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RESEARCH PAPER · Advanced Functional Materials · 2024

Designing Strong Polarity and High Configurational Entropy Flexible Units toward Excellent Ultraviolet Nonlinear Optical Materials

Haotian Tian, Chensheng Lin, Bingxuan Li, Xin Lei Zhao, Tao Yan, Ning Ye, Min Luo

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Designing Strong Polarity and High Configurational Entropy Flexible Units toward Excellent Ultraviolet Nonlinear Optical MaterialsOriginalSynergistic combination of different types of functional motif in Rb(NO 3 )(SO 3 NH 3 ) for realizing excellent ultraviolet optical nonlinearity18Learning From Nature: The Rational Non‐Centrosymmetric Structural Design in the Honeycomb‐Like Gaudefroyite Family23Rational Design of Novel Polar Nonlinear Optical Materials in Alkali Metal Rare Earth Iodates5The synthesis, structures and characterizations of (C5H12NO)4Cd3Cl10·2H2O and (C5H12NO)2BiCl6·H5O2 crystals0Unconventional Heterobidentate Coordination of 4‐Hydroxypyridine Leading to Remarkably Strong Second‐Harmonic Generation in Zn(C 5 H 4 NO) 267Unconventional Heterobidentate Coordination of 4‐Hydroxypyridine Leading to Remarkably Strong Second‐Harmonic Generation in Zn(C 5 H 4 NO) 221[C(NH2)3]2S2O6: A SBBO-Like Dithionate Crystal with Large Optical Anisotropy14Inch‐sized K[NH2(CH2COO)2]: a High‐Performance UV Nonlinear Optical Crystal Enabled by Novel Flexible π‐Conjugated Building Units, [NH2(CH2COO)2]−13(C6H10N2)ZnX4·H2O (X=Cl and Br): Excellent nonlinear optical properties and temperature induced photoluminescence for encryption23A Promising Deep Ultraviolet Nonlinear Optical Crystal Activated by the Ordered Structure Design40A Promising Deep Ultraviolet Nonlinear Optical Crystal Activated by the Ordered Structure Design3Synergically Assembling Advantageous Groups toward High‐Performance Infrared Nonlinear Optical Materials A II CdSiSe 4 (A II = Sr, Ba)40(3‐C6H10N2)ZnX4 (X = Cl and Br): Two Excellent UV Nonlinear Optical Crystals Designed by Combination of π‐conjugated and [ZnX4]2− Tetrahedral Units26Na[B3IO7(OH)] and Na2[B4IO9](IO3): Explorations of Boroiodates with Strong Second Harmonic Generation Response and Large Birefringence54Hg3(TeO3)2(NO3)2 and Hg3(Te2O5)2(NO3)2: The First Two Hg‐Based Tellurite Nitrate Unit‐Mixed Crystals with Large Optical Anisotropy16Hydrogen‐Bonded Assembly of Functional Units for Constructing Linear and Nonlinear Optical Crystals10The riddle of α-resorcinol revisited—New perspectives on “pocket-like” structure1Engineered Integration of Diverse Functional Units Induces Multifunctionality in Malonate‐Borate Hybrids44Synergistic Design of UV Nonlinear Optical Crystals: Harnessing Flexible π-Conjugated Anions and Guanidinium Cations for Enhanced Performance4Giant Birefringence Induced by Intermolecular Aromatic Interactions in Hydrogen‐Bonded Organic Frameworks37Deprotonation-Regulated Conformational Switching in Malonates Enables High-Performance Ultraviolet Polar Crystals3NaAg3Ga8S14: A new diamond-like framework infrared nonlinear optical material derived from AgGaS26A Band‐Orientation Co‐Anchoring Strategy for the Design of a High‐Performance Mid‐Infrared Nonlinear Optical Crystal2A Band‐Orientation Co‐Anchoring Strategy for the Design of a High‐Performance Mid‐Infrared Nonlinear Optical Crystal12Shape‐Topology‐Driven Design of Deep Ultraviolet Nonlinear Optical Crystals: Engineering [CH 3 PO 3 ]–Metal‐Oxo Layered Frameworks for Enhanced SHG, DUV Transparency3Ag(Te 2 O 3 )(PO 4 ): Linear and Nonlinear Optical Properties of a Noncentrosymmetric Phosphotellurite with P–O–Te Connection1Synergism of [C 2 N 4 H 7 S] cations and anionic modulators: tailoring second-order nonlinear optics and birefringence in organic–inorganic crystals6氢键组装的新型紫外非线性光学晶体（R/S‑DACH）Mal·H2O的设计及性能研究（特邀）0Enhanced tripling-performance in [C(NH2)3]4P2O7·H2O as UV nonlinear optical material due to π-conjugated cation and hydrogen bonding intervention1Anion Size‐Dependent Conformational Folding of Guanidinopropionate: Enabling Tunable Birefringence and Balanced Second‐Harmonic Generation Performance3Anion Size‐Dependent Conformational Folding of Guanidinopropionate: Enabling Tunable Birefringence and Balanced Second‐Harmonic Generation Performance0Local Conformational Confinement and Dipole Engineering for Phase-Matchable Solar-Blind Ultraviolet Nonlinear Optical Crystals11Reverse Weak Polarity‐Induced Ordered Layer Control for Enhanced Second‐Harmonic Generation in Ultraviolet Nonlinear Optical Crystals2Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0Rational Design of a Strong Nonlinear Optical Crystal With Ultrawide Bandgap via Fine‐Tuning of Channel Structures0Tailoring a Solar‐Blind Ultraviolet Ferroelectric for Nonlinear Optics Through a Local Symmetry‐Breaking Cascaded Strategy1K3Sr3Li2Ga4B6O20F: A Sr2Be2B2O7-Type Ultraviolet Nonlinear Optical Crystal0Charge and structural flexibility of tartrate groups enable high-performance ultraviolet nonlinear optical crystals0The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals1The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals0An Excellent Deep‐Ultraviolet Nonlinear Optical Crystal Realized via a Functional Group Based on a Two‐in‐One Strategy0

