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RESEARCH PAPER · Green Chemistry · 2023

Recent advances in plastic recycling and upgrading under mild conditions

Shengbo Zhang, Mei Li, Zhenyang Zuo, Zhiqiang Niu

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Recent advances in plastic recycling and upgrading under mild conditionsOriginalEfficient polyethylene terephthalate biodegradation by an engineered Ideonella sakaiensis PETase with a fixed substrate-binding W156 residue29Recent advances in the biological depolymerization and upcycling of polyethylene terephthalate28Advances in solar-driven, electro/photoelectrochemical, and microwave-assisted upcycling of waste polyesters15Design of depolymerizable polymers toward a circular economy69Efficient glycolysis of used PET bottles into a high-quality valuable monomer using a shape-engineered MnO x nanocatalyst27Embedding an esterase mimic inside polyesters to realize rapid and complete degradation without compromising their utility18Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook57A Unified View of Carbon Neutrality: Solar-Driven Selective Upcycling of Waste Plastics30Poly(vinyl chloride) Dechlorination Catalyzed by Zirconium10Tandem Chemical Depolymerization and Photoreforming of Waste PET Plastic to High-Value-Added Chemicals148Chemical recycling of waste plastics: Current challenges and perspectives37Photocatalytic Upcycling and Depolymerization of Vinyl Polymers19Photocatalytic Upcycling and Depolymerization of Vinyl Polymers74Enhancing H 2 O 2 Electrosynthesis at Industrial-Relevant Current in Acidic Media on Diatomic Cobalt Sites182Electro-Reforming of PET Plastic to C 2 Chemicals with Concurrent Generation of Hydrogen and Electric Energy188Spent Lithium‐Ion Batteries Derived Co 3 O 4 for Electrocatalytic Polyethylene Terephthalate Plastic Recycling22Grave-to-cradle photothermal upcycling of waste polyesters over spent LiCoO2111Coupling Waste Plastic Upgrading and CO 2 Photoreduction to High-Value Chemicals by a Binuclear Re–Ru Heterogeneous Catalyst77Brønsted-acid sites induced photocatalytic cracking of low-polarity polyethylene plastics17CO2-enhanced PET depolymerization by catalyst free methanolysis13Mg(OTf)2 as an Excellent Catalyst for the Reductive Depolymerization and Methanolysis of Polyesters and Polycarbonates17Photorefinery of Biomass and Plastics to Renewable Chemicals using Heterogeneous Catalysts96Photorefinery of Biomass and Plastics to Renewable Chemicals using Heterogeneous Catalysts4An efficient and scalable melt fiber spinning system to improve enzyme-based PET recycling3Methanolysis of Plastic Waste with Manganese Compounds10Photocatalytic upcycling of plastics containing aliphatic C–C bonds into versatile chemicals9Mechanism and performance of the hydrolytic chemical recycling of polylactide catalyzed by the protic ionic liquid 2-HEAA9Co-upcycling of Plastic Waste and Biowaste via Tandem Transesterification Reactions10Electrocatalytic upcycling of plastic waste: Progress, challenges, and future53Rapid hydrolysis of waste polyurethane and facile system separation16Oxidative degradation and upcycling of polyethylene wastes40Hydroborative Depolymerization of Polyesters and Polycarbonates to Diols Catalyzed by Heterogeneous Lanthanum Materials La(CH2C6H4NMe2-o)3@SBA-155Key Terms in Plastic Waste Transformation Reactions3Plastic-Degrading Enzymes from Marine Microorganisms and Their Potential Value in Recycling Technologies34Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials14Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials3Jogo Educacional sobre Reciclagem para Pessoas com Deficiência Intelectual2Photooxidation of Polystyrene into High‐Value Chemicals16Reassessing the Photochemical Upcycling of Polystyrene Using Acridinium Salts25Reassessing the Photochemical Upcycling of Polystyrene Using Acridinium Salts2Plastic waste valorization for formic acid production: A comparison between the electrolysis and hydrogenation process5Photocatalytic Upcycling of Plastic Waste into Syngas by ZnS/Ga 2 O 3 Z‐Scheme Heterojunction15Upcycling of Plastic Waste0Shape selective cracking of polypropylene on an H- MFI type zeolite catalyst with recovery of cyclooctane solvent4Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development23Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins44Selective solvothermal extraction of tetrabromobisphenol A to promote plastic recycling7Research progress on chemical upcycling of waste polyethylene terephthalate2Photoreforming of Plastic Waste to Sustainable Fuels and Chemicals: Waste to Energy59Efficient Photoredox Co-Upcycling of CO 2 and Plastic Waste by Band-Gap-Engineered Zn x Cd 1– x S Catalyst93Advances and Challenges for Catalytic Recycling and Upgrading of Real-World Mixed Plastic Waste100Recent Progress in Polyolefin Plastic: Polyethylene and Polypropylene Transformation and Depolymerization Techniques22A review of commercial plastic waste recycling into graphene materials14Advanced