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RESEARCH PAPER · Angewandte Chemie International Edition · 2019

Cs2Bi2O(Ge2O7) (CBGO): A Larger SHG Effect Induced by Synergistic Polarizations of BiO5 Polyhedra and GeO4 Tetrahedra

Ru‐Ling Tang, Chun‐Li Hu, Baolin Wu, Zhi Gang Fang, Yan Chen, Jiang‐Gao Mao

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Cs2Bi2O(Ge2O7) (CBGO): A Larger SHG Effect Induced by Synergistic Polarizations of BiO5 Polyhedra and GeO4 TetrahedraOriginalPolar polymorphism: α- and β-KCsWP 2 O 9 nonlinear optical materials with a strong second harmonic generation response25Ultraviolet nonlinear optical crystal: (NH4)ZnPO47Molecular Construction from AgGaS 2 to CuZnPS 4 : Defect-Induced Second Harmonic Generation Enhancement and Cosubstitution-Driven Band Gap Enlargement97Alignment of Polar Moieties Leading to Strong Second Harmonic Response in KCsMoP2O951Syntheses, characterization and calculations of LimAnM6O15 (A=Rb, Cs; M=Si, Ge; m+n=6)18A powder method for the high-efficacy evaluation of electro-optic crystals28A 2 Bi 2 (SeO 3 ) 3 F 2 (A = K and Rb): Excellent Mid-Infrared Nonlinear Optical Materials with Both Strong SHG Responses and Large Band Gaps64Series of Crystals with Giant Optical Anisotropy: A Targeted Strategic Research19Series of Crystals with Giant Optical Anisotropy: A Targeted Strategic Research140Sn2B5O9Br as an Outstanding Bifunctional Material with Strong Second‐Harmonic Generation Effect and Large Birefringence84The open-framework structure of KSbGe3O9 flux-grown crystals investigated by X-ray diffraction, vibrational spectroscopy, and DFT calculations5A new broad-band infrared window material CdPbOCl 2 with excellent comprehensive properties10Role of fluorine on the structure and second-harmonic-generation property of inorganic selenites and tellurites23Unexpected aliovalent cation substitution between two NLO materials LiBa 3 Bi 6 (SeO 3 ) 7 F 11 and Ba 3 Bi 6.5 (SeO 3 ) 7 F 10.5 O 0.518Cyanurates consisting of intrinsic planar π-conjugated 6-membered rings: An emerging source of optical functional materials112Vibrational and optical studies of a nonlinear optical crystal, Cs2Bi2O(Ge2O7)3High-Performance Second-Harmonic-Generation (SHG) Materials: New Developments and New Strategies324A3Te(Zn2Ge)Ge2O14 (A = Sr, Ba, and Pb): New Langasite Mid-infrared Nonlinear Optical Materials by Rational Chemical Substitution32A Congruent‐Melting Mid‐Infrared Nonlinear Optical Vanadate Exhibiting Strong Second‐Harmonic Generation22A Congruent‐Melting Mid‐Infrared Nonlinear Optical Vanadate Exhibiting Strong Second‐Harmonic Generation64CsCdGa3O6: A I-II-III-O (I = alkali metal, II = divalent metal, III = Al, Ga, In) type oxide featuring [Ga4O14]16− helical belts linked [Ga6O6]6+ and [Ga8O8]8+ cages11Structural, Electronic, Mechanical, Linear and Nonlinear Optical, and Piezoelectric Properties of CsIO\(_3\) Materials from Ab