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RESEARCH PAPER · Macromolecular Rapid Communications · 2022

Polyolefin Innovations toward Circularity and Sustainable Alternatives

Andrea H. Westlie, Eugene Y.‐X. Chen, Chris M. Holland, Shannon S. Stahl, Meredith Doyle, Scott R. Trenor, Katrina M. Knauer

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Polyolefin Innovations toward Circularity and Sustainable AlternativesOriginalPolyolefins Vitrimers: Design Principles and Applications108Catalytic Chemical Recycling of Post-Consumer Polyethylene188Mechanochemical Degradation and Recycling of Synthetic Polymers23Mechanochemical Degradation and Recycling of Synthetic Polymers167Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance63Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance4Polyethylene Incorporating Diels–Alder Comonomers: A “Trojan Horse” Strategy for Chemically Recyclable Polyolefins3Polyethylene Incorporating Diels–Alder Comonomers: A “Trojan Horse” Strategy for Chemically Recyclable Polyolefins87Alkane metathesis over immobilized pincer-ligated iridium complexes: Effect of support nature4Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook204Upcycling of polyethylenes by catalysis0Circular Polyolefins: Advances toward a Sustainable Future76Circular plastics technologies: open loop recycling of waste plastics into new chemicals0Copolymers0Current Advances and Challenges in Chemical Recycling of Polymeric Materials5Identifying methods to reduce emission intensity of centralised Photovoltaic deployment for net zero by 2050: Life cycle assessment case study of a 30 MW PV plant33C–H Functionalization of Polyolefins to Access Reprocessable Polyolefin Thermosets105Recent progress on UV-light barrier food packaging films – a systematic review125Amphiphilic Fibers Based on Polypropylene-G-Poly(Acrylic Acid) by Sequential Photo-Induced Metal-Free Atrp and Electrospinning0Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle106Degradable polyolefins prepared by integration of disulfides into metathesis polymerizations with 3,6-dihydro-1,2-dithiine9Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis19Design of depolymerizable polymers toward a circular economy69Mild aqueous metal catalyzed oxidative conversion of low-density polyethylene to low molecular weight aliphatic carboxylic acids15Ruthenium-catalyzed “open-loop” recycling of polyethylene via tandem isomerization-metathesis (ISOMET)12Sorting polyolefins with near-infrared spectroscopy: identification of optimal data analysis pipelines and machine learning classifiers19Recyclable, Reprocessable, Anticorrosive, and Hydrolysis-Resistant Long-Chain Aliphatic Polycarbonates as Polyethylene-like Materials15Chemically Recyclable Linear and Branched Polyethylenes Synthesized from Stoichiometrically Self-Balanced Telechelic Polyethylenes82Circular olefin copolymers made de novo from ethylene and α-olefins83Synthesis and Deconstruction of Polyethylene-type Materials194Towards effective recycling routes for polypropylene: Influence of a repair additive on flow characteristics and processability30Correlating Near-Infrared Spectra to Bulk Properties in Polyolefins25Plastic Waste Management During and Post COVID‐19 Pandemic: Challenges and Strategies9Topology-Accelerated and Selective Cascade Depolymerization of Architecturally Complex Polyesters19Assessing the circularity of post-consumer HDPE milk bottles through open-loop recycling and their environmental impact27Fabrication of polypropylene-g-poly(acrylic acid) based microfibers by combination of photo-induced metal-free ATRP and electrospinning process11To overcome the unconventional polymerization behavior of single-site symmetrical metallocene catalyst in the presence of borate10Catalytic chemical recycling and upcycling of polyolefin plastics27Ultra-high-molecular weight cyclic olefin copolymers with excellent all-round performance prepared via highly effective quasi-living copolymerization27Noncovalent Interactions in Late Transition Metal-Catalyzed Polymerization of Olefins49Sustainability pathways for perovskite photovoltaics80Synthesis, Characterization, and Application of High-Molecular-Weight Polyethylene-like Polycarbonates: Toward Sustainable and Recyclable Fibers20Untangling the chemical complexity of plastics to improve life cycle outcomes76Catalytic Upcycling of Polyolefins316Analyses of circular solutions for advanced plastics waste recycling88Assessment of Different Application Grades of Post-Consumer Recycled (PCR) Polyolefins from Material Recovery Facilities (MRFs) in the United States13Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties2Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties32Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials14Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials3An electricity-powered future for mixed plastic waste chemical recycling25Research progress and challenges in the upcycling of polyolefin plastics through chemical oxidation4The conformational preference of dynamic