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RESEARCH PAPER · Chemical Society Reviews · 2024

Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycle

Shuaiqi Yang, Shuai Du, Jin Zhu, Songqi Ma

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Closed-loop recyclable polymers: from monomer and polymer design to the polymerization–depolymerization cycleOriginalDirect Monomer Recovery from Ring-Closing Depolymerization of Thermosets17Chemically recyclable poly(thioether-thioester)s via ring-opening polymerization of seven-membered thiolactones4Hydrogenative Depolymerization of Polyesters Catalyzed by a PN3-Ruthenium Complex Using Both H2 and EtOH as Hydrogen Sources0Implementing a sulfur-substitution approach toward a high-performance recyclable polythioester9Reticular framework materials as versatile platforms for controllable polymer synthesis22Ring-opening Polymerization of Benzo-fused Caprolactone and its Copolymerization with Epoxides0Solvent-induced microstructure disruption and catalytic activation synergy toward mild and rapid degradation of epoxy thermosets4Upcycling of polymer waste to closed-loop recyclable polymers5Recent Advances in the Chemical Recycling of Polyamide for a Sustainable Circular Economy29Linear and Network-Forming Acetal Polymerization of Multifunctional Alcohols with Dichloromethane for Degradable and Recyclable Materials7Structure–Property Relationships of Elastomeric Vinylogous Urethane Thermosets and Their Application as Closed-Loop Recyclable Strain Sensors23Next-generation solar energy: Progress, stability, and prospects of polymer-modified Perovskite solar cells; A review39Ultratough Thermoplastic Elastomers Based on Chemically Recyclable Cycloalkyl-Substituted Polyhydroxyalkanoates30Synergetic “amine scissors” break down cured epoxy resins with nearly 100% degradation efficiency19Clusterization-triggered room-temperature phosphorescent synthetic polymeric materials18Viscoelastic Supramolecular Networks Based on Guanidinium‐Oxyanion Interactions0Modular Access to Aliphatic Polycarbonates with Tunable Properties and Dual Closed‐Loop Recyclability by Polycondensation–Depolymerization–Repolymerization Strategy2Modular Access to Aliphatic Polycarbonates with Tunable Properties and Dual Closed‐Loop Recyclability by Polycondensation–Depolymerization–Repolymerization Strategy13Catalyst‐Free Dynamic Covalent Knoevenagel/Hydrazide Condensation for Polyacylhydrazones and Covalent Adaptable Networks3Catalyst‐Free Dynamic Covalent Knoevenagel/Hydrazide Condensation for Polyacylhydrazones and Covalent Adaptable Networks14Kinetic modeling for radical polymerization and depolymerization9Acid-assisted strategy towards reuse of waste polyimide materials for multi-scenario thermally insulating and high-strength functional applications1A Synergistic Strategy Utilizing Amide Hydrogen Bonding and Naphthalene Conjugation to Develop High-Performance Polyamides5Performance-Guided Design of Chemically Recyclable Polymeric Materials: A Case Study on Thermoplastic Elastomers9Introducing Closed-Loop Chemically Recyclable Polymers in Undergraduate Polymer Chemistry Course2Revolutionizing water treatment: Polymerization pathways in advanced oxidation processes26Production of Polymer Monomers through Integrated Catalytic Approaches3Gem-dimethylation promotes reversible polymerization/deploymerization of thionolactones0Organocatalytic Ring-Opening Polymerization of Methyl-Substituted Glycolides0Upcycling of Polyethylene Terephthalate Waste into Closed-Loop Recyclable Carbon Fiber-Reinforced Polymer Composites with High Performance6Flexible strain sensor based on TPU internal ILs/CB conductive network for SOS emergency rescue1Enabling a Diversity‐Oriented Catalytic Atom Looping of a Biobased Polycarbonate3Stereospecific Hydroxyl–Yne Click Polymerization to Selectively Construct High-Performance Plastics and Elastomers4Mild and metal-free chemical recycling