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RESEARCH PAPER · Angewandte Chemie · 2008

Soluble Direct‐Band‐Gap Semiconductors LiAsS2 and NaAsS2: Large Electronic Structure Effects from Weak As⋅⋅⋅S Interactions and Strong Nonlinear Optical Response

Tarun Kumar Bera, Jung‐Hwan Song, Arthur J Freeman, Joon Ik Jang, John B. Ketterson, Mercouri G. Kanatzidis

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Soluble Direct‐Band‐Gap Semiconductors LiAsS2 and NaAsS2: Large Electronic Structure Effects from Weak As⋅⋅⋅S Interactions and Strong Nonlinear Optical ResponseOriginalStrong Second Harmonic Generation from the Tantalum Thioarsenates A3Ta2AsS11 (A = K and Rb)265Helical and linear [K(As11)]2− chains: Role of solvent on the conformation of chains formed by Zintl anions13Solution Processing of Chalcogenide Semiconductors via Dimensional Reduction239Soluble Semiconductors AAsSe2 (A = Li, Na) with a Direct-Band-Gap and Strong Second Harmonic Generation: A Combined Experimental and Theoretical Study241A Series of Novel Organically Templated Germanium Antimony Sulfides42(Ag2TeS3)2·A2S6 (A = Rb, Cs): Layers of Silver Thiotellurite Intergrown with Alkali-Metal Polysulfides28[Ni(en)3][InSbS4]: A One‐Dimensional Polymeric Indium Thioantimonate with a Polar Structure25Rb4Sn5P4Se20: A Semimetallic Selenophosphate23Rb4Sn5P4Se20: A Semimetallic Selenophosphate1NaSr3Be3B3O9F4: A Promising Deep‐Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F]10− Anionic Group369NaSr3Be3B3O9F4: A Promising Deep‐Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F]10− Anionic Group67Strongly Nonlinear Optical Chalcogenide Thin Films of APSe6 (A=K, Rb) from Spin‐Coating51Strongly Nonlinear Optical Chalcogenide Thin Films of APSe6 (A=K, Rb) from Spin‐Coating8Understanding Fluxes as Media for Directed Synthesis: In Situ Local Structure of Molten Potassium Polysulfides57On the Complexity of Crystallization of Thioantimonates: In‐situ Energy Dispersive X‐ray Diffraction (EDXRD) Studies of the Solvothermal Formation of the Isostructural Thioantimonates [TM(tren)Sb4S7] (TM = Fe, Zn)16Cs2B4SiO9: A Deep‐Ultraviolet Nonlinear Optical Crystal278Cs2B4SiO9: A Deep‐Ultraviolet Nonlinear Optical Crystal224Heterometallic Clusters [CuSn3S9]5− and [Cu6Sn6S20]10−: Solvothermal Synthesis and Characterization of 4f–3d Thiostannates26Noncentrosymmetric Cubic CsCdBO3 with Bichromophore23Exploring the influence of cationic skeletons on the arrangement of isolated BO 3 groups based on RbMgBO 3 , CsZn 4 (BO 3 ) 3 and Cs 4 Mg 4 (BO 3 ) 422Pr 3 S 2 Cl 2 [AsS 3 ]: A Praseodymium(III) Sulfide Chloride Thioarsenate(III) with Double Chains of Condensed [SPr 4 ] 10+ Tetrahedra9Tailored Synthesis of a Nonlinear Optical Phosphate with a Short Absorption Edge241Tailored Synthesis of a Nonlinear Optical Phosphate with a Short Absorption Edge60Na 2 BaMQ 4 (M=Ge, Sn; Q=S, Se): Infrared Nonlinear Optical Materials with Excellent Performances and that Undergo Structural Transformations202Na2BaMQ4 (M=Ge, Sn; Q=S, Se): Infrared Nonlinear Optical Materials with Excellent Performances and that Undergo Structural Transformations44Facile Hydrazine‐Hydrothermal Syntheses and Characterizations of Two Quaternary Thioarsenates(III): Two‐Dimensional SrAg4As2S6⋅2 H2O and One‐Dimensional BaAgAsS320Pb2BO3Cl: A Tailor‐Made Polar Lead Borate Chloride with Very Strong Second Harmonic Generation382Pb2BO3Cl: A Tailor‐Made Polar Lead Borate Chloride with Very Strong Second Harmonic Generation129MgSiAs: An Unexplored System with Promising Nonlinear Optical Properties53Sr 6 Cd 2 Sb 6 O 7 S 10 : Strong SHG Response Activated by Highly Polarizable Sb/O/S Groups124Sr6Cd2Sb6O7S10: Strong SHG Response Activated by Highly Polarizable Sb/O/S Groups22Large nonlinear optical effect in tungsten bronze structures via Li/Na cross-substitutions4

