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RESEARCH PAPER · Small · 2023

Cs4Zn5P6S18I2: the Largest Birefringence in Chalcohalide Achieved by Highly Polarizable Nonlinear Optical Functional Motifs

Xian‐Dan Chai, Mingze Li, Shujuan Lin, Wen‐Fa Chen, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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Cs4Zn5P6S18I2: the Largest Birefringence in Chalcohalide Achieved by Highly Polarizable Nonlinear Optical Functional MotifsOriginalACu4AsS4 (A = K, Rb): Two infrared nonlinear optical crystals with strong second-harmonic generation responses originating from multiple chromophores12[Sn 3 OF]PO 4 vs. [Sn 3 F 3 ]PO 4 : enhancing birefringence by breaking the R 3 symmetry and realigning lone pairs12Reconstructing nearly isotropic microstructures to construct a one-dimensional framework causing record birefringence in thiophosphates13β -CsHg 2 I 5 , a compound with rare [Hg 2 I 5 ] dimers and large optical anisotropy2Mixed Anionic M(S/X)6 Polyhedra as Symmetry-Breaking Motifs to Enhance the Infrared Nonlinear Optical Response in Y–M–S–X (M = Ga, Ge; X = Cl, Br)5A congruent-melting rubidium zinc vanadium oxychloride exhibiting strong mid-infrared second-harmonic generation and high laser-induced damage threshold6[Rb3BaCl][In8Se14]: Compressed chalcopyrite-type selenide achieved by polycationic substitution strategy toward excellent nonlinear optical property18Tin chalcohalide Sn 11 (PS 4 ) 4 I 10 obtained from structural-template-oriented synthesis: exhibiting balanced infrared nonlinear optical performance6Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances17BaSbBS 4 : a record-high-performance birefringent crystal identified by a target-driven closed-loop strategy28AgGaS2 and Derivatives: Design, Synthesis, and Optical Properties8P4Sn (n = 3, 5, 7): Large Birefringence Enhanced by 3D Aromaticity and Packing Effect Induced Directional π–π Noncovalent Interactions6A Series of Pentanary Rare-Earth Oxysulfides Obtained by Heterovalent Cation and Anion Cosubstitution Exhibiting Nonlinear Optical Activity and Ultrawide Band Gaps1Achieving giant optical anisotropy in the mid-far infrared region via ideal alignment of dual functional motifs0Optimal three-dimensional [Ag 4 P 2 S 6 ]-framework assembly directed by a threefold roto-inversion axis for enhanced birefringence0van der Waals layered CuInP 2 S 6 as infrared nonlinear optical material1Achieving High‐Birefringence Thiophosphates From Low Polarizability Anisotropy Units by an Axial Linear Matching Strategy1Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0Mineral‐Inspired and Computation‐Assisted Rational Design of Polar Gittinsite‐Type Thiophosphates With Exceptional Nonlinear Optical Performance3Birefringence and Photocurrent Response of A Series of Rare-Earth Selenophosphates Cs4RE2(PSe4)2(P2Se6) (RE = La–Nd, Sm, Gd, Tb) Synthesized by the Metal Oxide–Boron–Chalcogen (MOBQ) Method0Cation-Modulated Activation of Linear Units in an Ordered Arrangement Achieves the Largest Optical Anisotropy in Wide-Bandgap Metal Chalcogenides0

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  1. ACu4AsS4 (A = K, Rb): Two infrared nonlinear optical crystals with strong second-harmonic generation responses originating from multiple chromophores

    Scripta Materialia · 2023-12-20

    Xin Lei Zhao, Chensheng Lin, Chao Wang, Haotian Tian, Pengxiang Dong, Tao Yan, Bingxuan Li, Ning Ye, Min Luo

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  2. [Sn 3 OF]PO 4 vs. [Sn 3 F 3 ]PO 4 : enhancing birefringence by breaking the R 3 symmetry and realigning lone pairs

    Inorganic Chemistry Frontiers · 2024-01-01

    Yuhan Hu, Xi Xu, Ruixi Wang, Jingyun Han, Shunsong Zhang, Shuhui Zhan, Jingyu Guo, Li‐Ming Wu, Ling Chen

    Read original paper ↗ ·

  3. Reconstructing nearly isotropic microstructures to construct a one-dimensional framework causing record birefringence in thiophosphates

    Chemical Science · 2024-01-01

    Lin‐Tao Jiang, Xiao‐Ming Jiang, Yuhang Fan, Bin‐Wen Liu, Guo‐Cong Guo

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  4. β -CsHg 2 I 5 , a compound with rare [Hg 2 I 5 ] dimers and large optical anisotropy

    Dalton Transactions · 2024-01-01

    Yingying Kong, Hongshan Wang, Wang Zhao, Qi Sun, Junjie Li, Shilie Pan

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  5. Mixed Anionic M(S/X)6 Polyhedra as Symmetry-Breaking Motifs to Enhance the Infrared Nonlinear Optical Response in Y–M–S–X (M = Ga, Ge; X = Cl, Br)

    Chemistry of Materials · 2024-04-01

    Yan Jie Guo, Bin‐Wen Liu, Chao-Hong Xie, Wen‐Fa Chen, Mingxin Li, Xiao‐Ming Jiang, Guo‐Cong Guo

    Read original paper ↗ ·

  6. A congruent-melting rubidium zinc vanadium oxychloride exhibiting strong mid-infrared second-harmonic generation and high laser-induced damage threshold

