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RESEARCH PAPER · Inorganic Chemistry · 2020

Sr5Ga8O3S14: A Nonlinear Optical Oxysulfide with Melilite-Derived Structure and Wide Band Gap

Ruiqi Wang, Yangwu Guo, Xian Zhang, Yi Xiao, Jiyong Yao, Fuqiang Huang

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Sr5Ga8O3S14: A Nonlinear Optical Oxysulfide with Melilite-Derived Structure and Wide Band GapOriginalTwo Mixed-Anion Units of [GeOSe3] and [GeO3S] Originating from Partial Isovalent Anion Substitution and Inducing Moderate Second Harmonic Generation Response and Large Birefringence55A series of oxysulfides RE 2 M 2 S 3 O 4 (RE = Y, Tm; M = Zr, Hf) featuring a unique MS 3 O 4 motif and {[M 2 S 3 O 4 ] 8− } ∞ wrinkle layer13Recent progress in oxychalcogenides as IR nonlinear optical materials79Comparative study on the morphology, growth mechanism and luminescence property of RE2O2S:Eu3+ (RE = Lu, Gd, Y) phosphors23Structural Transformation and Second-Harmonic-Generation Activity in Rare-Earth and d0 Transition-Metal Oxysulfides RE3NbS3O4 (RE = Ce, Sm, Gd, Dy)38Highly polarized [GeOTe 3 ] motif-driven structural order promotion and an enhanced second harmonic generation response in the new nonlinear optical oxytelluride Ba 3 Ge 2 O 4 Te 334Complex coordinated functional groups: A great genes for nonlinear optical materials64Rational Crystal Structure Design and Nonlinear-Optical Properties of Noncentrosymmetric RbCu2NbS47Bridging oxygen atoms in trigonal prism units driven strong second-harmonic-generation efficiency in Sr 3 Ge 2 O 4 Te 318From oxides to oxysulfides: the mixed-anion GeS 3 O unit induces huge improvement in the nonlinear optical effect and optical anisotropy for potential nonlinear optical materials19Infrared nonlinear optical sulfide CsCd 4 In 5 S 12 exhibiting large second harmonic generation response16Rational design of a promising oxychalcogenide infrared nonlinear optical crystal60Structural dimension modulation in a new oxysulfide system of Ae 2 Sb 2 O 2 S 3 (Ae = Ca and Ba)4Synthesis, structural evolution and optical properties of a new family of oxychalcogenides [Sr 3 VO 4 ][MQ 3 ] (M = Ga, In, Q = S, Se)10Review of Heteroleptic Tetrahedra as Birefringent or Nonlinear Optical Motifs17Pb 4 SeBr 6 : A Congruently Melting Mid‐Infrared Nonlinear Optical Material with Excellent Comprehensive Performance39Sr3[SnOSe3][CO3]: A Heteroanionic Nonlinear Optical Material Containing Planar π‐conjugated [CO3] and Heteroleptic [SnOSe3] Anionic Groups78Sr3[SnOSe3][CO3]: A Heteroanionic Nonlinear Optical Material Containing Planar π‐conjugated [CO3] and Heteroleptic [SnOSe3] Anionic Groups7Heteroanionic Melilite Oxysulfide: A Promising Infrared Nonlinear Optical Candidate with a Strong Second-Harmonic Generation Response, Sufficient Birefringence, and Wide Bandgap65Improved Polarization in the Sr6Cd2Sb6O7Se10 Oxyselenide through Design of Lateral Sublattices for Efficient Photoelectric Conversion4Improved Polarization in the Sr6Cd2Sb6O7Se10 Oxyselenide through Design of Lateral Sublattices for Efficient Photoelectric Conversion16First Investigation of Nonlinear Optical Oxychalcogenide with Three‐Dimensional Anionic Framework and Special Windmill‐Like Functional Motifs †28[Ba2F2][Ge2O3S2]: An Unprecedented Heteroanionic Infrared Nonlinear Optical Material Containing Three Typical Anions47Mixed-Anion-Oriented Design of LnMGa3S6O (Ln = La, Pr, and Nd; M = Ca and Sr) Nonlinear Optical Oxysulfides with Targeted Property Balance56Recent developments on Bi-based oxychalcogenide materials with thermoelectric and optoelectronic applications: an overview33[Cs6Cl][Ga5GeQ12] (Q = S, Se): two novel porous layered chalcohalides exhibiting two-band emission and ion exchange properties6Oxychalcogenides as Promising Ultraviolet Nonlinear Optical Candidates: Experimental and Theoretical Studies of AEGeOS2(AE = Sr and Ba)24The Antiperovskite‐Type Oxychalcogenides Ae3Q[GeOQ3] (Ae = Ba, Sr; Q = S, Se) with Large Second Harmonic Generation Responses and Wide Band Gaps68Ba5Ga2SiO4S6: a Phase-Matching Nonlinear Optical Oxychalcogenide Design via Structural Regulation Originated from Heteroanion Introduction25Oxychalcogenides: A Promising Class of Materials for Nonlinear Optical Crystals with Mixed‐Anion Groups35Anisotropic structure building unit involving diverse chemical bonds: a new opportunity for high-performance second-order NLO materials181Comprehensive review on multiple mixed-anion ligands, physicochemical performances and application prospects in metal oxysulfides32Recent progress of newly developed functional building units and corresponding nonlinear optical materials14Zn 2 HgP 2 S 8 : A Wide Bandgap Hg‐Based Infrared Nonlinear Optical Material with Large Second‐Harmonic Generation Response75Heteroanionic LaBrVIO4 (VI = Mo, W): Excellence in Both Nonlinear Optical Properties and Photoluminescent Properties11Chiral and Polar Duality Design of Heteroanionic Compounds: Sr18Ge9O5S31 Based on [Sr3OGeS3]2+ and [Sr3SGeS3]2+ Groups20Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics7Heteroanionic [VO x S 4− x ] groups: tetrahedral units with large birefringence for mid-infrared nonlinear optical crystals9First-principles screening of metal–organic frameworks for entangled photon pair generation5Sr2HgGe2OS6: A Hg-Based Oxychalcogenide Infrared Nonlinear Optical Material Exhibiting Favorable Balance between a Large Band Gap and Strong Second Harmonic Generation Response10Ae3[TO3][SnOQ3] (Ae = Sr, Ba; T = Si, Ge; Q = S, Se) and Ba3[CO3][MQ4] (M = Ge, Sn; Q = S, Se): Design and Syntheses of a Series of Heteroanionic Antiperovskite-Type Oxychalcogenides29La 3 (Ga 3 S 3 O 3 )(Si 2 O 7 ): An Oxychalcogenide Demonstrating Ultrawide Optical Bandgap and Favorable Birefringence Propelled by Divergent Anionic Groups6Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances17Designing infrared nonlinear optical crystals, Sr 2 MgSn 2 OS 6 and Sr 2 SnGa 2 OS 6 , with hybrid anionic frameworks via a double substitution strategy4La 2 ZnGa 2 S 6 O: a melilite-type transition metal oxysulfide achieving a well-balanced nonlinear optical behavior5Hetero‐Anionic Oxychalcogenides with Structures and Properties Tuned by the O:S Ratio14Layered Anion‐Mixed Oxycompounds: Synthesis, Properties, and Applications29Halogenated Metal–Organic Frameworks for Entangled Photon Pair Generation0