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  1. Strong Second Harmonic Generation from the Tantalum Thioarsenates A3Ta2AsS11 (A = K and Rb)

    Journal of the American Chemical Society · 2008-12-17

    Tarun Kumar Bera, Joon Ik Jang, John B. Ketterson, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  2. Helical and linear [K(As11)]2− chains: Role of solvent on the conformation of chains formed by Zintl anions

    Chemical Physics Letters · 2009-04-03

    Arthur C. Reber, Angel Ugrinov, Ayusman Sen, Meichun Qian, S. N. Khanna

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  3. Solution Processing of Chalcogenide Semiconductors via Dimensional Reduction

    Advanced Materials · 2009-04-21

    David B. Mitzi

    Read original paper ↗ ·

  4. Soluble Semiconductors AAsSe2 (A = Li, Na) with a Direct-Band-Gap and Strong Second Harmonic Generation: A Combined Experimental and Theoretical Study

    Journal of the American Chemical Society · 2010-02-19

    Tarun K. Bera, Joon Ik Jang, Jung-Hwan Song, Christos D. Malliakas, Arthur J Freeman, John B. Ketterson, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  5. A Series of Novel Organically Templated Germanium Antimony Sulfides

    Chemistry - An Asian Journal · 2010-06-10

    Mei‐Ling Feng, Wei‐Wei Xiong, Dong Ye, Jian‐Rong Li, Xiao‐Ying Huang

    Read original paper ↗ ·

  6. (Ag2TeS3)2·A2S6 (A = Rb, Cs): Layers of Silver Thiotellurite Intergrown with Alkali-Metal Polysulfides

    Inorganic Chemistry · 2010-09-22

    Sandy L. Nguyen, Joon Ik Jang, John B. Ketterson, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  7. [Ni(en)3][InSbS4]: A One‐Dimensional Polymeric Indium Thioantimonate with a Polar Structure

    European Journal of Inorganic Chemistry · 2011-05-19

    Mei‐Ling Feng, Pei‐Xin Li, Ke‐Zhao Du, Xiao‐Ying Huang

    Read original paper ↗ ·

  8. Rb4Sn5P4Se20: A Semimetallic Selenophosphate

    Angewandte Chemie International Edition · 2011-08-02

    In Jae Chung, Kanishka Biswas, Jung‐Hwan Song, John Androulakis, Konstantinos Chondroudis, Konstantinos Paraskevopoulos, Arthur J Freeman, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  9. Rb4Sn5P4Se20: A Semimetallic Selenophosphate

    Angewandte Chemie · 2011-08-02

    In Jae Chung, Kanishka Biswas, Jung‐Hwan Song, John Androulakis, Konstantinos Chondroudis, Konstantinos Paraskevopoulos, Arthur J Freeman, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  10. NaSr3Be3B3O9F4: A Promising Deep‐Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F]10− Anionic Group

    Angewandte Chemie International Edition · 2011-08-24

    Hongwei Huang, Jiyong Yao, Zheshuai Lin, Xiaoyang Wang, Ran He, Wenjiao Yao, Naixia Zhai, Chuangtian Chen

    Read original paper ↗ ·

  11. NaSr3Be3B3O9F4: A Promising Deep‐Ultraviolet Nonlinear Optical Material Resulting from the Cooperative Alignment of the [Be3B3O12F]10− Anionic Group

    Angewandte Chemie · 2011-08-24

    Hongwei Huang, Jiyong Yao, Zheshuai Lin, Xiaoyang Wang, Ran He, Wenjiao Yao, Naixia Zhai, Chuangtian Chen