Initio Study0Enhancement of band gap and birefringence induced via π -conjugated chromophore with “tail effect”28Kyropoulos growth and characterization of monoclinic α-Bi 2 B 8 O 15 single crystal with a noncentrosymmetric structure4K6Bi13(PO4)15, K5Bi(P2O7)2, A5Bi5(PO4)4(P2O7)2 (A=K, Rb): New bismuth phosphates with different condensed phosphate groups8Anion-Tuned Synthesis of Ag Coordination Compounds: Approaches for Optimizing Second-Harmonic-Generation (SHG) Response5Hydrothermal synthesis of anisotropic SrGe 4 O 9 :Yb 3+ /Er 3+ nanorods and optimized upconversion luminescence for optical temperature sensing2Hydrothermal Synthesis of Anisotropic Srge4o9:Yb3+/Er3+ Nanorods and Optimized Upconvertion Luminescence for Fir Temperature Sensing0KRE(CO 3 ) 2 (RE = Eu, Gd, Tb): new mixed metal carbonates with strong photoluminescence and large birefringence15KSb(BeF 3 )F 3 : a totally fluorine strategy for achieving wide bandgap and large birefringence23Synthesis, Structure Determination, and Characterizations of a Polar Salt-Inclusion Scandium Germanate, Rb10Li3Sc4Ge12O36F7SrZnSnSe4: A quaternary selenide with large second harmonic generation and birefringence40Explorations of New SHG Materials in Mercury Iodate Sulfate System**9Cs2Bi2OSi2O7: A Promising Bismuth Silicate Nonlinear Optical Crystal with Face-Sharing BiO5 Polyhedra Exhibiting Strengthened Second Harmonic Generation Response and Birefringence43RbLiZn5(PO4)4 and BaLiZn3(PO4)3: two new zinc orthophosphates with all tetrahedra-based anion frameworks11Shedding Light on the Structure and Characterization of K2ZnGe2O6: A Phase-Matchable Nonlinear Optical Crystal19[Ba2F2][Ge2O3S2]: An Unprecedented Heteroanionic Infrared Nonlinear Optical Material Containing Three Typical Anions47Pb5(GeO4)(Ge2O7) and Pb3.32Ca1.68(GeO4)(Ge2O7): Two Nonlinear Optical Germanates Induced by Diverse PbOx Polyhedra17Enantiomeric Hydrogen-bonded Chains Driving Ferroelectric and Nonlinear Optical Behavior22Tailored Ordered Structures with Functional Units of Distorted [NbO6] and Antiparallel [GeO4] for Enhanced Birefringence in Germanate Crystal15Synthesis, structure, characterization, and electronic structure calculation of a new molecule-inclusion strontium gallate Sr6(Ga12O24)·Bi2O32Exploring Short-Wavelength Phase-Matching Nonlinear Optical Crystals by Employing KBe2BO3F2 as the Template96Single crystal growth and phase transition mechanism of KCsMoP 2 O 9 with efficient second harmonic generation via the emerging additional periodic phase technology4Synergistic coupling of interface ohmic contact and LSPR effects over Au/Bi 24 O 31 Br 10 nanosheets for visible-light-driven photocatalytic CO 2 reduction to CO38Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates51Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates7Polar Bismuth Selenite Iodate Oxide BiSeIO6 with Three Types of Lone Pair Cations in One Structure6Rational