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  1. Synergistic combination of different types of functional motif in Rb(NO 3 )(SO 3 NH 3 ) for realizing excellent ultraviolet optical nonlinearity

    Inorganic Chemistry Frontiers · 2024-01-01

    Yunxia Song, Chensheng Lin, Xin Yi Zhao, Tao Yan, Ning Ye, Haotian Tian, Min Luo

    Read original paper ↗ ·

  2. Learning From Nature: The Rational Non‐Centrosymmetric Structural Design in the Honeycomb‐Like Gaudefroyite Family

    Advanced Functional Materials · 2024-10-10

    Fanlu Bu, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  3. Rational Design of Novel Polar Nonlinear Optical Materials in Alkali Metal Rare Earth Iodates

    Inorganic Chemistry · 2024-10-23

    Lijuan Liu, Haotian Tian, Mingjun Xia, Xiaoyang Wang

    Read original paper ↗ ·

  4. The synthesis, structures and characterizations of (C5H12NO)4Cd3Cl10·2H2O and (C5H12NO)2BiCl6·H5O2 crystals

    Journal of Molecular Structure · 2024-10-25

    Chuanying Shen, Jie Liu, Xianzhe Wang, Xianzhe Wang, Chuanrui Zhu, Qiwei Xing, Chenyi Zhang, Kang Yang, Duanliang Wang

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  5. Unconventional Heterobidentate Coordination of 4‐Hydroxypyridine Leading to Remarkably Strong Second‐Harmonic Generation in Zn(C 5 H 4 NO) 2

    Angewandte Chemie International Edition · 2024-11-26

    Can Yang, Jie Gou, Yaolong Zhu, Yi Xiong, Zece Zhu, Ling Chen, Qi Wu

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  6. Unconventional Heterobidentate Coordination of 4‐Hydroxypyridine Leading to Remarkably Strong Second‐Harmonic Generation in Zn(C 5 H 4 NO) 2

    Angewandte Chemie · 2024-11-26

    Can Yang, Jie Gou, Yaolong Zhu, Yi Xiong, Zece Zhu, Ling Chen, Qi Wu

    Read original paper ↗ ·

  7. [C(NH2)3]2S2O6: A SBBO-Like Dithionate Crystal with Large Optical Anisotropy

    Inorganic Chemistry · 2024-12-11

    Siyu Li, Danyang Dou, Cheng Chen, Qi Shi, Bingbing Zhang, Ying Wang

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  8. Inch‐sized K[NH2(CH2COO)2]: a High‐Performance UV Nonlinear Optical Crystal Enabled by Novel Flexible π‐Conjugated Building Units, [NH2(CH2COO)2]−

