesis and Characterization of (H7C5N2)6(V10O28)·2H2O with Edge-Sharing VO6 Octahedra Exhibiting Large Birefringence2Designing hybrid zinc-based ultraviolet nonlinear optical crystal with strong NLO response and dual-color luminescence via the integration of two different SHG-active genes6Designing Hybrid Sb-Based Nonlinear Optical Crystals with Large Birefringence by Combining the Lone Pair and π-Conjugated Genes10Gradient cellulose-based separator with dual nano-confinement and ion-guiding functions for dendrite-free zinc-ion batteries6Ag(Te2O3)(PO4): The first Ag-containing phosphate-tellurite nonlinear optical crystal featuring novel zigzag layered structure0Sulfonated Module Aggregation for Ultrahigh Birefringence in Aqueous-Processable Crystals27Enhanced Second Harmonic Generation Response via Rational Design of Iodinated π-Conjugated Pyridine Group5Unlocking Strong Second‐Harmonic Generation in Deep‐UV‐Transparent Polar Organic Sulfonates through Connectivity Regulation6Chiral Lead-Oxyiodide Nonlinear Optical Crystals Constructed on l -Malate Groups5Achieving an optimal performance balance in UV nonlinear optical crystals via hydrogen-bond regulation1An organic–inorganic hybrid piezoelectric exhibiting high-temperature structural phase transition and moderate second harmonic generation response0From centrosymmetric (C 4 H 8 N 5 )(SbF 4 ) to polar (C 4 H 7 N 4 O)(SbF 4 ): a new UV nonlinear optical material achieved by functional group modulation8Stable lead succinate-iodides with strong second-harmonic generation response and large birefringence0Strong second-harmonic generation and wide temperature range switching behavior coexisting in an ultrawide-bandgap selenate0Suppressing antiparallel dipole alignment: A molecular engineering strategy toward sem-organic UV NLO crystals0Unit Symmetry‐Breaking and Layered Linear Ordering Enabling Superior Short‐Wave Ultraviolet Birefringent Crystal9C 6 H 7 NCl·X (X = Cl, Br): Outstanding Multifunctional Nonlinear Optical and Birefringent Crystals Enabled by Incorporation of π‐Conjugated Moieties2Conformational Editing Drives Covalent Hybridization for Nonlinear Optical Crystals2Rigid‐Flexible Coupling Units Enable Robust Large Birefringence2Persistent Second‐Harmonic Generation Enhancement Across an Unprecedented Pressure Range in a Hybrid Antimony Halide0An Ultra-Wide Bandgap Sulfonate with Two-Step Second-Harmonic Generation Switching2Cation‐Dominated Second‐Order Nonlinear Optical Response Enabled by π‐Conjugated Guanidinium Derivatives5Anion Size‐Dependent Conformational Folding of Guanidinopropionate: Enabling Tunable Birefringence and Balanced Second‐Harmonic Generation Performance3Reverse Weak Polarity‐Induced Ordered Layer Control for Enhanced Second‐Harmonic Generation in Ultraviolet Nonlinear Optical Crystals2Redox‐Driven Strategy Enabling Leapfrog Enhancement of Birefringence in Layered Tin‐Based Optical Crystals1Bio-inspired proton-conformation-coupled hydrogen-bond network reconfiguration for adaptive optical anisotropy0An Excellent Deep‐Ultraviolet Nonlinear Optical Crystal Realized via a Functional Group Based on a Two‐in‐One Strategy0Assembly of dual π-conjugated units toward enhanced birefringence in a 2D organic sulfonate crystal0A Hydrogen-Bonded Molecular Crystal with Strong Optical Anisotropy and Large Second-Harmonic Generation Response0Structural-Dynamic Synergy in Hydrogen-Bond Reconfiguration Enables Room-Temperature Tunable Nonlinear Optical Materials0

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  2. Hg[CS(NH 2 ) 2 ] 4 (SiF 6 ): a fluorosilicate crystal with large birefringence achieved via multi-functional group modification

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  3. Highly stable and reversible birefringence switching triggered by thermally stimulated phase transition

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  4. Optimizing optical anisotropy in low-dimensional structures via intralayer hydrogen bonding modulation and anionic substitution

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  5. Synergistic engineering of ultraviolet metal-free crystals with exceptional birefringence via pyridine-derived dimers

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  6. Zwitterionic Glycine-Based Antimony Fluorides with Exceptional Ultraviolet Nonlinear Optical Properties

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  7. Inch‐sized K[NH2(CH2COO)2]: a High‐Performance UV Nonlinear Optical Crystal Enabled by Novel Flexible π‐Conjugated Building Units, [NH2(CH2COO)2]−

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  8. Regulation of Refractive Index by Halogens in Two-Dimensional Layered Methylsulfonate Halides

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  9. (3‐C6H10N2)ZnX4 (X = Cl and Br): Two Excellent UV Nonlinear Optical Crystals Designed by Combination of π‐conjugated and [ZnX4]2− Tetrahedral Units

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  10. A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence

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  11. A 3D Hybrid Perovskite Ferroelastic with Triclinic‐to‐Cubic Phase Transition Boosts Temperature/Pressure Dual On/Off Switchable Birefringence

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  12. Metal Cation Engineered UV Birefringent Crystals in π‐Conjugated Sulfonates with Record‐High Optical Anisotropy

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  13. Sb2(TeO4)(SO4): An Anhydrous Tellurite Sulfate with Large Birefringence and Enhanced Thermal Stability

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  14. Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization

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    Yaolong Zhu, Jie Gou, Can Yang, Qingwen Zhu, Yi Xiong, Qi Wu

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  15. Decoupling the SHG‐Birefringence Trade‐off in UV NLO Materials via Triple‐Control Coordination Engineering: Achieving Synergistic Performance Optimization

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  16. Controllable Synthesis of a Strong Ultraviolet Nonlinear Optical Crystal by Tailoring the Lead Oxychloride Polyhedron

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  17. Unravelling the impact of octahedral distortion and non-covalent interactions on the hyperpolarizabilities of Co(II) and Ni(II) coordination complexes with uridine nucleotide

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  18. Mathematical Double‐Matrix Switchable Homochiral Ferroelectric

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  19. Mathematical Double‐Matrix Switchable Homochiral Ferroelectric

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  20. Breaking the Birefringence Barrier in B–O Crystals via B–C π-scaffolding

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  21. Synthesis and Characterization of (H7C5N2)6(V10O28)·2H2O with Edge-Sharing VO6 Octahedra Exhibiting Large Birefringence

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  22. Designing hybrid zinc-based ultraviolet nonlinear optical crystal with strong NLO response and dual-color luminescence via the integration of two different SHG-active genes

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  25. Ag(Te2O3)(PO4): The first Ag-containing phosphate-tellurite nonlinear optical crystal featuring novel zigzag layered structure

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