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  1. Two Mixed-Anion Units of [GeOSe3] and [GeO3S] Originating from Partial Isovalent Anion Substitution and Inducing Moderate Second Harmonic Generation Response and Large Birefringence

    Inorganic Chemistry · 2020-10-26

    Wenhao Xing, Pan Fang, Naizheng Wang, Zhuang Li, Zheshuai Lin, Jiyong Yao, Wenlong Yin, Bin Kang

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  2. A series of oxysulfides RE 2 M 2 S 3 O 4 (RE = Y, Tm; M = Zr, Hf) featuring a unique MS 3 O 4 motif and {[M 2 S 3 O 4 ] 8− } ∞ wrinkle layer

    Chemical Communications · 2021-01-01

    Zhen‐Tao Lu, Sihan Yang, Wenlong Liu, Sheng‐Ping Guo

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  3. Recent progress in oxychalcogenides as IR nonlinear optical materials

    Dalton Transactions · 2021-01-01

    Yang-Fang Shi, Wenbo Wei, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

    Read original paper ↗ ·

  4. Comparative study on the morphology, growth mechanism and luminescence property of RE2O2S:Eu3+ (RE = Lu, Gd, Y) phosphors

    Journal of Alloys and Compounds · 2021-03-10

    Benfu Qian, Ze Wang, Yulu Wang, Qianran Zhao, Xiuqing Zhou, Haifeng Zou, Yanhua Song, Ye Sheng

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  5. Structural Transformation and Second-Harmonic-Generation Activity in Rare-Earth and d0 Transition-Metal Oxysulfides RE3NbS3O4 (RE = Ce, Sm, Gd, Dy)