    Laser & Photonics Review · 2025-03-05

    Yujie Fan, Lingli Wu, Chensheng Lin, Haotian Tian, Chao Wang, Tao Yan, Min Luo

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  9. (C6H10N2)ZnX4·H2O (X=Cl and Br): Excellent nonlinear optical properties and temperature induced photoluminescence for encryption

    Chemical Engineering Journal · 2025-03-09

    Chuanying Shen, Chenyi Zhang, Chenyi Zhang, Qiwei Xing, Defu Sun, Kui Wu, Bingbing Zhang, Jiyang Wang, Jiyang Wang, Duanliang Wang

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  10. A Promising Deep Ultraviolet Nonlinear Optical Crystal Activated by the Ordered Structure Design

    Angewandte Chemie International Edition · 2025-03-11

    Haonan Liu, Xuming Zhai, Xinru Li, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  11. A Promising Deep Ultraviolet Nonlinear Optical Crystal Activated by the Ordered Structure Design

    Angewandte Chemie · 2025-03-11

    Haonan Liu, Xuming Zhai, Xinru Li, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  12. Synergically Assembling Advantageous Groups toward High‐Performance Infrared Nonlinear Optical Materials A II CdSiSe 4 (A II = Sr, Ba)

    Advanced Functional Materials · 2025-03-24

    Hongshan Wang, Ran An, Zhihua Yang, Shilie Pan, Junjie Li

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  13. (3‐C6H10N2)ZnX4 (X = Cl and Br): Two Excellent UV Nonlinear Optical Crystals Designed by Combination of π‐conjugated and [ZnX4]2− Tetrahedral Units

    Small · 2025-03-27

    Chuanying Shen, Jie Liu, Defu Sun, Kang Yang, Bingbing Zhang, Kui Wu, Jiyang Wang, Duanliang Wang

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  14. Na[B3IO7(OH)] and Na2[B4IO9](IO3): Explorations of Boroiodates with Strong Second Harmonic Generation Response and Large Birefringence

    Journal of the American Chemical Society · 2025-04-07

    Ya-Lan Deng, Chun‐Li Hu, Xiang Xu, Mingzhi Zhang, Jiang‐Gao Mao

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  15. Hg3(TeO3)2(NO3)2 and Hg3(Te2O5)2(NO3)2: The First Two Hg‐Based Tellurite Nitrate Unit‐Mixed Crystals with Large Optical Anisotropy

    Laser & Photonics Review · 2025-04-10

    Piao Tang, Xin Wen, Yuchen Yan, Cao Xue, Jindong Chen, Chensheng Lin, Min Luo, Ning Ye, Guang Peng

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  16. Hydrogen‐Bonded Assembly of Functional Units for Constructing Linear and Nonlinear Optical Crystals

    Advanced Optical Materials · 2025-04-29

    Ziqi Chen, Changyou Liu, Chenxu Li, Juanjuan Lu, Zhihua Yang, Shilie Pan, Miriding Mutailipu

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  17. The riddle of α-resorcinol revisited—New perspectives on “pocket-like” structure

    The Journal of Chemical Physics · 2025-07-08

    Zhenkai Cen, Lingyu Wang, Dongbo Wang, Junbo Gong, Junbo Gong

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  18. Engineered Integration of Diverse Functional Units Induces Multifunctionality in Malonate‐Borate Hybrids

    Aggregate · 2025-08-18

    Ziqi Chen, Chenxu Li, Xiaoyu Wu, Juanjuan Lu, Zhihua Yang, Xueling Hou, Miriding Mutailipu

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  19. Synergistic Design of UV Nonlinear Optical Crystals: Harnessing Flexible π-Conjugated Anions and Guanidinium Cations for Enhanced Performance

    Inorganic Chemistry · 2025-08-22

    Cheng Hu, Yujie Fan, Chensheng Lin, Yunxia Song, Chao Wang, Tao Yan, Min Luo

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  20. Giant Birefringence Induced by Intermolecular Aromatic Interactions in Hydrogen‐Bonded Organic Frameworks