crosslinker modulates the ‘closed-loop’ circular economy in polypropylene vitrimer11Depolymerization by transition metal complexes: strategic approaches to convert polymeric waste into feedstocks3Synthesis of butadiene-derived polyolefin graft copolymers and their crystallization behaviors4Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene1Ruthenium‐Catalyzed Deconstruction of Polyolefins: A Strategy to Up‐cycle Waste Polyethylene to Value‐Added Alkene20Circular Polymer Designed by Regulating Entropy: Spiro-Valerolactone-Based Polyesters with High Gas Barriers and Adhesion Strength22A Comprehensive Review on Barrelene-Derived α-Diimine Nickel and Palladium Olefin Polymerization Catalysts5Reactive Processing of Polyethylene with Azidotriazine: From Modified Thermoplastics to Injection Moldable Covalent Adaptable Networks7Catalytic closed-loop recycling of polyethylene-like materials produced by acceptorless dehydrogenative polymerization of bio-derived diols45A Useful Tool to Recycle Mixed Plastics Blends1A straightforward method to record the peak torque value when using a cantilever spring mechanical torque limiting device3Reductive Upcycling of Polyolefins, Polyesters and Mixed Plastic Wastes to Valuable Chemicals: Bridging Chemical Catalysis With Plastic Waste Management35Advanced characterization of 3D printed polyolefin elastomer-carbon black composites: cyclic mechanical behavior, thermophysical properties, and morphological analysis3Industrially Adaptable Way for Upcycling of Mixed i PP and PE via In Situ Compatibilization5Elucidating the enzymatic response of the white rot basidiomycete Abortiporus biennis for the downgrade of polystyrene5Thiol- and Disulfide-Functionalized Polycyclooctene: Metathesis Polymerization, Degradation, and Reformation6Polyethylene Hydrogenolysis over Ru Supported on Mesoporous MFI Zeolite: Effects of Mesoporosity and External Acid Sites16Biopolymers and their nanocomposites coated paper-based high barrier and sustainable food packaging materials56Ethylene-propylene block copolymers featuring dual crystalline networks: high-performance elastomers and sustainable high-density polyethylene/isotactic polypropylene blends upcycling10Investigating the Role of Molecular Structure on the Entanglement Behavior of Lignin-Derivable Polymethacrylates6Enhancing Mechanical Properties and Crystallization Kinetics of Isotactic Polypropylene by Boronic Acid-Cross-Linked Additives3Compatibilization of iPP/PS Blends with Diblock and Triblock Copolymers4Main-Chain Ketone Installation in Polyethylene Chains: A Metal-Free Strategy toward Photodegradable Plastics18Next‐Generation Sustainable Polyolefin Packaging Manufactured Using Flow‐Induced Crystallization0Chemoselective Sequential Polymerization: An Approach Toward Mixed Plastic Waste Recycling0Research progress on compatibilizers for physical blending recycling of polyolefins0Flame Retardant Polyolefins Using Fibers From Leather Waste: Adjusting Extrusion Variables to Balance the Property Profile2Thermodynamically driven closed-loop recyclable bridged polymers: from molecular design to high-performance materials0Fluorescently labelled polypropylene as a model microplastic for cellular imaging0Modifying Mechanical Performance of an LLDPE / PP Waste Blend During a Single Recycling Cycle Using Organometallic Complexes0Predicting Properties from Near-Infrared Spectra with Machine Learning for Improved Polyolefin Differentiation4Designing Resource-Efficient Polypropylene-Based Elastomers via Moderately Selective Catalyst for Toughening and Compatibilization0Unexpected Ductility Enhancement in Crystalline–Crystalline Polyolefin Diblock Copolymers without Introducing Soft Segments0Hot-Pressed Multicomponent Recycled Textile Polymer Blends Reinforced with Ground GFRP from Wind Turbine Blades: Microstructure–Property Relationships0True-to-life microplastics obtained from PP pasta bags for efficient removal of pharmaceutical contaminants in aqueous systems2Chemical recycling via precision depolymerization: fundamentals, design principles, and emerging frontiers for circular polymer systems3Photo-Oxidative Stability of Recycled Polypropylene: Effect of a Repair Additive on Degradation and Mechanical Retention0A Kinetic Model-Driven Techno-Economic Analysis of Plastic Pyrolysis: Linking Process Dynamics to Economic Viability2Electrospun chlorinated polypropylene microfibers modified with epoxidized soybean oil and gallic acid: morphological, thermal, and antioxidant characterization7Direct synthesis of non-migratory, intrinsically antioxidant ultra-high molecular weight polyethylene by nickel catalysis0Enabling Refinery Integration for Plastic Waste Recycling: A Probabilistic Techno-economic Analysis and Carbon Footprint Assessment of Poly-Crude Production0Masterbatch-enabled acceleration of polyolefin biodegradation under open air terrestrial environmental conditions0Bio‐Derived Phytic Acid‐Based Organic‐Inorganic Hybrid Coating for Flame‐Retardant and Thermally Stable Separators for Lithium‐Ion Batteries0