    Inorganic Chemistry · 2021-07-09

    Xin Lian, Zhen‐Tao Lu, Wen‐Dong Yao, Sihan Yang, Wenlong Liu, Ru‐Ling Tang, Sheng‐Ping Guo

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  6. Highly polarized [GeOTe 3 ] motif-driven structural order promotion and an enhanced second harmonic generation response in the new nonlinear optical oxytelluride Ba 3 Ge 2 O 4 Te 3

    Journal of Materials Chemistry C · 2021-11-18

    Mengran Sun, Xingyu Zhang, Chunxiao Li, Wenhao Liu, Zheshuai Lin, Jiyong Yao

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  7. Complex coordinated functional groups: A great genes for nonlinear optical materials

    Chinese Chemical Letters · 2021-12-03

    Weikang Wang, Dajiang Mei, Shaoguo Wen, Jian Wang, Yuandong Wu

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  8. Rational Crystal Structure Design and Nonlinear-Optical Properties of Noncentrosymmetric RbCu2NbS4

    Inorganic Chemistry · 2021-12-14

    Mengjia Luo, Chongxiang Huang, Feng Lin, Xiangli Che, Xian Zhang, Fuqiang Huang

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  9. Bridging oxygen atoms in trigonal prism units driven strong second-harmonic-generation efficiency in Sr 3 Ge 2 O 4 Te 3

    Chemical Communications · 2022-01-01

    Mengran Sun, Wenhao Xing, Ming‐Hsien Lee, Jiyong Yao

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  10. From oxides to oxysulfides: the mixed-anion GeS 3 O unit induces huge improvement in the nonlinear optical effect and optical anisotropy for potential nonlinear optical materials

    RSC Advances · 2022-01-01

    Xinyu Tian, Xiaodong Zhang, Yan Xiao, Xiaowen Wu, Bingbing Zhang, Daqing Yang, Kui Wu

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  11. Infrared nonlinear optical sulfide CsCd 4 In 5 S 12 exhibiting large second harmonic generation response

    Journal of Materials Chemistry C · 2022-01-01

    Yang Wang, Ruiqi Wang, Xiangli Che, Fei Liang, Min Luo, Yufeng Tang, Yunzhen Cao, Fuqiang Huang

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  12. Rational design of a promising oxychalcogenide infrared nonlinear optical crystal

    Chemical Science · 2022-01-01

    Yansong Cheng, Hongping Wu, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  13. Structural dimension modulation in a new oxysulfide system of Ae 2 Sb 2 O 2 S 3 (Ae = Ca and Ba)

    Inorganic Chemistry Frontiers · 2022-01-01

    Ruiqi Wang, Yantao Zhao, Xian Zhang, Fuqiang Huang

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  14. Synthesis, structural evolution and optical properties of a new family of oxychalcogenides [Sr 3 VO 4 ][MQ 3 ] (M = Ga, In, Q = S, Se)

    Inorganic Chemistry Frontiers · 2022-01-01

    Ruiqi Wang, Fei Liang, Xian Zhang, Yunjia Yang, Fuqiang Huang

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  15. Review of Heteroleptic Tetrahedra as Birefringent or Nonlinear Optical Motifs

    Crystal Growth & Design · 2022-01-18

    Junben Huang, Shan Shu, Gemei Cai

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  16. Pb 4 SeBr 6 : A Congruently Melting Mid‐Infrared Nonlinear Optical Material with Excellent Comprehensive Performance

    Advanced Optical Materials · 2022-01-29

    Jiankang Wang, Hongping Wu, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  17. Sr3[SnOSe3][CO3]: A Heteroanionic Nonlinear Optical Material Containing Planar π‐conjugated [CO3] and Heteroleptic [SnOSe3] Anionic Groups

    Angewandte Chemie International Edition · 2022-03-10

    Jiankang Wang, Yansong Cheng, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  18. Sr3[SnOSe3][CO3]: A Heteroanionic Nonlinear Optical Material Containing Planar π‐conjugated [CO3] and Heteroleptic [SnOSe3] Anionic Groups

    Angewandte Chemie · 2022-03-10

    Jiankang Wang, Yansong Cheng, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  19. Heteroanionic Melilite Oxysulfide: A Promising Infrared Nonlinear Optical Candidate with a Strong Second-Harmonic Generation Response, Sufficient Birefringence, and Wide Bandgap

    ACS Applied Materials & Interfaces · 2022-05-11

    Ruiqi Wang, Fei Liang, Xin Liu, Yi Xiao, Qianqian Liu, Xian Zhang, Li‐Ming Wu, Ling Chen, Fuqiang Huang