    Advanced Materials · 2025-08-29

    Yayong Sun, Hongyuan Sha, Yanqiang Li, Yayu Yan, Weiqi Huang, Tao Ouyang, Liyang Qin, Siwen Zhang, Hao Huang, Qiaohong Li, Sangen Zhao, Chao He, Rongjian Sa, Jianguo Zhang, Tianhua Zhou

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  21. Deprotonation-Regulated Conformational Switching in Malonates Enables High-Performance Ultraviolet Polar Crystals

    Inorganic Chemistry · 2025-10-03

    Zhengyan Lin, Huili Liu, Liling Cao, Ling Huang, Xuehua Dong, Yuqiao Zhou, Daojiang Gao, Ning Ye

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  22. NaAg3Ga8S14: A new diamond-like framework infrared nonlinear optical material derived from AgGaS2

    Chinese Journal of Structural Chemistry · 2025-10-15

    Hongshan Wang, Zhenglong Li, Zhenglong Li, Ran An, Zhenyou Wang, Juanjuan Lu, Guansong Zheng, Zhihua Yang, Yu Chu, Junjie Li

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  23. A Band‐Orientation Co‐Anchoring Strategy for the Design of a High‐Performance Mid‐Infrared Nonlinear Optical Crystal

    Angewandte Chemie · 2025-10-17

    Haochen Li, Haotian Tian, Pifu Gong, Tianyu Wang, Hongyu Liu, Bing Li, Qian Wu, Mingjun Xia

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  24. A Band‐Orientation Co‐Anchoring Strategy for the Design of a High‐Performance Mid‐Infrared Nonlinear Optical Crystal

    Angewandte Chemie International Edition · 2025-10-17

    Haochen Li, Haotian Tian, Pifu Gong, Tianyu Wang, Hongyu Liu, Bing Li, Qian Wu, Mingjun Xia

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  25. Shape‐Topology‐Driven Design of Deep Ultraviolet Nonlinear Optical Crystals: Engineering [CH 3 PO 3 ]–Metal‐Oxo Layered Frameworks for Enhanced SHG, DUV Transparency

    Laser & Photonics Review · 2025-11-03

    Cheng Hu, Lingli Wu, Chensheng Lin, Yujie Fan, Chao Wang, Huixin Fan, Tao Yan, Min Luo

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  26. Ag(Te 2 O 3 )(PO 4 ): Linear and Nonlinear Optical Properties of a Noncentrosymmetric Phosphotellurite with P–O–Te Connection

    Inorganic Chemistry · 2025-12-03

    Wei Chen, Zi-Xuan Zhao, Chao He, Mengjiao Xu, Hui‐Yan Zhao, Qi Wei, Guo‐Ming Wang

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  27. Synergism of [C 2 N 4 H 7 S] cations and anionic modulators: tailoring second-order nonlinear optics and birefringence in organic–inorganic crystals

    Inorganic Chemistry Frontiers · 2026-01-01

    Wenxiao Zhang, Yumeng Cui, Siyu Li, Bingbing Zhang, Ying Wang

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  28. 氢键组装的新型紫外非线性光学晶体（R/S‑DACH）Mal·H2O的设计及性能研究（特邀）

    Chinese Journal of Lasers · 2026-01-01

    阚子钧 Kan Zijun, 李雷鸣 Li Leiming, 吴红萍 Wu Hongping, 张玉杰 ZHANG Yujie, 俞洪伟 Yu Hongwei, 吴以成 Wu Yicheng

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  29. Enhanced tripling-performance in [C(NH2)3]4P2O7·H2O as UV nonlinear optical material due to π-conjugated cation and hydrogen bonding intervention

    Chinese Journal of Structural Chemistry · 2026-03-07

    Lei Wu, Enshen Wang, Bao Jiang, Xueyin Fu, Kechen Sun, Maierhaba Abudoureheman, Zhaohui Chen, Qun Jing, Yuhong Su

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  30. Anion Size‐Dependent Conformational Folding of Guanidinopropionate: Enabling Tunable Birefringence and Balanced Second‐Harmonic Generation Performance

