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RESEARCH PAPER · Science · 2023

Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylation

Wei Zhang, Sung Min Kim, Lennart Wahl, Rachit Khare, Lillian Hale, Jian Zhi Hu, Donald M. Camaioni, Oliver Y. Gutiérrez, Yue Liu, Johannes A. Lercher

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Low-temperature upcycling of polyolefins into liquid alkanes via tandem cracking-alkylationOriginalChemical sciences, technological innovations, and resource circulation2Functionalization of polyethylene with hydrolytically-stable ester groups6Recent advances in plastic recycling and upgrading under mild conditions147Selective oxidative upgrade of waste polystyrene plastics by nitric acid to produce benzoic acid43A highly ionic reaction environment achieving low-temperature polyethylene upcycling3Notizen aus der Chemie0Boosting the aqueous-phase production of lactic acid via dual-site activation of carbohydrates2Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide69Mechanistic Understanding of Efficient Polyethylene Hydrocracking over Two‐Dimensional Platinum‐Anchored Tungsten Trioxide4Unraveling the catalytic activity of CaClOH-rich incineration fly ash in the pyrolysis of single-use plastics10Upcycling contaminated plastics21A new strategy to achieve the recycling of plastic waste by catalysis under mild conditions10Self‐Growing Organic Materials26Self‐Growing Organic Materials1Upcycling of polyethylenes by catalysis0Ionic-Liquid-Mediated Deconstruction of Polymers for Advanced Recycling and Upcycling45Chemical recycling of polyolefins: a closed-loop cycle of waste to olefins126Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes to Liquid Organic Hydrogen Carriers94Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes to Liquid Organic Hydrogen Carriers14Mechanistic Insights Enable Divergent Product Selectivity in Catalyst-Controlled Photooxidative Degradation of Polystyrene90Chemical upcycling of polyethylene, polypropylene, and mixtures to high-value surfactants349From Plastic Waste to Treasure: Selective Upcycling through Catalytic Technologies100Upcycling of Polypropylene Wastes via Catalytically C−H Modification with Polar Olefins12Solvent‐Free Depolymerization of Plastic Waste Enabled by Plastic‐Catalyst Interfacial Engineering55Solvent‐Free Depolymerization of Plastic Waste Enabled by Plastic‐Catalyst Interfacial Engineering3Stapler Strategies for Upcycling Mixed Plastics0Boosting the catalytic performance of metal–zeolite catalysts in the hydrocracking of polyolefin wastes by optimizing the nanoscale proximity56Co-upcycling of polyvinyl chloride and polyesters199Low‐Temperature Upcycling of Polypropylene Waste into H2 Fuel via a Novel Tandem Hydrothermal Process7Recent Advances in the Functionalized Poly(α-Hydroxy Acids) Synthesized fromO-Carboxyanhydrides4Molecular design and experimental study on the alkylation of benzene with C6 olefin dimer with Lewis acidic monoamine ionic liquids and its sulfonate surfactant properties9End-of-Life Plastics Management: A Review7Acidic ionic liquid-functionalized ordered mesoporous polymers: Highly efficient solid acid catalysts for water-medium organic reactions15Precise activation of C–C bonds for recycling and upcycling of plastics81Numerical study on waste polyethylene pyrolysis driven by self-sustaining smoldering9Ultrasmall Zeolite Subcrystal Catalyst Devoid of Intracrystalline Diffusion Limitation for Bulk Molecule Conversion14Beyond biodegradation: upcycling of polylactic acid plastic waste into amino acids via cascade catalysis under mild conditions60Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Efficient Degradation of Oxidized Polyethylene Containing Ester Bonds by Cutinase or Lipase in Aqueous Phase0Hydroxyl carboxylate anion catalyzed depolymerization of biopolyesters and transformation to chemicals8Influence of temperatures and loadings on olefin diffusion in MFI-type zeolites in one- to three-dimensions6Plastic as Fuel of the Future1Role of the hydrocarbon molecular structure in CNT growth on Fe–Al catalysts6Selective Recovery of Para-Xylene from Polyethylene Terephthalate Plastic26Selectivity descriptors of the catalytic n -hexane cracking process over 10-membered ring zeolites32A general strategy for recycling polyester wastes into carboxylic acids and hydrocarbons75Catalytic Hydrogenolysis of Polyethylene Under Reactive Separation46Solar reforming as an emerging technology for circular chemical industries182A Unified View of Carbon Neutrality: Solar-Driven Selective