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RESEARCH PAPER · Inorganic Chemistry · 2021

α-Ca2CdP2 and β-Ca2CdP2: Two Polymorphic Phosphide-Based Infrared Nonlinear Crystals with Distorted NLO-Active Tetrahedral Motifs Realizing Large Second Harmonic Generation Effects and Suitable Band Gaps

Yingshuang Sun, Chensheng Lin, Jindong Chen, Feng Xu, Shunda Yang, Bingxuan Li, Guangsai Yang, Min Luo, Ning Ye

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α-Ca2CdP2 and β-Ca2CdP2: Two Polymorphic Phosphide-Based Infrared Nonlinear Crystals with Distorted NLO-Active Tetrahedral Motifs Realizing Large Second Harmonic Generation Effects and Suitable Band GapsOriginalApplying band gap engineering to tune the linear optical and nonlinear optical properties of noncentrosymmetric chalcogenides La 4 Ge 3 Se x S 12− x ( x = 0, 2, 4, 6, 8, 10)21The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks36Pnictides: An emerging class of infrared nonlinear optical material candidates47Hg 2 (SeO 3 )(SO 4 ): the first sulfate selenite with large birefringence explored from d 10 transition metal compounds36Uncovering a Vital Band Gap Mechanism of Pnictides49The Kurtz-Perry powder technique revisited: A case study on the importance of reference quality and broadband nonlinear optical measurements using LiInSe232BaSi7P10 and SrSi7P10: Two Infrared Nonlinear Optical Phosphides with T2 Supertetrahedra Exhibiting Strong Second‐Harmonic Generation Effects22Structural Complexity and Tuned Thermoelectric Properties of a Polymorph of the Zintl Phase Ca2CdSb2 with a Non-centrosymmetric Monoclinic Structure16(C4H10NO)PbX3 (X = Cl, Br): Design of Two Lead Halide Perovskite Crystals with Moderate Nonlinear Optical Properties35Synthesis and Crystal Structure of the Zintl Phases Na2CaCdSb2, Na2SrCdSb2 and Na2EuCdSb26Inherent law of SHG and phase-matching in 0D NLO materials: Permutation tetra-coordinated groups2The Electronic and Thermoelectric Transport Properties of Zintl Pnictides2Halogen-assisted octet binding electrons construction of pnictogens towards wide-bandgap nonlinear optical pnictides17Enhancing Properties with Distortion: A Comparative Study of Two Iron Phosphide Fe2P Polymorphs15β-Yb2CdSb2—A Complex Non-Centrosymmetric Zintl Polymorph3Achieving strong optical nonlinearity and wide bandgap of pnictides via ionic motif–driven directed assembly of covalent groups40Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 1131Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 116Multifunctional Cd‐based Hybrid with Large Birefringence Achieving Excellent Second Harmonic Generation and Reversible Temperature‐Activated Fluorescence for Anti‐counterfeiting16Pnictides: An Overview of Crystal Structures, Properties and Applications5Inorganic Ge-based ferroelectric perovskites towards quasi-phase-matching in the infrared region0Mid-Infrared Transparent Materials: from Mechanisms to Cutting-Edge Applications10Design of a High-Performance Infrared Nonlinear Optical Crystal via a Multiple Flexible-Group Synergistic Polarization Strategy12First Principles Study of Electronic and Thermoelectric Properties of Ca2CdP23Mid‐ to Far‐Infrared Nonlinear Optical Crystals: Design Strategies, Structure–Property Relationships and Engineering Prospects0CaM 3 Si 4 P 11 (M = Al, Ga): [P 2 ] Motifs‐Modified Quasi‐T 3 Supertetrahedra Drive Superior Infrared Nonlinear Optical Performances1Topology‐Preserving Ionic‐Unit Substitution Enables Sphalerite‐Like Phosphides Achieving Superior Infrared Optical Nonlinearity0Topology‐Preserving Ionic‐Unit Substitution Enables Sphalerite‐Like Phosphides Achieving Superior Infrared Optical Nonlinearity0Beyond the bandgap bottleneck: structure–property design principles for infrared nonlinear optical phosphides0Homologous lattice coupling drives the formation of tetrahedra-ordered phase exhibiting enhanced optical nonlinearity and band gap0

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  1. Applying band gap engineering to tune the linear optical and nonlinear optical properties of noncentrosymmetric chalcogenides La 4 Ge 3 Se x S 12− x ( x = 0, 2, 4, 6, 8, 10)

    Inorganic Chemistry Frontiers · 2021-01-01

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  2. The Rise of Infrared Nonlinear Optical Pnictides: Advances and Outlooks

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  3. Pnictides: An emerging class of infrared nonlinear optical material candidates

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    Jindong Chen, Xiaotian Jiang, Qingchen Wu, Zheshuai Lin, Min Luo, Ning Ye

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  4. Hg 2 (SeO 3 )(SO 4 ): the first sulfate selenite with large birefringence explored from d 10 transition metal compounds

    Materials Chemistry Frontiers · 2022-01-01

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  5. Uncovering a Vital Band Gap Mechanism of Pnictides

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  6. The Kurtz-Perry powder technique revisited: A case study on the importance of reference quality and broadband nonlinear optical measurements using LiInSe2

    Journal of Alloys and Compounds · 2022-05-13

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  7. BaSi7P10 and SrSi7P10: Two Infrared Nonlinear Optical Phosphides with T2 Supertetrahedra Exhibiting Strong Second‐Harmonic Generation Effects

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  8. Structural Complexity and Tuned Thermoelectric Properties of a Polymorph of the Zintl Phase Ca2CdSb2 with a Non-centrosymmetric Monoclinic Structure

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  9. (C4H10NO)PbX3 (X = Cl, Br): Design of Two Lead Halide Perovskite Crystals with Moderate Nonlinear Optical Properties

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  10. Synthesis and Crystal Structure of the Zintl Phases Na2CaCdSb2, Na2SrCdSb2 and Na2EuCdSb2

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  11. Inherent law of SHG and phase-matching in 0D NLO materials: Permutation tetra-coordinated groups

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  12. The Electronic and Thermoelectric Transport Properties of Zintl Pnictides

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  13. Halogen-assisted octet binding electrons construction of pnictogens towards wide-bandgap nonlinear optical pnictides

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  14. Enhancing Properties with Distortion: A Comparative Study of Two Iron Phosphide Fe2P Polymorphs

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  15. β-Yb2CdSb2—A Complex Non-Centrosymmetric Zintl Polymorph

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  16. Achieving strong optical nonlinearity and wide bandgap of pnictides via ionic motif–driven directed assembly of covalent groups

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  17. Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 11

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  18. Reinforced Nonlinear Optical Performances Induced by P‐P Homoatomic Bond in Phosphide SrIn 3 Si 4 P 11

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  19. Multifunctional Cd‐based Hybrid with Large Birefringence Achieving Excellent Second Harmonic Generation and Reversible Temperature‐Activated Fluorescence for Anti‐counterfeiting

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  20. Pnictides: An Overview of Crystal Structures, Properties and Applications

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  21. Inorganic Ge-based ferroelectric perovskites towards quasi-phase-matching in the infrared region

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