Design of a Rare‐Earth Oxychalcogenide Nd3[Ga3O3S3][Ge2O7] with Superior Infrared Nonlinear Optical Performance64Optimal Design of Mid-Infrared Nonlinear-Optical Crystals: From SrZnSnSe 4 to SrZnSiSe 423Cd2Nb2Te4O15: A Novel Pseudo‐Aurivillius‐Type Tellurite with Unprecedented Nonlinear Optical Properties and Excellent Stability40Centrosymmetric Rb2Sb(C2O4)2.5(H2O)3 and Noncentrosymmetric RbSb2(C2O4)F5: Two Antimony (III) Oxalates as UV Optical Materials20Giant Mid‐Infrared Second‐Harmonic Generation Response in a Densely‐Stacked Van Der Waals Transition‐Metal Oxychloride39Giant Mid‐Infrared Second‐Harmonic Generation Response in a Densely‐Stacked Van Der Waals Transition‐Metal Oxychloride8Two Noncentrosymmetric Bismuth Phosphates: Rational Design Synthesis and Optical Properties4CsSn2(HPO3)2I: The first inorganic metal phosphite iodide as a promising birefringent material exhibits a large birefringence with ideally layered framework25K(NH4)Zn2(PO4)2: a Beryllium-Free Sr2Be2B2O7 Derivative with Enhanced Interlayer Connectivity7Designing excellent UV birefringent materials through the synergistic interaction of two highly distorted functional groups23Absorption and emission properties of Eu3+ doped Cs2Bi2O(Ge2O7) acentric biaxial single crystal3Li13YGe4O16: A Mid-infrared Rare-Earth Germanate Nonlinear Optical Crystal Featuring a Broad Transmission Range and an Enlarged Band Gap10MgHg(SeO3)2(H2O)2: A magnesium mercury selenite with large birefringence7Enhanced UV Nonlinear Optical Properties in Layered Germanous Phosphites through Functional Group Sequential Construction11Enhanced UV Nonlinear Optical Properties in Layered Germanous Phosphites through Functional Group Sequential Construction118Ba3Zn4Si4O15: A Novel Centrosymmetric Silicate with Isolated SiO4 and Si2O7 Units0Achieving balanced UV SHG responses, optical band gaps and birefringence in rare earth compounds Ln(IO 3 )(SO 4 )·3H 2 O (Ln = Y, Gd, Er, Ho, Dy, Eu)4A Wide Band Gap Germanate with the Largest Second Harmonic Generation Response Created by Hypoxic Strategy22A Wide Band Gap Germanate with the Largest Second Harmonic Generation Response Created by Hypoxic Strategy6Synergistic triple-site engineering in ABX-type hybrid halides for high-performance nonlinear optical crystals14Recent Progress in the Design and Synthesis of Nonlinear Optical Crystals with Stereochemically Active Lone Pairs8Growth, structure and optical properties of PbBi3PO8 crystals0Oxygen Vacancies and Electric Poling Synergistically Modulate c ‐Axis Built‐in Electric Field in Bi 2 TeO 5 for Efficient H 2 O 2 Production under Real Water Motion7Single-crystal Ca 3 Ge 3 O 9 calcium germanate: structure, thermal and optical properties from experimental and first-principles analyses0中红外氧化物非线性光学晶体研究进展（特邀）0CaM 3 Si 4 P 11 (M = Al, Ga): [P 2 ] Motifs‐Modified Quasi‐T 3 Supertetrahedra Drive Superior Infrared Nonlinear Optical Performances1