strategies for plastic upcycling: unlocking sustainable waste valorization pathways for a green and sustainable environment7Catalysis in sustainable energy resources: overview studies of hydrogen, methane, biomass and plastics21Closed-loop electro-upcycling of PET waste into formate and hydrogen via self-supported NiCo 2 O 4 spinel arrays12Recent advances in catalytic hydrogenolysis of polyester1Reengineering waste PET bottles into BiOBr/Bi 4 O 5 Br 2 heterojunction materials for highly selective photocatalytic oxidation of benzyl alcohol4Sustainable base-mediated chemical upcycling of poly (propylene carbonate) to β-hydroxy sulfides and oxides1Theory-guided multifunctional Zn-Salen molecular catalyst for sustainable polyester plastic recycling12Upcycling of poly(ethylene terephthalate) waste plastics to terephthalonitrile6Visible-light-driven photocatalytic depolymerization of post-consumer PET to terephthalic acid via cerium catalysis with batch-to-flow scalability14Photocatalytic upcycling of polylactic acid to alanine by sulfur vacancy-rich cadmium sulfide103Photoreforming of waste plastic by B‐doped carbon nitride nanotube: Atomic‐level modulation and mechanism insights44Visible light–triggered depolymerization of commercial polymethacrylates128Kinetic analysis of PET methanolysis by using biomass-based heterogeneous catalysts. Towards sustainable chemical plastic recycling11Morphology Optimization of Spinel Catalysts for High‐Efficiency Photothermal Catalytic Upcycling of Polyethylene Terephthalate47Activating Molybdenum Peroxide Scissors for Converting Polyamide Plastic into Low Carbon Alcohols9Activating Molybdenum Peroxide Scissors for Converting Polyamide Plastic into Low Carbon Alcohols0Efficient Bioprocess for Mixed PET Waste Depolymerization Using Crude Cutinase8Catalytic Upgrading of Plastic Wastes into High-Value Carbon Nanomaterials: Synthesis and Applications59Catalytic Reforming of PET Plastic Waste for Efficient Hydrogen Production Using Bifunctional Ru Catalyst4In vivo and in vitro degradation and biological toxicity studies of polyesters with varying degradation rates17Asymmetric Atomic Pt–B Dual-Site Catalyst for Efficient Photoreforming of Waste Polylactic Acid Plastics in Seawater56Synergetic effects of p-toluenesulfonic acid and acetic acid on the catalytic depolymerization of bisphenol A polycarbonate waste into valuable chemicals2A comprehensive mechanism of polyester enzymatic depolymerization: A novel singular key parameter for streamlined eco-design2Microplastics in Weras Ganga, Bolgoda North Lake, Sri Lanka: A Reflection of Urban Waste Mismanagement8Polyethyleneketones with Controlled Spacer Units: Synthesis, Characterization, and Photodegradation13Photoreforming for upcycling of plastics into energy, chemicals and materials: a review7Reductive depolymerization of polycarbonates and polyesters using alkaline earth catalysts6Unlocking the Potential of Mn‐based Catalyst for Durable Two‐electron Oxygen Reduction in Acid at High Current Densities17Unlocking the Potential of Mn‐based Catalyst for Durable Two‐electron Oxygen Reduction in Acid at High Current Densities5Sustainable Treatment of Plastic Wastes with Photocatalytic Technologies: A Review7Upcycling of Waste Polyester Plastic to Carboxylic Acids and Hydrogen by a Ru δ+ –Ru 0 Dual-Site Catalyst28Ni/Nb2O5 as a noble-metal-free catalyst for the chemical upcycling of waste polyolefin plastics9Photocatalytic Waste Polystyrene Plastic Conversion: Reaction Mechanism and Catalyst Design38Binuclear Metal-Based Covalent Organic Framework Mimicking Metallohydrolases for Direct Photoreforming of PET Plastic48Efficient and Sustainable Electrochemical System for Alkali Ion Recovery from Alkaline Polyester Waste Hydrolysis0Electrochemical Upgrading Plastic to Organosulfurs Through Fe‐N 3 Single Atom Catalyst Under Ambient Conditions7Electrochemical Upgrading Plastic to Organosulfurs Through Fe‐N 3 Single Atom Catalyst Under Ambient Conditions26Fabricated double Z-scheme heterojunction photocatalyst for highly selective photocatalytic conversion of polylactic acid plastics6Effects of Conduction Band Edge Regulation on the Photoreforming Efficiency of Plastic Waste: Taking BPNS/TiO 2 as a Photocatalyst21Tandem Catalysis to Mitigate Coke Formation in the Upcycling of Mixed Polyolefin Wastes11Waste plastic-derived carbon materials for supercapacitors and rechargeable batteries27From waste to value: Synthesis of diols from polyester and polycarbonate plastics using commercial iron catalysts0Highly Stable Heterometallic Catalysts for Polyester Depolymerization and Polymerization at High Temperatures19Recycle Learning: um Jogo Educacional com Agentes Inteligentes para a Conscientização Ambiental0Orchestrating catalytic hotspots and macromolecular architectures: molecular engineering toward zero-waste polymer circularity4Sustainable, ultrafast, and solvent-free thiol–ene reactions promoted by a triazatruxene-based initiator2Toward Sustainable Plastic