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  20. Improved Polarization in the Sr6Cd2Sb6O7Se10 Oxyselenide through Design of Lateral Sublattices for Efficient Photoelectric Conversion

    Angewandte Chemie · 2022-06-18

    Ruiqi Wang, Fakun Wang, Xian Zhang, Xinliang Feng, Chendong Zhao, Kejun Bu, Zhuang Zhang, Tianyou Zhai, Fuqiang Huang

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  21. Improved Polarization in the Sr6Cd2Sb6O7Se10 Oxyselenide through Design of Lateral Sublattices for Efficient Photoelectric Conversion

    Angewandte Chemie International Edition · 2022-06-18

    Ruiqi Wang, Fakun Wang, Xian Zhang, Xinliang Feng, Chendong Zhao, Kejun Bu, Zhuang Zhang, Tianyou Zhai, Fuqiang Huang

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  22. First Investigation of Nonlinear Optical Oxychalcogenide with Three‐Dimensional Anionic Framework and Special Windmill‐Like Functional Motifs †

    Chinese Journal of Chemistry · 2022-07-14

    Jia-Nuo Li, Xiaohui Li, Ying‐Xuan Xu, Wenlong Liu, Sheng‐Ping Guo

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  23. [Ba2F2][Ge2O3S2]: An Unprecedented Heteroanionic Infrared Nonlinear Optical Material Containing Three Typical Anions

    ACS Materials Letters · 2022-07-25

    Haonan Liu, Zhongfu Song, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  24. Mixed-Anion-Oriented Design of LnMGa3S6O (Ln = La, Pr, and Nd; M = Ca and Sr) Nonlinear Optical Oxysulfides with Targeted Property Balance

    ACS Applied Materials & Interfaces · 2022-08-11

    Jingjing Xu, Kui Wu, Yan Xiao, Bingbing Zhang, Haohai Yu, Huaijin Zhang

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  25. Recent developments on Bi-based oxychalcogenide materials with thermoelectric and optoelectronic applications: an overview

    Materials Today Chemistry · 2022-09-13

    A. Parida, Subrata Senapati, Rajesh R. Naik

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  26. [Cs6Cl][Ga5GeQ12] (Q = S, Se): two novel porous layered chalcohalides exhibiting two-band emission and ion exchange properties

    Science China Chemistry · 2022-09-15

    Ruiqi Wang, Xian Zhang, Fuqiang Huang

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  27. Oxychalcogenides as Promising Ultraviolet Nonlinear Optical Candidates: Experimental and Theoretical Studies of AEGeOS2(AE = Sr and Ba)

    Inorganic Chemistry · 2022-09-21

    Hedi Yang, Shenghua Zhou, Mao‐Yin Ran, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  28. The Antiperovskite‐Type Oxychalcogenides Ae3Q[GeOQ3] (Ae = Ba, Sr; Q = S, Se) with Large Second Harmonic Generation Responses and Wide Band Gaps

    Advanced Science · 2022-12-05

    Shaoxin Cui, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  29. Ba5Ga2SiO4S6: a Phase-Matching Nonlinear Optical Oxychalcogenide Design via Structural Regulation Originated from Heteroanion Introduction

    Inorganic Chemistry · 2022-12-16

    Yong‐Fang Shi, Shenghua Zhou, Bingxuan Li, Yi Liu, Xintao Wu, Hua Lin, Qi‐Long Zhu

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  30. Oxychalcogenides: A Promising Class of Materials for Nonlinear Optical Crystals with Mixed‐Anion Groups

    Chemistry - A European Journal · 2022-12-16

    Yu-Jie Zhang, Hongping Wu, Zhanggui Hu, Hongwei Yu

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  31. Anisotropic structure building unit involving diverse chemical bonds: a new opportunity for high-performance second-order NLO materials

    Chemical Society Reviews · 2023-01-01

    Xin Liu, Yi‐Chang Yang, Mengyue Li, Ling Chen, Li‐Ming Wu

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  32. Comprehensive review on multiple mixed-anion ligands, physicochemical performances and application prospects in metal oxysulfides

    Coordination Chemistry Reviews · 2023-04-05

    Jing Xu, Kui Wu

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  33. Recent progress of newly developed functional building units and corresponding nonlinear optical materials

    Chinese Journal of Structural Chemistry · 2023-05-11

    Wenjing Tan, Chenyang Zhang, Chenyang Zhang, Tingting Huang, Bingbing Zhang

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  34. Zn 2 HgP 2 S 8 : A Wide Bandgap Hg‐Based Infrared Nonlinear Optical Material with Large Second‐Harmonic Generation Response