    Read original paper ↗ ·

  12. Strongly Nonlinear Optical Chalcogenide Thin Films of APSe6 (A=K, Rb) from Spin‐Coating

    Angewandte Chemie International Edition · 2011-09-20

    In Jae Chung, Myung‐Gil Kim, Joon Ik Jang, Jiaqing He, John B. Ketterson, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  13. Strongly Nonlinear Optical Chalcogenide Thin Films of APSe6 (A=K, Rb) from Spin‐Coating

    Angewandte Chemie · 2011-09-20

    In Jae Chung, Myung‐Gil Kim, Joon Ik Jang, Jiaqing He, John B. Ketterson, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  14. Understanding Fluxes as Media for Directed Synthesis: In Situ Local Structure of Molten Potassium Polysulfides

    Journal of the American Chemical Society · 2012-05-14

    Daniel P. Shoemaker, Duck Young Chung, John F. Mitchell, Travis H. Bray, L. Soderholm, Peter J. Chupas, Mercouri G. Kanatzidis

    Read original paper ↗ ·

  15. On the Complexity of Crystallization of Thioantimonates: In‐situ Energy Dispersive X‐ray Diffraction (EDXRD) Studies of the Solvothermal Formation of the Isostructural Thioantimonates [TM(tren)Sb4S7] (TM = Fe, Zn)

    Zeitschrift für anorganische und allgemeine Chemie · 2012-09-26

    Beatrix Seidlhofer, Е. А. Антонова, Jing Wang, Diana Schinkel, Wolfgang Bensch

    Read original paper ↗ ·

  16. Cs2B4SiO9: A Deep‐Ultraviolet Nonlinear Optical Crystal

    Angewandte Chemie International Edition · 2013-02-13

    Hongping Wu, Hao Yu, Shilie Pan, Zhenjun Huang, Zhihua Yang, Xin Su, Kenneth Reinhard Poeppelmeier

    Read original paper ↗ ·

  17. Cs2B4SiO9: A Deep‐Ultraviolet Nonlinear Optical Crystal

    Angewandte Chemie · 2013-02-13

    Hongping Wu, Hongwei Yu, Shilie Pan, Zhenjun Huang, Zhihua Yang, Xin Su, Kenneth Reinhard Poeppelmeier

    Read original paper ↗ ·

  18. Heterometallic Clusters [CuSn3S9]5− and [Cu6Sn6S20]10−: Solvothermal Synthesis and Characterization of 4f–3d Thiostannates

    Chemistry - A European Journal · 2013-04-24

    Ruihong Chen, Fang Wang, Chunying Tang, Yong Zhang, Dingxian Jia

    Read original paper ↗ ·

  19. Noncentrosymmetric Cubic CsCdBO3 with Bichromophore

    European Journal of Inorganic Chemistry · 2013-10-02

    Hongwei Yu, Hongping Wu, Shilie Pan, Bingbing Zhang, Ming Wen, Zhihua Yang, Hongyi Li, Xiangzhan Jiang

    Read original paper ↗ ·

  20. Exploring the influence of cationic skeletons on the arrangement of isolated BO 3 groups based on RbMgBO 3 , CsZn 4 (BO 3 ) 3 and Cs 4 Mg 4 (BO 3 ) 4

    New Journal of Chemistry · 2014-01-01

    Zheng Wang, Min Zhang, Shilie Pan, Zhihua Yang, Hui Zhang, Bingbing Zhang, Ying Wang, Jing Kang, Xiaoxia Nina Lin

    Read original paper ↗ ·

  21. Pr 3 S 2 Cl 2 [AsS 3 ]: A Praseodymium(III) Sulfide Chloride Thioarsenate(III) with Double Chains of Condensed [SPr 4 ] 10+ Tetrahedra

    Zeitschrift für anorganische und allgemeine Chemie · 2015-01-26

    Dong‐Hee Kang, Florian Ledderboge, Holger Kleinke, Thomas Schleid

    Read original paper ↗ ·

  22. Tailored Synthesis of a Nonlinear Optical Phosphate with a Short Absorption Edge

    Angewandte Chemie International Edition · 2015-02-09

    Sangen Zhao, Pifu Gong, Siyang Luo, Lei Bai, Zheshuai Lin, Yuan‐Yuan Tang, Yuelan Zhou, Maochun Hong, Junhua Luo