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  1. Polyolefins Vitrimers: Design Principles and Applications

    Chemistry of Materials · 2022-11-21

    Mostafa Ahmadi, Ahad Hanifpour, Sina Ghiassinejad, Evelyne van Ruymbeke

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  2. Catalytic Chemical Recycling of Post-Consumer Polyethylene

    Journal of the American Chemical Society · 2022-12-16

    Alejandra Arroyave, Shilin Cui, Jaqueline C. Lopez, Andrew L. Kocen, Anne M. LaPointe, Massimiliano Delferro, Geoffrey W. Coates

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  3. Mechanochemical Degradation and Recycling of Synthetic Polymers

    Angewandte Chemie · 2023-04-01

    Junfeng Zhou, Tze‐Gang Hsu, Junpeng Wang

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  4. Mechanochemical Degradation and Recycling of Synthetic Polymers

    Angewandte Chemie International Edition · 2023-04-01

    Junfeng Zhou, Tze‐Gang Hsu, Junpeng Wang

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  5. Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance

    Angewandte Chemie International Edition · 2023-04-18

    Changxia Shi, Liam T. Reilly, Eugene Y.‐X. Chen

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  6. Hybrid Monomer Design Synergizing Property Trade‐offs in Developing Polymers for Circularity and Performance

    Angewandte Chemie · 2023-04-19

    Changxia Shi, Liam T. Reilly, Eugene Y.‐X. Chen

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  7. Polyethylene Incorporating Diels–Alder Comonomers: A “Trojan Horse” Strategy for Chemically Recyclable Polyolefins

    Angewandte Chemie · 2023-05-10

    Sarah M. Parke, Jaqueline C. Lopez, Shilin Cui, Anne M. LaPointe, Geoffrey W. Coates

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  8. Polyethylene Incorporating Diels–Alder Comonomers: A “Trojan Horse” Strategy for Chemically Recyclable Polyolefins

    Angewandte Chemie International Edition · 2023-05-10

    Sarah M. Parke, Jaqueline C. Lopez, Shilin Cui, Anne M. LaPointe, Geoffrey W. Coates

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  9. Alkane metathesis over immobilized pincer-ligated iridium complexes: Effect of support nature

    Applied Catalysis B: Environmental · 2023-06-19

    Cristina Megías‐Sayago, Ignacio Centeno-Vega, Luis Francisco Bobadilla, Svetlana Ivanova, Nuria Rendón, Andrés Suárez

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  10. Sustainable developments in polyolefin chemistry: Progress, challenges, and outlook

    Progress in Polymer Science · 2023-06-25

    Xiaoyan Wang, Yanshan Gao, Yong Jin Tang

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  11. Upcycling of polyethylenes by catalysis

    Unknown journal · 2023-07-20

    Adamu Aminu Idris

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  12. Circular Polyolefins: Advances toward a Sustainable Future

    Macromolecules · 2023-07-21

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  13. Circular plastics technologies: open loop recycling of waste plastics into new chemicals

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  14. Copolymers

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  15. Current Advances and Challenges in Chemical Recycling of Polymeric Materials

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  16. Identifying methods to reduce emission intensity of centralised Photovoltaic deployment for net zero by 2050: Life cycle assessment case study of a 30 MW PV plant

    Progress in Photovoltaics Research and Applications · 2023-10-19

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  17. C–H Functionalization of Polyolefins to Access Reprocessable Polyolefin Thermosets

    Journal of the American Chemical Society · 2023-12-11

    Eliza K. Neidhart, Mutian Hua, Zhengxing Peng, Logan T. Kearney, Vittal Bhat, Foad Vashahi, Erik J. Alexanian, Sergei S. Sheiko, Cheng Wang, Brett A. Helms, Frank A. Leibfarth

