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RESEARCH PAPER · Angewandte Chemie International Edition · 2025

Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency Conversion

Xiangyu Long, Fuming Li, Haotian Qiu, Xueling Hou, Juanjuan Lu, Junjie Li, Zhihua Yang, Jinhui Cao, Shilie Pan, Miriding Mutailipu

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Integrating Fluorinated [BF 4 ] Anion With π‐Conjugated Six‐Membered Rings for Short‐Wavelength UV Frequency ConversionOriginalA mercury-based selenite with wide bandgap and moderate birefringence via cation substitution and partial fluorination1Bandgap tuning through the substitution of alkali metal cations in A 2 AlCuF 6 (A = K, Rb, and Cs) for optoelectronic and renewable energy applications2Experimental measurements and density functional theory analysis of a novel Mannich base: structural and nonlinear optical perspectives1Synergistic Enhancement of Birefringence in Metal Benzoxazolium Complexes by π-Conjugated [C 9 H 10 NO] + and Triangular [HgI 3 ] − Motifs3Structural Anion Geometry-Regulated Molecular Alignment in [C 10 H 8 NO 2 ]-Based Crystals for Enhancing Ultraviolet Birefringence0Hydrogen‐Bond‐Directed Assembly of Urea Derivatives: Exceptional Birefringence Achieved by π ‐Conjugated Unit Alignment3From Coplanarity to Coaxiality: A Linearity-Oriented Design Paradigm for Ultrahigh Ultraviolet Birefringent Inorganic Crystals5Linear [ICl 2 ] Units Induced Giant Optical Anisotropy in AICl 2 (A = NH 4 , Rb): A Pathway to Advanced Birefringent Materials4Peroxide‐Assisted Solvate Engineering Enables Record‐High Birefringence in a Solar‐Blind Transparent Crystal0Tuning Second‐Order Nonlinear Optical Properties via Electronic Interaction Engineering: Distinct Roles of Nonconjugation, σ–π Conjugation, and Intramolecular Charge Transfer in Chalcogen‑Functionalized Closo ‐Carborane Hybrids0The First Silver Lead Borate, AgPb[B5O9]0From High Symmetry to High Symmetry: A Self‐Assembly Strategy for Synthesizing Large Birefringent Borates0[CN4H8]SiF6: Fluorination-guided design of deep-UV crystal with large birefringence0A novel tetrafluoroborate with giant birefringence assembled from biocompatible adenine0Rational Construction of Fluoride Crystals With Record Birefringence via Water‐Regulated Hydrogen‐Bond Network Reconfiguration0An Excellent Deep‐Ultraviolet Nonlinear Optical Crystal Realized via a Functional Group Based on a Two‐in‐One Strategy0Dual‐Role BF 3 Anchoring Enables Giant Birefringence in Short‐Wave UV‐Transparent Fluoroborates0

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  1. A mercury-based selenite with wide bandgap and moderate birefringence via cation substitution and partial fluorination

    Dalton Transactions · 2026-01-01

    Chen Zhu, Xiao-Min Wu, Xiao-Xue Wang, Si-Qi Zhou, Jing-Jing Wu, Xin-Lei Liu, You-Qian Wu, Jiannian Yao, Peng-Fei Li, Yu-Wu Zhong

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  2. Bandgap tuning through the substitution of alkali metal cations in A 2 AlCuF 6 (A = K, Rb, and Cs) for optoelectronic and renewable energy applications

    RSC Advances · 2026-01-01

    Muhammad Yaqoob, Nora Mobark Farhan, Hudabia Murtaza, Quratul Ain, Rawiyah A. Alkahtani, Junaid Munir, Mohammed Sultan Al-Buriahi

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  3. Experimental measurements and density functional theory analysis of a novel Mannich base: structural and nonlinear optical perspectives

    CrystEngComm · 2026-01-01

    Dennis A. Raj, Mani Jeeva, R. Purusothaman, I. Vetha Potheher

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  4. Synergistic Enhancement of Birefringence in Metal Benzoxazolium Complexes by π-Conjugated [C 9 H 10 NO] + and Triangular [HgI 3 ] − Motifs

    Inorganic Chemistry · 2026-03-19

    Bin Li, Xinyuan Zhang, Fei Liang, Zhanggui Hu, Ning Ye

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  5. Structural Anion Geometry-Regulated Molecular Alignment in [C 10 H 8 NO 2 ]-Based Crystals for Enhancing Ultraviolet Birefringence