Upcycling of Waste Plastics30Highly Selective Upgrading of Polyethylene into Light Aromatics via a Low-Temperature Melting-Catalysis Strategy55Catalytic conversion of mixed polyolefins under mild atmospheric pressure48Microwave-intensified catalytic upcycling of plastic waste into hydrogen and carbon nanotubes over self-dispersing bimetallic catalysts80Emerging green approaches for valorization of plastics with saturated carbon backbones42Upcycling Waste Plastics with a C–C Backbone by Heterogeneous Catalysis45Catalytic Strategies for the Upcycling of Polyolefin Plastic Waste30Circular olefin copolymers made de novo from ethylene and α-olefins83Ring-Opening Polymerization of Lactones to Prepare Closed-Loop Recyclable Polyesters116Recent Progresses and Challenges in Upcycling of Plastics through Selective Catalytic Oxidation15Synthesis and Deconstruction of Polyethylene-type Materials194Enhanced biodegradation activity toward polyethylene by fusion protein of anchor peptide and Streptomyces sp. strain K30 latex clearing protein13Catalytic upcycling plastics with CO2: A novel strategy for carbon waste valorization0Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes3Chloride and Hydride Transfer as Keys to Catalytic Upcycling of Polyethylene into Liquid Alkanes29CO2-facilitated upcycling of polyolefin plastics to aromatics at low temperature56Upcycling of Carbon Fiber/Thermoset Composites into High‐Performance Elastomers and Repurposed Carbon Fibers58Upcycling of Carbon Fiber/Thermoset Composites into High‐Performance Elastomers and Repurposed Carbon Fibers5Light-driven polymer recycling to monomers and small molecules112Research Progress in Fuel Oil Production by Catalytic Pyrolysis Technologies of Waste Plastics29Catalytic fast pyrolysis over heavy metals-containing livestock manure biochar catalyst for polystyrene upcycling22Hierarchical FAU Zeolites Boosting the Hydrocracking of Polyolefin Waste into Liquid Fuels38Upcycling of polyethylene to gasoline through a self-supplied hydrogen strategy in a layered self-pillared zeolite166Conversion of Polyethylene to Low-Molecular-Weight Oil Products at Moderate Temperatures Using Nickel/Zeolite Nanocatalysts6Complete hydrogenolysis of mixed plastic wastes101Complete Degradation of Polyolefin Plastic Wastes to High‐Value Products7Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling3Micelles Cascade Assembly to Tandem Porous Catalyst for Waste Plastics Upcycling50Hydrodeoxygenation of Oxygen‐Containing Aromatic Plastic Wastes into Cycloalkanes and Aromatics11Catalytic performance and acidic analysis of chloroaluminate ionic liquid with various impurities in the synthesis of multi-octylnaphthalene base oil1Thermodynamic and economic analysis of a deployable and scalable process to recover Monomer-Grade styrene from waste polystyrene22Conversion of Post-Refining Waste MONG to Gaseous Fuel in a Rotary Gasifier1Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst12Oxidative Upcycling of Polyethylene to Long Chain Diacid over Co‐MCM‐41 Catalyst58Synthesis and structure–property relationship of coal-based isomeric alkylbenzene sulfonate surfactants19Upgrading Polyolefin Plastic Waste into Multifunctional Porous Graphene using Silicone‐Assisted Direct Laser Writing14Recent progress of waste plastic upcycling based on multifunctional zeolite catalysts13Polyethylene to gasoline via a self-supplied hydrogen strategy0Lifecycle Management for Sustainable Plastics: Recent Progress from Synthesis, Processing to Upcycling87Catalytic chemical recycling and upcycling of polyolefin plastics27Room-Temperature Upcycling of Mixed PVC and Polyolefin Waste1Recent advances in polyolefin plastic waste upcycling via mild heterogeneous catalysis route from catalyst development to process design25Mild Catalytic Degradation of Crystalline Polyethylene Units in a Solid State Assisted by Carboxylic Acid Groups23Stapler Strategies for Upcycling Mixed Plastics49Active species in chloroaluminate ionic liquids catalyzing low-temperature polyolefin deconstruction22Bimetal-carbon engineering for polypropylene conversion into hydrocarbons and ketones in a Fenton-like system10Sustainable Plastics with High Performance and Convenient Processibility19Manipulating Dual-Metal Catalytic Activities toward Organic Upgrading in Upcycling Plastic Wastes with Inhibited Oxygen Evolution52Catalyst‐ and Solvent‐Free Upcycling of Poly(Ethylene Terephthalate) Waste to Biodegradable Plastics52Fabrication of MnAlNiO to boost the conversion of plastic wastes to CNTs for the supercapacitor