of polyureas via acylation-activated bond cleavage2The photocatalytic synthesis and closed-loop recycling of poly(semi-aromatic 1,2-ethanediol)s1Sulfur-containing sustainable polymers: synthetic pathways, degradation mechanisms, and multifunctional applications16Programmed recycling of triblock copolymers1Supramolecular chemical recycling of dynamic polymers20Semirenewable Polyamides Containing Disulfide Bonds: Synthesis, Degradation, Self-Healing, and Triboelectric Properties6[(Salen*)Co(OAc)] as a robust initiator for the immortal bulk ring-opening (co)polymerization of l -lactide and ε-caprolactone1Recent advances in plastic upcycling enabled by dynamic covalent cross-linking strategies0Synthesis and Upcycling of All‐Carbon‐Backbone Degradable Polyethylene with Dispersed On‐Chain Ketones5Synthesis and Upcycling of All‐Carbon‐Backbone Degradable Polyethylene with Dispersed On‐Chain Ketones0Closed-loop recyclable and flame-retardant coating toward engineered multifunctional electromagnetic shielding2Entropy-driven toughening and closed-loop recycling of polymers via divergent metal-pyrazole interactions9New Biocatalytic Approaches for Plastic Depolymerization3A new paradigm for closed-loop recyclable plastics: the sulfur-substitution strategy0Electrochemical recovery and regeneration of polyethylene terephthalate materials7Chemically recyclable films from thermoplastic ABA-triblock copolymers containing polylactide A-blocks and easily degradable polydioxolane B-block - towards the novel type of sustainable plastics1Sustainable Design of Dynamic Poly(disulfide)s29Closed-Loop and Precision Synthesis of Polymuconates via Organocatalyzed Group Transfer Polymerization0Environmental performance of single-use plastic packaging: A life cycle assessment of end-of-life scenarios in the agri-food sector2Benzo-Fused Monomer Design toward Semiaromatic Polymers for a Circular Plastic Economy13Controlled ring-opening polymerization of xylose-derived lactones towards sustainable polyesters0Converting natural biopolymers to sustainable bioplastics via structure engineering15Designing recyclable inorganic–organic hybrid polymer coatings through integrating silicone-based molecular scission points0Fully bio-based monopyrrolidone-containing monomers towards the synthesis of renewable polyesters with high T g and hydrolyzable closed-loop recycling0Photopolymerizable green composite biomaterials for potential 3D printing applications1Selectively controlled ring-opening copolymerization to chemically recyclable thermoplastic elastomers1Substituent engineering of dynamic covalent bonds enables simultaneous enhancement of performance and recyclability1α-Lipoic acid: from a mitochondrial cofactor to a versatile platform for dynamic biomaterials and translational biomedicine0Depolymerization of Vinyl Polymers18Rapid Chemical Recycling of Eugenol-Derived Epoxy Thermosets via Cleavable Silyl Ether Linkages with High Chemical Recovery1On-demand underwater adhesion and self-healing superhydrophilic/underwater superoleophobic coating1Recyclable Self‐Healing Polymer Materials With Enhanced Mechanical Properties1A Biobased Bicyclic Monomer toward Poly(butylene terephthalate) Copolyesters with Dual Closed-Loop Recyclability and Improved Performance0Fluorinated dynamic imine-based porous materials with excellent hydrophobicity and closed-loop recycling2High-Performance, Closed-Loop Recyclable Polyimine Elastomers Based on Covalent Adaptive Networks for Polyimine/Carbon Fiber Elastomeric Composites6Thermodynamics, Closed-Loop Recycling, and Marine Degradation of Poly(alkylene oxalate)s Synthesized through Ring-Opening Polymerization3Hierarchical Dynamic Network Reconfiguration for Co-Rrecycling of Mixed Biodegradable Polyesters0Unveiling the Electrochemical Reactivity of Urethane Toward Different Bond Formations and Application to Polyurethane Deconstruction via C─N Bond Formation3Unveiling the