    Crystal Growth & Design · 2026-04-07

    YaoGuo Shen, Yiman Yang, Jiajia Xiong, Xinyi Wang

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  6. Hydrogen‐Bond‐Directed Assembly of Urea Derivatives: Exceptional Birefringence Achieved by π ‐Conjugated Unit Alignment

    Small · 2026-04-14

    Peng Jiang, Yuqi Qin, Junwei Feng, Minqiang Gai, Shilie Pan

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  7. From Coplanarity to Coaxiality: A Linearity-Oriented Design Paradigm for Ultrahigh Ultraviolet Birefringent Inorganic Crystals

    Journal of the American Chemical Society · 2026-05-04

    Congcong Jin, Yang Li, Chong‐An Chen, Wei Zeng, S. D. Lee, Kang Min Ok

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  8. Linear [ICl 2 ] Units Induced Giant Optical Anisotropy in AICl 2 (A = NH 4 , Rb): A Pathway to Advanced Birefringent Materials

    Advanced Functional Materials · 2026-05-22

    Du Yinxia, C J Huang, Hongshan Wang, Linan Wang, Z Chen, Miriding Mutailipu, Shilie Pan, Junjie Li

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  9. Peroxide‐Assisted Solvate Engineering Enables Record‐High Birefringence in a Solar‐Blind Transparent Crystal

    Angewandte Chemie International Edition · 2026-06-22

    Yang Li, Congcong Jin, Kang Min Ok

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  10. Tuning Second‐Order Nonlinear Optical Properties via Electronic Interaction Engineering: Distinct Roles of Nonconjugation, σ–π Conjugation, and Intramolecular Charge Transfer in Chalcogen‑Functionalized Closo ‐Carborane Hybrids

    Chemistry - A European Journal · 2026-07-09

    Jia-Qi Wen, Ran Tao, Jia-Huan Li, Yi Miao, Jia-Yi Zhang, Yong‐Qing Qiu, Hong-Qiang Wang, Chun‐Guang Liu

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  11. The First Silver Lead Borate, AgPb[B5O9]

    Journal of Chemical Crystallography · 2026-07-30

    V. E. Kireev, D. O. Charkin, Yu.O. Kopylova, A. N. Gosteva, M. Yu. Arsent’ev, Kompanchenko A.A., M.G. Krzhizhanovskaya, S. N. Volkov, Sergey M. Aksenov

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  12. From High Symmetry to High Symmetry: A Self‐Assembly Strategy for Synthesizing Large Birefringent Borates

    Small · 2026-08-03

    Chunjie Shen, Junwei Feng, Zhihua Yang, Shilie Pan, Feng Zhang

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  13. [CN4H8]SiF6: Fluorination-guided design of deep-UV crystal with large birefringence

    Inorganic Chemistry Communications · 2026-08-23

    Piaoyu Yan, Bao Jiang, Jing Zhou, Jiawen Liu, Wanxiu Xi, Ensheng Wang, Xiuhua Cui, Zhaohui Chen

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  14. A novel tetrafluoroborate with giant birefringence assembled from biocompatible adenine

    Journal of Molecular Structure · 2026-09-06

    Guangzhizhen Fan, Yuze Li, Lixiang Qin, Zhou Yanling, Hongming Liu

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  15. Rational Construction of Fluoride Crystals With Record Birefringence via Water‐Regulated Hydrogen‐Bond Network Reconfiguration

    Angewandte Chemie International Edition · 2026-09-11

    Ru‐Ling Tang, Bing-Wei Miao, Ling Wang, Zheng-Yu Yang, Guo-Ren Zhu, Wenlong Liu, Sheng‐Ping Guo

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  16. An Excellent Deep‐Ultraviolet Nonlinear Optical Crystal Realized via a Functional Group Based on a Two‐in‐One Strategy

    Energy & environment materials · 2026-09-15

    Xiliang Jiang, Hongyuan Sha, Xieming Xu, Chenrui Wang, Luying Zheng, Haotian Tian, Binwen Liu, Shuai‐Hua Wang, Guo‐Cong Guo

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  17. Dual‐Role BF 3 Anchoring Enables Giant Birefringence in Short‐Wave UV‐Transparent Fluoroborates

    Advanced Functional Materials · 2026-09-30

    Jin Chen, Jia‐Min Lian, Huai‐Yu Wu, Yun‐Xia Hu, Jinyu Luo, Yiru Fu, Cai‐Yi Liu, Ke‐Zhao Du

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