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  1. Polar polymorphism: α- and β-KCsWP 2 O 9 nonlinear optical materials with a strong second harmonic generation response

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  2. Ultraviolet nonlinear optical crystal: (NH4)ZnPO4

    Inorganic Chemistry Communications · 2020-01-21

    Xun Chen, Yue Han, Qi Wei, Jie Pan, Song‐De Han, Li Wei, Guo‐Ming Wang

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  3. Molecular Construction from AgGaS 2 to CuZnPS 4 : Defect-Induced Second Harmonic Generation Enhancement and Cosubstitution-Driven Band Gap Enlargement

    Chemistry of Materials · 2020-03-05

    Zhuang Li, Shengzi Zhang, Zhiwei Huang, Li‐Dong Zhao, Ece Uykur, Wenhao Xing, Zheshuai Lin, Jiyong Yao, Yicheng Wu

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  4. Alignment of Polar Moieties Leading to Strong Second Harmonic Response in KCsMoP2O9

    Chemistry of Materials · 2020-03-13

    Tuohetijiang Baiheti, Shujuan Han, Abudukadi Tudi, Zhihua Yang, Shilie Pan

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  5. Syntheses, characterization and calculations of LimAnM6O15 (A=Rb, Cs; M=Si, Ge; m+n=6)

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  6. A powder method for the high-efficacy evaluation of electro-optic crystals

    National Science Review · 2020-05-16

    Feng Xu, Ge Zhang, Min Luo, Guang Peng, Yu Chen, Tao Yan, Ning Ye

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  7. A 2 Bi 2 (SeO 3 ) 3 F 2 (A = K and Rb): Excellent Mid-Infrared Nonlinear Optical Materials with Both Strong SHG Responses and Large Band Gaps

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    Shuangshuang Shi, Chensheng Lin, Guangsai Yang, Liling Cao, Bingxuan Li, Tao Yan, Min Luo, Ning Ye

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  8. Series of Crystals with Giant Optical Anisotropy: A Targeted Strategic Research

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  9. Series of Crystals with Giant Optical Anisotropy: A Targeted Strategic Research

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  10. Sn2B5O9Br as an Outstanding Bifunctional Material with Strong Second‐Harmonic Generation Effect and Large Birefringence

    Advanced Optical Materials · 2020-12-16

    Jingyu Guo, Shichao Cheng, Shujuan Han, Zhihua Yang, Shilie Pan

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  11. The open-framework structure of KSbGe3O9 flux-grown crystals investigated by X-ray diffraction, vibrational spectroscopy, and DFT calculations

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  12. A new broad-band infrared window material CdPbOCl 2 with excellent comprehensive properties

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  13. Role of fluorine on the structure and second-harmonic-generation property of inorganic selenites and tellurites

    Chemical Communications · 2021-01-01

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  14. Unexpected aliovalent cation substitution between two NLO materials LiBa 3 Bi 6 (SeO 3 ) 7 F 11 and Ba 3 Bi 6.5 (SeO 3 ) 7 F 10.5 O 0.5

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  15. Cyanurates consisting of intrinsic planar π-conjugated 6-membered rings: An emerging source of optical functional materials

    Coordination Chemistry Reviews · 2021-04-14

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  16. Vibrational and optical studies of a nonlinear optical crystal, Cs2Bi2O(Ge2O7)

    Spectrochimica Acta Part A Molecular and Biomolecular Spectroscopy · 2021-04-20

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  17. High-Performance Second-Harmonic-Generation (SHG) Materials: New Developments and New Strategies

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  18. A3Te(Zn2Ge)Ge2O14 (A = Sr, Ba, and Pb): New Langasite Mid-infrared Nonlinear Optical Materials by Rational Chemical Substitution

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  19. A Congruent‐Melting Mid‐Infrared Nonlinear Optical Vanadate Exhibiting Strong Second‐Harmonic Generation

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  20. A Congruent‐Melting Mid‐Infrared Nonlinear Optical Vanadate Exhibiting Strong Second‐Harmonic Generation

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  21. CsCdGa3O6: A I-II-III-O (I = alkali metal, II = divalent metal, III = Al, Ga, In) type oxide featuring [Ga4O14]16− helical belts linked [Ga6O6]6+ and [Ga8O8]8+ cages

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  22. Structural, Electronic, Mechanical, Linear and Nonlinear Optical, and Piezoelectric Properties of CsIO\(_3\) Materials from Ab Initio Study

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  23. Enhancement of band gap and birefringence induced via π -conjugated chromophore with “tail effect”

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  24. Kyropoulos growth and characterization of monoclinic α-Bi 2 B 8 O 15 single crystal with a noncentrosymmetric structure

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  25. K6Bi13(PO4)15, K5Bi(P2O7)2, A5Bi5(PO4)4(P2O7)2 (A=K, Rb): New bismuth phosphates with different condensed phosphate groups

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  26. Anion-Tuned Synthesis of Ag Coordination Compounds: Approaches for Optimizing Second-Harmonic-Generation (SHG) Response

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  27. Hydrothermal synthesis of anisotropic SrGe 4 O 9 :Yb 3+ /Er 3+ nanorods and optimized upconversion luminescence for optical temperature sensing