Electrochemical Reactivity of Urethane Toward Different Bond Formations and Application to Polyurethane Deconstruction via C─N Bond Formation0A Multifunctional Tetracyclic Monomer toward Bio-Based Polyesters with Excellent Performance and Facile Chemical Closed-Loop Recycling3Dual-Pathway Strategy for Click-Type Functionalization and Programmable Polymer Deconstruction10Selective Synthesis and Polymerization of Methyl-1,4-dioxan-2-one toward Closed-Loop Recyclable Poly(ether- alt -ester) from Methyl Glycolate and Propylene Oxide2All-Hydrocarbon Polymers with Chemical Recyclability via a Catalyst-Free and Solvent-Free Method1Depolymerization and Reuse of Polycarbonates: Emerging Classes, Mechanisms and Challenges5Lattice distortion-induced eg* band broadening of a nickel-based electrocatalyst for boosting electrocatalytic PBS plastic upcycling1Depolymerization and Reuse of Polycarbonates: Emerging Classes, Mechanisms and Challenges1Synthesis and reversible photoisomerization of Thiol-yne-Derived Poly(vinyl thioether ester)s0Chemically Recyclable Polymers: Tunable Performance Enabled by Precision Ring-Opening (Co)polymerization1High‐Performance Recycling Biobased Photopolymers for 3D Printing2The mechanism of reactions of diphenyl carbonate with methylamine under the action of acid-base and metal-containing catalysts0A hierarchical dynamic network enables closed-loop recyclable solid-solid phase change materials with high toughness and infrared stealth capability1Closed-loop recycling of disulfide-based vitrimers enabled by ambient-temperature depolymerization2Closed-Loop Chemical Recycling of Poly(butylene succinate) Using Organocatalysts0Tailoring electronic delocalization via fluorinated hyperbranched polysiloxane for colorless, transparent, and degradable cyanate ester resin1One-Step Fabrication of a PEDOT:PSS-Integrated Stretchable, Elastic, and Adhesive Conductive Hydrogel for Wearable Soft Sensors0A mechanistic understanding of how weak links enhance polymer recyclability uncovers emergent doping strategy3Intramolecularly Synergic Catalysis Enables Efficient Closed‐Loop Recycling of Polyesters and Polycarbonates0Intramolecularly Synergic Catalysis Enables Efficient Closed‐Loop Recycling of Polyesters and Polycarbonates0Li–Ti–P–Si hybrid char networks in lithium titanate reinforced intumescent epoxy coatings for enhanced fire protection0Dynamic Polymers Based on Coordination Bonds0In-situ polymerization-induced thixotropy of cement paste under shear histories: A theoretical model0Well-defined polymer electrolytes via controlled polymerizations0Liquid Metal‐Based Bifunctional Catalysis: Bridging Lactone Polymerization, Polyester Recycling, and Sustainable Flexible Electronics0Green Production of Para ‐Dioxanone for Sustainable Polymers0Covalent Organic Framework Mediated Polymerization for Multifunctional Applications0Covalent Organic Framework Mediated Polymerization for Multifunctional Applications0Closed‐Loop Recyclable Solid Polymer Electrolytes via Dynamic Lipoate Cross‐Linking1Closed‐Loop Recyclable Solid Polymer Electrolytes via Dynamic Lipoate Cross‐Linking1Initiator-Free In Situ Photocuration for Constructing Degradable and Closed-Loop Recyclable Poly(disulfide)s from Renewable Biomass0Nonpolar Polysiloxane with 100% Self-Healability, Closed-Loop Recyclability, and Antifouling0Strong, Hydrophobic, and Recyclable Materials Enabled by Nacre‐Like Multiple Interactions0From mechanism to practice: Structure-activity relationships and engineering feasibility of metal-free carbon materials for pollutant polymerization in low-carbon water treatment0Controlled Ring-Opening Polymerization of 5-Phenyl-1,4-dioxan-2-one toward Stereochemically Tunable and Closed-Loop Recyclable Polyesters0

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  1. Direct Monomer Recovery from Ring-Closing Depolymerization of Thermosets

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