Waste Valorization: Green Synergistic Catalytic Strategies for Plastic Upcycling12Electrocatalytic valorization of biomass-derived alcohols and aldehydes: Mechanistic insights and innovative catalyst design11Electronic regulation via dual-defect synergy for boosting electro-reforming of polyethylene terephthalate waste to value-added formate and hydrogen4From waste plastic to hydrogen fuel: selective conversion through advanced catalytic technologies20Upcycling of PET waste: from one polymer to another polymer22Tandem depolymerization-electrocatalysis for plastic waste upcycling6Optimization of Fenton-like-driven waste plastic upgrading processes: Trade-off strategies between environmental and techno-economic benefits1Surface and Interface Properties of Metal Species for Waste Plastic Hydroconversion6Electrochemical recovery and regeneration of polyethylene terephthalate materials7WO2Cl2-promoted chemical recycling of plastics into valuable products0Beyond mechanical recycling: artificial photosynthesis enables polyester plastic upcycling into valuable chemicals5Advanced catalyst design and mechanistic insights in electrocatalytic upcycling of PET-derived ethylene glycol and coupled electrolysis systems4Chemically recyclable polyester materials0Depolymerization of crystalline PET under mild conditions by a serine-incorporated copper azolate hydrolase mimic0Electrochemical depolymerization of polycarbonates under catalyst-free conditions0Integrating chemical and biological conversion for waste plastics recycling and upcycling toward a circular bioeconomy0Photoreforming of plastic waste into value-added chemicals with hydrogen production4Recent Advances in Earth-Abundant Metal-Catalyzed Oxidative Degradation of Polyolefins0Research Progress on Reductive Defluorination of Polytetrafluoroethylene (PTFE)0Solubility-limited depolymerization kinetics in the glycolysis of carbonyl-containing polymers2Solvent-mediated contaminant removal from plastic waste using thermodynamic modeling4Recovery technology for waste plastics based on electrocatalytic reforming: From mechanism understanding to catalyst design2Nanozymes for Energy and Environmental Sustainability5Sustainable co-upcycling of waste PET plastic and ethylene glycol to high-value carboxylic acids on a carbon-encapsulated RuNi bimetallic catalyst4Chain Flexibility as a Fundamental Descriptor for Mild Depolymerization of Polyesters and Polycarbonates3Process intensification driven by non-conventional energy fields in emerging plastic recycling: A systematic review2Electrocatalytic degradation strategies for plastic fibers with sustainable resource recovery potential4Conversion of waste micro/nano plastics into carbon materials: A new trend for renewable energy and environmental applications0Bioinspired Design of F–Zn Sites in Layered Double Hydroxides for Photothermal Catalytic Upcycling of Polyethylene Terephthalate9Bioinspired Design of F–Zn Sites in Layered Double Hydroxides for Photothermal Catalytic Upcycling of Polyethylene Terephthalate0Rational catalyst design and coupled electrolysis for electrocatalytic upcycling of waste polyester plastics1Green and Sustainable Chemistry for a Circular Economy2Selective Photocatalytic Upcycling of Polystyrene Plastic to High-Value Chemicals by a Single-Atom Fe Catalyst7Scalable Upcycling of Mixed Plastics into High-Performance Covalent Adaptable Networks5Well‐Defined Heterocatalysts for Plastic Upcycling: From Design to Applications3Waste plastic recycling and upgrading via electro- and photocatalytic C−X bond coupling1Natural Sunlight‐Driven Synthesis of Conjugated Microporous Polymers via Electron Donor‐Acceptor Complexes for Highly Efficient Catalytic Upcycling of Real‐World Plastic Waste0Natural Sunlight‐Driven Synthesis of Conjugated Microporous Polymers via Electron Donor‐Acceptor Complexes for Highly Efficient Catalytic Upcycling of Real‐World Plastic Waste1Photocatalytic Depolymerization of Commercial Polymethacrylates via a Solvent-Independent Pathway1Photoreforming and Photoelectroreforming of Waste‐Derived Feedstocks for Solar‐Driven Production of Fuels and Chemicals0Photocatalytic Upcycling of Polyester Waste to Organonitrogen Compounds0AI-driven de novo protein design coupled with high-throughput screening: Challenges and opportunities0Solar‐Driven Upcycling of Waste Polyethylene Terephthalate0Pt/Mo Cocatalyst-Modified g-C3N4/ZnIn2S4 Heterojunctions: Electron–Hole Separation Boosted Selective Photocatalytic Plastic Upcycling0Nonpolar Polysiloxane with 100% Self-Healability, Closed-Loop Recyclability, and Antifouling0Emerging Catalytic Platforms for Plastic Waste Recycling and Upcycling Over MOFs and COFs: Catalyst Engineering and Reaction Mechanisms0Mixed plastic waste in the sustainable road: Thermal stability, mechanical properties, economic and environmental assessment0Bridging Science and Policy on Terrestrial Plastic Pollution: A Bibliometric Analysis of Global Research Trends and African Governance Gaps0

