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RESEARCH PAPER · Angewandte Chemie International Edition · 2023

Solvent‐Free Depolymerization of Plastic Waste Enabled by Plastic‐Catalyst Interfacial Engineering

Xiaoshen Bai, Divakar Reddy Aireddy, Amitava D. Roy, Kunlun Ding

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Solvent‐Free Depolymerization of Plastic Waste Enabled by Plastic‐Catalyst Interfacial EngineeringOriginalClosed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle106CO 2 catalyzed recycling of polyester and polycarbonate plastics16Selective Recovery of Para-Xylene from Polyethylene Terephthalate Plastic26Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst94Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst5Chemical Recycling of Polycarbonates via Ammonolysis and Polycaprolactones by KOH‐Catalyzed Methanolysis22From Polyester Plastics to Diverse Monomers via Low‐Energy Upcycling65Catalytic Hydroxyethylation of Phenols with Renewable Ethylene Glycol Diester as an Alternative to Ethylene Oxide4Recent advances in the chemical recycling of polyesters44Molecular Recognition in Mechanochemistry: Insights from Solid‐State NMR Spectroscopy4Molecular Recognition in Mechanochemistry: Insights from Solid‐State NMR Spectroscopy2Depolymerization mechanisms and closed-loop assessment in polyester waste recycling144Biotechnology for the degradation and upcycling of traditional plastics10Upconversion Phosphor-Driven Photodegradation of Plastics11Circular Economy and Chemical Conversion for Polyester Wastes23Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins44Stabilization of ZnO Catalysts for Polyesters Hydrolytic Depolymerization by Incorporation into ZrO2 Lattice: A Polylactic Acid Case Study5Advances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design6Toward Sustainable Polydienes26Molecular Details of Polyester Decrystallization via Molecular Simulation6Selective Asymmetric Hydrogenation of Waste Polyethylene Terephthalate via Controlled Sorption through Precisely Tuned Moderate Acid Sites50One-Pot Conversion of Polyethylene Terephthalate into 1,4-Cyclohexanedicarboxylic Acid without External H219Chemical recycling of waste polyester plastics1An effective strategy for degrading waste PET plastic into regenerated DMT with nearly equivalent methanol at relatively low temperature10Atomic Cu–O–Zr Sites for Highly Selective Production of p ‐xylene from Tandem Upcycling of PET and CO 216Atomic Cu–O–Zr Sites for Highly Selective Production of p ‐xylene from Tandem Upcycling of PET and CO 20Advancements in Catalytic Depolymerization Technologies10Sustainable Closed‐Loop Recycling of Polyester Waste Using Reconstructed Defective‐Metal–Organic Frameworks18Sustainable Closed‐Loop Recycling of Polyester Waste Using Reconstructed Defective‐Metal–Organic Frameworks5Synergistic Catalysis Driven by Solvent Effect: Efficient Glycolysis of Polyethylene Terephthalate (PET) by the Zn(OAc) 2 /DBU-DMSO System15Catalytic Upcycling of PET: From Waste to Chemicals and Degradable Polymers48Catalytic Depolymerization of Polyester Waste via Zinc Oxide‐Decorated Silica3Integrated Conversion of Polyesters, CO 2 , and Glycerol via Ethylene Oxide‐Mediated Tandem Process9Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives11Depolymerization of polyesters catalyzed by binuclear metal complexes0One‐Pot Upcycling of Heterogeneous Polyester Waste to Biodegradable Thermoplastics: A Cost‐Effective Solution for a Circular Economy6Cutting-Edge advances in chemical depolymerization-based recycling of waste polyethylene terephthalate plastics0Photocatalytic Upcycling of Polyethylene Terephthalate via Formate-Mediated Non-Hydrogen Deoxygenative Reduction4Efficient glycolysis of PET waste with Zn-mediated ionic liquid catalyst: Uncovering the mechanism of dimolecular activation and kinetic acceleration8Valorization of waste polyolefins to butene, unsaturated fatty alcohols, and branched alkenes using CO2 and plasma catalyst2Precision bond cleavage in waste plastics: Directed catalytic upcycling1Bimetallic Synergistic Catalysis Enabling Efficient Chemical Recycling of Commercial Polyesters1Low-temperature polyethylene terephthalate upcycling by phenolic ionic liquids6Mechanochemical Recycling of Polyethylene Terephthalate with Monohydrate Barium-Hydroxide0Stepwise Hydrodeoxygenation of Mixed Oxygenated Plastics Enables Sequential Production of Jet- and Gasoline-Range Fuels0Conversion of all polyester units to amines: Ruthenium-catalyzed, acid-assisted hydrogenative amination0Dynamic Self‐Focusing Photothermal Localization Induced Mild Solvent‐Free Upcycling of Polystyrene0Study on Methanolysis of Polyethylene Terephthalate to Dimethyl Terephthalate Over Titanate Nanostructured Materials0Chemical Recycling of Polyester Wastes: Emerging Upcycling Technologies, Fundamental Mechanisms, Process Analysis, and Machine Learning1Air-Oxidizing, Solvent-Free Depolymerization of Plastic Waste to Produce Valuable Chemicals0Enhanced Catalytic Dechlorination of Polyvinyl Chloride (PVC) and H2 Production Enabled by Synergistic Gaδ+/Ga0 Active Sites in Liquid Metal Particles0Continuous-Flow Vapor-Phase Methanolysis in a Fixed-Bed Enables PET Recycling with In Situ Decolorization and Purification0Noncovalent Interaction-Catalyzed High Conversion of Waste PET Plastics into Organic Esters under Mild Conditions0Selective Consecutive Decarboxylation Enables Skeletal Contraction of Waste PET0

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  5. Selective Upcycling of Polyethylene Terephthalate towards High‐valued Oxygenated Chemical Methyl p‐Methyl Benzoate using a Cu/ZrO2 Catalyst

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  6. Chemical Recycling of Polycarbonates via Ammonolysis and Polycaprolactones by KOH‐Catalyzed Methanolysis

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  7. From Polyester Plastics to Diverse Monomers via Low‐Energy Upcycling

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  8. Catalytic Hydroxyethylation of Phenols with Renewable Ethylene Glycol Diester as an Alternative to Ethylene Oxide

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  9. Recent advances in the chemical recycling of polyesters

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  12. Depolymerization mechanisms and closed-loop assessment in polyester waste recycling

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  14. Upconversion Phosphor-Driven Photodegradation of Plastics

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  15. Circular Economy and Chemical Conversion for Polyester Wastes

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  16. Challenges and opportunities in catalytic hydrogenolysis of oxygenated plastics waste: polyesters, polycarbonates, and epoxy resins

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  17. Stabilization of ZnO Catalysts for Polyesters Hydrolytic Depolymerization by Incorporation into ZrO2 Lattice: A Polylactic Acid Case Study

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  18. Advances in heterogeneous catalysts for sustainable PET upcycling: from mechanistic understanding to catalyst design

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  22. One-Pot Conversion of Polyethylene Terephthalate into 1,4-Cyclohexanedicarboxylic Acid without External H2

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  34. Plasma Catalysis for Plastic Waste Conversion into Value‐Added Products: Advancements and Perspectives

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  37. Cutting-Edge advances in chemical depolymerization-based recycling of waste polyethylene terephthalate plastics

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