    Angewandte Chemie International Edition · 2026-04-13

    Si‐Qian Jiang, Shuang Zhao, Yi‐Chang Yang, Jingyu Guo, Wenkai Zhao, Xuefei Wang, Li‐Ming Wu, Ling Chen

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  31. Anion Size‐Dependent Conformational Folding of Guanidinopropionate: Enabling Tunable Birefringence and Balanced Second‐Harmonic Generation Performance

    Angewandte Chemie · 2026-04-13

    Si‐Qian Jiang, Shuang Zhao, Yi‐Chang Yang, Jingyu Guo, Wenkai Zhao, Xuefei Wang, Li‐Ming Wu, Ling Chen

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  32. Local Conformational Confinement and Dipole Engineering for Phase-Matchable Solar-Blind Ultraviolet Nonlinear Optical Crystals

    Journal of the American Chemical Society · 2026-04-13

    Guangsheng Xu, Junwei Feng, Luyong Zhang, Zhihua Yang, Jian Wei Han, Shilie Pan

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  33. Reverse Weak Polarity‐Induced Ordered Layer Control for Enhanced Second‐Harmonic Generation in Ultraviolet Nonlinear Optical Crystals

    Advanced Science · 2026-05-11

    Lingli Wu, Chensheng Lin, Bo Li, Huixin Fan, Lingfei Lv, Shunda Yang, Tao Yan, Min Luo

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  34. Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects

    Advanced Optical Materials · 2026-07-21

    Xiangran Kong, Jingdong Yan, Zi Wang, Hongwei Leng, Shichao Cheng, Sue Hao, Xiaoran Niu, Zuotao Lei, Chunhui Yang

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  35. Rational Design of a Strong Nonlinear Optical Crystal With Ultrawide Bandgap via Fine‐Tuning of Channel Structures

    Laser & Photonics Review · 2026-08-15

    Zilong Geng, Zuju Ma, Ruibiao Fu, Xin-Tao Wu

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  36. Tailoring a Solar‐Blind Ultraviolet Ferroelectric for Nonlinear Optics Through a Local Symmetry‐Breaking Cascaded Strategy

    Advanced Materials · 2026-08-17

    Hongyuan Sha, Bingxuan Li, Xiaoming Yang, Lingfei Lv, Chao He, Jiangang He, Zujian Wang, Yali Yang, Zhihua Yang, Fangfang Zhang, Xifa Long, Shilie Pan

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  37. K3Sr3Li2Ga4B6O20F: A Sr2Be2B2O7-Type Ultraviolet Nonlinear Optical Crystal

    Inorganic Chemistry · 2026-08-28

    Bing Li, Aoge Yao, Jianqiao Wang, Zhengyang Zhou, Hongrui Liu, Haochen Li, Haotian Tian, Qian Wu, Ying Zhao, Lei Kang, Shu Hai Guo, Mingjun Xia

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  38. Charge and structural flexibility of tartrate groups enable high-performance ultraviolet nonlinear optical crystals

    Chinese Journal of Structural Chemistry · 2026-09-01

    Hongbo Huang, Yinsong Zhao, Yining Wang, Jiaxing Wang, Hanyu Chen, Daqing Yang, Ying Wang, Bingbing Zhang

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  39. The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals

    Angewandte Chemie International Edition · 2026-09-10

    Xiangqing Cao, Haotian Qiu, Juanjuan Lu, Yun Mo Yang, Xueling Hou, Junjie Li, Shilie Pan, Miriding Mutailipu

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  40. The Multi‐Scale Paradigm: An Integrated Design Logic for Nonlinear Optical Crystals

    Angewandte Chemie · 2026-09-10

    Xiangqing Cao, Haotian Qiu, Juanjuan Lu, Yun Mo Yang, Xueling Hou, Junjie Li, Shilie Pan, Miriding Mutailipu

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  41. An Excellent Deep‐Ultraviolet Nonlinear Optical Crystal Realized via a Functional Group Based on a Two‐in‐One Strategy

    Energy & environment materials · 2026-09-15

    Xiliang Jiang, Hongyuan Sha, Xieming Xu, Chenrui Wang, Luying Zheng, Haotian Tian, Binwen Liu, Shuai‐Hua Wang, Guo‐Cong Guo

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