    Read original paper ↗ ·

  23. Tailored Synthesis of a Nonlinear Optical Phosphate with a Short Absorption Edge

    Angewandte Chemie · 2015-02-09

    Sangen Zhao, Pifu Gong, Siyang Luo, Lei Bai, Zheshuai Lin, Yuan‐Yuan Tang, Yuelan Zhou, Maochun Hong, Junhua Luo

    Read original paper ↗ ·

  24. Na 2 BaMQ 4 (M=Ge, Sn; Q=S, Se): Infrared Nonlinear Optical Materials with Excellent Performances and that Undergo Structural Transformations

    Angewandte Chemie International Edition · 2016-04-21

    Kui Wu, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  25. Na2BaMQ4 (M=Ge, Sn; Q=S, Se): Infrared Nonlinear Optical Materials with Excellent Performances and that Undergo Structural Transformations

    Angewandte Chemie · 2016-04-21

    Kui Wu, Zhihua Yang, Shilie Pan

    Read original paper ↗ ·

  26. Facile Hydrazine‐Hydrothermal Syntheses and Characterizations of Two Quaternary Thioarsenates(III): Two‐Dimensional SrAg4As2S6⋅2 H2O and One‐Dimensional BaAgAsS3

    Chemistry - An Asian Journal · 2016-04-28

    Dongming Yan, Chang Liu, Wen‐Xiang Chai, Xuerong Zheng, Luodong Zhang, Mingjia Zhi, Chunmei Zhou, Qichun Zhang, Yi Liu

    Read original paper ↗ ·

  27. Pb2BO3Cl: A Tailor‐Made Polar Lead Borate Chloride with Very Strong Second Harmonic Generation

    Angewandte Chemie International Edition · 2016-08-24

    Guohong Zou, Chensheng Lin, Hongil Jo, Gnu Nam, Tae‐Soo You, Kang Min Ok

    Read original paper ↗ ·

  28. Pb2BO3Cl: A Tailor‐Made Polar Lead Borate Chloride with Very Strong Second Harmonic Generation

    Angewandte Chemie · 2016-08-24

    Guohong Zou, Chensheng Lin, Hongil Jo, Gnu Nam, Tae‐Soo You, Kang Min Ok

    Read original paper ↗ ·

  29. MgSiAs: An Unexplored System with Promising Nonlinear Optical Properties

    Advanced Functional Materials · 2018-05-21

    Katherine E. Woo, Jian Wang, Kui Wu, Kathleen Lee, Juli‐Anna Dolyniuk, Shilie Pan, Kirill A. Kovnir

    Read original paper ↗ ·

  30. Sr 6 Cd 2 Sb 6 O 7 S 10 : Strong SHG Response Activated by Highly Polarizable Sb/O/S Groups

    Angewandte Chemie International Edition · 2019-04-15

    Ruiqi Wang, Fei Liang, Fakun Wang, Yangwu Guo, Xian Zhang, Yi Xiao, Kejun Bu, Zheshuai Lin, Jiyong Yao, Tianyou Zhai, Fuqiang Huang

    Read original paper ↗ ·

  31. Sr6Cd2Sb6O7S10: Strong SHG Response Activated by Highly Polarizable Sb/O/S Groups

    Angewandte Chemie · 2019-04-15

    Ruiqi Wang, Fei Liang, Fakun Wang, Yangwu Guo, Xian Zhang, Yi Xiao, Kejun Bu, Zheshuai Lin, Jiyong Yao, Tianyou Zhai, Fuqiang Huang

    Read original paper ↗ ·

  32. Large nonlinear optical effect in tungsten bronze structures via Li/Na cross-substitutions

    Chemical Communications · 2020-01-01

    Shihang Chu, Kun Lin, Tao Yang, Chengyi Yu, Yili Cao, Yujuan Zhang, Yujiao Sun, Zerui Li, Xingxing Jiang, Zheshuai Lin, Qiang Li, Jun Chen, Kenichi Kato, Hui Wu, Qingzhen Huang, Xianran Xing

    Read original paper ↗ ·
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