    Journal of Alloys and Compounds · 2024-04-14

    Lei Geng, Wenfei Li, Chang‐Yu Meng, You‐Zhao Lan, Baozhu Zhu, Shihua Ma, Qi Wu

    Read original paper ↗ ·

  7. [Rb3BaCl][In8Se14]: Compressed chalcopyrite-type selenide achieved by polycationic substitution strategy toward excellent nonlinear optical property

    Science China Materials · 2024-05-16

    Fan Wu, Wen‐Fa Chen, Zixuan Wu, Xiao‐Ming Jiang, Bin‐Wen Liu, Guo‐Cong Guo

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  8. Tin chalcohalide Sn 11 (PS 4 ) 4 I 10 obtained from structural-template-oriented synthesis: exhibiting balanced infrared nonlinear optical performance

    Inorganic Chemistry Frontiers · 2024-12-19

    Cuier Deng, Xi Qing Xu, Yuhan Hu, Jingyu Guo, Li‐Ming Wu, Ling Chen

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  9. Emergent Mid‐Infrared Nonlinear Optical Candidates With Targeted Balance Performances

    Small · 2024-12-23

    Junben Huang, Ailijiang Abudurusuli, Zhihua Yang, Shilie Pan

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  10. BaSbBS 4 : a record-high-performance birefringent crystal identified by a target-driven closed-loop strategy

    Chemical Science · 2025-01-01

    Ming‐Zhi Zhang, Yue Zhao, Chun‐Li Hu, Jiang‐Gao Mao

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  11. AgGaS2 and Derivatives: Design, Synthesis, and Optical Properties

    Nanomaterials · 2025-01-20

    Guansheng Xing, Bing Chen

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  12. P4Sn (n = 3, 5, 7): Large Birefringence Enhanced by 3D Aromaticity and Packing Effect Induced Directional π–π Noncovalent Interactions

    Advanced Optical Materials · 2025-04-11

    Wei Wu, Yi‐Bing Huang, Si‐Fan Lu, Jia Gao, Yan Guo, Wei‐Qi Huang, Meng‐Na Jing, Xiao‐Ming Jiang, Guo‐Cong Guo

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  13. A Series of Pentanary Rare-Earth Oxysulfides Obtained by Heterovalent Cation and Anion Cosubstitution Exhibiting Nonlinear Optical Activity and Ultrawide Band Gaps

    Inorganic Chemistry · 2025-07-10

    Zhi Bing Deng, Qiu-Yang Du, Fang-Xu Tian, Zong-Ze Li, Mingyang Li, Mao‐Yin Ran, Wenlong Liu, Sheng‐Ping Guo

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  14. Achieving giant optical anisotropy in the mid-far infrared region via ideal alignment of dual functional motifs

    Inorganic Chemistry Frontiers · 2026-01-01

    Yi-Wen Shan, Ming‐Zhi Zhang, C Hu, Jiang‐Gao Mao

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  15. Optimal three-dimensional [Ag 4 P 2 S 6 ]-framework assembly directed by a threefold roto-inversion axis for enhanced birefringence

    Inorganic Chemistry Frontiers · 2026-01-01

    MF Zhang, C Hu, Jiang‐Gao Mao

    Read original paper ↗ ·

  16. van der Waals layered CuInP 2 S 6 as infrared nonlinear optical material

    Chemical Communications · 2026-01-01

    Zheng-Tao Hu, 马祖驹, Xin‐Tao Wu, Qi‐Long Zhu, Hua Lin

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  17. Achieving High‐Birefringence Thiophosphates From Low Polarizability Anisotropy Units by an Axial Linear Matching Strategy

    Advanced Optical Materials · 2026-05-18

    Ming‐Zhi Zhang, C Hu, Yi‐Wen Shan, Jiang‐Gao Mao

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  18. Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects

    Advanced Optical Materials · 2026-07-21

    Xiangran Kong, Jingdong Yan, Zi Wang, Hongwei Leng, Shichao Cheng, Sue Hao, Xiaoran Niu, Zuotao Lei, Chunhui Yang

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  19. Mineral‐Inspired and Computation‐Assisted Rational Design of Polar Gittinsite‐Type Thiophosphates With Exceptional Nonlinear Optical Performance

    Advanced Functional Materials · 2026-08-06

    Mao‐Yin Ran, Shao-Peng Gui, Jian Cheng, Yu‐Xuan Zhang, Wen‐Dong Yao, Wenlong Liu, Sheng‐Ping Guo

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  20. Birefringence and Photocurrent Response of A Series of Rare-Earth Selenophosphates Cs4RE2(PSe4)2(P2Se6) (RE = La–Nd, Sm, Gd, Tb) Synthesized by the Metal Oxide–Boron–Chalcogen (MOBQ) Method

    Inorganic Chemistry · 2026-08-10

    Si Yang, Zong-Ze Li, Ning Wang, Xin Lei Zhao, Sheng‐Ping Guo

    Read original paper ↗ ·

  21. Cation-Modulated Activation of Linear Units in an Ordered Arrangement Achieves the Largest Optical Anisotropy in Wide-Bandgap Metal Chalcogenides

    Chemistry of Materials · 2026-09-09

    Wen‐Dong Yao, Xiao Huang, Qiu-Yang Du, Xu‐Bin Ni, Wenlong Liu, Sheng‐Ping Guo

    Read original paper ↗ ·
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