application15Catalytic Upcycling of Polyolefins316Recovering Valuable Chemicals from Polypropylene Waste via a Mild Catalyst-Free Hydrothermal Process20Selective Upcycling of Polyolefins into High-Value Nitrogenated Chemicals80Catalytic recycling of plastics into value-added products28Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization12Ultra‐Narrow Alkane Product Distribution in Polyethylene Waste Hydrocracking by Zeolite Micro‐Mesopore Diffusion Optimization66Synthesis and characterization of bioplastics based on silyated starch and acrylated epoxidized soybean oil10Task‐Specific Deep Eutectic Solvent for Efficient Dissolution and Further Accelerating Alkaline Hydrolysis of Polyesters Into Their Monomers18Upcycling Polyethylene into Poly(3-hydroxybutyrate) via a Chemo-Enzymatic-Microbial Cascade0Review of key issues and potential strategies in bio-degradation of polyolefins5Influence of Trace Metal in Plastics on Catalyst Activity and Reusability during Polyolefins Upcycling with Polyoxometalates2Catalytic Hydrodeoxygenation of Mixed Plastic Wastes into Sustainable Naphthenes47Noble metal-free tandem catalysis enables efficient upcycling plastic waste into liquid fuel components22Polyethylene Recycling via Water Activation by Ball Milling5Polyethylene Recycling via Water Activation by Ball Milling23Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials14Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials3One-pot catalytic conversion of polyethylene wastes to gasoline through a dual-catalyst system41Valorization of Polycaprolactone to γ-Caprolactone over Lewis Acidic Ionic Liquids5Upcycling Polyethylene to High‐Purity Hydrogen under Ambient Conditions via Mechanocatalysis2Upcycling Polyethylene to High‐Purity Hydrogen under Ambient Conditions via Mechanocatalysis15Engineering noble metal-free nickel catalysts for highly efficient liquid fuel production from waste polyolefins under mild conditions16Aqu‐Thermoplastics: Recycling Plastics with Water9A better fate for PVC2Room-temperature co-upcycling of polyvinyl chloride and polypropylene50Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development23Understanding the Role of the Surface Acidity of MFI Zeolites during LDPE Cracking: Decomposition Temperature and Product Distribution26Research progress on chemical recycling of waste plastics mediated by ionic liquids0Chemical transformation of polyurethane into valuable polymers26Upcycling of Polyethylene Wastes to Valuable Chemicals over Group VIII Metal‐decorated WO 3 Nanosheets6An electricity-powered future for mixed plastic waste chemical recycling25Ionic liquids with multiple hydrogen bonds as metal-free catalysts for efficient hydrolysis of PET under relatively mild conditions6Heterogeneous catalysis strategies for polyolefin plastic upcycling: co-reactant-assisted and direct transformation under mild conditions15Microwave‐Powered Liquid Metal Degradation of Polyolefins30Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100Product Oriented Upcycling of Waste Polyethylene Terephthalate Plastic and Carbon Dioxide via Decoupled Electrolysis9Upcycling of waste plastics: strategies, status-quo, and prospects3Alkylation technology0Can mixed plastics be recycled and upcycled without separation?11Highly adaptable oxidative upcycling of polyolefins to multifunctional chemicals containing oxygen and nitrogen9Low temperature polyolefin deconstruction via tandem cracking-hydrogenation2Recycling of polystyrene waste to mono-aromatic hydrocarbons via intermittent thermal scission5Theoretical determination of a model molecule for the catalytic upcycling of polyethylene and polypropylene0Transforming polystyrene wastes into aromatic products near ambient temperature with aluminium chloride6Upcycling of poly(ethylene terephthalate) waste plastics to terephthalonitrile6Upcycling polyethersulfones to luminescent materials by aminolysis4Upgrading of waste polyolefins with non-noble metal catalysts21Nitrogenative Degradation of Polystyrene Waste44Conversion of Polypropylene to Light Olefins by HMFI Catalysts below Pyrolytic Temperature: Catalytic, Spectroscopic, and Theoretical Studies3Molecular Design for Dual Circularity: Polyester with Complementary Mechanical and Chemical Recyclability under Mild Conditions3Molecular Design for Dual Circularity: Polyester with Complementary Mechanical and Chemical Recyclability under Mild Conditions1Co-upcycling of polyethylene terephthalate and polyoxymethylene into valuable chemicals13

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