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RESEARCH PAPER · Chemical Science · 2025

Synergistic engineering of ultraviolet metal-free crystals with exceptional birefringence via pyridine-derived dimers

Jiachen Lu, Kang Min Ok

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Synergistic engineering of ultraviolet metal-free crystals with exceptional birefringence via pyridine-derived dimersOriginalMetal Cation Engineered UV Birefringent Crystals in π‐Conjugated Sulfonates with Record‐High Optical Anisotropy17Breaking the Birefringence Barrier in B–O Crystals via B–C π-scaffolding36A novel metal-free crystal demonstrating superior birefringence attributed to the synergistic interaction of dual π-conjugated units8Optimizing the Hydrogen-Bond Network Drives Cadmium Ce(IV) Fluoride Hydrate with Significantly Enhanced Optical Anisotropy8Exceptional Enhancement of Optical Anisotropy Achieved via the Strategy of Combining Rigid Groups with High Symmetry and π‐Conjugated Organic Groups in Hybrid Fluorides33Sulfonated Module Aggregation for Ultrahigh Birefringence in Aqueous-Processable Crystals26Hybrid Zinc‒Based Halides with Giant Optical Anisotropy via Protonation‒Engineered π ‒Conjugated Organic Group24Hydrogen‐Bond‐Driven Metal‐Free Crystal (C 6 H 7 N 2 O)(NH 2 SO 3 ) with Giant Birefringence and Solar‐Blind Ultraviolet Transmission0Achieving record birefringence in metal-free semiorganic sulfate crystals via tetrahedral anionic group substitution0Overcoming the Bandgap‐Birefringence Trade‐Off: Proton‐Transfer Engineering of High‐Performance Ultraviolet‐Transparent Organic Crystal5Rigid‐Flexible Coupling Units Enable Robust Large Birefringence2Ce(2,2′-bipyridyl)3(SCN)3: Lanthanide Coordination- and Hydrogen-Bond-Directed Binary π-Conjugated Assemblies with Synergistic Large Birefringence and Broad Transparency0Assembly of dual π-conjugated units toward enhanced birefringence in a 2D organic sulfonate crystal0Dual‐Role BF 3 Anchoring Enables Giant Birefringence in Short‐Wave UV‐Transparent Fluoroborates0

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  1. Metal Cation Engineered UV Birefringent Crystals in π‐Conjugated Sulfonates with Record‐High Optical Anisotropy

    Small · 2025-04-07

    Zichang Wang, Qing‐Yu Liu, Zhihua Yang, Xueling Hou, Minqiang Gai

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  2. Breaking the Birefringence Barrier in B–O Crystals via B–C π-scaffolding

    Journal of the American Chemical Society · 2025-07-04

    Jiajia Li, Miao‐Bin Xu, Mingchang Wang, Zhi Wei Lin, Yuan Hua Lin, Yun-Xia Hu, Jia-Min Lian, Jin Chen, Ke‐Zhao Du

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  3. A novel metal-free crystal demonstrating superior birefringence attributed to the synergistic interaction of dual π-conjugated units

    Science China Materials · 2025-07-07

    Die-Xue Yang, Ru‐Ling Tang, Yi‐Lei Lv, Bing-Wei Miao, Wenlong Liu, Sheng‐Ping Guo

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  4. Optimizing the Hydrogen-Bond Network Drives Cadmium Ce(IV) Fluoride Hydrate with Significantly Enhanced Optical Anisotropy

    Inorganic Chemistry · 2025-07-25

    Wen-Ye Gao, Siyu Ma, Bing-Wei Miao, Wenfeng Zhou, Wenlong Liu, Ru‐Ling Tang

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  5. Exceptional Enhancement of Optical Anisotropy Achieved via the Strategy of Combining Rigid Groups with High Symmetry and π‐Conjugated Organic Groups in Hybrid Fluorides

    Advanced Science · 2025-10-06

    Ru‐Ling Tang, Bing-Wei Miao, Guo-Ren Zhu, Wenlong Liu, Sheng‐Ping Guo

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  6. Sulfonated Module Aggregation for Ultrahigh Birefringence in Aqueous-Processable Crystals

    Journal of the American Chemical Society · 2025-10-14

    Congcong Jin, Yang Li, Chong‐An Chen, Jihyun Lee, Chanhee Ko, Soo‐Yeon Lee, Kang Min Ok

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  7. Hybrid Zinc‒Based Halides with Giant Optical Anisotropy via Protonation‒Engineered π ‒Conjugated Organic Group

    Advanced Functional Materials · 2025-11-20

    Ruo‐Nan Li, Zhen‐Cheng Wu, Wen‐Dong Yao, Yi‐Fan Fu, Yu‐Mei Zhang, Wenlong Liu, Jiajing Wu, Sheng‐Ping Guo

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  8. Hydrogen‐Bond‐Driven Metal‐Free Crystal (C 6 H 7 N 2 O)(NH 2 SO 3 ) with Giant Birefringence and Solar‐Blind Ultraviolet Transmission

    Advanced Optical Materials · 2025-12-10

    Zhenkai Cen, Z.-Y. Li, Guang Peng, Junbo Gong, Junbo Gong

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  9. Achieving record birefringence in metal-free semiorganic sulfate crystals via tetrahedral anionic group substitution

    Chemical Science · 2026-01-01

    Yan-Zhen Xie, Hai-Yan Jiang, Yi Zhang, Hui‐Ping Xiao, Qing‐Yan Liu, Yu‐Ling Wang

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  10. Overcoming the Bandgap‐Birefringence Trade‐Off: Proton‐Transfer Engineering of High‐Performance Ultraviolet‐Transparent Organic Crystal

    Angewandte Chemie · 2026-03-05

    Lin Qiu, Xing‐Yu Li, Bing-Wei Miao, Hongjian Yu, Wenlong Liu, Yifan Sun, Ru‐Ling Tang

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  11. Rigid‐Flexible Coupling Units Enable Robust Large Birefringence

    Advanced Science · 2026-03-26

    Jie Zhou, Yanqiang Li, Ji Qi, Wei Huang, Liangmeng Zhu, Zhiyong Bai, Yang Zhou, Junhua Luo, Sangen Zhao

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  12. Ce(2,2′-bipyridyl)3(SCN)3: Lanthanide Coordination- and Hydrogen-Bond-Directed Binary π-Conjugated Assemblies with Synergistic Large Birefringence and Broad Transparency

    Inorganic Chemistry · 2026-07-24

    Quan-Wei Zhang, Zi-Han Tian, Ming-Xing Wu, Chenyuan Ma, Xing-Yu Bi, Zhi Gang Fang, Meihong Duan

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  13. Assembly of dual π-conjugated units toward enhanced birefringence in a 2D organic sulfonate crystal

    Science China Chemistry · 2026-09-15

    Longyun Xu, Hanjing Huang, Conggang Li, Huijian Zhao, Conghe Liu, Kaidong Xu, Jina Wang, Ning Ye, Zhanggui Hu

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  14. Dual‐Role BF 3 Anchoring Enables Giant Birefringence in Short‐Wave UV‐Transparent Fluoroborates

    Advanced Functional Materials · 2026-09-30

    Jin Chen, Jia‐Min Lian, Huai‐Yu Wu, Yun‐Xia Hu, Jinyu Luo, Yiru Fu, Cai‐Yi Liu, Ke‐Zhao Du

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