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  18. Recent progress on UV-light barrier food packaging films – a systematic review

    Innovative Food Science & Emerging Technologies · 2023-12-19

    Swarup Roy, Rejish Ramakrishnan, Gülden Gökşen, Sunita Singh, Łukasz Łopusiewicz

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  19. Amphiphilic Fibers Based on Polypropylene-G-Poly(Acrylic Acid) by Sequential Photo-Induced Metal-Free Atrp and Electrospinning

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  20. Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle

    Chemical Society Reviews · 2024-01-01

    Shuaiqi Yang, Shuai Du, Jin Zhu, Songqi Ma

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  21. Degradable polyolefins prepared by integration of disulfides into metathesis polymerizations with 3,6-dihydro-1,2-dithiine

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    Hong-Gyu Seong, Thomas P. Russell, Todd S. Emrick

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  22. Depolymerization of waste polyethylene to linear alkenes via sequential dehydrogenation and metathesis

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    Kishor V. Khopade, Nikhita S. Rajput, Raghavendrakumar Rangappa, Nagaraju Barsu, Samir H. Chikkali

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  23. Design of depolymerizable polymers toward a circular economy

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  24. Mild aqueous metal catalyzed oxidative conversion of low-density polyethylene to low molecular weight aliphatic carboxylic acids

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  25. Ruthenium-catalyzed “open-loop” recycling of polyethylene via tandem isomerization-metathesis (ISOMET)

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  26. Sorting polyolefins with near-infrared spectroscopy: identification of optimal data analysis pipelines and machine learning classifiers

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  27. Recyclable, Reprocessable, Anticorrosive, and Hydrolysis-Resistant Long-Chain Aliphatic Polycarbonates as Polyethylene-like Materials

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  28. Chemically Recyclable Linear and Branched Polyethylenes Synthesized from Stoichiometrically Self-Balanced Telechelic Polyethylenes

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  29. Circular olefin copolymers made de novo from ethylene and α-olefins

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  30. Synthesis and Deconstruction of Polyethylene-type Materials

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  31. Towards effective recycling routes for polypropylene: Influence of a repair additive on flow characteristics and processability

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  32. Correlating Near-Infrared Spectra to Bulk Properties in Polyolefins

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  33. Plastic Waste Management During and Post COVID‐19 Pandemic: Challenges and Strategies

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  34. Topology-Accelerated and Selective Cascade Depolymerization of Architecturally Complex Polyesters

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  35. Assessing the circularity of post-consumer HDPE milk bottles through open-loop recycling and their environmental impact

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  36. Fabrication of polypropylene-g-poly(acrylic acid) based microfibers by combination of photo-induced metal-free ATRP and electrospinning process

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  37. To overcome the unconventional polymerization behavior of single-site symmetrical metallocene catalyst in the presence of borate

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  38. Catalytic chemical recycling and upcycling of polyolefin plastics

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  39. Ultra-high-molecular weight cyclic olefin copolymers with excellent all-round performance prepared via highly effective quasi-living copolymerization

    Chemical Engineering Journal · 2024-06-17

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  40. Noncovalent Interactions in Late Transition Metal-Catalyzed Polymerization of Olefins

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  41. Sustainability pathways for perovskite photovoltaics

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  42. Synthesis, Characterization, and Application of High-Molecular-Weight Polyethylene-like Polycarbonates: Toward Sustainable and Recyclable Fibers

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  43. Untangling the chemical complexity of plastics to improve life cycle outcomes

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  44. Catalytic Upcycling of Polyolefins

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  45. Analyses of circular solutions for advanced plastics waste recycling

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  46. Assessment of Different Application Grades of Post-Consumer Recycled (PCR) Polyolefins from Material Recovery Facilities (MRFs) in the United States

    ACS Applied Polymer Materials · 2024-10-19

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  47. Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties

    Angewandte Chemie · 2024-10-29

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  48. Photooxidation of Polyolefins to Produce Materials with In‐Chain Ketones and Improved Materials Properties

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  49. Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials

    Angewandte Chemie International Edition · 2024-10-30

    Saeed Ataie, Amir Malmir, Sabrina S. Scott, James T. Goettel, Steven N. Clemens, Darryl J. Morrison, Cyrus Mackie, Belinda Heyne, Savvas George Hatzikiriakos, Laurel L. Schafer

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  50. Hydroaminoalkylation for Amine Functionalization of Vinyl‐Terminated Polyethylene Enables Direct Access to Responsive Functional Materials

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