    Small · 2023-07-20

    Yu Chu, Hongshan Wang, Tudi Abutukadi, Zhi Li, Miriding Mutailipu, Xin Su, Zhihua Yang, Junjie Li, Shilie Pan

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  35. Heteroanionic LaBrVIO4 (VI = Mo, W): Excellence in Both Nonlinear Optical Properties and Photoluminescent Properties

    Chemistry of Materials · 2023-08-14

    Zixian Jiao, Osvaldo Medina Mireles, Kevin Ensz, Fei Wang, Mingli Liang, P. Shiv Halasyamani, Bingbing Zhang, D. Paul Rillema, Jian Wang

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  36. Chiral and Polar Duality Design of Heteroanionic Compounds: Sr18Ge9O5S31 Based on [Sr3OGeS3]2+ and [Sr3SGeS3]2+ Groups

    Advanced Science · 2023-12-08

    Shaoxin Cui, Hongping Wu, Xinkang Dong, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Kenneth Reinhard Poeppelmeier, Hongwei Yu

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  37. Chemical perspectives on heteroanionic compounds: a potential playground for multiferroics

    Materials Chemistry Frontiers · 2024-01-01

    Karishma Prasad, Vivian Nguyen, Bingheng Ji, Jasmine Quah, Danielle Goodwin, Jian Wang

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  38. Heteroanionic [VO x S 4− x ] groups: tetrahedral units with large birefringence for mid-infrared nonlinear optical crystals

    Inorganic Chemistry Frontiers · 2024-01-01

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  39. First-principles screening of metal–organic frameworks for entangled photon pair generation

    Materials for Quantum Technology · 2024-02-23

    S. Shanmuga Sundara Raj, Simón Paiva, Rubén A. Fritz, Felipe Herrera, Yamil J. Colón

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  40. Sr2HgGe2OS6: A Hg-Based Oxychalcogenide Infrared Nonlinear Optical Material Exhibiting Favorable Balance between a Large Band Gap and Strong Second Harmonic Generation Response

    Inorganic Chemistry · 2024-05-23

    Guili Wang, Chunxiao Li, Ming‐Hsien Lee, Jiyong Yao

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  41. Ae3[TO3][SnOQ3] (Ae = Sr, Ba; T = Si, Ge; Q = S, Se) and Ba3[CO3][MQ4] (M = Ge, Sn; Q = S, Se): Design and Syntheses of a Series of Heteroanionic Antiperovskite-Type Oxychalcogenides

    Journal of the American Chemical Society · 2024-09-16

    Yuanding Yu, Shiyi Zhang, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  42. La 3 (Ga 3 S 3 O 3 )(Si 2 O 7 ): An Oxychalcogenide Demonstrating Ultrawide Optical Bandgap and Favorable Birefringence Propelled by Divergent Anionic Groups

    ACS Materials Letters · 2024-12-19

    Ming‐Shu Zhang, Shao‐Min Pei, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  43. Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances

    Small · 2024-12-23

    Junben Huang, Ailijiang Abudurusuli, Zhihua Yang, Shilie Pan

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  44. Designing infrared nonlinear optical crystals, Sr 2 MgSn 2 OS 6 and Sr 2 SnGa 2 OS 6 , with hybrid anionic frameworks via a double substitution strategy

    Materials Chemistry Frontiers · 2025-01-01

    Zhen Qian, Deman Kong, Hongping Wu, Hongwei Yu, Zhanggui Hu, Jiyang Wang, Yicheng Wu

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  45. La 2 ZnGa 2 S 6 O: a melilite-type transition metal oxysulfide achieving a well-balanced nonlinear optical behavior

    Dalton Transactions · 2025-01-01

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  46. Hetero‐Anionic Oxychalcogenides with Structures and Properties Tuned by the O:S Ratio

    Advanced Functional Materials · 2025-01-17

    Shaoxin Cui, Shuoxing Yang, Hongping Wu, Zhanggui Hu, Jiyang Wang, Yicheng Wu, Hongwei Yu

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  47. Layered Anion‐Mixed Oxycompounds: Synthesis, Properties, and Applications

    Advanced Science · 2025-02-07

    Yange Luan, Yumin Li, Zhong Li, Baoyue Zhang, Jian Zhen Ou

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  48. Halogenated Metal–Organic Frameworks for Entangled Photon Pair Generation

    Chemistry of Materials · 2025-12-14

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