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  5. Efficient glycolysis of used PET bottles into a high-quality valuable monomer using a shape-engineered MnO x nanocatalyst

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  7. Review on Catalytic Depolymerization of Polyolefin Waste by Hydrogenolysis: State-of-the-Art and Outlook

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  14. Enhancing H 2 O 2 Electrosynthesis at Industrial-Relevant Current in Acidic Media on Diatomic Cobalt Sites

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  15. Electro-Reforming of PET Plastic to C 2 Chemicals with Concurrent Generation of Hydrogen and Electric Energy

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  17. Grave-to-cradle photothermal upcycling of waste polyesters over spent LiCoO2

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  36. Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials

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  37. Jogo Educacional sobre Reciclagem para Pessoas com Deficiência Intelectual

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  38. Photooxidation of Polystyrene into High‐Value Chemicals

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  39. Reassessing the Photochemical Upcycling of Polystyrene Using Acridinium Salts

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  43. Upcycling of Plastic Waste

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  45. Catalytic materials based on metals (ions) used in the upcycling of plastics and polymers into fuels and valuable chemicals as part of sustainable development

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  46. Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins

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  47. Selective solvothermal extraction of tetrabromobisphenol A to promote plastic recycling

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  48. Research progress on chemical upcycling of waste polyethylene terephthalate

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  49. Photoreforming of Plastic Waste to Sustainable Fuels and Chemicals: Waste to Energy

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  50. Efficient Photoredox Co-Upcycling of CO 2 and Plastic Waste by Band-Gap-Engineered Zn x Cd 1– x S Catalyst

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