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  28. Hydrothermal Synthesis of Anisotropic Srge4o9:Yb3+/Er3+ Nanorods and Optimized Upconvertion Luminescence for Fir Temperature Sensing

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  29. KRE(CO 3 ) 2 (RE = Eu, Gd, Tb): new mixed metal carbonates with strong photoluminescence and large birefringence

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  30. KSb(BeF 3 )F 3 : a totally fluorine strategy for achieving wide bandgap and large birefringence

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  31. Synthesis, Structure Determination, and Characterizations of a Polar Salt-Inclusion Scandium Germanate, Rb10Li3Sc4Ge12O36F

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  32. SrZnSnSe4: A quaternary selenide with large second harmonic generation and birefringence

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  33. Explorations of New SHG Materials in Mercury Iodate Sulfate System**

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  34. Cs2Bi2OSi2O7: A Promising Bismuth Silicate Nonlinear Optical Crystal with Face-Sharing BiO5 Polyhedra Exhibiting Strengthened Second Harmonic Generation Response and Birefringence

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  35. RbLiZn5(PO4)4 and BaLiZn3(PO4)3: two new zinc orthophosphates with all tetrahedra-based anion frameworks

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  36. Shedding Light on the Structure and Characterization of K2ZnGe2O6: A Phase-Matchable Nonlinear Optical Crystal

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  37. [Ba2F2][Ge2O3S2]: An Unprecedented Heteroanionic Infrared Nonlinear Optical Material Containing Three Typical Anions

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  38. Pb5(GeO4)(Ge2O7) and Pb3.32Ca1.68(GeO4)(Ge2O7): Two Nonlinear Optical Germanates Induced by Diverse PbOx Polyhedra

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  40. Tailored Ordered Structures with Functional Units of Distorted [NbO6] and Antiparallel [GeO4] for Enhanced Birefringence in Germanate Crystal

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  41. Synthesis, structure, characterization, and electronic structure calculation of a new molecule-inclusion strontium gallate Sr6(Ga12O24)·Bi2O3

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  42. Exploring Short-Wavelength Phase-Matching Nonlinear Optical Crystals by Employing KBe2BO3F2 as the Template

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  43. Single crystal growth and phase transition mechanism of KCsMoP 2 O 9 with efficient second harmonic generation via the emerging additional periodic phase technology

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  44. Synergistic coupling of interface ohmic contact and LSPR effects over Au/Bi 24 O 31 Br 10 nanosheets for visible-light-driven photocatalytic CO 2 reduction to CO

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  45. Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates

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  46. Intense d‐p Hybridization in Nb3O15 Tripolymer Induced the Largest Second Harmonic Generation Response and Birefringence in Germanates

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  47. Polar Bismuth Selenite Iodate Oxide BiSeIO6 with Three Types of Lone Pair Cations in One Structure

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  48. Rational Design of a Rare‐Earth Oxychalcogenide Nd3[Ga3O3S3][Ge2O7] with Superior Infrared Nonlinear Optical Performance

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    Mao‐Yin Ran, Shenghua Zhou, Wenbo Wei, Bingxuan Li, Xin‐Tao Wu, Hua Lin, Qi‐Long Zhu

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  49. Optimal Design of Mid-Infrared Nonlinear-Optical Crystals: From SrZnSnSe 4 to SrZnSiSe 4

    Inorganic Chemistry · 2023-04-16

    Mengjie Ma, Junhui Dang, Yuandong Wu, Xiao‐Ming Jiang, Dajiang Mei

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  50. Cd2Nb2Te4O15: A Novel Pseudo‐Aurivillius‐Type Tellurite with Unprecedented Nonlinear Optical Properties and Excellent Stability

    Small · 2023-05-28

    Qiang Wang, Xuehua Dong, Ling Huang, Kang Min Ok, Zhien Lin, Guohong Zou

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